arXiv subjects

G. Wang

Publications and source records attributed to G. Wang.

At least 127 records · Page 7Linked to original sources

arXiv2016

Exciton Radiative Lifetime in Transition Metal Dichalcogenide Monolayers

We have investigated the exciton dynamics in transition metal dichalcogenide mono-layers using time-resolved photoluminescence experiments performed with optimized time-resolution. For MoSe2 monolayers, we measure $τ_{rad}=1.8\pm0.2$ ps that we interpret as the intrinsic radiative recombination time. Similar values are found for WSe2 mono-layers. Our detailed analysis suggests the following scenario: at low temperature (T $\leq$ 50 K), the exciton oscillator strength is so large that the entire light can be emitted before the time required for the establishment of a thermalized exciton distribution. For higher lattice temperatures, the photoluminescence dynamics is characterized by two regimes with very different characteristic times. First the PL intensity drops drastically with a decay time in the range of the picosecond driven by the escape of excitons from the radiative window due to exciton- phonon interactions. Following this first non-thermal regime, a thermalized exciton population is established gradually yielding longer photoluminescence decay times in the nanosecond range. Both the exciton effective radiative recombination and non-radiative recombination channels including exciton-exciton annihilation control the latter. Finally the temperature dependence of the measured exciton and trion dynamics indicates that the two populations are not in thermodynamical equilibrium.

cond-mat.mtrl-sci↗

arXiv2015

Spin transport in molybdenum disulfide multilayer channel

Molybdenum disulfide has recently emerged as a promising two-dimensional semiconducting material for nano-electronic, opto-electronic and spintronic applications. However, demonstrating spin-transport through a semiconducting MoS2 channel is challenging. Here we demonstrate the electrical spin injection and detection in a multilayer MoS2 semiconducting channel. A magnetoresistance (MR) around 1% has been observed at low temperature through a 450nm long, 6 monolayer thick channel with a Co/MgO spin injector and detector. From a systematic study of the bias voltage, temperature and back-gate voltage dependence of MR, it is found that the hopping via localized states in the contact depletion region plays a key role for the observation of the two-terminal MR. Moreover, the electron spin-relaxation is found to be greatly suppressed in the multilayer MoS2 channel for in-plan spin injection. The underestimated long spin diffusion length (~235nm) and large spin lifetime (~46ns) open a new avenue for spintronic applications using multilayer transition metal dichalcogenides.

cond-mat.mtrl-sci↗

arXiv2015

Magneto-spectroscopy of excited states in charge-tunable GaAs/AlGaAs [111] quantum dots

We present a combined experimental and theoretical study of highly charged and excited electron-hole complexes in strain-free (111) GaAs/AlGaAs quantum dots grown by droplet epitaxy. We address the complexes with one of the charge carriers residing in the excited state, namely, the ``hot'' trions X$^{-*}$ and X$^{+*}$, and the doubly negatively charged exciton X$^{2-}$. Our magneto-photoluminescence experiments performed on single quantum dots in the Faraday geometry uncover characteristic emission patterns for each excited electron-hole complex, which are very different from the photoluminescence spectra observed in (001)-grown quantum dots. We present a detailed theory of the fine structure and magneto-photoluminescence spectra of X$^{-*}$, X$^{+*}$ and X$^{2-}$ complexes, governed by the interplay between the electron-hole Coulomb exchange interaction and the heavy-hole mixing, characteristic for these quantum dots with a trigonal symmetry. Comparison between experiment and theory of the magneto-photoluminescence allows for precise charge state identification, as well as extraction of electron-hole exchange interaction constants and $g$-factors for the charge carriers occupying excited states.

