arXiv subjects

G. Sangiovanni

Publications and source records attributed to G. Sangiovanni.

71 records · Page 4Linked to original sources

arXiv2010

High-temperature optical spectral weight and Fermi liquid renormalization in Bi-based cuprates

The optical conductivity and the spectral weight W(T) of two superconducting cuprates at optimum doping, Bi2Sr2-xLaxCuO6 and Bi2Sr2CaCu2O8, have been first measured up to 500 K. Above 300 K, W(T) deviates from the usual T2 behavior in both compounds, even though the zero-frequency extrapolation of the optical conductivity remains larger than the Ioffe-Regel limit. The deviation is surprisingly well described by the T4 term of the Sommerfeld expansion, but its coefficients are enhanced by strong correlation. This renormalization is due to strong correlation, as shown by the good agreement with dynamical mean field calculations.

cond-mat.supr-con↗

arXiv2010

Dichotomy between large local and small ordered magnetic moment in Iron-based superconductors

We study a four band model for iron-based superconductors within local density approximation + dynamical mean field theory (LDA+DMFT). This successfully reproduces the results of models which take As p degrees of freedom explicitly into account and has several physical advantages over the standard five d-band model. Our findings reveal that the new superconductors are more strongly correlated than their single-particle properties suggest. Two-particle correlation functions unveil the dichotomy between local and ordered magnetic moments in these systems, calling for further experiments to better resolve the short time scale spin dynamics.

cond-mat.supr-con↗

arXiv2010

Analytical continuation of imaginary axis data using maximum entropy

We study the maximum entropy (MaxEnt) approach for analytical continuation of spectral data from imaginary times to real frequencies. The total error is divided in a statistical error, due to the noise in the input data, and a systematic error, due to deviations of the default function, used in the MaxEnt approach, from the exact spectrum. We find that the MaxEnt approach in its classical formulation can lead to a nonoptimal balance between the two types of errors, leading to an unnecessary large statistical error. The statistical error can be reduced by splitting up the data in several batches, performing a MaxEnt calculation for each batch and averaging. This can outweigh an increase in the systematic error resulting from this approach. The output from the MaxEnt result can be used as a default function for a new MaxEnt calculation. Such iterations often lead to worse results due to an increase in the statistical error. By splitting up the data in batches, the statistical error is reduced and and the increase resulting from iterations can be outweighed by a decrease in the systematic error. Finally we consider a linearized version to obtain a better understanding of the method.

physics.data-an↗

arXiv2010

Inequivalent routes across the Mott transition in V2O3 explored by X-ray absorption

The changes in the electronic structure of V2O3 across the metal-insulator transition induced by temperature, doping and pressure are identified using high resolution x-ray absorption spectroscopy at the V pre K-edge. Contrary to what has been taken for granted so far, the metallic phase reached under pressure is shown to differ from the one obtained by changing doping or temperature. Using a novel computational scheme, we relate this effect to the role and occupancy of the a1g orbitals. This finding unveils the inequivalence of different routes across the Mott transition in V2O3

cond-mat.str-el↗

arXiv2009

Pressure and alloying effects on the metal to insulator transition in NiS{2-x}Se{x} studied by infrared spectroscopy

The metal to insulator transition in the charge transfer NiS{2-x}Se{x} compound has been investigated through infrared reflectivity. Measurements performed by applying pressure to pure NiS2 (lattice contraction) and by Se-alloying (lattice expansion) reveal that in both cases an anomalous metallic state is obtained. We find that optical results are not compatible with the linear Se-alloying vs Pressure scaling relation previously established through transport, thus pointing out the substantially different microscopic origin of the two transitions.

cond-mat.str-el↗

arXiv2008

Photoemission kinks and phonons in cuprates

One of the possible mechanisms of high Tc superconductivity is Cooper pairing with the help of bosons, which change the slope of the electronic dispersion as observed by photoemission. Giustino et al. calculated that in the high temperature superconductor La1.85Sr0.15CuO4 crystal lattice vibrations (phonons) should have a negligible effect on photoemission spectra and concluded that phonons do not play an important role. We show that the calculations employed by Giustino et al. fail to reproduce huge influence of electron-phonon coupling on important phonons observed in experiments. Thus one would expect these calculations to similarly fail in explaining the role of electron-phonon coupling for the electronic dispersion.

