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G. S. Tucker

Publications and source records attributed to G. S. Tucker.

At least 19 recordsLinked to original sources

Proposal for a new spectrometer at ESS: Njord and Remora

Many of the most interesting scientific subjects are also the hardest to study with neutrons. Metal-organic frameworks, organic superconductors, quantum magnets, pressure-tuned materials, are systems where the relevant signals are weak, the samples are tiny, or the experiments need extreme sample environments such as pressure cells and high-field cryomagnets. Existing instruments often run into practical limits before the science is exhausted. For some questions the samples are simply too small; for others, the signal is buried in background or the required measurement time becomes prohibitive. This is both a scientific opportunity and a challenge for the European neutron scattering community. We present Njord and Remora as a paired instrument concept for the European Spallation Source (ESS). The proposal focuses on two linked problems: important science cases are being limited by neutron flux and sample geometry, and the community also needs more beamtime. Njord addresses the first by pushing the available brightness into a tightly focused beam, while Remora uses the remaining spectral window to add a complementary spectrometer on the same beamport.

physics.ins-det

On the pseudo-doublet ground state of the non-Kramers compound SrTm2O4 and its frustrated antiferromagnetic interactions

Here we present experimental evidence of the pseudo-doublet ground state of the non-Kramers compound SrTm2O4, based on specific heat, magnetic entropy and electron paramagnetic resonance. We demonstrate that the two crystallographic Tm3+ sites give rise to distinct single-ion anisotropies, and by extension, SrTm2O4 hosts two magnetic sublattices. Inelastic neutron scattering reveals low-lying dispersing crystal-field excitations, which we modelled using an effective charge model and mean field random phase approximation. The extracted magnetic exchange interactions are both antiferromagnetic and frustrated for both chains. Interchain magnetic exchange interactions are negligible. The strength of the magnetic exchange interactions in relation to the size of crystal field gaps, together with the frustration and low dimensionality, force the system to remain paramagnetic down to the lowest experimentally reachable temperature despite the pseudo-doublet nature of its ground state.

cond-mat.str-el

Short-range magnetic correlations in quasicrystalline i-Tb-Cd

We report on elastic and inelastic neutron scattering from single-grain isotopically-enriched samples to elucidate the local magnetic correlations between Tb$^{3+}$ moments in quasicrystalline i-Tb-Cd. The inelastic neutron scattering measurements of the CEF excitations demonstrated that the Tb$^{3+}$ moments are directed primarily along the local five-fold axes of the Tsai-type cluster as was found for the TbCd6 approximant phase. Based on the inelastic measurements, we consider of a simple Ising-type model for the moment configurations on a single Tb$^{3+}$ icosahedron and enumerate the lowest energy moment configurations. We then calculate the diffuse scattering from these configurations and compare with the experimental magnetic diffuse scattering measurements to identify the most likely single cluster moment configurations and find reasonable agreement between the broad features observed in our scattering simulations. We further consider the role of higher-order (longer range) intercluster correlations for the magnetic scattering.

cond-mat.str-el

Early Release Science of the exoplanet WASP-39b with JWST NIRSpec PRISM

Transmission spectroscopy of exoplanets has revealed signatures of water vapor, aerosols, and alkali metals in a few dozen exoplanet atmospheres. However, these previous inferences with the Hubble and Spitzer Space Telescopes were hindered by the observations' relatively narrow wavelength range and spectral resolving power, which precluded the unambiguous identification of other chemical species$-$in particular the primary carbon-bearing molecules. Here we report a broad-wavelength 0.5-5.5 $μ$m atmospheric transmission spectrum of WASP-39 b, a 1200 K, roughly Saturn-mass, Jupiter-radius exoplanet, measured with JWST NIRSpec's PRISM mode as part of the JWST Transiting Exoplanet Community Early Release Science Team program. We robustly detect multiple chemical species at high significance, including Na (19$σ$), H$_2$O (33$σ$), CO$_2$ (28$σ$), and CO (7$σ$). The non-detection of CH$_4$, combined with a strong CO$_2$ feature, favours atmospheric models with a super-solar atmospheric metallicity. An unanticipated absorption feature at 4$μ$m is best explained by SO$_2$ (2.7$σ$), which could be a tracer of atmospheric photochemistry. These observations demonstrate JWST's sensitivity to a rich diversity of exoplanet compositions and chemical processes.

astro-ph.EP

Topological magnon band structure of emergent Landau levels in a skyrmion lattice

