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G. Saxena

Publications and source records attributed to G. Saxena.

At least 19 recordsLinked to original sources

Impact of Shape Coexistence on Nuclear Stability

Nuclear decay properties are conventionally predicted assuming nuclei decay from their ground-state configurations. However, this often neglects a fundamental structural complexity which is the phenomenon of shape coexistence, where nuclei possess multiple competing configurations at nearly degenerate energies. When both parent and daughter nuclei can exist in different energy minima, multiple decay pathways become possible. We systematically investigate how shape coexistence influences nuclear decay for approximately 1500 even-even nuclei ($8 \leq Z \leq 118$, $8 \leq N \leq 184$) using the Nilsson-Strutinsky method and relativistic mean-field calculations with NL3$^*$, DD-ME2, and DD-PC1 functionals. We identify around 400 nuclei exhibiting competing energy minima separated by less than 1 MeV. For these shape-coexisting nuclei, we calculate $\alpha$, $\beta^+$ and $\beta^-$ decay half-lives considering all possible transition pathways between the competing minima. Our results demonstrate that shape coexistence substantially impacts decay predictions, with half-lives showing variations up to nearly one logarithmic unit depending on which configurations participate in the transition. Comparison with experimental data from NUBASE2020 shows that pathways involving the second minimum sometimes reproduce measured lifetimes more closely than conventional ground-state to ground-state assumptions. Branching ratios exhibit even stronger sensitivity, with certain nuclei displaying complete inversions of the dominant decay mode depending on configuration choice. These pathway-dependent variations are not due to model uncertainties but reflect inherent structural effects. The correlation between the shape dynamics and nuclear stability establishes the shape coexistence as an essential component in predictive nuclear structure and astrophysics studies.

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Impact of microscopic structural transitions on particle stability and lifetimes of hot nuclei

The impact of temperature-induced deformations and shape fluctuations on the particle stability and decay processes has been investigated across the isotopes of hot nuclear systems with $Z = 28$ to $50$, with focus on astrophysically crucial pathways at excitation energies relevant to stellar environments. We perform global finite-temperature analysis using the statistical theory of hot nuclei combined with the triaxially deformed Nilsson Hamiltonian and Strutinsky's prescription, and explore the interplay between deformation, shell quenching, separation energies, and $\beta$-decay characteristics at finite temperatures. Our results show that around critical temperatures $T_c \approx 1$--$2$ MeV, where the shell quenching effects become predominant, the nuclear deformation reduces and the shape undergoes a transition to the spherical configuration. Our computed neutron and proton separation energies, which usually decrease with increasing temperature, implying the reduced binding in hot nuclei, occasionally show an enhancement in some nuclei at reduced deformation around $T_c$ that shifts the last unbound nucleon to the bound, stabilizing the nucleus by shifting the drip-line boundaries. A few nuclei are found to show one- and two-neutron drip line expansion with temperature. Moreover, the temperature-induced changes in deformation strongly correlate with the marked variations in our calculated $Q_\beta$ values and lifetimes, underscoring their impact on weak interaction rates. These findings provide insight into the sensitivity of particle stability and weak-interaction observables to thermal effects and may serve as complementary inputs for modeling nuclear processes in hot astrophysical environments.

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Thermal Evolution of Shape Coexistence in Mo and Ru Isotopes

The temperature-driven shape dynamics of isotopic chains of Mo and Ru elements and their impact on decay modes have been investigated in a statistical theoretical framework with macroscopic-microscopic apporach. These isotopes located at the key points in r-process path are known for the rapid structural changes, shape instabilities and shape coexistence that impact the nuclear processes, decay modes and lifetimes. At high temperatures that may exist in stars or in various nuclear reaction processes, these nuclei undergo a variety of shape and deformation changes due to thermal shell quenching effects influencing the decay energies (Q value), and eventually life-time have been studied in detail. Our findings provide insight into the observed shift in the deformation, shapes and coexisting states due to the diminishing nuclear shell effects in hot nuclei, revealing that the structural changes influence the decay processes and significantly in the astrophysically relevant Mo-Ru region especially around A = 100.

