arXiv subjects

G. Woltersdorf

Publications and source records attributed to G. Woltersdorf.

18 recordsLinked to original sources

arXiv2026

Observation of Ultrafast Coherent and Incoherent Spin Torques via Terahertz Spin-Hall Magnetoresistance

Spin Hall magnetoresistance (SMR) is a cornerstone effect in spintronics, enabling the electrical readout of magnetic states through spin-orbit coupling at interfaces. Despite its widespread use, experimental studies of SMR are limited to static (DC) or low-frequency (GHz) regimes, leaving the ultrafast dynamics of interfacial spin transport in the terahertz (THz) frequency window entirely unexplored. Here, we report the observation of SMR spanning from DC to 1.5 THz in the model SMR system YIG/Pt, bridging the divide between electronic transport and THz optics. We demonstrate that the SMR response exhibits a pronounced low-pass behavior, decreasing significantly with frequency and vanishing above 1.5 THz. Through a dynamic model, we reveal that this unexpected spectral decay arises from a fundamental competition between two distinct interfacial spin-magnetization coupling mechanisms: the frequency-independent coherent spin torque, and an incoherent torque mediated by thermal magnons. Our analysis shows that the reduced THz SMR signal reflects the nonzero response time of the magnon chemical potential, which facilitates the increased outflow of incoherent magnons through the interface at high frequencies. These results resolve the microscopic nature of spin-torque generation at ultrafast timescales. Crucially, this work establishes THz SMR as a powerful, non-contact methodology capable of probing spin-magnon coupling in magnetic thin films, providing the essential tool for advancing the next generation of spintronic devices, particularly those based on high-frequency antiferromagnets and emerging altermagnetic materials.

cond-mat.mes-hall↗

arXiv2026

Magneto-optical evidence for single-crystal-like magnetic switching of epitaxial antiferromagnetic LaFeO3 films

Strained epitaxial films of the antiferromagnetic orthoferrite LaFeO3 offer a promising platform for antiferromagnetic spintronics, yet their magnetic switching behavior and domain structure have remained largely unexplored due to the small magnitude of the weak ferromagnetic moment. Here, we demonstrate that longitudinal magneto-optical Kerr effect (MOKE) measurements provide a sensitive and direct probe of magnetic switching and domain processes in coherently strained LaFeO3 thin films grown on orthorhombic substrates. By employing DyScO3(110), GdScO3(110), and NdGaO3(110) substrates, we achieve straincontrolled, largely twin-free growth and identify the orientation of the orthorhombic c-axis through the presence or absence of a longitudinal MOKE signal. Compressively strained films exhibit large Kerr signals, rectangular hysteresis loops, and magnetic single-domain remanence over macroscopic areas. Tensile strain on orthorhombic substrates is associated with two competing structural effects on thin film orientation; in-plane magnetization has been identified in some films on GdScO3(110) by MOKE. Angle-dependent MOKE hysteresis follows the Kondorsky model, indicating domain-wall-controlled switching analogous to bulk single crystals. Kerr microscopy reveals abrupt domain nucleation and rapid domain-wall motion, with defects acting as pinning centers and governing the coercive field. Our results establish MOKE as an efficient optical tool for identifying orthorhombic orientation, probing magnetic switching of coupled weak magnetization and Neel vectors, and accessing domain dynamics in LaFeO3 films. This provides a foundation for strain-engineered orthoferrite thin films in antiferromagnetic spintronics and magnonics.

cond-mat.mtrl-sci↗

arXiv2024

Laser patterning of magnonic structure via local crystallization of Yittrium Iron Garnet

The fabrication and integration of high-quality structures of Yttrium Iron Garnet (YIG) is critical for magnonics.Films with excellent properties are obtained only on single crystal Gadolinium Gallium Garnet (GGG) substrates using high-temperature processes. The subsequent realization of magnonic structures via lithography and etching is not straightforward as it requires a tight control of the edge roughness, to avoid magnon scattering, and planarization in case of multilayer devices. In this work we describe a different approach based on local laser annealing of amorphous YIG films, avoiding the need for subjecting the entire sample to high thermal budgets and for physical etching. Starting from amorphous and paramagnetic YIG films grown by pulsed laser deposition at room temperature on GGG, a 405 nm laser is used for patterning arbitrary shaped ferrimagnetic structures by local crystallization. In thick films (160 nm) the laser induced surface corrugation prevents the propagation of spin-wave modes in patterned conduits. For thinner films (80 nm) coherent propagation is observed in 1.2 micron wide conduits displaying an attenuation length of 5 micron which is compatible with a damping coefficient of about 5e-3. Possible routes to achieve damping coefficients compatible with state-of-the art epitaxial YIG films are discussed.