The motion of a spin excitation across topologically non-trivial magnetic order exhibits a deflection that is analogous to the effect of the Lorentz force on an electrically charged particle in an orbital magnetic field. We used polarized inelastic neutron scattering to investigate the propagation of magnons (i.e., bosonic collective spin excitations) in a lattice of skyrmion tubes in manganese silicide. For wave vectors perpendicular to the skyrmion tubes, the magnon spectra are consistent with the formation of finely spaced emergent Landau levels that are characteristic of the fictitious magnetic field used to account for the nontrivial topological winding of the skyrmion lattice. This provides evidence of a topological magnon band structure in reciprocal space, which is borne out of the nontrivial real-space topology of a magnetic order.

cond-mat.str-el

Multiple Magnetic Bilayers and Unconventional Criticality without Frustration in BaCuSi$_2$O$_6$

The dimerized quantum magnet BaCuSi$_2$O$_6$ was proposed as an example of "dimensional reduction" arising near the magnetic-field-induced quantum critical point (QCP) due to perfect geometrical frustration of its inter-bilayer interactions. We demonstrate by high-resolution neutron spectroscopy experiments that the effective intra-bilayer interactions are ferromagnetic, thereby excluding frustration. We explain the apparent dimensional reduction by establishing the presence of three magnetically inequivalent bilayers, with ratios 3:2:1, whose differing interaction parameters create an extra field-temperature scaling regime near the QCP with a non-trivial but non-universal exponent. We demonstrate by detailed quantum Monte Carlo simulations that the magnetic interaction parameters we deduce can account for all the measured properties of BaCuSi$_2$O$_6$, opening the way to a quantitative understanding of non-universal scaling in any modulated layered system.

cond-mat.str-el

Multiphase Magnetism in Yb2Ti2O7

We document the coexistence of ferro- and anti-ferromagnetism in pyrochlore $\rm Yb_2Ti_2O_7$ using three neutron scattering techniques on stoichiometric crystals: elastic neutron scattering shows a canted ferromagnetic ground state, neutron scattering shows spin wave excitations from both a ferro-and an antiferro-magnetic state, and field and temperature dependent small angle neutron scattering reveals the corresponding anisotropic magnetic domain structure. High-field $\langle 111 \rangle$ spin wave fits show that $\rm Yb_2Ti_2O_7$ is extremely close to an antiferromagnetic phase boundary. Classical Monte Carlo simulations based on the interactions inferrred from high field spin wave measurements confirm $ψ_2$ antiferromagnetism is metastable within the FM ground state.

cond-mat.str-el

Magnetic structure of Ba(TiO)Cu$_4$(PO$_4$)$_4$ probed using spherical neutron polarimetry

The antiferromagnetic compound Ba(TiO)Cu$_4$(PO$_4$)$_4$ contains square cupola of corner-sharing CuO$_4$ plaquettes, which were proposed to form effective quadrupolar order. To identify the magnetic structure, we have performed spherical neutron polarimetry measurements. Based on symmetry analysis and careful measurements we conclude that the orientation of the Cu$^{2+}$ spins form a non-collinear in-out structure with spins approximately perpendicular to the CuO$_4$ motif. Strong Dzyaloshinskii-Moriya interaction naturally lends itself to explain this phenomenon. The identification of the ground state magnetic structure should serve well for future theoretical and experimental studies into this and closely related compounds.

cond-mat.str-el

On the relation between the column density structures and the magnetic field orientation in the Vela C molecular complex

We statistically evaluate the relative orientation between gas column density structures, inferred from Herschel submillimetre observations, and the magnetic field projected on the plane of sky, inferred from polarized thermal emission of Galactic dust observed by BLASTPol at 250, 350, and 500 micron, towards the Vela C molecular complex. First, we find very good agreement between the polarization orientations in the three wavelength-bands, suggesting that, at the considered common angular resolution of 3.0 arcminutes that corresponds to a physical scale of approximately 0.61 pc, the inferred magnetic field orientation is not significantly affected by temperature or dust grain alignment effects. Second, we find that the relative orientation between gas column density structures and the magnetic field changes progressively with increasing gas column density, from mostly parallel or having no preferred orientation at low column densities to mostly perpendicular at the highest column densities. This observation is in agreement with previous studies by the Planck collaboration towards more nearby molecular clouds. Finally, we find a correspondence between the trends in relative orientation and the shape of the column density probability distribution functions. In the sub-regions of Vela C dominated by one clear filamentary structure, or "ridges", we find a sharp transition from preferentially parallel or having no preferred relative orientation at low column densities to preferentially perpendicular at highest column densities. In the sub-regions of Vela C dominated by several filamentary structures with multiple orientations, or "nests", such a transition is also present, but it is clearly less sharp than in the ridge-like sub-regions. Both of these results suggest that the magnetic field is dynamically important for the formation of density structures in this region.

astro-ph.GA

Magnetodielectric detection of magnetic quadrupole order in Ba(TiO)Cu$_4$(PO$_4$)$_4$ with Cu$_4$O$_{12}$ square cupolas

