arXiv subjects

G. V. Budkin

Publications and source records attributed to G. V. Budkin.

At least 19 recordsLinked to original sources

arXiv2026

Photogalvanic effect in monolayers of transition metal dichalcogenides

We present a theoretical study of photocurrents generated by direct optical transitions induced by linearly polarized radiation in monolayers of transition metal dichalcogenides. A microscopic theory of both the ballistic and shift contributions to the photocurrent is developed that accounts for Coulomb attraction between photoexcited electrons and holes. It is demonstrated that, in typical 2D semiconductors, the Coulomb correlation causes the ballistic contribution to dominate over the shift photocurrent.

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arXiv2024

Influence of Coulomb interaction on interband photogalvanic effect in semiconductors

The ballistic and shift contributions to the interband linear photogalvanic effect are calculated in the same band structure model of a noncentrosymmetric semiconductor. The calculation uses a two-band generalized Dirac effective Hamiltonian with the off-diagonal components containing $\mathbf{ k}$-dependent terms of the first and second order. The developed theory takes into account the Coulomb interaction between the photoexited electron and hole. It is shown that in typical semiconductors the ballistic photocurrent $j^{({\rm bal})}$ significantly exceeds the shift current $j^{({\rm sh})}$: the ratio $j^{({\rm sh})}/j^{({\rm bal})}$ has the order of $a_B/ \ell$, where $a_B$ is the Bohr radius and $\ell$ is the mean free path of photocarriers due to their quasi-momentum scattering.

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arXiv2022

Splitting of Dirac cones in HgTe quantum wells: Effects of crystallographic orientation, interface-, bulk-, and structure-inversion asymmetry

We develop a microscopic theory of the fine structure of Dirac states in $(0lh)$-grown HgTe/CdHgTe quantum wells (QWs), where $l$ and $h$ are the Miller indices. It is shown that bulk, interface, and structure inversion asymmetry causes the anticrossing of levels even at zero in-plane wave vector and lifts the Dirac state degeneracy. In the QWs of critical thickness, the two-fold degenerate Dirac cone gets split into non-degenerate Weyl cones. The splitting and the Weyl point positions dramatically depend on the QW crystallographic orientation. We calculate the splitting parameters related to bulk, interface, and structure inversion asymmetry and derive the effective Hamiltonian of the Dirac states. Further, we obtain an analytical expression for the energy spectrum and discuss the spectrum for (001)-, (013)- and (011)-grown QWs.

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arXiv2022

THz ratchet effect in HgTe interdigitated structures

The emergence of ratchet effects in two-dimensional materials is strongly correlated with the introduction of asymmetry into the system. In general, dual-grating-gate structures forming lateral asymmetric superlattices provide a suitable platform for studying this phenomenon. Here, we report on the observation of ratchet effects in HgTe-based dual-grating-gate structures hosting different band structure properties. Applying polarized terahertz laser radiation we detected linear and polarization independent ratchets, as well as an radiation-helicity driven circular ratchet effect. Studying the ratchet effect in devices made of quantum wells (QWs) of different thickness we observed that the magnitude of the signal substantially increases with decreasing QW width with a maximum value for devices made of QWs of critical thickness hosting Dirac fermions. Furthermore, sweeping the gate voltage amplitude we observed sign-alternating oscillations for gate voltages corresponding to p-type conductivity. The amplitude of the oscillations is more than two orders of magnitude larger than the signal for n-type conducting QWs. The oscillations and the signal enhancement are shown to be caused by the complex valence band structure of HgTe-based QWs. These peculiar features of the ratchet currents make these materials an ideal platform for the development of THz applications.

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arXiv2022

Spin splitting in low-symmetry quantum wells beyond Rashba and Dresselhaus terms

Spin-orbit interaction in semiconductor structures with broken space inversion symmetry leads to spin splitting of electron and hole states even in the absence of magnetic field. We discover that, beyond the Rashba and Dresselhaus contributions, there is an additional type of the zero-field spin splitting which is caused by the interplay of the cubic shape of crystal unit cell and macroscopic structure asymmetry. In quantum wells grown along low-symmetry crystallographic axes, this type of spin-orbit interaction couples the out-of-plane component of carrier's spin with the in-plane momentum while the coupling strength is controlled by structure inversion asymmetry. We carry out numerical calculations and develop an analytical theory, which demonstrate that this interaction can dominate $\boldsymbol{k}$-linear spin splitting of heavy-hole subbands.