cond-mat.mes-hall↗

arXiv2015

Dependable Structural Helath Monitoring Using Wireless Sensor Networks

As an alternative to current wired-based networks, wireless sensor networks (WSNs) are becoming an increasingly compelling platform for engineering structural health monitoring (SHM) due to relatively low-cost, easy installation, and so forth. However, there is still an unaddressed challenge: the application-specific dependability in terms of sensor fault detection and tolerance. The dependability is also affected by a reduction on the quality of monitoring when mitigating WSN constrains (e.g., limited energy, narrow bandwidth). We address these by designing a dependable distributed WSN framework for SHM (called DependSHM) and then examining its ability to cope with sensor faults and constraints. We find evidence that faulty sensors can corrupt results of a health event (e.g., damage) in a structural system without being detected. More specifically, we bring attention to an undiscovered yet interesting fact, i.e., the real measured signals introduced by one or more faulty sensors may cause an undamaged location to be identified as damaged (false positive) or a damaged location as undamaged (false negative) diagnosis. This can be caused by faults in sensor bonding, precision degradation, amplification gain, bias, drift, noise, and so forth. In DependSHM, we present a distributed automated algorithm to detect such types of faults, and we offer an online signal reconstruction algorithm to recover from the wrong diagnosis. Through comprehensive simulations and a WSN prototype system implementation, we evaluate the effectiveness of DependSHM.

cs.DC↗

arXiv2015

Spin and valley dynamics of excitons in transition metal dichalcogenides monolayers

Monolayers of transition metal dichalcogenides, namely, molybdenum and tungsten disulfides and diselenides demonstrate unusual optical properties related to the spin-valley locking effect. Particularly, excitation of monolayers by circularly polarized light selectively creates electron-hole pairs or excitons in non-equivalent valleys in momentum space, depending on the light helicity. This allows studying the inter-valley dynamics of charge carriers and Coulomb complexes by means of optical spectroscopy. Here we present a concise review of the neutral exciton fine structure and its spin and valley dynamics in monolayers of transition metal dichalcogenides. It is demonstrated that the long-range exchange interaction between an electron and a hole in the exciton is an efficient mechanism for rapid mixing between bright excitons made of electron-hole pairs in different valleys. We discuss the physical origin of the long-range exchange interaction and outline its derivation in both the electrodynamical and $\mathbf k \cdot \mathbf p$ approaches. We further present a model of bright exciton spin dynamics driven by an interplay between the long-range exchange interaction and scattering. Finally, we discuss the application of the model to describe recent experimental data obtained by time-resolved photoluminescence and Kerr rotation techniques.

cond-mat.mes-hall↗

arXiv2015

A Measurement of the Cosmic Microwave Background Gravitational Lensing Potential from 100 Square Degrees of SPTpol Data

We present a measurement of the cosmic microwave background (CMB) gravitational lensing potential using data from the first two seasons of observations with SPTpol, the polarization-sensitive receiver currently installed on the South Pole Telescope (SPT). The observations used in this work cover 100 deg$^2$ of sky with arcminute resolution at 150 GHz. Using a quadratic estimator, we make maps of the CMB lensing potential from combinations of CMB temperature and polarization maps. We combine these lensing potential maps to form a minimum-variance (MV) map. The lensing potential is measured with a signal-to-noise ratio of greater than one for angular multipoles between $100< L <250$. This is the highest signal-to-noise mass map made from the CMB to date and will be powerful in cross-correlation with other tracers of large-scale structure. We calculate the power spectrum of the lensing potential for each estimator, and we report the value of the MV power spectrum between $100< L <2000$ as our primary result. We constrain the ratio of the spectrum to a fiducial $Λ$CDM model to be $A_{\rm MV}=0.92 \pm 0.14 {\rm\, (Stat.)} \pm 0.08 {\rm\, (Sys.)}$. Restricting ourselves to polarized data only, we find $A_{\rm POL}=0.92 \pm 0.24 {\rm\, (Stat.)} \pm 0.11 {\rm\, (Sys.)}$. This measurement rejects the hypothesis of no lensing at $5.9 σ$ using polarization data alone, and at $14 σ$ using both temperature and polarization data.

astro-ph.CO↗

arXiv2015

Double resonant Raman scattering and valley coherence generation in monolayer WSe2

