arXiv subjects

G. S. Uhrig

Publications and source records attributed to G. S. Uhrig.

At least 55 records · Page 3Linked to original sources

arXiv2006

One- and Two-Triplon Spectra of a Cuprate Ladder

We have performed inelastic neutron scattering on the near ideal spin-ladder compound La4Sr10Cu24O41, which will serve as a model system for the investigation of doped ladders. A key feature in the analysis was the separation of one-triplon and two-triplon scattering contributions due to an antiphase rung modulation. This enabled extraction of the one-triplon dispersion which has a spin gap of 26.4+/-0.3 meV, and for the first time two-triplon scattering is clearly observed. The exchange constants are determined by fitting the data to be Jleg=186 meV and Jrung=124 meV along the leg and the rung respectively. In addition to the surprisingly large difference between Jleg and Jrung a substantial ring exchange of Jcyc=31 meV was confirmed.

cond-mat.str-el↗

arXiv2006

Neutron scattering from a coordination polymer quantum paramagnet

Inelastic neutron scattering measurements are reported for a powder sample of the spin-1/2 quantum paramagnet $\rm Cu(Quinoxaline)Br_2$. Magnetic neutron scattering is identified above an energy gap of 1.9 meV. Analysis of the sharp spectral maximum at the onset indicates that the material is magnetically quasi-one-dimensional. Consideration of the wave vector dependence of the scattering and polymeric structure further identifies the material as a two-legged spin-1/2 ladder. Detailed comparison of the data to various models of magnetism in this material based on the single mode approximation and the continuous unitary transformation are presented. The latter theory provides an excellent account of the data with leg exchange $J_{\parallel}=2.0$ meV and rung exchange $J_{\perp}=3.3$ meV.

cond-mat.str-el↗

arXiv2005

Thermodynamics of Adiabatically Loaded Cold Bosons in the Mott Insulating Phase of One-Dimensional Optical Lattices

In this work we give a consistent picture of the thermodynamic properties of bosons in the Mott insulating phase when loaded adiabatically into one-dimensional optical lattices. We find a crucial dependence of the temperature in the optical lattice on the doping level of the Mott insulator. In the undoped case, the temperature is of the order of the large onsite Hubbard interaction. In contrast, at a finite doping level the temperature jumps almost immediately to the order of the small hopping parameter. These two situations are investigated on the one hand by considering limiting cases like the atomic limit and the case of free fermions. On the other hand, they are examined using a quasi-particle conserving continuous unitary transformation extended by an approximate thermodynamics for hardcore particles.

cond-mat.stat-mech↗

arXiv2005

Temperature in One-Dimensional Bosonic Mott insulators

The Mott insulating phase of a one-dimensional bosonic gas trapped in optical lattices is described by a Bose-Hubbard model. A continuous unitary transformation is used to map this model onto an effective model conserving the number of elementary excitations. We obtain quantitative results for the kinetics and for the spectral weights of the low-energy excitations for a broad range of parameters in the insulating phase. By these results, recent Bragg spectroscopy experiments are explained. Evidence for a significant temperature of the order of the microscopic energy scales is found.

cond-mat.stat-mech↗

arXiv2005

Zero-field incommensurate spin-Peierls phase with interchain frustration in TiOCl

We report on the magnetic, thermodynamic and optical properties of the quasi-one-dimensional quantum antiferromagnets TiOCl and TiOBr, which have been discussed as spin-Peierls compounds. The observed deviations from canonical spin-Peierls behavior, e.g. the existence of two distinct phase transitions, have been attributed previously to strong orbital fluctuations. This can be ruled out by our optical data of the orbital excitations. We show that the frustration of the interchain interactions in the bilayer structure gives rise to incommensurate order with a subsequent lock-in transition to a commensurate dimerized state. In this way, a single driving force, the spin-Peierls mechanism, induces two separate transitions.

cond-mat.str-el↗

arXiv2005

Magnetic Excitations in Bilayer High-Temperature Superconductors with Stripe Correlations

