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G. W. Kim

Publications and source records attributed to G. W. Kim.

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A study of neutrinoless double electron capture in $^{40}$Ca from the AMoRE experiment

The search for neutrinoless double electron capture ($0ν\mathrm{2EC}$) provides a sensitive probe of lepton-number violation and the Majorana nature of neutrinos. We investigate the $0ν\mathrm{2EC}$ decay of $^{40}$Ca using cryogenic detectors equipped with metallic magnetic calorimeters in the AMoRE-I experiment. The analysis is based on a physics dataset corresponding to a total exposure of 7.32 kg$\cdot$yr from thirteen $^{40}$Ca$^{100}$MoO$_4$ crystals. No significant excess is observed, and a lower limit on the half-life is obtained as $T^{0ν}_{1/2} > 1.7 \times 10^{22}$ yr at 90$\%$ confidence level. An improved sensitivity is expected for the upcoming AMoRE-II experiment. These results demonstrate the potential of CaMoO$_4$ detectors to explore rare decay processes beyond the primary $^{100}$Mo $0νββ$ search program.

nucl-ex

Improved limit on neutrinoless double beta decay of $^{100}$Mo from AMoRE-I

AMoRE searches for the signature of neutrinoless double beta decay of $^{100}$Mo with a 100 kg sample of enriched $^{100}$Mo. Scintillating molybdate crystals coupled with a metallic magnetic calorimeter operate at milli-Kelvin temperatures to measure the energy of electrons emitted in the decay. As a demonstration of the full-scale AMoRE, we conducted AMoRE-I, a pre-experiment with 18 molybdate crystals, at the Yangyang Underground Laboratory for over two years. The exposure was 8.02 kg$\cdot$year (or 3.89 kg$_{\mathrm{^{100}Mo}}\cdot$year) and the total background rate near the Q-value was 0.025 $\pm$ 0.002 counts/keV/kg/year. We observed no indication of $0νββ$ decay and report a new lower limit of the half-life of $^{100}$Mo $0νββ$ decay as $ T^{0ν}_{1/2}>2.9\times10^{24}~\mathrm{yr}$ at 90\% confidence level. The effective Majorana mass limit range is $m_{ββ}<$(210--610) meV using nuclear matrix elements estimated in the framework of different models, including the recent shell model calculations.

nucl-ex

Development of MMC-based lithium molybdate cryogenic calorimeters for AMoRE-II

The AMoRE collaboration searches for neutrinoless double beta decay of $^{100}$Mo using molybdate scintillating crystals via low temperature thermal calorimetric detection. The early phases of the experiment, AMoRE-pilot and AMoRE-I, have demonstrated competitive discovery potential. Presently, the AMoRE-II experiment, featuring a large detector array with about 90 kg of $^{100}$Mo isotope, is under construction. This paper discusses the baseline design and characterization of the lithium molybdate cryogenic calorimeters to be used in the AMoRE-II detector modules. The results from prototype setups that incorporate new housing structures and two different crystal masses (316 g and 517 - 521 g), operated at 10 mK temperature, show energy resolutions (FWHM) of 7.55 - 8.82 keV at the 2.615 MeV $^{208}$Tl $γ$ line, and effective light detection of 0.79 - 0.96 keV/MeV. The simultaneous heat and light detection enables clear separation of alpha particles with a discrimination power of 12.37 - 19.50 at the energy region around $^6$Li(n, $α$)$^3$H with Q-value = 4.785 MeV. Promising detector performances were demonstrated at temperatures as high as 30 mK, which relaxes the temperature constraints for operating the large AMoRE-II array.

physics.ins-det

Projected background and sensitivity of AMoRE-II

AMoRE-II aims to search for neutrinoless double beta decay with an array of 423 Li$_2$$^{100}$MoO$_4$ crystals operating in the cryogenic system as the main phase of the Advanced Molybdenum-based Rare process Experiment (AMoRE). AMoRE has been planned to operate in three phases: AMoRE-pilot, AMoRE-I, and AMoRE-II. AMoRE-II is currently being installed at the Yemi Underground Laboratory, located approximately 1000 meters deep in Jeongseon, Korea. The goal of AMoRE-II is to reach up to $T^{0νββ}_{1/2}$ $\sim$ 6 $\times$ 10$^{26}$ years, corresponding to an effective Majorana mass of 15 - 29 meV, covering all the inverted mass hierarchy regions. To achieve this, the background level of the experimental configurations and possible background sources of gamma and beta events should be well understood. We have intensively performed Monte Carlo simulations using the GEANT4 toolkit in all the experimental configurations with potential sources. We report the estimated background level that meets the 10$^{-4}$counts/(keV$\cdot$kg$\cdot$yr) requirement for AMoRE-II in the region of interest (ROI) and show the projected half-life sensitivity based on the simulation study.

physics.ins-det

Background study of the AMoRE-pilot experiment

We report a study on the background of the Advanced Molybdenum-Based Rare process Experiment (AMoRE), a search for neutrinoless double beta decay (\znbb) of $^{100}$Mo. The pilot stage of the experiment was conducted using $\sim$1.9 kg of \CAMOO~ crystals at the Yangyang Underground Laboratory, South Korea, from 2015 to 2018. We compared the measured $β/γ$ energy spectra in three experimental configurations with the results of Monte Carlo simulations and identified the background sources in each configuration. We replaced several detector components and enhanced the neutron shielding to lower the background level between configurations. A limit on the half-life of $0νββ$ decay of $^{100}$Mo was found at $T_{1/2}^{0ν} \ge 3.0\times 10^{23}$ years at 90\% confidence level, based on the measured background and its modeling. Further reduction of the background rate in the AMoRE-I and AMoRE-II are discussed.