The electronic states at the direct band gap of monolayer WSe2 at the $K^+$ and $K^-$ valleys are related by time reversal and may be viewed as pseudo-spins. The corresponding optical interband transitions are governed by robust excitons. In double resonant Raman spectroscopy, we uncover that the 2s exciton state energy differs from the 1s state energy by exactly the energy of the combination of several prominent phonons. Superimposed on the exciton photoluminescence (PL) we observe the double resonant Raman signal. This spectrally narrow peak shifts with the excitation laser energy as incoming photons match the 2s and outgoing photons the 1s exciton transition. The multi-phonon resonance has important consequences: Following linearly polarized excitation of the 2s exciton a superposition of valley states is generated which can relax fast via phonon emission and with minimal loss of coherence from the 2s to 1s state. This explains the high degree of valley coherence measured for the 1s exciton PL.

cond-mat.mtrl-sci↗

arXiv2015

The First Data Release (DR1) of the LAMOST general survey

The Large sky Area Multi-Object Spectroscopic Telescope (LAMOST) General Survey is a spectroscopic survey that will eventually cover approximately half of the celestial sphere and collect 10 million spectra of stars, galaxies and QSOs. Objects both in the pilot survey and the first year general survey are included in the LAMOST First Data Release (DR1). The pilot survey started in October 2011 and ended in June 2012, and the data have been released to the public as the LAMOST Pilot Data Release in August 2012. The general survey started in September 2012, and completed its first year of operation in June 2013. The LAMOST DR1 includes a total of 1202 plates containing 2,955,336 spectra, of which 1,790,879 spectra have observed signal-to-noise S/N >10. All data with S/N>2 are formally released as LAMOST DR1 under the LAMOST data policy. This data release contains a total of 2,204,696 spectra, of which 1,944,329 are stellar spectra, 12,082 are galaxy spectra and 5,017 are quasars. The DR1 includes not only spectra, but also three stellar catalogues with measured parameters: AFGK-type stars with high quality spectra (1,061,918 entries), A-type stars (100,073 entries), and M stars (121,522 entries). This paper introduces the survey design, the observational and instrumental limitations, data reduction and analysis, and some caveats. Description of the FITS structure of spectral files and parameter catalogues is also provided.

astro-ph.GA↗

arXiv2015

Exciton states in monolayer MoSe2: impact on interband transitions

We combine linear and non-linear optical spectroscopy at 4K with ab initio calculations to study the electronic bandstructure of MoSe2 monolayers. In 1-photon photoluminescence excitation (PLE) and reflectivity we measure a separation between the A- and B-exciton emission of 220 meV. In 2-photon PLE we detect for the A- and B-exciton the 2p state 180meV above the respective 1s state. In second harmonic generation (SHG) spectroscopy we record an enhancement by more than 2 orders of magnitude of the SHG signal at resonances of the charged exciton and the 1s and 2p neutral A- and B-exciton. Our post-Density Functional Theory calculations show in the conduction band along the $K-Γ$ direction a local minimum that is energetically and in k-space close to the global minimum at the K-point. This has a potentially strong impact on the polarization and energy of the excitonic states that govern the interband transitions and marks an important difference to MoS2 and WSe2 monolayers.

cond-mat.mtrl-sci↗

arXiv2015

Magneto-optics in transition metal diselenide monolayers

We perform photoluminescence experiments at 4K on two different transition metal diselenide monolayers, namely MoSe2 and WSe2 in magnetic fields $B_z$ up to 9T applied perpendicular to the sample plane. In MoSe2 monolayers the valley polarization of the neutral and the charged exciton (trion) can be tuned by the magnetic field, independent of the excitation laser polarization. In the investigated WSe2 monolayer sample the evolution of the trion valley polarization depends both on the applied magnetic field and the excitation laser helicity, while the neutral exciton valley polarization depends only on the latter. Remarkably we observe a reversal of the sign of the trion polarization between WSe2 and MoSe2. For both systems we observe a clear Zeeman splitting for the neutral exciton and the trion of about $\pm2$meV at $B_z\mp9$T. The extracted Landé-factors for both exciton complexes in both materials are $g\approx -4$.