physics.app-ph↗

arXiv2023

Terahertz spin conductance probes of coherent and incoherent spin tunneling through MgO tunnel junctions

We study femtosecond spin currents through MgO tunneling barriers in CoFeB(2 nm)|MgO($d$)|Pt(2 nm) stacks by terahertz emission spectroscopy. To obtain transport information independent of extrinsic experimental factors, we determine the complex-valued spin conductance $\tilde{G}_d (ω)$ of the MgO layer (thickness d= 0-6 Å over a wide frequency range $(ω/2π=$ 0.5-8 THz). In the time $(t)$ domain,$ G_d (t)$ has an instantaneous and delayed component that point to (i) spin transport through Pt pinholes in MgO, (ii) coherent spin tunneling and (iii) incoherent resonant spin tunneling mediated by defect states in MgO. A remarkable signature of (iii) is its relaxation time that grows monotonically with $d$ to as much as 270 fs at $d= 6$ Å, in full agreement with an analytical model. Our results indicate that terahertz spin conductance spectroscopy will yield new and relevant insights into ultrafast spin transport for a wide range of materials.

physics.app-ph↗

arXiv2021

Spin transport-induced damping of coherent THz spin dynamics in iron

We study the damping of perpendicular standing spin-waves (PSSWs) in ultrathin Fe films at frequencies up to 2.4 THz. The PSSWs are excited by optically generated ultrashort spin current pulses, and probed optically in the time domain. Analyzing the wavenumber and thickness dependence of the damping, we demonstrate that at sufficiently large wave vectors $k$ the damping is dominated by spin transport effects scaling with k^4 and limiting the frequency range of observable PSSWs. Although this contribution is known to originate in the spin diffusion, we argue that at moderate and large k a more general description is necessary and develop a model where the 'transverse spin mean free path' is the a key parameter, and estimate it to be ~0.5 nm.

cond-mat.mes-hall↗

arXiv2021

Laser-induced terahertz spin transport in magnetic nanostructures arises from the same force as ultrafast demagnetization

Laser-induced terahertz spin transport (TST) and ultrafast demagnetization (UDM) are central but so far disconnected phenomena in femtomagnetism and terahertz spintronics. Here, we use broadband terahertz emission spectroscopy to reliably measure both processes in one setup. We find that the rate of UDM of a single ferromagnetic metal film F has the same time evolution as the flux of TST from F into an adjacent normal-metal layer N. This remarkable agreement shows that UDM and TST are driven by the same force, which is fully determined by the state of the ferromagnet. An analytical model consistently and quantitatively explains our observations. It reveals that both UDM in F and TST in the F|N stack arise from a generalized spin voltage, which is defined for arbitrary, nonthermal electron distributions. We also conclude that contributions due to a possible temperature difference between F and N are minor and that the spin-current amplitude can, in principle, be increased by one order of magnitude. In general, our findings allow one to apply the vast knowledge of UDM to TST, thereby opening up new pathways toward large-amplitude terahertz spin currents and, thus, energy-efficient ultrafast spintronic devices.

cond-mat.mes-hall↗

arXiv2020

Integration and characterization of micron-sized YIG structures with very low Gilbert damping on arbitrary substrates

We present a novel process that allows the transfer of monocrystalline yttrium-iron-garnet microstructures onto virtually any kind of substrate. The process is based on a recently developed method that allows the fabrication of freestanding monocrystalline YIG bridges on gadolinium-gallium-garnet. Here the bridges' spans are detached from the substrate by a dry etching process and immersed in a watery solution. Using drop casting the immersed YIG platelets can be transferred onto the substrate of choice, where the structures finally can be reattached and thus be integrated into complex devices or experimental geometries. Using time resolved scanning Kerr microscopy and inductively measured ferromagnetic resonance we can demonstrate that the structures retain their excellent magnetic quality. At room temperature we find a ferromagnetic resonance linewidth of $μ_0ΔH_{HWHM}\approx 195\,μT$ and we were even able to inductively measure magnon spectra on a single micron-sized yttrium-iron-garnet platelet at a temperature of 5 K. The process is flexible in terms of substrate material and shape of the structure. In the future this approach will allow for new types of spin dynamics experiments up to now unthinkable.