nucl-ex

Alpha backgrounds in the AMoRE-Pilot experiment

The Advanced Mo-based Rare process Experiment (AMoRE)-Pilot experiment is an initial phase of the AMoRE search for neutrinoless double beta decay of $^{100}$Mo, with the purpose of investigating the level and sources of backgrounds. Searches for neutrinoless double beta decay generally require ultimately low backgrounds. Surface $α$ decays on the crystals themselves or nearby materials can deposit a continuum of energies that can be as high as the $Q$-value of the decay itself and may fall in the region of interest (ROI). To understand these background events, we studied backgrounds from radioactive contaminations internal to and on the surface of the crystals or nearby materials with Geant4-based Monte Carlo simulations. In this study, we report on the measured $α$ energy spectra fitted with the corresponding simulated spectra for six crystal detectors, where sources of background contributions could be identified through high energy $α$ peaks and continuum parts in the energy spectrum for both internal and surface contaminations. We determine the low-energy contributions from internal and surface $α$ contaminations by extrapolating from the $α$ background fitting model.

physics.ins-det

Measurement of the Background Activities of a 100Mo-enriched Powder Sample for an AMoRE Crystal Material by using Fourteen High-Purity Germanium Detectors

The Advanced Molybdenum-based Rare process Experiment in its second phase (AMoRE-II) will search for neutrinoless double-beta (0ν\b{eta}\b{eta}) decay of 100Mo in 200 kg of molybdate crystals. To achieve the zero-background level in the energy range of the double-beta decay Q-value of 100Mo, the radioactive contamination levels in AMoRE crystals should be low. 100EnrMoO3 powder, which is enriched in the 100Mo isotope, is used to grow the AMoRE crystals. A shielded array of fourteen high-purity germanium detectors with 70% relative efficiency each was used for the measurement of background activities in a sample of 9.6-kg powder. The detector system named CAGe located at the Yangyang underground laboratory was designed for measuring low levels of radioactivity from natural radioisotopes or cosmogenic nuclides such as 228Ac, 228Th, 226Ra, 88Y, and 40K. The activities of 228Ac and 228Th in the powder sample were 0.88 \pm 0.12 mBq/kg and 0.669 \pm 0.087 mBq/kg, respectively. The activity of 226Ra was measured to be 1.50 \pm 0.23 mBq/kg. The activity of 88Y was 0.101 \pm 0.016 mBq/kg. The activity of 40K was found as 36.0 \pm 4.1 mBq/kg.

physics.ins-det

Development of an array of HPGe detectors with 980% relative efficiency

Searches for new physics push experiments to look for increasingly rare interactions. As a result, detectors require increasing sensitivity and specificity, and materials must be screened for naturally occurring, background-producing radioactivity. Furthermore the detectors used for screening must approach the sensitivities of the physics-search detectors themselves, thus motivating iterative development of detectors capable of both physics searches and background screening. We report on the design, installation, and performance of a novel, low-background, fourteen-element high-purity germanium detector named the CAGe (CUP Array of Germanium), installed at the Yangyang underground laboratory in Korea.

physics.ins-det

Growth and development of pure Li2MoO4 crystals for rare event experiment at CUP

The Center for Underground Physics (CUP) of the Institute for Basic Science (IBS) is searching for the neutrinoless double-beta decay (0ν\b{eta}\b{eta}) of 100Mo in the molybdate crystals of the AMoRE experiment. The experiment requires pure scintillation crystals to minimize internal backgrounds that can affect the 0ν\b{eta}\b{eta} signal. For the last few years, we have been growing and studying Li2MoO4 crystals in a clean-environment facility to minimize external contamination during the crystal growth. Before growing Li2100MoO4 crystal, we have studied Li2natMoO4 crystal growth by a conventional Czochralski (CZ) grower. We grew a few different kinds of Li2natMO4 crystals using different raw materials in a campaign to minimize impurities. We prepared the fused Al2O3 refractories for the growth of ingots. Purities of the grown crystals were measured with high purity germanium detectors and by inductively coupled plasma mass spectrometry. The results show that the Li2MoO4 crystal has purity levels suitable for rare-event experiments. In this study, we present the growth of Li2MoO4 crystals at CUP and their purities.

physics.ins-det

First Results from the AMoRE-Pilot neutrinoless double beta decay experiment

The Advanced Molybdenum-based Rare process Experiment (AMoRE) aims to search for neutrinoless double beta decay (0$νββ$) of $^{100}$Mo with $\sim$100 kg of $^{100}$Mo-enriched molybdenum embedded in cryogenic detectors with a dual heat and light readout. At the current, pilot stage of the AMoRE project we employ six calcium molybdate crystals with a total mass of 1.9 kg, produced from $^{48}$Ca-depleted calcium and $^{100}$Mo-enriched molybdenum ($^{48\textrm{depl}}$Ca$^{100}$MoO$_4$). The simultaneous detection of heat(phonon) and scintillation (photon) signals is realized with high resolution metallic magnetic calorimeter sensors that operate at milli-Kelvin temperatures. This stage of the project is carried out in the Yangyang underground laboratory at a depth of 700 m. We report first results from the AMoRE-Pilot $0νββ$ search with a 111 kg$\cdot$d live exposure of $^{48\textrm{depl}}$Ca$^{100}$MoO$_4$ crystals. No evidence for $0νββ$ decay of $^{100}$Mo is found, and a upper limit is set for the half-life of 0$νββ$ of $^{100}$Mo of $T^{0ν}_{1/2} > 9.5\times10^{22}$ y at 90% C.L.. This limit corresponds to an effective Majorana neutrino mass limit in the range $\langle m_{ββ}\rangle\le(1.2-2.1)$ eV.

hep-ex