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G. Schütz

Publications and source records attributed to G. Schütz.

9 recordsLinked to original sources

Nanoscale imaging of spin textures with locally varying altermagnetic response in $α$-Fe$_2$O$_3$

Altermagnetism is a recently identified magnetic state in which time-reversal symmetry is broken despite a collinear compensated spin structure. The response of altermagnets is determined not only by their $d$-, $g$-, or $i$-wave spin order, but also the orientation of their Néel vector $\mathbf{L}$. Therefore, accessing a response that fundamentally depends on the orientation of $\mathbf{L}$, such as the anomalous Hall effect, remains experimentally challenging in particular at the nanoscale. Here, we harness nano-spectroscopic X-ray magnetic circular dichroism (XMCD) to investigate nanoscale modulated altermagnetic responses in $α$-Fe$_2$O$_3$ (Hematite). By performing spectroscopy across the temperature-induced $\mathbf{L}$-reorientation Morin transition, we observe the on-and-off switching of XMCD, in agreement with our theoretical calculations. Although the bulk XMCD vanishes below the Morin temperature, we confirm the reorientation of $\mathbf{L}$ by harnessing polarization-independent X-ray absorption spectroscopy. Moreover, we observe a finite XMCD signal in nanoscale domain walls with locally modulated Néel vectors, while the surrounding domains exhibit no XMCD. At room temperature, we instead identify altermagnetic meron spin textures that exhibit XMCD in their planar regions but no XMCD in their nanoscopic cores. Our results establish a pathway to harness complex spin textures with nanoscale functionalities in a broader class of altermagnets with various $\mathbf{L}$-orientations and using light, earth-abundant elements.

cond-mat.mtrl-sci↗

Real-space imaging of confined magnetic skyrmion tubes

Magnetic skyrmions are topologically nontrivial particles with a potential application as information elements in future spintronic device architectures. While they are commonly portrayed as two dimensional objects, in reality magnetic skyrmions are thought to exist as elongated, tube-like objects extending through the thickness of the sample. Study of this skyrmion tube (SkT) state is highly relevant for investigating skyrmion metastability and for implementation in recently proposed magnonic computing. However, direct experimental imaging of skyrmion tubes has yet to be reported. Here, we demonstrate the first real-space observation of skyrmion tubes in a lamella of FeGe using resonant magnetic x-ray imaging and comparative micromagnetic simulations, confirming their extended structure. The formation of these structures at the edge of the sample highlights the importance of confinement and edge effects in the stabilisation of the SkT state, opening the door to further investigations into this unexplored dimension of the skyrmion spin texture.

cond-mat.str-el↗

On the quest of low temperature nitrogen infusion relevant for superconducting Nb based radio-frequency cavities

A detailed study of the near-surface structure and composition of Nb, the material of choice for Superconducting Radio Frequency accelerator (SRF) cavities, is of great importance in order to understand the effects of different treatments applied during cavity production. By means of surface-sensitive techniques such as grazing incidence diffuse X-ray scattering, X-ray reflectivity and X-ray photoelectron spectroscopy, single-crystalline Nb(100) samples were investigated in and ex-situ during annealing in UHV as well as in nitrogen atmospheres with temperatures and pressures similar to the ones employed in real Nb cavity treatments. Annealing of Nb specimens up to 800°C in vacuum promotes partial reduction of the natural surface oxides (Nb2O5, NbO2, NbO) into NbO. Upon cooling to 120°C, no evidence of nitrogen-rich layers was detected after nitrogen exposure times of up to 48 hours. Oxygen enrichment below the Nb/oxide interface and posterior diffusion of oxygen species towards the Nb matrix, along with a partial reduction of the natural surface oxides was observed upon a stepwise annealing up to 250°C. Nitrogen introduction to the system at 250°C neither promotes N diffusion into the Nb matrix nor the formation of new surface layers. Upon further heating to 500°C in a nitrogen atmosphere, the growth of a new subsurface Nb$_x$N$_y$ layer was detected. These results shed light on the composition of the near-surface region of Nb after low-temperature nitrogen treatments, which are reported to lead to a performance enhancement of SRF cavities.

cond-mat.mtrl-sci↗

Nanoscale X-Ray Imaging of Spin Dynamics in Yttrium Iron Garnet

Time-resolved scanning transmission x-ray microscopy (TR-STXM) has been used for the direct imaging of spin wave dynamics in thin film yttrium iron garnet (YIG) with spatial resolution in the sub 100 nm range. Application of this x-ray transmission technique to single crystalline garnet films was achieved by extracting a lamella (13x5x0.185 $\mathrm{μm^3}$) of liquid phase epitaxy grown YIG thin film out of a gadolinium gallium garnet substrate. Spin waves in the sample were measured along the Damon-Eshbach and backward volume directions of propagation at gigahertz frequencies and with wavelengths in a range between 100~nm and 10~$\mathrmμ$m. The results were compared to theoretical models. Here, the widely used approximate dispersion equation for dipole-exchange spin waves proved to be insufficient for describing the observed Damon-Eshbach type modes. For achieving an accurate description, we made use of the full analytical theory taking mode-hybridization effects into account.