cond-mat.mes-hall↗

arXiv2019

Monocrystalline free standing 3D yttrium iron garnet magnon nano resonators

Nano resonators in which mechanical vibrations and spin waves can be coupled are an intriguing concept that can be used in quantum information processing to transfer information between different states of excitation. Until now, the fabrication of free standing magnetic nanostructures which host long lived spin wave excitatons and may be suitable as mechanical resonators seemed elusive. We demonstrate the fabrication of free standing monocrystalline yttrium iron garnet (YIG) 3D nanoresonators with nearly ideal magnetic properties. The freestanding 3D structures are obtained using a complex lithography process including room temperature deposition and lift-off of amorphous YIG and subsequent crystallization by annealing. The crystallization nucleates from the substrate and propagates across the structure even around bends over distances of several micrometers to form e.g. monocrystalline resonators as shown by transmission electron microscopy. Spin wave excitations in individual nanostructures are imaged by time resolved scanning Kerr microscopy. The narrow linewidth of the magnetic excitations indicates a Gilbert damping constant of only $α= 2.6 \times 10^{-4}$ rivalling the best values obtained for epitaxial YIG thin film material. The new fabrication process represents a leap forward in magnonics and magnon mechanics as it provides 3D YIG structures of unprecedented quality. At the same time it demonstrates a completely new route towards the fabrication of free standing crystalline nano structures which may be applicable also to other material systems.

cond-mat.mes-hall↗

arXiv2018

Magneto-optical properties of Au upon the injection of hot spin-polarized electrons across Fe/Au(001) interfaces

We demonstrate a novel method for the excitation of sizable magneto-optical effects in Au by means of the laser-induced injection of hot spin-polarized electrons in Au/Fe/MgO(001) heterostructures. It is based on the energy- and spin-dependent electron transmittance of Fe/Au interface which acts as a spin filter for non-thermalized electrons optically excited in Fe. We show that after crossing the interface, majority electrons propagate through the Au layer with the velocity on the order of 1 nm/fs (close to the Fermi velocity) and the decay length on the order of 100 nm. Featuring ultrafast functionality and requiring no strong external magnetic fields, spin injection results in a distinct magneto-optical response of Au. We develop a formalism based on the phase of the transient complex MOKE response and demonstrate its robustness in a plethora of experimental and theoretical MOKE studies on Au, including our ab initio calculations. Our work introduces a flexible tool to manipulate magneto-optical properties of metals on the femtosecond timescale that holds high potential for active magneto-photonics, plasmonics, and spintronics.

cond-mat.mes-hall↗

arXiv2018

Femtosecond formation dynamics of the spin Seebeck effect revealed by terahertz spectroscopy

Understanding the transfer of spin angular momentum is essential in modern magnetism research. A model case is the generation of magnons in magnetic insulators by heating an adjacent metal film. Here, we reveal the initial steps of this spin Seebeck effect with <27fs time resolution using terahertz spectroscopy on bilayers of ferrimagnetic yttrium-iron garnet and platinum. Upon exciting the metal with an infrared laser pulse, a spin Seebeck current $j_\textrm{s}$ arises on the same ~100fs time scale on which the metal electrons thermalize. This observation highlights that efficient spin transfer critically relies on carrier multiplication and is driven by conduction electrons scattering off the metal-insulator interface. Analytical modeling shows that the electrons' dynamics are almost instantaneously imprinted onto $j_\textrm{s}$ because their spins have a correlation time of only ~4fs and deflect the ferrimagnetic moments without inertia. Applications in material characterization, interface probing, spin-noise spectroscopy and terahertz spin pumping emerge.

cond-mat.mes-hall↗

arXiv2016

Observation of orbital two-channel Kondo effect in a ferromagnetic L10-MnGa film

The experimental existence and stability of the quantum criticality point of the two-channel Kondo (2CK) effect displaying exotic non-Fermi liquid physics has been buried in persistent confusion despite the intensive theoretical and experimental efforts in past three decades. Here we report an experimental realization of the two-level system scattering-induced orbital 2CK effect in a ferromagnetic L10-MnGa film, which is signified by a magnetic field-independent resistivity upturn that has a logarithmic and square-root temperature dependence beyond and below the Kondo temperature of ~14.5 K, respectively. Our result not only evidences the robust existence of orbital 2CK effect even in the presence of strong magnetic fields and long-range ferromagnetic ordering but also extends the scope of 2CK host materials from nonmagnetic nanoscale point contacts to diffusive conductors of disordered alloys.

cond-mat.str-el↗

arXiv2016

Composition-tuned magneto-optical Kerr effect in L10-MnxGa films with giant perpendicular anisotropy