cond-mat.supr-con↗

arXiv2008

Quasiparticle evolution and pseudogap formation in V2O3: An infrared spectroscopy study

The infrared conductivity of V2O3 is measured in the whole phase diagram. Quasiparticles appear above the Neel temperature TN and eventually disappear further enhancing the temperature, leading to a pseudogap in the optical spectrum above 425 K. Our calculations demonstrate that this loss of coherence can be explained only if the temperature dependence of lattice parameters is considered. V2O3 is therefore effectively driven from the metallic to the insulating side of the Mott transition as the temperature is increased.

cond-mat.str-el↗

arXiv2006

Sum rules and vertex corrections for electron-phonon interactions

We derive sum rules for the phonon self-energy and the electron-phonon contribution to the electron self-energy of the Holstein-Hubbard model in the limit of large Coulomb interaction U. Their relevance for finite U is investigated using exact diagonalization and dynamical mean-field theory. Based on these sum rules, we study the importance of vertex corrections to the electron-phonon interactionin a diagrammatic approach. We show that they are crucial for a sum rule for the electron self-energy in the undoped system while a sum rule related to the phonon self-energy of doped systems is satisfied even if vertex corrections are neglected. We provide explicit results for the vertex function of a two-site model.

cond-mat.str-el↗

arXiv2006

Static vs. dynamical mean field theory of Mott antiferromagnets

Studying the antiferromagnetic phase of the Hubbard model by dynamical mean field theory, we observe striking differences with static (Hartree-Fock) mean field: The Slater band is strongly renormalized and spectral weight is transferred to spin-polaron side bands. Already for intermediate values of the interaction $U$ the overall bandwidth is larger than in Hartree-Fock, and the gap is considerably smaller. Such differences survive any renormalization of $U$. Our photoemission experiments for Cr-doped V$_2$O$_3$ show spectra qualitatively well described by dynamical mean field theory.

cond-mat.str-el↗

arXiv2006

Electron-phonon interaction and antiferromagnetic correlations

We study effects of the Coulomb repulsion on the electron-phonon interaction (EPI) in a model of cuprates at zero and finite doping. We find that antiferromagnetic correlations strongly enhance EPI effects on the electron Green's function with respect to the paramagnetic correlated system, but the net effect of the Coulomb interaction is a moderate suppression of the EPI. Doping leads to additional suppression, due to reduced antiferromagnetic correlations. In contrast, the Coulomb interaction strongly suppresses EPI effects on phonons, but the suppression weakens with doping.

cond-mat.str-el↗

arXiv2005

Polarons and Bipolarons in Holstein and Holstein $t-J$ models by Dynamical Mean Field Theory

The results of a comparative study of electronic spectral properties as well as phonon Probability Distribution Function (PDF) are reported. The study is done using Dynamical Mean Field Theory for the half-filled spinless and spinful Holstein model and for a single hole in Holstein t-J model. Qualitative changes in phonon PDF signals a polaronic crossover while an electronic Metal Insulator Transition (MIT) due to pairing into a bipolaronic state can be seen from a gap in the electronic DOS or by the vanishing of the quasi particle spectral weight. MIT can be observed only at sufficiently high density provided the Coulomb repulsion is neglected. In the limit of low density the carrier show a polaronic behavior trough the development of a definite polarization shifting the average value of the phonon PDF. At large densities occupied and empty sites result an a bimodal the phonon PDF. At the polaron crossover fluctuation of phonon coordinates tends to be larger than those at any other coupling. In this regime Born-Oppenheimer approximation is shown to fail also when phonon frequency is much less then electron bandwidth. For a single hole in the t-J model a further source of localization is due to magnetic superexchange energy which tends to localize the spin-defect spreading due to the presence of the hole.

cond-mat.str-el↗

arXiv2005

Pairing and polarization in systems with retarded interactions

In a system where a boson (e.g, a phonon) of finite frequency $ω_0$ is coupled to electrons, two phenomena occur as the coupling is increased: electron pairing and polarization of the boson field. Within a path integral formalism and a Dynamical Mean-Field approach, we introduce {\it ad hoc} distribution function which allow us to pinpoint the two effects. When $ω_0$ is smaller than the bandwidth $D$, pairing and polarization occur for fairly similar couplings for all considered temperatures. When $ω_0 > D$, the two phenomena tend to coincide only for $T \gg ω_0$, but are no longer tied for low temperatures so that a state of paired particles without finite polarization is stabilized.