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arXiv2020

The drag of photons by electric current in quantum wells

The flow of electric current in quantum well breaks the space inversion symmetry, which leads to the dependence of the radiation transmission on the relative orientation of current and photon wave vector, this phenomenon can be named current drag of photons. We have developed a microscopic theory of such an effect for intersubband transitions in quantum wells taking into account both depolarization and exchange-correlation effects. It is shown that the effect of the current drag of photons originates from the asymmetry of intersubband optical transitions due to the redistribution of electrons in momentum space. We show that the presence of dc electric current leads to the shift of intersubband resonance position and affects both transmission coefficient and absorbance in quantum wells.

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arXiv2020

Impact ionization induced by terahertz radiation in HgTe quantum wells of critical thickness

We report on the observation of terahertz (THz) radiation induced band-to-band impact ionization in \HgTe quantum well (QW) structures of critical thickness, which are characterized by a nearly linear energy dispersion. The THz electric field drives the carriers initializing electron-hole pair generation. The carrier multiplication is observed for photon energies less than the energy gap under the condition that the product of the radiation angular frequency $ω$ and momentum relaxation time $τ_{\text l}$ larger than unity. In this case, the charge carriers acquire high energies solely because of collisions in the presence of a high-frequency electric field. The developed microscopic theory shows that the probability of the light impact ionization is proportional to $\exp(-E_0^2/E^2)$, with the radiation electric field amplitude $E$ and the characteristic field parameter $E_0$. As observed in experiment, it exhibits a strong frequency dependence for $ωτ\gg 1$ characterized by the characteristic field $E_0$ linearly increasing with the radiation frequency $ω$.

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arXiv2020

Terahertz Magnetospectroscopy of Cyclotron Resonances from Topological Surface States in Thick Films of Cd$_x$Hg$_{1-x}$Te

We present studies of the cyclotron resonance (CR) in thick Cd$_x$Hg$_{1-x}$Te films with different cadmium concentrations corresponding to inverted and normal band order, as well as to an almost linear energy dispersion. Our results demonstrate that formation of two-dimensional topological surface states requires sharp interfaces between layers with inverted and normal band order, in which case the corresponding CR is clearly observed for the out-of-plane orientation of magnetic field, but does not show up for an in-plane orientation. By contrast, all samples having more conventional technological design with smooth interfaces (i.e., containing regions of Cd$_x$Hg$_{1-x}$Te with gradually changing Cd content $x$) show equally pronounced CR in both in-plane and out-of-plane magnetic field revealing that CR is excited in three-dimensional states. Modeling of the surface states for different film designs supports our main observations. In all samples, we observe additional broad helicity-independent resonances which are attributed to photo-ionization and magnetic freeze-out of impurity states.

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arXiv2019

Symmetry breaking and circular photogalvanic effect in epitaxial Cd$_x$Hg$_{1-x}$Te films

We report on the observation of symmetry breaking and the circular photogalvanic effect in Cd$_x$Hg$_{1-x}$Te alloys. We demonstrate that irradiation of bulk epitaxial films with circularly polarized terahertz radiation leads to the circular photogalvanic effect (CPGE) yielding a photocurrent whose direction reverses upon switching the photon helicity. This effect is forbidden in bulk zinc-blende crystals by symmetry arguments, therefore, its observation indicates either the symmetry reduction of bulk material or that the photocurrent is excited in the topological surface states formed in a material with low Cadmium concentration. We show that the bulk states play a crucial role because the CPGE was also clearly detected in samples with non-inverted band structure. We suggest that strain is a reason of the symmetry reduction. We develop a theory of the CPGE showing that the photocurrent results from the quantum interference of different pathways contributing to the free-carrier absorption (Drude-like) of monochromatic radiation.