cond-mat.mes-hall↗

Coherent excitation of heterosymmetric spin waves with ultrashort wavelengths

In the emerging field of magnonics, spin waves are foreseen as signal carriers for future spintronic information processing and communication devices, owing to both the very low power losses and a high device miniaturisation potential predicted for short-wavelength spin waves. Yet, the efficient excitation and controlled propagation of nanoscale spin waves remains a severe challenge. Here, we report the observation of high-amplitude, ultrashort dipole-exchange spin waves (down to 80 nm wavelength at 10 GHz frequency) in a ferromagnetic single layer system, coherently excited by the driven dynamics of a spin vortex core. We used time-resolved x-ray microscopy to directly image such propagating spin waves and their excitation over a wide range of frequencies. By further analysis, we found that these waves exhibit a heterosymmetric mode profile, involving regions with anti-Larmor precession sense and purely linear magnetic oscillation. In particular, this mode profile consists of dynamic vortices with laterally alternating helicity, leading to a partial magnetic flux closure over the film thickness, which is explained by a strong and unexpected mode hybridisation. This spin-wave phenomenon observed is a general effect inherent to the dynamics of sufficiently thick ferromagnetic single layer films, independent of the specific excitation method employed.

cond-mat.mes-hall↗

Emission and Propagation of Multi-Dimensional Spin Waves with nanoscale wavelengths in Anisotropic Spin Textures

Spin waves offer intriguing novel perspectives for computing and signal processing, since their damping can be lower than the Ohmic losses in conventional CMOS circuits. For controlling the spatial extent and propagation of spin waves on the actual chip, magnetic domain walls show considerable potential as magnonic waveguides. However, low-loss guidance of spin waves with nanoscale wavelengths, in particular around angled tracks, remains to be shown. Here we experimentally demonstrate that such advanced control of propagating spin waves can be obtained using natural features of magnetic order in an interlayer exchange-coupled, anisotropic ferromagnetic bilayer. Using Scanning Transmission X-Ray Microscopy, we image generation of spin waves and their propagation across distances exceeding multiple times the wavelength, in extended planar geometries as well as along one-dimensional domain walls, which can be straight and curved. The observed range of wavelengths is between 1 μm and 150 nm, at corresponding excitation frequencies from 250 MHz to 3 GHz. Our results show routes towards practical implementation of magnonic waveguides employing domain walls in future spin wave logic and computational circuits.

cond-mat.mes-hall↗

Transmission x-ray microscopy at low temperatures - analyzing supercurrents with high spatial resolution

Scanning transmission x-ray microscopy has been used to image electric currents in superconducting films at temperatures down to 20 K. The magnetic stray field of supercurrents in a thin YBaCuO film is mapped into a soft-magnetic coating of permalloy. The so created local magnetization of the ferromagnetic film can be detected by dichroic absorption of polarized x-rays. To enable high-quality measurements in transmission geometry the whole heterostructure of ferromagnet, superconductor and single-crystalline substrate has been thinned to an overall thickness of less than 1 micron. With this novel technique local supercurrents can be analyzed in a wide range of temperatures and magnetic fields. A magnetic resolution of less than 100nm together with simultaneously obtained nanostructural data allow the correlation of local supercurrents with the micro- and nanostructure of the superconducting film.

cond-mat.supr-con↗

Chiral symmetry breaking of magnetic vortices by sample roughness

Finite-element micromagnetic simulations are employed to study the chiral symmetry breaking of magnetic vortices, caused by the surface roughness of thin-film magnetic structures. An asymmetry between vortices with different core polarizations has been experimentally observed for square-shaped platelets. E.g., the threshold fields for vortex core switching were found to differ for core up and down. This asymmetry was however not expected for these symmetrically-shaped structures, where both core polarizations should behave symmetrically. Three-dimensional finite element simulations are employed to show that a small surface roughness can break the symmetry between vortex cores pointing up and down. A relatively small sample roughness is found sufficient to reproduce the experimentally observed asymmetries. It arises from the lack of mirror-symmetry of the rough thin-film structures, which causes vortices with different handedness to exhibit asymmetric dynamics.

cond-mat.other↗

X-ray imaging of the dynamic magnetic vortex core deformation

Magnetic platelets with a vortex configuration are attracting considerable attention. The discovery that excitation with small in-plane magnetic fields or spin polarised currents can switch the polarisation of the vortex core did not only open the possibility of using such systems in magnetic memories, but also initiated the fundamental investigation of the core switching mechanism itself. Micromagnetic models predict that the switching is mediated by a vortex-antivortex pair, nucleated in a dynamically induced vortex core deformation. In the same theoretical framework, a critical core velocity is predicted, above which switching occurs. Although these models are extensively studied and generally accepted, experimental support has been lacking until now. In this work, we have used high-resolution time-resolved X-ray microscopy to study the detailed dynamics in vortex structures. We could reveal the dynamic vortex core deformation preceding the core switching. Also, the threshold velocity could be measured, giving quantitative comparison with micromagnetic models.

cond-mat.other↗