arXiv subjects

G. Timothy Noe II

Publications and source records attributed to G. Timothy Noe II.

9 recordsLinked to original sources

arXiv2026

Limited coincidence between ultrahigh-field superconductivity and line of metamagnetic endpoints in UTe$_2$

The field-dependent magnetization of UTe$_2$ was measured through the metamagnetic transition at a variety of field angles, tracking how the step in magnetization evolves with fields tilted away from the $b$ axis. For fields oriented within the $ab$ plane, jumps in both $M_a$ and $M_b$ vanish approximately 18° away from the $b$ axis. From contactless conductivity measurements, we find that the halo-like high-field superconducting region extends to the $ab$ plane, where it exists only within a very narrow ($<$1°) angular range near the termination of the metamagnetic phase boundary and extends beyond the highest measured field of 73 T. As the field orientation tilts towards the $c$ axis, the superconducting and metamagnetic phase boundaries no longer coincide and exhibit distinct trends.

cond-mat.supr-con↗

arXiv2022

Tunable Plasmonic Ultrastrong Coupling: Emulating Dicke Physics at Room Temperature

A system of N two-level atoms cooperatively interacting with a photonic field can be described as a single giant atom coupled to the field with interaction strength ~N^0.5. This enhancement, known as Dicke cooperativity in quantum optics, has recently become an indispensable element in quantum information technology based on strong light-matter coupling. Here, we extend the coupling beyond the standard light-matter interaction paradigm, emulating Dicke cooperativity in a terahertz metasurface with N meta-atoms. Cooperative enhancement manifested in the form of matter-matter coupling, through the hybridization of localized surface plasmon resonance in individual meta-atoms and surface lattice resonance due to the periodic array of the meta-atoms. By varying the lattice constant of the array, we observe a clear anticrossing behavior, a signature of strong coupling. Furthermore, through engineering of the capacitive split-gap in the meta-atoms, the coupling rate was cooperatively enhanced into the ultrastrong coupling regime by a factor of N^0.5. This room-temperature technology serves as a convenient quantum emulator of the dynamics of a qubit with a giant dipole moment coherently driven by a single bosonic field.

physics.optics↗

arXiv2022

Magnetically Tuned Continuous Transition from Weak to Strong Coupling in Terahertz Magnon Polaritons

Depending on the relative rates of coupling and dissipation, a light-matter coupled system is either in the weak- or strong-coupling regime. Here, we present a unique system where the coupling rate continuously increases with an externally applied magnetic field while the dissipation rate remains constant, allowing us to monitor a weak-to-strong coupling transition as a function of magnetic field. We observed a Rabi splitting of a terahertz magnon mode in yttrium orthoferrite above a threshold magnetic field of ~14 T. Based on a microscopic theoretical model, we show that with increasing magnetic field the magnons transition into magnon polaritons through an exceptional point, which will open up new opportunities for in situ control of non-Hermitian systems.

cond-mat.mes-hall↗

arXiv2022

Magnetic Control of Soft Chiral Phonons in PbTe

PbTe crystals have a soft transverse optical phonon mode in the terahertz frequency range, which is known to efficiently decay into heat-carrying acoustic phonons, resulting in anomalously low thermal conductivity. Here, we studied this phonon via polarization-dependent terahertz spectroscopy. We observed softening of this mode with decreasing temperature, indicative of incipient ferroelectricity, which we explain through a model including strong anharmonicity with a quartic displacement term. In magnetic fields up to 25T, the phonon mode split into two modes with opposite handedness, exhibiting circular dichroism. Their frequencies displayed Zeeman splitting together with an overall diamagnetic shift with increasing magnetic field. Using a group-theoretical approach, we demonstrate that these observations are results of magnetic field-induced morphic changes in the crystal symmetries through the Lorentz force exerted on the lattice ions. This study thus reveals a novel process of controlling phonon properties in a soft ionic lattice by a strong magnetic field.

physics.optics↗

arXiv2021

Giant Terahertz Polarization Rotation in Ultrathin Films of Aligned Carbon Nanotubes

For facile manipulation of polarization states of light for applications in communications, imaging, and information processing, an efficient mechanism is desired for rotating light polarization with a minimum interaction length. Here, we report giant polarization rotations for terahertz (THz) electromagnetic waves in ultrathin (~45 nm), high-density films of aligned carbon nanotubes. We observed polarization rotations of up to ~20° and ~110° for transmitted and reflected THz pulses, respectively. The amount of polarization rotation was a sensitive function of the angle between the incident THz polarization and the nanotube alignment direction, exhibiting a `magic' angle at which the total rotation through transmission and reflection becomes exactly 90°. Our model quantitatively explains these giant rotations as a result of extremely anisotropic optical constants, demonstrating that aligned carbon nanotubes promise ultrathin, broadband, and tunable THz polarization devices.