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arXiv2019

Thermal generation of shift electric current

It is shown that the dissipation of energy in an electron gas confined in a quantum well made of non-centrosymmetric crystal leads to a direct electric current. The current originates from the real-space shift of the wavepackets of Bloch electrons at the electron scattering by phonons, which tends to restore thermal equilibrium between the electron and phonon subsystems. We develop a microscopic theory of such a phonogalvanic effect for narrow band gap zinc-blende quantum wells.

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arXiv2019

Cyclotron resonance induced photogalvanic effect in surface states of 200 nm thick strained HgTe films

We report on the study of magneto-photogalvanic and magnetotransport phenomena in 200 nm partially strained HgTe films. This thickness is slightly larger than the estimated critical thickness of lattice relaxation leaving the film partially relaxed with the value of the energy gap close to zero. We show that illumination of HgTe films with monochromatic terahertz laser radiation results in a giant resonant photocurrent caused by the cyclotron resonance in the surface states. The resonant photocurrent is also detected in the reference fully strained 80 nm HgTe films previously shown to be fully gapped 3D topological insulators. We show that the resonance positions in both types of films almost coincide demonstrating the existence of topologically protected surface states in thick HgTe films. The conclusion is supported by magnetotransport experiments.

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arXiv2018

High frequency impact ionization and nonlinearity of photocurrent induced by intense terahertz radiation in HgTe-based quantum well structures

We report on a strong nonlinear behavior of the photogalvanics and photoconductivity under excitation of HgTe quantum wells (QWs) by intense terahertz (THz) radiation. The increasing radiation intensity causes an inversion of the sign of the photocurrent and transition to its superlinear dependence on the intensity. The photoconductivity also shows a superlinear raise with the intensity. We show that the observed photoresponse nonlinearities are caused by the band-to-band \emph{light} impact ionization under conditions of a photon energy less than the forbidden gap. The signature of this kind of impact ionization is that the angular radiation frequency $ω=2πf$ is much higher than the reciprocal momentum relaxation time. Thus, the impact ionization takes place solely because of collisions in the presence of a high-frequency electric field. The effect has been measured on narrow HgTe/CdTe QWs of 5.7\,nm width; the nonlinearity is detected for linearly and circularly polarized THz radiation with different frequencies ranging from $f=0.6$ to 1.07\,THz and intensities up to hundreds of kW/cm$^2$. We demonstrate that the probability of the impact ionization is proportional to the exponential function, $\exp(-E_0^2/E^2)$, of the radiation electric field amplitude $E$ and the characteristic field parameter $E_0$. The effect is observable in a wide temperature range from 4.2 to 90\,K, with the characteristic field increasing with rising temperature.

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arXiv2017

Circular and linear magnetic quantum ratchet effects in dual-grating-gate CdTe-based nanostructures

We report on the observation and systematic study of polarization sensitive magnetic quantum ratchet effects induced by alternating electric fields in the terahertz frequency range. The effects are detected in (Cd,Mn)Te-based quantum well (QW) structures with inter-digitated dual-grating-gate (DGG) lateral superlattices. A dc electric current excited by cw terahertz laser radiation shows 1/B-periodic oscillations with an amplitude much larger than the photocurrent at zero magnetic field. Variation of gate voltages applied to individual grating gates of the DGG enables us to change the degree and the sign of the lateral asymmetry in a controllable way. The data reveal that the photocurrent reflects the degree of lateral asymmetry induced by different gate potentials. We show that the magnetic ratchet photocurrent includes the Seebeck thermoratchet effect as well as the effects of "linear" and "circular" ratchets, which are sensitive to the corresponding polarization of the driving electromagnetic force. Theoretical analysis performed in the framework of semiclassical approach and taking into account Landau quantization describes the experimental results well.