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Conflation of Ensemble-Learned Nuclear Mass Models for Enhanced Precision

Ensemble learning algorithms, the gradient boosting and bagging regressors, are employed to correct the residuals of nuclear mass excess for a diverse set of six nuclear mass models. The weighted average of these corrected residuals reduces due to their partial cancellation, yielding a significant improvement in nuclear mass predictions. Our conflated model, which integrates ensemble learning and model averaging (ELMA), achieves a root mean square error of approximately 65 keV, well below the critical threshold of 100 keV, for the complete data set of Atomic Mass Evaluation (AME2020). The validity of ELMA is demonstrated through the evaluation of $Q$ values for $\alpha$ decay, showing a marked decrease in deviations from experimental data relative to predictions from individual nuclear mass models. We have also compiled a table of nuclear mass excesses and binding energies for about 6,300 nuclei, which serves as a valuable resource for various nuclear physics applications and is publicly accessible via the ELMA web interface (https://ddnp.in).

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Theoretical Investigation of {\alpha}-decay in Heavy and Superheavy Isomers

The heavy and superheavy elements of the periodic table predominately disintegrate by {\alpha}-decay, facilitating transitions mainly between ground states and occasionally involving isomeric states. This study focuses on estimating the half-lives of {\alpha}-transitions both from and to isomeric states, using a recently refined formula which shows excellent agreement with experimental data when isospin of parent nucleus as well as angular momentum taken away by the {\alpha} particle are incorporated. These findings provide valuable insights for upcoming experimental investigations of isomeric states. Additionally, the study predicts potential {\alpha}-decay in several yet-unobserved isomeric nuclei, contributing to a deeper understanding of nuclear structure in heavy and superheavy elements.

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Impact of Nuclear Deformation of Parent and Daughter Nuclei on One Proton Radioactivity Lifetimes

The influence of nuclear deformation on proton-decay half-lives has been systematically studied in microscopic theoretical frameworks for a wide range of nuclei with Z<82. Correlation between 1p-decay half-lives and the deformed nuclear shapes of both the parent and daughter nuclei has been investigated. Since the deformations of proton emitters and their residual nuclei impact the potential barrier and disintegration energy which are crucial for the accurate determination of half-lives, we incorporate the nuclear deformations of both the emitters and residues in a phenomenological manner and propose a new semi-empirical formula to estimate the 1p-decay half-lives. The robustness of this formula is demonstrated by the accurate predictions of the measured values while making it reliable for forecasting the properties of other potential proton emitters. The phenomenon of shape coexistence as observed in several proton emitters and their respective daughter nuclei, is particularly signicant in this context due to secondary minima in the potential energy surfaces of both the nuclei. Accounting for these factors signicantly affects the estimation of half-lives and branching ratios by introducing additional decay pathways and altering transition probabilities between different nuclear shapes.

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Superheavy Magic Nuclei: Ground-State Properties, Bubble Structure and {\alpha}-Decay Chains

A systematic investigation of superheavy nuclei in the isotopic chains of proton numbers Z=106, 114, 120, and 126 together with isotonic chains of neutron numbers N=162, 172, and 184 is presented in the theoretical framework of relativistic mean-field density functionals based on density-dependent meson-nucleon couplings. Ground-state properties, including binding energy, shape, deformation, density profile, and radius, are estimated to provide compelling evidence of magicity in these even-even nuclei, aligning with the concept of the 'island of stability'. The analysis reveals central depletion in the charge density, indicating a bubble-like structure, primarily attributed to the substantial repulsive Coulomb field and the influence of higher l-states. A thorough examination of potential decay modes, employing various semi-empirical formulas, is presented. The probable alpha-decay chains are evaluated, demonstrating excellent agreement with available experimental data

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Theoretical investigation of heavy cluster decay from Z=118 and 120 isotopes: A search for an empirical formula in superheavy region