cond-mat.str-el↗

arXiv2005

Phonon softening and dispersion in the 1D Holstein model of spinless fermions

We investigate the effect of electron-phonon interaction on the phononic properties in the one-dimensional half-filled Holstein model of spinless fermions. By means of determinantal Quantum Monte Carlo simulation we show that the behavior of the phonon dynamics gives a clear signal of the transition to a charge-ordered phase, and the phase diagram obtained in this way is in excellent agreement with previous DMRG results. By analyzing the phonon propagator we extract the renormalized phonon frequency, and study how it first softens as the transition is approached and then subsequently hardens in the charge-ordered phase. We then show how anharmonic features develop in the phonon propagator, and how the interaction induces a sizable dispersion of the dressed phonon in the non-adiabatic regime.

cond-mat.str-el↗

arXiv2005

Electron-phonon Interaction close to a Mott transition

The effect of Holstein electron-phonon interaction on a Hubbard model close to a Mott-Hubbard transition at half-filling is investigated by means of Dynamical Mean-Field Theory. We observe a reduction of the effective mass that we interpret in terms of a reduced effective repulsion. When the repulsion is rescaled to take into account this effect, the quasiparticle low-energy features are unaffected by the electron-phonon interaction. Phonon features are only observed within the high-energy Hubbard bands. The lack of electron-phonon fingerprints in the quasiparticle physics can be explained interpreting the quasiparticle motion in terms of rare fast processes.

cond-mat.str-el↗

arXiv2004

Phase Separation close to the density-driven Mott transition in the Hubbard-Holstein model

The density driven Mott transition is studied by means of Dynamical Mean-Field Theory in the Hubbard-Holstein model, where the Hubbard term leading to the Mott transition is supplemented by an electron-phonon (e-ph) term. We show that an intermediate e-ph coupling leads to a first-order transition at T=0, which is accompanied by phase separation between a metal and an insulator. The compressibility in the metallic phase is substantially enhanced. At quite larger values of the coupling a polaronic phase emerges coexisting with a non-polaronic metal.

cond-mat.str-el↗

arXiv2004

Doping-driven transition to a time-reversal breaking state in the phase diagram of the cuprates

Motivated by recent tunnelling and Andreev-reflection experiments, we study the conditions for a quantum transition within the superconducting phase of the cuprates,in which a bulk imaginary (time-reversal breaking) $id_{xy}$component appears in addition to the $d_{x^2 - y^2}$ order parameter. We examine in detail the role of some important physical features of the cuprates.In particular we show that a closed Fermi surface,a bilayer splitting, an orthorhombic distortion,and the proximity to a quantum critical point around optimal doping favor the appearance of the imaginary component. These findings could explain why the mixed $d_{x^2 - y^2}+ id_{xy}$ order parameter is observed in YBCO and LSCO, and suggest that it could appear also in Bi2212. We also predict that, in all cuprates, the mixed state should be stable only in a limited doping region all contained beneath the $d_{x^2 - y^2}$ dome. The behavior of the specific heat at the secondary transition is discussed.

cond-mat.supr-con↗

arXiv2002

Time Reversal Breaking Superconducting State in the Phase Diagram of the Cuprates

We review and extend a previous study on the symmetry of the superconducting state, stimulated by recent tunneling and Andreev reflection measurements giving robust evidences for the existence of a $d_{x^2-y^2}+id_{xy}$ order parameter in the overdoped regime of two different cuprates. Looking for a possible second-order phase transition from a standard $d_{x^2-y^2}$ to a mixed and time reversal breaking state, we confirm the results of our previous analysis on La$_{2-x}$Sr$_{x}$CuO$_{4}$. In the case of Y$_{1-y}$Ca$_y$Ba$_2$Cu$_3$O$_{7-x}$ as well, among all the allowed symmetries, the $d_{x^2-y^2}+id_{xy}$ is the most favored one and the unconventional state is likely to occur in a small dome of the phase diagram located in the optimal-overdoped region and at very low temperatures.

cond-mat.supr-con↗