arXiv subjects

G. Rempe

Publications and source records attributed to G. Rempe.

At least 37 records · Page 2Linked to original sources

arXiv2009

Controlling a magnetic Feshbach resonance with laser light

The capability to tune the strength of the elastic interparticle interaction is crucial for many experiments with ultracold gases. Magnetic Feshbach resonances are a tool widely used for this purpose, but future experiments would benefit from additional flexibility such as spatial modulation of the interaction strength on short length scales. Optical Feshbach resonances offer this possibility in principle, but suffer from fast particle loss due to light-induced inelastic collisions. Here we show that light near-resonant with a molecular bound-to-bound transition can be used to shift the magnetic field at which a magnetic Feshbach resonance occurs. This makes it possible to tune the interaction strength with laser light and at the same time induce considerably less loss than an optical Feshbach resonance would do.

cond-mat.other↗

arXiv2009

Lieb-Liniger model of a dissipation-induced Tonks-Girardeau gas

We show that strong inelastic interactions between bosons in one dimension create a Tonks-Girardeau gas, much as in the case of elastic interactions. We derive a Markovian master equation that describes the loss caused by the inelastic collisions. This yields a loss rate equation and a dissipative Lieb-Liniger model for short times. We obtain an analytic expression for the pair correlation function in the limit of strong dissipation. Numerical calculations show how a diverging dissipation strength leads to a vanishing of the actual loss rate and renders an additional elastic part of the interaction irrelevant.

cond-mat.other↗

arXiv2009

Electrostatic extraction of cold molecules from a cryogenic reservoir

We present a method which delivers a continuous, high-density beam of slow and internally cold polar molecules. In our source, warm molecules are first cooled by collisions with a cryogenic helium buffer gas. Cold molecules are then extracted by means of an electrostatic quadrupole guide. For ND$_3$ the source produces fluxes up to $(7 \pm ^{7}_{4}) \times 10^{10}$ molecules/s with peak densities up to $(1.0 \pm ^{1.0}_{0.6}) \times 10^9$ molecules/cm$^3$. For H$_2$CO the population of rovibrational states is monitored by depletion spectroscopy, resulting in single-state populations up to $(82 \pm 10)%$.

physics.chem-ph↗

arXiv2009

Cold guided beams of water isotopologs

Electrostatic velocity filtering and guiding is an established technique to produce high fluxes of cold polar molecules. In this paper we clarify different aspects of this technique by comparing experiments to detailed calculations. In the experiment, we produce cold guided beams of the three water isotopologs H2O, D2O and HDO. Their different rotational constants and orientations of electric dipole moments lead to remarkably different Stark shift properties, despite the molecules being very similar in a chemical sense. Therefore, the signals of the guided water isotopologs differ on an absolute scale and also exhibit characteristic electrode voltage dependencies. We find excellent agreement between the relative guided fractions and voltage dependencies of the investigated isotopologs and predictions made by our theoretical model of electrostatic velocity filtering.

physics.chem-ph↗

arXiv2008

Fast Excitation and Photon Emission of a Single-Atom-Cavity System

We report on the fast excitation of a single atom coupled to an optical cavity using laser pulses that are much shorter than all other relevant processes. The cavity frequency constitutes a control parameter that allows the creation of single photons in a superposition of two tunable frequencies. Each photon emitted from the cavity thus exhibits a pronounced amplitude modulation determined by the oscillatory energy exchange between the atom and the cavity. Our technique constitutes a versatile tool for future quantum networking experiments.

quant-ph↗

arXiv2008

Photon-Photon Entanglement with a Single Trapped Atom

An experiment is performed where a single rubidium atom trapped within a high-finesse optical cavity emits two independently triggered entangled photons. The entanglement is mediated by the atom and is characterized both by a Bell inequality violation of S=2.5, as well as full quantum-state tomography, resulting in a fidelity exceeding F=90%. The combination of cavity-QED and trapped atom techniques makes our protocol inherently deterministic - an essential step for the generation of scalable entanglement between the nodes of a distributed quantum network.