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arXiv2017

Magnetic quantum ratchet effect in (Cd,Mn)Te- and CdTe-based quantum well structures with a lateral asymmetric superlattice

We report on the observation of magnetic quantum ratchet effect in (Cd,Mn)Te- and CdTe-based quantum well structures with an asymmetric lateral dual grating gate superlattice subjected to an external magnetic field applied normal to the quantum well plane. A dc electric current excited by cw terahertz laser radiation shows 1/B-oscillations with an amplitude much larger as compared to the photocurrent at zero magnetic field. We show that the photocurrent is caused by the combined action of a spatially periodic in-plane potential and the spatially modulated radiation due to the near field effects of light diffraction. Magnitude and direction of the photocurrent are determined by the degree of the lateral asymmetry controlled by the variation of voltages applied to the individual gates. The observed magneto-oscillations with enhanced photocurrent amplitude result from Landau quantization and, for (Cd,Mn)Te at low temperatures, from the exchange enhanced Zeeman splitting in diluted magnetic heterostructures. Theoretical analysis, considering the magnetic quantum ratchet effect in the framework of semiclassical approach, describes quite well the experimental results.

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arXiv2015

Ratchet transport of a two-dimensional electron gas at cyclotron resonance

The driving of charge carriers confined in a quantum well lacking the center of space inversion by an alternating electric field leads to the formation of a direct electric current. We develop a microscopic theory of such a quantum ratchet effect for quantum wells subjected to a static magnetic field. We show that the ratchet current emerges for a linearly polarized alternating electric field as well as a rotating electric field and drastically increases at the cyclotron resonance conditions. For the magnetic field tilted with respect to the quantum well normal, the ratchet current contains an additional resonance at the first subharmonic of the cyclotron resonance.

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arXiv2015

Cyclotron Resonance Assisted Photocurrents in Surface States of a 3D Topological Insulator Based on a Strained High Mobility HgTe Film

We report on the observation of cyclotron resonance induced photocurrents, excited by continuous wave terahertz radiation, in a 3D topological insulator (TI) based on an 80 nm strained HgTe film. The analysis of the photocurrent formation is supported by complimentary measurements of magneto-transport and radiation transmission. We demonstrate that the photocurrent is generated in the topologically protected surface states. Studying the resonance response in a gated sample we examined the behavior of the photocurrent, which enables us to extract the mobility and the cyclotron mass as a function of the Fermi energy. For high gate voltages we also detected cyclotron resonance (CR) of bulk carriers, with a mass about two times larger than that obtained for the surface states. The origin of the CR assisted photocurrent is discussed in terms of asymmetric scattering of TI surface carriers in the momentum space. Furthermore, we show that studying the photocurrent in gated samples provides a sensitive method to probe the effective masses and the mobility of 2D Dirac surface states, when the Fermi level lies in the bulk energy gap or even in the conduction band.

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arXiv2014

Orbital magnetic ratchet effect

Magnetic ratchets -- two-dimensional systems with superimposed non-centrosymmetric ferromagnetic gratings -- are considered theoretically. It is demonstrated that excitation by radiation results in a directed motion of two-dimensional carriers due to pure orbital effect of the periodic magnetic field. Magnetic ratchets based on various two-dimensional systems like topological insulators, graphene and semiconductor heterostructures are investigated. The mechanisms of the electric current generation caused by both radiation-induced heating of carriers and by acceleration in the radiation electric field in the presence of space-oscillating Lorentz force are studied in detail. The electric currents sensitive to the linear polarization plane orientation as well as to the radiation helicity are calculated. It is demonstrated that the frequency dependence of the magnetic ratchet currents is determined by the dominant elastic scattering mechanism of two-dimensional carriers and differs for the systems with linear and parabolic energy dispersions.

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arXiv2013

Cyclotron-resonance-assisted photon drag effect in InSb/InAlSb quantum wells excited by terahertz radiation

We report on the observation of the cyclotron-resonance-assisted photon drag effect. Resonant photocurrent is detected in InSb/InAlSb quantum wells structures subjected to a static magnetic field and excited by terahertz radiation at oblique incidence. The developed theory based on Boltzmann's kinetic equation is in a good agreement with the experimental findings. We show that the resonant photocurrent originates from the transfer of photon momentum to free electrons drastically enhanced at cyclotron resonance.

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