Various decay modes in superheavy nuclei have been of significant interest among which cluster radioactivity has recently gained sizable attention. The {\alpha}-decay being a predominant decay mode in the superheavy region, the accurate determination of cluster decay half-lives is also crucial in this region as it has tremendous potential to be explored as one of the major decay channels. The usability of the Royer analytical formula [Nuclear Physics A 683 (2001) 182], which is based on the asymmetric fission model, has been investigated for the cluster and {\alpha} decay in superheavy region, by comparing it with several other (semi)empirical/analytical formulas. After fitting the formula on around 100 cluster-decay data and around 423 {\alpha}-decay data, the refitted Royer formula (RRF) is found to be very robust which is able to estimate the cluster decay and {\alpha}-decay half-lives with good accuracy. In fact, a comparison of the half-lives of both the decay modes using the same formula points towards a substantial chance of heavy cluster (Kr and Sr) decay from various isotopes of Z=118 and 120. Hence, the formula proposed in this study works fairly well for the estimation of cluster decay half-lives in superheavy regions where most empirical formulas fail to match with the half-lives from the various established theories.

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Indispensability of cross-shell contributions in neutron resonance spacing

Spin and parity dependent nuclear level densities (NLDs) are obtained for configuration interaction shell model using a numerically efficient spectral distribution method. The calculations are performed for $^{24}$Na, $^{25,26,27}$Mg nuclei using full $sd$-$pf$ model space that incorporates the cross-shell excitations from $sd$ to $pf$-shell. The NLDs so obtained are then employed to determine the s-wave neutron resonance spacing (D$_0$) which is one of the crucial inputs for the predictions of astrophysical reaction rates. Though the considered nuclei are not neutron-rich, the contributions from cross-shell excitations to $pf$-shell are indispensable to explain the experimental data for D$_0$ which otherwise are significantly overestimated.

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Correlation between the Shape Coexistence and Stability in Mo and Ru isotopes

In a rapidly changing shape phase region, the presence of shape coexistence and its possible impact on the decay modes and half$-$lives, has been explored in astrophysically interesting Mo and Ru isotopes, in an extensive study within the microscopic theoretical framework using Nilsson Strutinsky Method and Relativistic Mean Field Model. The isotopic chains of Mo and Ru exhibit rapid shape phase transitions, triaxial $\gamma$ softness, shape instability along with many coexisting states mostly with oblate and triaxial shapes. Proton and neutron separation energies have been calculated and compared with the available data. Results obtained from both the formalisms are in good agreement with each other as well as the available experimental data. Our computed $\beta-$decay half$-$lives and separation energy for nuclei exhibiting shape coexistence were examined for the decay mode from second minima state of the parent nuclei to the ground or excited state of the daughter nuclei. The second minima state of the coexisting shapes in Mo and Ru isotopes, were seen to impact the structural properties, $\beta-$decay half$-$lives, separation energy and hence the stability of the nuclei.

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A global study of $\alpha$-clusters decay in heavy and superheavy nuclei with half-life and preformation factor

A detailed study of $\alpha$-clusters decay is exhibited by incorporating crucial microscopic nuclear structure information into the estimations of half-life and preformation factor. For the first time, using the k-cross validation approach, two semi-empirical formulas for (i) $\alpha$-decay half-life and (ii) $\alpha$-particle preformation factor, are picked out and subsequently modified by including shell, odd-nucleon blocking, and asymmetry effects along with the usual dependence on $\alpha$-decay energy ($Q_{\alpha}$) and angular momentum of $\alpha$-particle. Both the formulas are fitted for the two different regions separated by neutron number N$=$126, as from the experimental systematics the role of N$=$126 shell closure is found decisive in determining the trends of $Q_{\alpha}$, $\alpha$-decay half-life, and $\alpha$-particle preformation factor. It is found that the inclusion of the above-mentioned degrees of freedom significantly reduces the errors in the estimations when compared with several other similar modified/refitted semi-empirical relations indicating the robustness of the proposed formulas. The predictions of $\alpha$-decay half-life throughout the periodic chart have been made including the unknown territory, future probable decay chain of self-conjugate nucleus $^{112}$Ba terminated on $^{100}$Sn, decay chain of $^{208}$Pa through new isotope $^{204}$Ac as well as decay chains of awaiting superheavy nuclei $^{298}$Og and $^{299}$120.