In vortex-like spin arrangements, multiple spins can combine into emergent multipole moments. Such multipole moments have broken space-inversion and time-reversal symmetries, and can therefore exhibit linear magnetoelectric (ME) activity. Three types of such multipole moments are known: toroidal, monopole, and quadrupole moments. So far, however, the ME-activity of these multipole moments has only been established experimentally for the toroidal moment. Here, we propose a magnetic square cupola cluster, in which four corner-sharing square-coordinated metal-ligand fragments form a noncoplanar buckled structure, as a promising structural unit that carries an ME-active multipole moment. We substantiate this idea by observing clear magnetodielectric signals associated with an antiferroic ME-active magnetic quadrupole order in the real material Ba(TiO)Cu$_4$(PO$_4$)$_4$. The present result serves as a useful guide for exploring and designing new ME-active materials based on vortex-like spin arrangements.

cond-mat.str-el

Spin dynamics near a putative antiferromagnetic quantum critical point in Cu substituted BaFe$_2$As$_2$ and its relation to high-temperature superconductivity

We present the results of elastic and inelastic neutron scattering measurements on non-superconducting Ba(Fe${_{0.957}}$Cu${_{0.043}}$)${_2}$As${_2}$, a composition close to a quantum critical point between AFM ordered and paramagnetic phases. By comparing these results with the spin fluctuations in the low Cu composition as well as the parent compound BaFe$_2$As$_2$ and superconducting Ba(Fe$_{1-x}$Ni$_x$)$_2$As$_2$ compounds, we demonstrate that paramagnon-like spin fluctuations are evident in the antiferromagnetically ordered state of Ba(Fe$_{0.957}$Cu$_{0.043}$)$_2$As$_2$, which is distinct from the AFM-like spin fluctuations in the superconducting compounds. Our observations suggest that Cu substitution decouples the interaction between quasiparticles and the spin fluctuations. We also show that the spin-spin correlation length, ${ξ(T)}$, increases rapidly as the temperature is lowered and find ${ω/T}$ scaling behavior, the hallmark of quantum criticality, at an antiferromagnetic quantum critical point.

cond-mat.str-el

Attitude determination for balloon-borne experiments

An attitude determination system for balloon-borne experiments is presented. The system provides pointing information in azimuth and elevation for instruments flying on stratospheric balloons over Antarctica. In-flight attitude is given by the real-time combination of readings from star cameras, a magnetometer, sun sensors, GPS, gyroscopes, tilt sensors and an elevation encoder. Post-flight attitude reconstruction is determined from star camera solutions, interpolated by the gyroscopes using an extended Kalman Filter. The multi-sensor system was employed by the Balloon-borne Large Aperture Submillimeter Telescope for Polarimetry (BLASTPol), an experiment that measures polarized thermal emission from interstellar dust clouds. A similar system was designed for the upcoming flight of SPIDER, a Cosmic Microwave Background polarization experiment. The pointing requirements for these experiments are discussed, as well as the challenges in designing attitude reconstruction systems for high altitude balloon flights. In the 2010 and 2012 BLASTPol flights from McMurdo Station, Antarctica, the system demonstrated an accuracy of <5' rms in-flight, and <5" rms post-flight.

astro-ph.IM

The Balloon-borne Large Aperture Submillimeter Telescope for Polarimetry-BLASTPol: Performance and results from the 2012 Antarctic flight

The Balloon-borne Large Aperture Submillimeter Telescope for Polarimetry (BLASTPol) is a suborbital mapping experiment, designed to study the role played by magnetic fields in the star formation process. BLASTPol observes polarized light using a total power instrument, photolithographic polarizing grids, and an achromatic half-wave plate to modulate the polarization signal. During its second flight from Antarctica in December 2012, BLASTPol made degree scale maps of linearly polarized dust emission from molecular clouds in three wavebands, centered at 250, 350, and 500 microns. The instrumental performance was an improvement over the 2010 BLASTPol flight, with decreased systematics resulting in a higher number of confirmed polarization vectors. The resultant dataset allows BLASTPol to trace magnetic fields in star-forming regions at scales ranging from cores to entire molecular cloud complexes.

astro-ph.IM

Thermal design and performance of the balloon-borne large aperture submillimeter telescope for polarimetry BLASTPol