cond-mat.mtrl-sci↗

arXiv2015

Measurements of Sub-degree B-mode Polarization in the Cosmic Microwave Background from 100 Square Degrees of SPTpol Data

We present a measurement of the $B$-mode polarization power spectrum (the $BB$ spectrum) from 100 $\mathrm{deg}^2$ of sky observed with SPTpol, a polarization-sensitive receiver currently installed on the South Pole Telescope. The observations used in this work were taken during 2012 and early 2013 and include data in spectral bands centered at 95 and 150 GHz. We report the $BB$ spectrum in five bins in multipole space, spanning the range $300 \le \ell \le 2300$, and for three spectral combinations: 95 GHz $\times$ 95 GHz, 95 GHz $\times$ 150 GHz, and 150 GHz $\times$ 150 GHz. We subtract small ($< 0.5 σ$ in units of statistical uncertainty) biases from these spectra and account for the uncertainty in those biases. The resulting power spectra are inconsistent with zero power but consistent with predictions for the $BB$ spectrum arising from the gravitational lensing of $E$-mode polarization. If we assume no other source of $BB$ power besides lensed $B$ modes, we determine a preference for lensed $B$ modes of $4.9 σ$. After marginalizing over tensor power and foregrounds, namely polarized emission from galactic dust and extragalactic sources, this significance is $4.3 σ$. Fitting for a single parameter, $A_\mathrm{lens}$, that multiplies the predicted lensed $B$-mode spectrum, and marginalizing over tensor power and foregrounds, we find $A_\mathrm{lens} = 1.08 \pm 0.26$, indicating that our measured spectra are consistent with the signal expected from gravitational lensing. The data presented here provide the best measurement to date of the $B$-mode power spectrum on these angular scales.

astro-ph.CO↗

arXiv2015

Carbon p Electron Ferromagnetism in Silicon Carbide

Ferromagnetism can occur in wide-band gap semiconductors as well as in carbon-based materials when specific defects are introduced. It is thus desirable to establish a direct relation between the defects and the resulting ferromagnetism. Here, we contribute to revealing the origin of defect-induced ferromagnetism using SiC as a prototypical example. We show that the long-range ferromagnetic coupling can be attributed to the p electrons of the nearest-neighbor carbon atoms around the VSiVC divacancies. Thus, the ferromagnetism is traced down to its microscopic, electronic origin.

cond-mat.mtrl-sci↗

arXiv2015

Polarization and time-resolved photoluminescence spectroscopy of excitons in MoSe2 monolayers

We investigate valley exciton dynamics in MoSe2 monolayers in polarization- and time-resolved photoluminescence (PL) spectroscopy at 4K. Following circularly polarized laser excitation, we record a low circular polarization degree of the PL of typically $\leq5\%$. This is about 10 times lower than the polarization induced under comparable conditions in MoS2 and WSe2 monolayers. The evolution of the exciton polarization as a function of excitation laser energy and power is monitored in PL excitation (PLE) experiments. Fast PL emission times are recorded for both the neutral exciton of $\leq3$ ps and for the charged exciton (trion) of 12 ps.

cond-mat.mtrl-sci↗

arXiv2014

eRHIC Design Study: An Electron-Ion Collider at BNL

This document presents BNL's plan for an electron-ion collider, eRHIC, a major new research tool that builds on the existing RHIC facility to advance the long-term vision for Nuclear Physics to discover and understand the emergent phenomena of Quantum Chromodynamics (QCD), the fundamental theory of the strong interaction that binds the atomic nucleus. We describe the scientific requirements for such a facility, following up on the community-wide 2012 white paper, 'Electron-Ion Collider: the Next QCD Frontier', and present a design concept that incorporates new, innovative accelerator techniques to provide a cost-effective upgrade of RHIC with polarized electron beams colliding with the full array of RHIC hadron beams. The new facility will deliver electron-nucleon luminosity of 10^33-10^34 cm-1sec-1 for collisions of 15.9 GeV polarized electrons on either 250 GeV polarized protons or 100 GeV/u heavy ion beams. The facility will also be capable of providing an electron beam energy of 21.2 GeV, at reduced luminosity. We discuss the on-going R&D effort to realize the project, and present key detector requirements and design ideas for an experimental program capable of making the 'golden measurements' called for in the EIC White Paper.