quant-ph↗

arXiv2008

Two-photon gateway in one-atom cavity quantum electrodynamics

Single atoms absorb and emit light from a resonant laser beam photon by photon. We show that a single atom strongly coupled to an optical cavity can absorb and emit resonant photons in pairs. The effect is observed in a photon correlation experiment on the light transmitted through the cavity. We find that the atom-cavity system transforms a random stream of input photons into a correlated stream of output photons, thereby acting as a two-photon gateway. The phenomenon has its origin in the quantum anharmonicity of the energy structure of the atom-cavity system. Future applications could include the controlled interaction of two photons by means of one atom.

quant-ph↗

arXiv2008

A Dissipative Tonks-Girardeau Gas of Molecules

Strongly correlated states in many-body systems are traditionally created using elastic interparticle interactions. Here we show that inelastic interactions between particles can also drive a system into the strongly correlated regime. This is shown by an experimental realization of a specific strongly correlated system, namely a one-dimensional molecular Tonks-Girardeau gas.

cond-mat.other↗

arXiv2008

Dissipation induced Tonks-Girardeau gas in an optical lattice

We present a theoretical investigation of a lattice Tonks-gas that is created by inelastic, instead of elastic interactions. An analytical calculation shows that in the limit of strong two-body losses, the dynamics of the system is effectively that of a Tonks gas. We also derive an analytic expression for the effective loss rate. We find good agreement between these analytical results and results from a rigorous numerical calculation. The Tonks character of the gas is visible both in a reduced effective loss rate and in the momentum distribution of the gas.

cond-mat.other↗

arXiv2008

Strong dissipation inhibits losses and induces correlations in cold molecular gases

Atomic quantum gases in the strong-correlation regime offer unique possibilities to explore a variety of many-body quantum phenomena. Reaching this regime has usually required both strong elastic and weak inelastic interactions, as the latter produce losses. We show that strong inelastic collisions can actually inhibit particle losses and drive a system into a strongly-correlated regime. Studying the dynamics of ultracold molecules in an optical lattice confined to one dimension, we show that the particle loss rate is reduced by a factor of 10. Adding a lattice along the one dimension increases the reduction to a factor of 2000. Our results open up the possibility to observe exotic quantum many-body phenomena with systems that suffer from strong inelastic collisions.

cond-mat.other↗

arXiv2008

Nonlinear spectroscopy of photons bound to one atom

Optical nonlinearities typically require macroscopic media, thereby making their implementation at the quantum level an outstanding challenge. Here we demonstrate a nonlinearity for one atom enclosed by two highly reflecting mirrors. We send laser light through the input mirror and record the light from the output mirror of the cavity. For weak laser intensity, we find the vacuum-Rabi resonances. But for higher intensities, we find an additional resonance. It originates from the fact that the cavity can accommodate only an integer number of photons and that this photon number determines the characteristic frequencies of the coupled atom-cavity system. We selectively excite such a frequency by depositing at once two photons into the system and find a transmission which increases with the laser intensity squared. The nonlinearity differs from classical saturation nonlinearities and is direct spectroscopic proof of the quantum nature of the atom-cavity system. It provides a photon-photon interaction by means of one atom, and constitutes a step towards a two-photon gateway or a single-photon transistor.

quant-ph↗

arXiv2007

Doppler-Free Spectroscopy of Weak Transitions: An Analytical Model Applied to Formaldehyde

Experimental observation of Doppler-free signals for weak transitions can be greatly facilitated by an estimate for their expected amplitudes. We derive an analytical model which allows the Doppler-free amplitude to be estimated for small Doppler-free signals. Application of this model to formaldehyde allows the amplitude of experimentally observed Doppler-free signals to be reproduced to within the experimental error.