We present the thermal model of the Balloon-borne Large-Aperture Submillimeter Telescope for Polarimetry (BLASTPol). This instrument was successfully flown in two circumpolar flights from McMurdo, Antarctica in 2010 and 2012. During these two flights, BLASTPol obtained unprecedented information about the magnetic field in molecular clouds through the measurement of the polarized thermal emission of interstellar dust grains. The thermal design of the experiment addresses the stability and control of the payload necessary for this kind of measurement. We describe the thermal modeling of the payload including the sun-shielding strategy. We present the in-flight thermal performance of the instrument and compare the predictions of the model with the temperatures registered during the flight. We describe the difficulties of modeling the thermal behavior of the balloon-borne platform and establish landmarks that can be used in the design of future balloon-borne instruments.

astro-ph.IM

BLASTbus electronics: general-purpose readout and control for balloon-borne experiments

We present the second generation BLASTbus electronics. The primary purposes of this system are detector readout, attitude control, and cryogenic housekeeping, for balloon-borne telescopes. Readout of neutron transmutation doped germanium (NTD-Ge) bolometers requires low noise and parallel acquisition of hundreds of analog signals. Controlling a telescope's attitude requires the capability to interface to a wide variety of sensors and motors, and to use them together in a fast, closed loop. To achieve these different goals, the BLASTbus system employs a flexible motherboard-daughterboard architecture. The programmable motherboard features a digital signal processor (DSP) and field-programmable gate array (FPGA), as well as slots for three daughterboards. The daughterboards provide the interface to the outside world, with versions for analog to digital conversion, and optoisolated digital input/output. With the versatility afforded by this design, the BLASTbus also finds uses in cryogenic, thermometry, and power systems. For accurate timing control to tie everything together, the system operates in a fully synchronous manner. BLASTbus electronics have been successfully deployed to the South Pole, and flown on stratospheric balloons.

astro-ph.IM

Lattice distortion and stripe-like antiferromagnetic order in Ca10(Pt3As8)(Fe2As2)5

Ca10(Pt3As8)(Fe2As2)5 is the parent compound for a class of Fe-based high-temperature superconductors where superconductivity with transition temperatures up to 30 K can be introduced by partial element substitution. We present a combined high-resolution high-energy x-ray diffraction and elastic neutron scattering study on a Ca10(Pt3As8)(Fe2As2)5 single crystal. This study reveals the microscopic nature of two distinct and continuous phase transitions to be very similar to other Fe-based high-temperature superconductors: an orthorhombic distortion of the high-temperature tetragonal Fe-As lattice below T_S = 110(2) K followed by stripe-like antiferromagnetic ordering of the Fe moments below T_N = 96(2) K. These findings demonstrate that major features of the Fe-based high-temperature superconductors are very robust against variations in chemical constitution as well as structural imperfection of the layers separating the Fe-As layers from each other and confirms that the Fe-As layers primarily determine the physics in this class of material.

cond-mat.supr-con

Comparison of Prestellar Core Elongations and Large-Scale Molecular Cloud Structures in the Lupus I Region

Turbulence and magnetic fields are expected to be important for regulating molecular cloud formation and evolution. However, their effects on subparsec to 100 parsec scales, leading to the formation of starless cores, is not well understood. We investigate the prestellar core structure morphologies obtained from analysis of the Herschel-SPIRE 350 $μ$m maps of the Lupus I cloud. This distribution is first compared on a statistical basis to the large scale shape of the main filament. We find the distribution of the elongation position angle of the cores to be consistent with a random distribution, which means no specific orientation of the morphology of the cores is observed with respect to a large-scale filament shape model for Lupus I, or relative to a large-scale bent filament model. This distribution is also compared to the mean orientation of the large-scale magnetic fields probed at 350 $μ$m with the Balloon-borne Large Aperture Telescope for Polarimetry (BLASTPol) during its 2010 campaign. Here again we do not find any correlation between the core morphology distribution and the average orientation of the magnetic fields on parsec scales. Our main conclusion is that the local filament dynamics - including secondary filaments that often run orthogonally to the primary filament - and possibly small-scale variations in the local magnetic field direction, could be the dominant factors for explaining the final orientation of each core.

astro-ph.GA

Crossover from spin-waves to diffusive spin excitations in underdoped Ba(Fe$_{1-x}$Co$_{x}$)$_{2}$As$_{2}$

Using inelastic neutron scattering, we show that the onset of superconductivity in underdoped Ba(Fe$_{1-x}$Co$_{x}$)$_{2}$As$_{2}$ coincides with a crossover from well-defined spin waves to overdamped and diffusive spin excitations. This crossover occurs despite the presence of long-range stripe antiferromagnetic order for samples in a compositional range from x=0.04-0.055, and is a consequence of the shrinking spin-density wave gap and a corresponding increase in the particle-hole (Landau) damping. The latter effect is captured by a simple itinerant model relating Co doping to changes in the hot spots of the Fermi surface. We argue that the overdamped spin fluctuations provide a pairing mechanism for superconductivity in these materials.

cond-mat.supr-con