The universal behaviour of the magnetic excitations in high-temperature superconductors is described in a model with static stripes retaining only the localized spin degrees of freedom. The stripes are represented by a model of coupled two-leg spin ladders. We start from the results obtained previously by continuous unitary transformations for an isolated spin ladder. A quantitative description of neutron scattering data is reached, using a model for a single cuprate layer with well established values of the exchange coupling constants. The neutron resonance peak is explained in terms of a saddle point in the dispersion of the magnetic excitations. Here we make predictions for bilayer systems with in-phase or out-of-phase stripe correlations. The results may serve as a guide for future experimental analyses.

cond-mat.supr-con↗

arXiv2004

Magnetic excitations in the stripe phase of high-T_c superconductors

The magnetic excitations in the stripe phase of high-T_c superconductors are investigated in a model of spin ladders which are effectively coupled via charged stripes. Starting from the effective single-triplon model for the isolated spin ladder, the quasi-one-dimensional spin system can be described straightforwardly. Very good agreement is obtained with recent neutron scattering data on La_(15/8)Ba_(1/8)CuO_4 (no spin gap) and YBa_2Cu_3O_(6.6) (gapped). The signature of quasi-one-dimensional spin physics in a single-domain stripe phase is predicted.

cond-mat.supr-con↗

arXiv2004

Unifying Magnons and Triplons in Stripe-Ordered Cuprate Superconductors

Based on a two-dimensional model of coupled two-leg spin ladders, we derive a unified picture of recent neutron scattering data of stripe-ordered La_(15/8)Ba_(1/8)CuO_4, namely of the low-energy magnons around the superstructure satellites and of the triplon excitations at higher energies. The resonance peak at the antiferromagnetic wave vector Q_AF in the stripe-ordered phase corresponds to a saddle point in the dispersion of the magnetic excitations. Quantitative agreement with the neutron data is obtained for J= 130-160 meV and J_cyc/J = 0.2-0.25.

cond-mat.supr-con↗

arXiv2003

Charge order induced sharp Raman peak in Sr_14Cu_24O_41

In the two-leg S=1/2 ladders of Sr_14Cu_24O_41 a modulation of the exchange coupling arises from the charge order within the other structural element, the CuO_2 chains. In general, breaking translational invariance by modulation causes gaps within the dispersion of elementary excitations. We show that the gap induced by the charge order can drastically change the magnetic Raman spectrum leading to the sharp peak observed in Sr_14Cu_24O_41. This sharp Raman line gives insight in the charge-order periodicity and hence in the distribution of carriers. The much broader spectrum of La_6Ca_8Cu_24O$_41 reflects the response of an undoped ladder in the absence of charge order.

cond-mat.str-el↗

arXiv2003

Evidence for a large magnetic heat current in insulating cuprates

The in-plane thermal conductivity $k$ of the two-dimensional antiferromagnetic monolayer cuprate Sr$_2$CuO$_2$Cl$_2$ is studied. Analysis of the unusual temperature dependence of $k$ reveals that at low temperatures the heat is carried by phonons, whereas at high temperatures magnetic excitations contribute significantly. Comparison with other insulating layered cuprates suggests that a large magnetic contribution to the thermal conductivity is an intrinsic property of these materials.

cond-mat.str-el↗

arXiv2002

Rung-singlet phase of the S=1/2 two-leg spin-ladder with four-spin cyclic exchange

Using continuous unitary transformations (CUT) we calculate the one-triplet gap for the antiferromagnetic S=1/2 two-leg spin ladder with additional four-spin exchange interactions in a high order series expansion about the limit of isolated rungs. By applying a novel extrapolation technique we calculate the transition line between the rung-singlet phase and a spontaneously dimerized phase with dimers on the legs. Using this efficient extrapolation technique we are able to analyze the crossover from strong rung coupling to weakly coupled chains.

cond-mat.str-el↗

arXiv2002

Novel Extrapolation for Strong Coupling Expansions

We present a novel extrapolation scheme for high order series expansions. The idea is to express the series, obtained in orders of an external variable, in terms of an internal parameter of the system. Here we apply this method to the 1-triplet dispersion in an antiferromagnetic $S=1/2$ Heisenberg ladder. By the use of the internal parameter the accuracy of the truncated series is enhanced tremendously.