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Cluster radioactivity from trans-tin to superheavy region using an improved empirical formula

A simple relation $(aZ_{c} + b)(Z_{d}/Q)^{1/2} + (cZ_{c} + d)$ of estimation of the half-life of cluster emission is further improved for cluster and $\alpha$-decays, separately, by incorporating isospin of parent nucleus as well as angular momentum taken away by the emitted particle. This improved version is not only found robust in producing experimental half-lives belonging to the trans-tin and trans-lead regions but also elucidates cluster emission in superheavy nuclei over the usual $\alpha$-decay. Considering daughter nuclei around the doubly magic $^{100}$Sn and $^{208}$Pb nuclei for trans-tin and trans-lead (including superheavy) parents, respectively, a systematic and extensive study of 56$\leq$Z$\leq$120 isotopes is performed for the light and heavy cluster emissions. A fair competition among cluster emission, $\alpha$-decay, spontaneous fission, and $\beta$-decay is observed in this broad range resulting in a substantial probability of C to Sr clusters from several nuclei, which demonstrates the adequacy of shell effects. The present article proposes a single, improved, latest-fitted, and effective formula of cluster radioactivity that can be used to estimate precise half-lives for a wide range of the periodic chart from trans-tin to superheavy nuclei.

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Decay properties of undetected superheavy nuclei with Z>110

A comprehensive study of favoured and unfavoured $\alpha$-decay, cluster decay, weak-decay along with spontaneous fission in undetected superheavy nuclei within the range for proton number 111$\leq$Z$\leq$118 and neutron number 161$\leq$N$\leq$192 is performed. Half-lives for various mentioned decays are estimated with good accuracy on the basis of NUBASE2020 and are found in excellent match with the known half-lives. $\alpha$-decay mode is found most probable in this wide range and correspondingly potential $\alpha$-decay chains are reckoned. Peculiarly, the chances of cluster emission, as well as weak-decay, are also anticipated in this region of the periodic chart which open new pathways of detection of superheavy nuclei.

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Neutron Skin Thickness Dependence of Astrophysical $S$-factor

Background: The density dependence of nuclear symmetry energy is crucial in determining several properties of finite nuclei to the neutron stars with mass $\sim$ 1.4 $M_\odot$. The values of neutron skin thickness, isovector giant dipole resonances energies and various nuclear reaction cross-sections in asymmetric nuclei have been utilized to determine the slope of symmetry energy ($L_0$) at the saturation density. Recent PREX-II and CREX measurements of neutron skin thickness in $^{208}$Pb and $^{48}$Ca nuclei yield very different values of $L_0$ which overlap marginally within 90$\%$ confidence interval. Purpose: Our objective is to demonstrate the role of symmetry energy on the sub-barrier fusion cross-section and the astrophysical $S$-factor for asymmetric nuclei. Method: The nucleus nucleus potentials are generated using the double folding model (DFM) for three different nucleon-nucleon interactions. These DFM potentials are used for the calculation of the sub-barrier fusion cross-section and the astrophysical $S$-factor. The nucleon densities required for DFM potentials are generated from different families of non-relativistic and relativistic mean-field models which correspond to a wide range of neutron skin thickness or $L_0$. Results: We have calculated the sub-barrier fusion cross-section for several asymmetric nuclei involving O, Ca, Ni, and Sn isotopes. The results are presented for the barrier parameters, cross-section, and astrophysical $S$-factor for $^{54}$Ca+$^{54}$Ca and $^{124}$Sn+$^{124}$Sn as a function of neutron skin thickness. Conclusions: The cross-section for the neutron-rich nuclei show a strong dependence on the behavior of symmetry energy or the neutron skin thickness. The increase in skin thickness lowers the height of the barrier as well as its width which enhances the values of the $S$-factor by more than an order of magnitude.