physics.optics↗

arXiv2007

Internal-state thermometry by depletion spectroscopy in a cold guided beam of formaldehyde

We present measurements of the internal state distribution of electrostatically guided formaldehyde. Upon excitation with continuous tunable ultraviolet laser light the molecules dissociate, leading to a decrease in the molecular flux. The population of individual guided states is measured by addressing transitions originating from them. The measured populations of selected states show good agreement with theoretical calculations for different temperatures of the molecule source. The purity of the guided beam as deduced from the entropy of the guided sample using a source temperature of 150K corresponds to that of a thermal ensemble with a temperature of about 30 K.

physics.chem-ph↗

arXiv2007

Trapping of Neutral Rubidium with a Macroscopic Three-Phase Electric Trap

We trap neutral ground-state rubidium atoms in a macroscopic trap based on purely electric fields. For this, three electrostatic field configurations are alternated in a periodic manner. The rubidium is precooled in a magneto-optical trap, transferred into a magnetic trap and then translated into the electric trap. The electric trap consists of six rod-shaped electrodes in cubic arrangement, giving ample optical access. Up to 10^5 atoms have been trapped with an initial temperature of around 20 microkelvin in the three-phase electric trap. The observations are in good agreement with detailed numerical simulations.

physics.atom-ph↗

arXiv2007

Atom-molecule Rabi oscillations in a Mott insulator

We observe large-amplitude Rabi oscillations between an atomic and a molecular state near a Feshbach resonance. The experiment uses 87Rb in an optical lattice and a Feshbach resonance near 414 G. The frequency and amplitude of the oscillations depend on magnetic field in a way that is well described by a two-level model. The observed density dependence of the oscillation frequency agrees with the theoretical expectation. We confirmed that the state produced after a half-cycle contains exactly one molecule at each lattice site. In addition, we show that for energies in a gap of the lattice band structure, the molecules cannot dissociate.

cond-mat.stat-mech↗

arXiv2007

Trapping and observing single atoms in the dark

A single atom strongly coupled to a cavity mode is stored by three-dimensional confinement in blue-detuned cavity modes of different longitudinal and transverse order. The vanishing light intensity at the trap center reduces the light shift of all atomic energy levels. This is exploited to detect a single atom by means of a dispersive measurement with 95% confidence in 0.010 ms, limited by the photon-detection efficiency. As the atom switches resonant cavity transmission into cavity reflection, the atom can be detected while scattering about one photon.

quant-ph↗

arXiv2007

Preparation of a quantum state with one molecule at each site of an optical lattice

Ultracold gases in optical lattices are of great interest, because these systems bear a great potential for applications in quantum simulations and quantum information processing, in particular when using particles with a long-range dipole-dipole interaction, such as polar molecules. Here we show the preparation of a quantum state with exactly one molecule at each site of an optical lattice. The molecules are produced from an atomic Mott insulator with a density profile chosen such that the central region of the gas contains two atoms per lattice site. A Feshbach resonance is used to associate the atom pairs to molecules. Remaining atoms can be removed with blast light. The technique does not rely on the molecule-molecule interaction properties and is therefore applicable to many systems.

cond-mat.stat-mech↗

arXiv2007

Light force fluctuations in a strongly coupled atom-cavity system

Between mirrors, the density of electromagnetic modes differs from the one in free space. This changes the radiation properties of an atom as well as the light forces acting on an atom. It has profound consequences in the strong-coupling regime of cavity quantum electrodynamics. For a single atom trapped inside the cavity, we investigate the atom-cavity system by scanning the frequency of a probe laser for various atom-cavity detunings. The avoided crossing between atom and cavity resonance is visible in the transmission of the cavity. It is also visible in the loss rate of the atom from the intracavity dipole trap. On the normal-mode resonances, the dominant contribution to the loss rate originates from dipole-force fluctuations which are dramatically enhanced in the cavity. This conclusion is supported by Monte-Carlo simulations.

quant-ph↗