cond-mat.str-el↗

arXiv2001

Strong damping of phononic heat current by magnetic excitations in SrCu_2(BO_3)_2

Measurements of the thermal conductivity as a function of temperature and magnetic field in the 2D dimer spin system SrCu$_2$(BO$_3$)$_2$ are presented. In zero magnetic field the thermal conductivity along and perpendicular to the magnetic planes shows a pronounced double-peak structure as a function of temperature. The low-temperature maximum is drastically suppressed with increasing magnetic field. Our quantitative analysis reveals that the heat current is due to phonons and that the double-peak structure arises from pronounced resonant scattering of phonons by magnetic excitations.

cond-mat.str-el↗

arXiv2001

Fractional and Integer Excitations in Quantum Antiferromagnetic Spin 1/2 Ladders

Spectral densities are computed in unprecedented detail for quantum antiferromagnetic spin 1/2 two-leg ladders. These results were obtained due to a major methodical advance achieved by optimally chosen unitary transformations. The approach is based on dressed integer excitations. Considerable weight is found at high energies in the two-particle sector. Precursors of fractional spinon physics occur implying that there is no necessity to resort to fractional excitations in order to describe features at higher energies.

cond-mat.str-el↗

arXiv2001

Magnetic excitations in two-leg spin 1/2 ladders: experiment and theory

Magnetic excitations in two-leg S=1/2 ladders are studied both experimentally and theoretically. Experimentally, we report on the reflectivity, the transmission and the optical conductivity sigma(omega) of undoped La_x Ca_14-x Cu_24 O_41 for x=4, 5, and 5.2. Using two different theoretical approaches (Jordan-Wigner fermions and perturbation theory), we calculate the dispersion of the elementary triplets, the optical conductivity and the momentum-resolved spectral density of two-triplet excitations for 0.2 <= J_parallel/J_perpendicular <= 1.2. We discuss phonon-assisted two-triplet absorption, the existence of two-triplet bound states, the two-triplet continuum, and the size of the exchange parameters.

cond-mat.str-el↗

arXiv2001

Heat transport in SrCu_2(BO_3)_2 and CuGeO_3

In the low dimensional spin systems $SrCu_2(BO_3)_2$ and $CuGeO_3$ the thermal conductivities along different crystal directions show pronounced double-peak structures and strongly depend on magnetic fields. For $SrCu_2(BO_3)_2$ the experimental data can be described by a purely phononic heat current and resonant scattering of phonons by magnetic excitations. A similar effect seems to be important in $CuGeO_3$, too but, in addition, a magnetic contribution to the heat transport may be present.

cond-mat.str-el↗

arXiv2001

Optical spectroscopy of (La,Ca)14Cu24O41 spin ladders: comparison of experiment and theory

Transmission and reflectivity of La_x Ca_14-x Cu_24 O_41 two-leg spin-1/2 ladders were measured in the mid-infrared regime between 500 and 12000 1/cm. This allows us to determine the optical conductivity sigma_1 directly and with high sensitivity. Here we show data for x=4 and 5 with the electrical field polarized parallel to the rungs (E||a) and to the legs (E||c). Three characteristic peaks are identified as magnetic excitations by comparison with two different theoretical calculations.

cond-mat.str-el↗

arXiv2001

Observation of two-magnon bound states in the two-leg ladders of (Ca,La)14Cu24O41

Phonon-assisted 2-magnon absorption is studied at T=4 K in the spin-1/2 two-leg ladders of Ca_14-x La_x Cu_24 O_41 (x=5 and 4) for polarization of the electrical field parallel to the legs and the rungs, respectively. Two peaks at about 2140 and 2800 1/cm reflect van-Hove singularities in the density of states of the strongly dispersing 2-magnon singlet bound state, and a broad peak at about 4000 1/cm is identified with the 2-magnon continuum. Two different theoretical approaches (Jordan-Wigner fermions and perturbation theory) describe the data very well for J_parallel = 1050 - 1100 1/cm and J_parallel / J_perp = 1 - 1.1. A striking similarity of the high-energy continuum absorption of the ladders and of the undoped high T_c cuprates is observed.

cond-mat.str-el↗