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G. Royer

Publications and source records attributed to G. Royer.

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Spontaneous fission half-lives of heavy and superheavy nuclei within a generalized liquid drop model

We systematically calculate the spontaneous fission half-lives for heavy and superheavy nuclei between U and Fl isotopes. The spontaneous fission process is studied within the semi-empirical WKB approximation. The potential barrier is obtained using a generalized liquid drop model, taking into account the nuclear proximity, the mass asymmetry, the phenomenological pairing correction, and the microscopic shell correction. Macroscopic inertial-mass function has been employed for the calculation of the fission half-life. The results reproduce rather well the experimental data. Relatively long half-lives are predicted for many unknown nuclei, sufficient to detect them if synthesized in a laboratory.

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Fusion excitation function revisited

We report on a comprehensive systematics of fusion-evaporation and/or fusion-fission cross sections for a very large variety of systems over an energy range 4-155 A.MeV. Scaled by the reaction cross sections, fusion cross sections do not show a universal behavior valid for all systems although a high degree of correlation is present when data are ordered by the system mass asymmetry.For the rather light and close to mass-symmetric systems the main characteristics of the complete and incomplete fusion excitation functions can be precisely determined. Despite an evident lack of data above 15A.MeV for all heavy systems the available data suggests that geometrical effects could explain the persistence of incomplete fusion at incident energies as high as 155A.MeV.

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Clusters in Light Nuclei

A great deal of research work has been undertaken in the alpha-clustering study since the pioneering discovery, half a century ago, of 12C+12C molecular resonances. Our knowledge of the field of the physics of nuclear molecules has increased considerably and nuclear clustering remains one of the most fruitful domains of nuclear physics, facing some of the greatest challenges and opportunities in the years ahead. In this work, the occurence of "exotic" shapes in light N=Z alpha-like nuclei is investigated. Various approaches of superdeformed and hyperdeformed bands associated with quasimolecular resonant structures are presented. Results on clustering aspects are also discussed for light neutron-rich Oxygen isotopes.

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Binary reaction decays from 24Mg+12C

Charged particle and gamma decays in 24Mg* are investigated for excitation energies where quasimolecular resonances appear in 12C+12C collisions. Various theoretical predictions for the occurence of superdeformed and hyperdeformed bands associated with resonance structures with low spin are discussed within the measured 24Mg* excitation energy region. The inverse kinematics reaction 24Mg+12C is studied at E_lab(24Mg) = 130 MeV, an energy which enables the population of 24Mg states decaying into 12C+12C resonant break-up states. Exclusive data were collected with the Binary Reaction Spectrometer in coincidence with EUROBALL IV installed at the VIVITRON Tandem facility at Strasbourg. Specific structures with large deformation were selectively populated in binary reactions and their associated gamma decays studied. Coincident events associated with inelastic and alpha-transfer channels have been selected by choosing the excitation energy or the entry point via the two-body Q-values. The analysis of the binary reaction channels is presented with a particular emphasis on 24Mg-gamma, 20Ne-gamma and 16O-gamma coincidences. New information (spin and branching ratios) is deduced on high-energy states in 24Mg and 16O, respectively.

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Proton radioactivity within a generalized liquid drop model

The proton radioactivity half-lives of spherical proton emitters are investigated theoretically. The potential barriers preventing the emission of protons are determined in the quasimolecular shape path within a generalized liquid drop model (GLDM) including the proximity effects between nuclei in a neck and the mass and charge asymmetry. The penetrability is calculated with the WKB approximation. The spectroscopic factor has been taken into account in half-life calculation, which is obtained by employing the relativistic mean field (RMF) theory combined with the BCS method with the force NL3. The half-lives within the GLDM are compared with the experimental data and other theoretical values. The GLDM works quite well for spherical proton emitters when the spectroscopic factors are considered, indicating the necessity of introducing the spectroscopic factor and the success of the GLDM for proton emission. Finally, we present two formulas for proton emission half-life calculation similar to the Viola-Seaborg formulas and Royer's formulas of alpha decay.

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Branching ratios of $α$-decay to excited states of even-even nuclei

Branching ratios of $α$-decay to members of the ground state rotational band and excited 0$^{+}$ states of even-even nuclei are calculated in the framework of the generalized liquid drop model (GLDM) by taking into account the angular momentum of the $α$-particle and the excitation probability of the daughter nucleus. The calculation covers isotopic chains from Hg to Fm in the mass regions $180< A <202$ and A$\geq 224$. The calculated branching ratios of the $α$-transitions are in good agreement with the experimental data and some useful predictions are provided for future experiments.