physics.acc-ph↗

arXiv2014

Measurements of E-Mode Polarization and Temperature-E-Mode Correlation in the Cosmic Microwave Background from 100 Square Degrees of SPTpol Data

We present measurements of $E$-mode polarization and temperature-$E$-mode correlation in the cosmic microwave background (CMB) using data from the first season of observations with SPTpol, the polarization-sensitive receiver currently installed on the South Pole Telescope (SPT). The observations used in this work cover 100~\sqdeg\ of sky with arcminute resolution at $150\,$GHz. We report the $E$-mode angular auto-power spectrum ($EE$) and the temperature-$E$-mode angular cross-power spectrum ($TE$) over the multipole range $500 < \ell \leq5000$. These power spectra improve on previous measurements in the high-$\ell$ (small-scale) regime. We fit the combination of the SPTpol power spectra, data from \planck\, and previous SPT measurements with a six-parameter \LCDM cosmological model. We find that the best-fit parameters are consistent with previous results. The improvement in high-$\ell$ sensitivity over previous measurements leads to a significant improvement in the limit on polarized point-source power: after masking sources brighter than 50\,mJy in unpolarized flux at 150\,GHz, we find a 95\% confidence upper limit on unclustered point-source power in the $EE$ spectrum of $D_\ell = \ell (\ell+1) C_\ell / 2 π< 0.40 \ μ{\mbox{K}}^2$ at $\ell=3000$, indicating that future $EE$ measurements will not be limited by power from unclustered point sources in the multipole range $\ell < 3600$, and possibly much higher in $\ell.$

astro-ph.CO↗

arXiv2014

Exciton dynamics in WSe2 bilayers

We investigate exciton dynamics in 2H-WSe2 bilayers in time-resolved photoluminescence (PL) spectroscopy. Fast PL emission times are recorded for both the direct exciton with $τ_{D}$ ~ 3 ps and the indirect optical transition with $τ_{i}$ ~ 25 ps. For temperatures between 4 to 150 K $τ_{i}$ remains constant. Following polarized laser excitation, we observe for the direct exciton transition at the K point of the Brillouin zone efficient optical orientation and alignment during the short emission time $τ_{D}$. The evolution of the direct exciton polarization and intensity as a function of excitation laser energy is monitored in PL excitation (PLE) experiments.

cond-mat.mtrl-sci↗

arXiv2014

Charge tuning in [111] grown GaAs droplet quantum dots

We demonstrate charge tuning in strain free GaAs/AlGaAs quantum dots (QDs) grown by droplet epitaxy on a GaAs(111)A substrate. Application of a bias voltage allows the controlled charging of the QDs from $-3|e|$ to $+2|e|$. The resulting changes in QD emission energy and exciton fine-structure are recorded in micro-photoluminescence experiments at T=4K. We uncover the existence of excited valence and conduction states, in addition to the s-shell-like ground state. We record a second series of emission lines about 25meV above the charged exciton emission coming from excited charged excitons. For these excited interband transitions a negative diamagnetic shift of large amplitude is uncovered in longitudinal magnetic fields.

cond-mat.mes-hall↗

arXiv2014

Electron Spin Dephasing and Optical Pumping of Nuclear Spins in GaN

We have measured the donor-bound electron spin dynamics in cubic GaN by time-resolved Kerr rotation experiments. The ensemble electron spin dephasing time in this quantum dot like system characterized by a Bohr radius of 2.5 nm is of the order of 1.5 ns as a result of the interaction with the fluctuating nuclear spins. It increases drastically when an external magnetic field as small as 10 mT is applied. We extract a dispersion of the nuclear hyperfine field δBn $\sim$ 4 mT, in agreement with calculations. We also demonstrate for the first time in GaN based systems the optical pumping of nuclear spin yielding the build-up of a significant nuclear polarization.

cond-mat.mes-hall↗