physics.optics↗

arXiv2021

Ultrastrong Magnon-Magnon Coupling Dominated by Antiresonant Interactions

Exotic quantum vacuum phenomena are predicted in cavity quantum electrodynamics (QED) systems with ultrastrong light-matter interactions. Their ground states are predicted to be vacuum squeezed states with suppressed quantum fluctuations. The source of such phenomena are antiresonant terms in the Hamiltonian, yet antiresonant interactions are typically negligible compared to resonant interactions in light-matter systems. We report an unusual coupled matter-matter system of magnons that can simulate a unique cavity QED Hamiltonian with coupling strengths that are easily tunable into the ultrastrong coupling regime and with dominant antiresonant terms. We found a novel regime where vacuum Bloch-Siegert shifts, the hallmark of antiresonant interactions, greatly exceed analogous frequency shifts from resonant interactions. Further, we theoretically explored the system's ground state and calculated up to 5.9 dB of quantum fluctuation suppression. These observations demonstrate that magnonic systems provide an ideal platform for simulating exotic quantum vacuum phenomena predicted in ultrastrongly coupled light-matter systems.

quant-ph↗

arXiv2019

Terahertz Faraday and Kerr rotation spectroscopy of Bi$_{1-x}$Sb$_x$ films in high magnetic fields up to 30 Tesla

We report results of terahertz Faraday and Kerr rotation spectroscopy measurements on thin films of $\text{Bi}_{1-x}\text{Sb}_{x}$, an alloy system that exhibits a semimetal-to-topological-insulator transition as the Sb composition $x$ increases. By using a single-shot time-domain terahertz spectroscopy setup combined with a table-top pulsed mini-coil magnet, we conducted measurements in magnetic fields up to 30~T, observing distinctly different behaviors between semimetallic ($x < 0.07$) and topological insulator ($x > 0.07$) samples. Faraday and Kerr rotation spectra for the semimetallic films showed a pronounced dip that blue-shifted with the magnetic field, whereas spectra for the topological insulator films were positive and featureless, increasing in amplitude with increasing magnetic field and eventually saturating at high fields ($>$20~T). Ellipticity spectra for the semimetallic films showed resonances, whereas the topological insulator films showed no detectable ellipticity. To explain these observations, we developed a theoretical model based on realistic band parameters and the Kubo formula for calculating the optical conductivity of Landau-quantized charge carriers. Our calculations quantitatively reproduced all experimental features, establishing that the Faraday and Kerr signals in the semimetallic films predominantly arise from bulk hole cyclotron resonances while the signals in the topological insulator films represent combined effects of surface carriers originating from multiple electron and hole pockets. These results demonstrate that the use of high magnetic fields in terahertz magnetopolarimetry, combined with detailed electronic structure and conductivity calculations, allows us to unambiguously identify and quantitatively determine unique contributions from different species of carriers of topological and nontopological nature in Bi$_{1-x}$Sb$_x$.

cond-mat.mes-hall↗

arXiv2016

Single-Shot Terahertz Time-Domain Spectroscopy in Pulsed High Magnetic Fields

We have developed a single-shot terahertz time-domain spectrometer to perform optical-pump/terahertz-probe experiments in pulsed, high magnetic fields up to 30 T. The single-shot detection scheme for measuring a terahertz waveform incorporates a reflective echelon to create time-delayed beamlets across the intensity profile of the optical gate beam before it spatially and temporally overlaps with the terahertz radiation in a ZnTe detection crystal. After imaging the gate beam onto a camera, we can retrieve the terahertz time-domain waveform by analyzing the resulting image. To demonstrate the utility of our technique, we measured cyclotron resonance absorption of optically excited carriers in the terahertz frequency range in intrinsic silicon at high magnetic fields, with results that agree well with published values.

physics.ins-det↗

arXiv2016

Dicke Superradiance in Solids

Recent advances in optical studies of condensed matter have led to the emergence of phenomena that have conventionally been studied in the realm of quantum optics. These studies have not only deepened our understanding of light-matter interactions but also introduced aspects of many-body correlations inherent in optical processes in condensed matter systems. This article is concerned with superradiance (SR), a profound quantum optical process predicted by Dicke in 1954. The basic concept of SR applies to a general $N$-body system where constituent oscillating dipoles couple together through interaction with a common light field and accelerate the radiative decay of the system. In the most fascinating manifestation of SR, known as superfluorescence (SF), an incoherently prepared system of $N$ inverted atoms spontaneously develops macroscopic coherence from vacuum fluctuations and produces a delayed pulse of coherent light whose peak intensity $\propto N^2$. Such SF pulses have been observed in atomic and molecular gases, and their intriguing quantum nature has been unambiguously demonstrated. Here, we focus on the rapidly developing field of research on SR in solids, where not only photon-mediated coupling but also strong Coulomb interactions and ultrafast scattering exist. We describe SR and SF in molecular centers in solids, molecular aggregates and crystals, quantum dots, and quantum wells. In particular, we will summarize a series of studies we have recently performed on quantum wells in strong magnetic fields. These studies show that cooperative effects in solid-state systems are not merely small corrections that require exotic conditions to be observed; rather, they can dominate the nonequilibrium dynamics and light emission processes of the entire system of interacting electrons.

cond-mat.quant-gas↗