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Reaction mechanisms in 24Mg+12C and 32S+24Mg

The occurence of "exotic" shapes in light N=Z alpha-like nuclei is investigated for 24Mg+12C and 32S+24Mg. Various approaches of superdeformed and hyperdeformed bands associated with quasimolecular resonant structures with low spin are presented. For both reactions, exclusive data were collected with the Binary Reaction Spectrometer in coincidence with EUROBALL IV installed at the VIVITRON Tandem facility of Strasbourg. Specific structures with large deformation were selectively populated in binary reactions and their associated $γ$-decays studied. The analysis of the binary and ternary reaction channels is discussed.

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Fission decay of N = Z nuclei at high angular momentum: $^{60}$Zn

Using a unique two-arm detector system for heavy ions (the BRS, binary reaction spectrometer) coincident fission events have been measured from the decay of $^{60}$Zn compound nuclei formed at 88MeV excitation energy in the reactions with $^{36}$Ar beams on a $^{24}$Mg target at $E_{lab}(^{36}$Ar) = 195 MeV. The detectors consisted of two large area position sensitive (x,y) gas telescopes with Bragg-ionization chambers. From the binary coincidences in the two detectors inclusive and exclusive cross sections for fission channels with differing losses of charge were obtained. Narrow out-of-plane correlations corresponding to coplanar decay are observed for two fragments emitted in binary events, and in the data for ternary decay with missing charges from 4 up to 8. After subtraction of broad components these narrow correlations are interpreted as a ternary fission process at high angular momentum through an elongated shape. The lighter mass in the neck region consists dominantly of two or three-particles. Differential cross sections for the different mass splits for binary and ternary fission are presented. The relative yields of the binary and ternary events are explained using the statistical model based on the extended Hauser-Feshbach formalism for compound nucleus decay. The ternary fission process can be described by the decay of hyper-deformed states with angular momentum around 45-52 $hbar$.

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$α$ particle preformation in heavy nuclei and penetration probability

The $α$ particle preformation in the even-even nuclei from $^{108}$Te to $^{294}$118 and the penetration probability have been studied. The isotopes from Pb to U have been firstly investigated since the experimental data allow us to extract the microscopic features for each element. The assault frequency has been estimated using classical methods and the penetration probability from tunneling through the Generalized Liquid Drop Model (GLDM) potential barrier. The preformation factor has been extracted from experimental $α$ decay energies and half-lives. The shell closure effects play the key role in the $α$ preformation. The more the nucleon number is close to the magic numbers, the more the formation of $α$ cluster is difficult inside the mother nucleus. The penetration probabilities reflect that 126 is a neutron magic number. The penetration probability range is very large compared to that of the preformation factor. The penetration probability determines mainly the $α$ decay half-life while the preformation factor allows us to obtain information on the nuclear structure. The study has been extended to the newly observed heaviest nuclei.

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Ternary cluster decay within the liquid drop model

Longitudinal ternary and binary fission barriers of $^{36}$Ar, $^{56}$Ni and $^{252}$Cf nuclei have been determined within a rotational liquid drop model taking into account the nuclear proximity energy. For the light nuclei the heights of the ternary fission barriers become competitive with the binary ones at high angular momenta since the maximum lies at an outer position and has a much higher moment of inertia.

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On the coefficients of the liquid drop model mass formulae and nuclear radii

The coefficients of different mass formulae derived from the liquid drop model and including or not the curvature energy, the diffuseness correction to the Coulomb energy, the charge exchange correction term, different forms of the Wigner term and different powers of the relative neutron excess $I=(N-Z)/A$ have been determined by a least square fitting procedure to 2027 experimental atomic masses. The Coulomb diffuseness correction $Z^2/A$ term or the charge exchange correction $Z^{4/3}/A^{1/3}$ term plays the main role to improve the accuracy of the mass formula. The Wigner term and the curvature energy can also be used separately for the same purpose. The introduction of an $|I|$ dependence in the surface and volume energies improves slightly the efficiency of the expansion and is more effective than an $I^4$ dependence. Different expressions reproducing the experimental nuclear charge radius are provided. The different fits lead to a surface energy coefficient of around 17-18 MeV and a relative equivalent rms charge radius r$_0$ of 1.22-1.23 fm.