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Cluster radioactivity in trans-lead region: A systematic study with modified empirical formulas

The possibility of cluster emission from trans-lead (86$\leq$Z$\leq$96) region of periodic chart has been explored comprehensively by employing few empirical formulas which are modified by adding angular momentum ($l$) or isospin-dependent ($I=(N-Z)/A$) or both terms for the calculation of cluster decay half-lives. These modified versions of the formulas are found with lesser ${\chi}^2$ per degree of freedom and root mean-square error, in addition to the smaller values of some other statistical parameters, while compared to their corresponding old versions on available 61 experimental data of cluster radioactivity. By applying the modified version of the formula given by Balasubramaniam \textit{et al.} [PRC 70 (2004) 017301], the most accurate formula among these, half-lives of several clusters i.e. isotopes of Be, B, C, N, O, F, Ne, Na, Mg, and Si are predicted systematically for the several isotopes in the trans-lead region. The contest of cluster emission with $\alpha$-decay has been investigated in form of branching ratio which brings several potential cluster emissions into the probable decay modes of these nuclei. The accurate prediction of half-lives of such clusters is expected to be crucial for the future experimental observations where $\alpha$-decay is observed dominantly.

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Deformation dependence of 2p-radioactivity half-lives: Probe with a new formula across the mass region with Z<82

Effect of deformation on half-life of two-proton (2p) radioactivity is investigated across the periodic chart for nuclei with Z$<$82. 2p-decay half-lives are estimated by employing our newly proposed semi-empirical formula wherein the nuclear deformation has been incorporated in a phenomenological way. Robustness of the formula is demonstrated as it estimates the measured values quite accurately and, hence, reliably applied to predict the other possible 2p-emitters. For many proton rich nuclei for which experimental data on the decay energies are not available, we have used the theoretical values obtained from our calculations using the relativistic mean-field (RMF) approach. The uncertainties in the theoretical decay energy values are minimised by machine learning (ML) technique. Correlation of 2p-radioactivity with 2p-halo and deformation is probed. Our calculations show the phenomenon of shape coexistence in several 2p-emitters, wherein the prolate shape is found to be more predominant for the ground state.

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Astrophysical reaction rates with realistic nuclear level densities

Realistic nuclear level densities (NLDs) obtained within the spectral distribution method (SDM) are employed to study nuclear processes of astrophysical interest. The merit of SDM lies in the fact that the NLDs corresponding to many body shell model Hamiltonian consisting of residual interaction can be obtained for the full configurational space without recourse to the exact diagnolization of huge matrices. We calculate NLDs and s-wave neutron resonance spacings which agree reasonably well with the available experimental data. By employing these NLDs, we compute reaction cross-sections and astrophysical reaction rates for radiative neutron capture in few Fe-group nuclei, and compare them with experimental data as well as with those obtained with NLDs from phenomenological and microscopic mean-field models. The results obtained for the NLDs from SDM are able to explain the experimental data quite well. These results are of particular importance since the configuration mixing through the residual interaction naturally accounts for the collective excitations. In the mean-field models, the collective effects are included through the vibrational and rotational enhancement factors and their NLDs are further normalized at low energies with neutron resonance data.

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A comprehensive study of decay modes associated with Pb isotopes

Decay modes in Pb isotopes within the range 176$\leq$A$\leq$266 are investigated by the calculation of half-lives using several empirical formulas. These formulas along with various theoretical treatments are first tested to reproduce experimental half-lives and known decay modes of Pb isotopes, which are in consequence applied to estimate half-lives and decay modes of unknown Pb isotopes. A comparison between $α$-decay and weak-decay from the stable to drip-line isotopes is canvassed which leads to the excellent match with experimental data and applicability of applied empirical formulas. In addition, the full chain of Pb isotopes is probed as potential daughter candidates of cluster emission from superheavy nuclei which ensued the predominant role of $^{208}$Pb and nearby isotopes in probable cluster emission.

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