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Recent $α$ decay half-lives and analytic expression predictions including superheavy nuclei

New recent experimental $α$ decay half-lives have been compared with the results obtained from previously proposed formulas depending only on the mass and charge numbers of the $α$ emitter and the Q$α$ value. For the heaviest nuclei they are also compared with calculations using the Density-Dependent M3Y (DDM3Y) effective interaction and the Viola-Seaborg-Sobiczewski (VSS) formulas. The correct agreement allows us to make predictions for the $α$ decay half-lives of other still unknown superheavy nuclei from these analytic formulas using the extrapolated Q$α$ of G. Audi, A. H. Wapstra, and C. Thibault [Nucl. Phys. A729, 337 (2003)].

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On the mass formula and Wigner and curvature energy terms

The efficiency of different mass formulas derived from the liquid drop model including or not the curvature energy, the Wigner term and different powers of the relative neutron excess $I$ has been determined by a least square fitting procedure to the experimental atomic masses assuming a constant R$_{0,charge}$/A$^{1/3}$ ratio. The Wigner term and the curvature energy can be used independently to improve the accuracy of the mass formula. The different fits lead to a surface energy coefficient of around 17-18 MeV, a relative sharp charge radius r$_0$ of 1.22-1.23 fm and a proton form-factor correction to the Coulomb energy of around 0.9 MeV.

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Theoretical and experimental αdecay half-lives of the heaviest odd-Z elements and general predictions

Theoretical decay half-lives of the heaviest odd-Z nuclei are calculated using the experimental Q value. The barriers in the quasimolecular shape path are determined within a Generalized Liquid Drop Model (GLDM) and the WKB approximation is used. The results are compared with calculations using the Density-Dependent M3Y (DDM3Y) effective interaction and the Viola-Seaborg-Sobiczewski (VSS) formulas. The calculations provide consistent estimates for the half-lives of the decay chains of these superheavy elements. The experimental data stand between the GLDM calculations and VSS ones in the most time. Predictions are provided for the decay half-lives of other superheavy nuclei within the GLDM and VSS approaches using the recent extrapolated Q of Audi, Wapstra, and Thibault [Nucl. Phys. A729, 337 (2003)], which may be used for future experimental assignment and identification.

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Coefficients and terms of the liquid drop model and mass formula

The coefficients of different combinations of terms of the liquid drop model have been determined by a least square fitting procedure to the experimental atomic masses. The nuclear masses can also be reproduced using a Coulomb radius taking into account the increase of the ratio $R\_0/A^{1/3}$ with increasing mass, the fitted surface energy coefficient remaining around 18 MeV.

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alpha decay half-lives of new superheavy nuclei within a generalized liquid drop model

The alpha decay half-lives of the recently produced isotopes of the 112, 114, 116 and 118 nuclei and decay products have been calculated in the quasi-molecular shape path using the experimental Qalpha value and a Generalized Liquid Drop Model including the proximity effects between nucleons in the neck or the gap between the nascent fragments. Reasonable estimates are obtained for the observed alpha decay half-lives. The results are compared with calculations using the Density-Dependent M3Y effective interaction and the Viola-Seaborg-Sobiczewski formulae. Generalized Liquid Drop Model predictions are provided for the alpha decay half-lives of other superheavy nuclei using the Finite Range Droplet Model Qalpha and compared with the values derived from the VSS formulae.

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On the double and triple-humped fission barriers and half-lives of actinide elements

The deformation barriers standing in the quasi-molecular shape path have been determined in the actinide region within a macroscopic-microscopic energy derived from a generalized liquid drop model, the algebraic droplet model shell corrections and analytic expressions for the pairing energies. Double and triple-humped fission barriers appear. The second barrier corresponds to the transition from one-body shapes to two touching ellipsoids. The third minimum and third peak, when they exist, come from shell rearrangements in the deformed fragment. The shape of the other almost magic one is close to the sphere. The barrier heights agreewith the experimental results, the energy of the second minimum being a little too high. The predicted half-lives follow the experimental data trend.

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Entrance channels and alpha decay half-lives of the heaviest elements

The barriers standing against the formation of superheavy elements and their consecutive $α$ decay have been determined in the quasimolecular shape path within a Generalized Liquid Drop Model including the proximity effects between nucleons in a neck, the mass and charge asymmetry, a precise nuclear radius and the shell effects given by the Droplet Model. For moderately asymmetric reactions double-hump potential barriers stand and fast fission of compact shapes in the outer well is possible. Very asymmetric reactions lead to one hump barriers which can be passed only with a high energy relatively to the superheavy element energy. Then, only the emission of several neutrons or an $α$ particle can allow to reach an eventual ground state. For almost symmetric heavy-ion reactions, there is no more external well and the inner barrier is higher than the outer one.

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