We report the large polar magnetooptical Kerr effect in L10-MnxGa epitaxial films with giant perpendicular magnetic anisotropy in a wide composition range. The Kerr rotation was enhanced by a factor of up to 10 by decreasing Mn atomic concentration, which most likely arises from the variation of the effective spin-orbit coupling strength, compensation effect of magnetic moments at different Mn atom sites, and overall strain. The Kerr ellipticity and the magnitude of the complex Kerr angle is found to have more complex composition-dependence that varies with the photon energy. These L10-MnxGa films show large Kerr rotation of up to 0.10o, high reflectivity of 35%-55% in a wide wavelength range of 400~850 nm, and giant magnetic anisotropic field of up to 210 kOe, making them an interesting material system for emerging spintronics and terahertz modulator applications.

cond-mat.mtrl-sci↗

arXiv2016

Extremely Nonperturbative Nonlinearities in GaAs Driven by Atomically Strong Terahertz Fields in Gold Metamaterials

Terahertz near fields of gold metamaterials resonant at a frequency of $0.88\,\rm THz$ allow us to enter an extreme limit of non-perturbative ultrafast THz electronics: Fields reaching a ponderomotive energy in the keV range are exploited to drive nondestructive, quasi-static interband tunneling and impact ionization in undoped bulk GaAs, injecting electron-hole plasmas with densities in excess of $10^{19}\,\rm cm^{-3}$. This process causes bright luminescence at energies up to $0.5\,\rm eV$ above the band gap and induces a complete switch-off of the metamaterial resonance accompanied by self-amplitude modulation of transmitted few-cycle THz transients. Our results pave the way towards highly nonlinear THz optics and optoelectronic nanocircuitry with sub-picosecond switching times.

physics.optics↗

arXiv2013

Inverse Spin Hall Effect in NiFe / Normal Metal Bilayers

Spin pumping in ferromagnets provides a source of pure spin currents. Via the inverse spin Hall effect a spin current is converted into a charge current and a corresponding detectable DC-voltage. The ratio of injected spin current to resulting charge current is given by the spin Hall angle. However, the number of experiments more or less equals the number of different values for spin Hall angles, even for the most studied normal metal platinum. This publication provides a full study of inverse spin Hall effect and anisotropic magnetoresistance for different NiFe(Py) / normal metal bilayers using a coplanar waveguide structure. Angle and frequency dependent measurements strongly suggest that spin pumping and inverse spin Hall effect can be used to quantify spin Hall angles only if certain conditions are met. Ruling out the anisotropic magnetoresistance as a parasitic voltage generating effect measurements of the inverse spin Hall effect in Py/Pt and Py/Au yield spin Hall angles of 0.09 and 0.008 respectively. Furthermore, DC-voltages at ferromagnetic resonance for Py/Pt are studied as a function of temperature and the results are compared to theoretical models.

cond-mat.mes-hall↗

arXiv2013

First-principles calculation of the Gilbert damping parameter via the linear response formalism with application to magnetic transition-metals and alloys

A method for the calculations of the Gilbert damping parameter $α$ is presented, which based on the linear response formalism, has been implemented within the fully relativistic Korringa-Kohn-Rostoker band structure method in combination with the coherent potential approximation alloy theory. To account for thermal displacements of atoms as a scattering mechanism, an alloy-analogy model is introduced. This allows the determination of $α$ for various types of materials, such as elemental magnetic systems and ordered magnetic compounds at finite temperature, as well as for disordered magnetic alloys at $T = 0$ K and above. The effects of spin-orbit coupling, chemical and temperature induced structural disorder are analyzed. Calculations have been performed for the 3$d$ transition-metals bcc Fe, hcp Co, and fcc Ni, their binary alloys bcc Fe$_{1-x}$Co$_{x}$, fcc Ni$_{1-x}$Fe$_x$, fcc Ni$_{1-x}$Co$_x$ and bcc Fe$_{1-x}$V$_{x}$, and for 5d impurities in transition-metal alloys. All results are in satisfying agreement with experiment.

cond-mat.other↗

arXiv2009

Damping by slow relaxing rare earth impurities in Ni80Fe20

Doping NiFe by heavy rare earth atoms alters the magnetic relaxation properties of this material drastically. We show that this effect can be well explained by the slow relaxing impurity mechanism. This process is a consequence of the anisotropy of the on site exchange interaction between the 4f magnetic moments and the conduction band. As expected from this model the magnitude of the damping effect scales with the anisotropy of the exchange interaction and increases by an order of magnitude at low temperatures. In addition our measurements allow us to determine the relaxation time of the 4f electrons as a function of temperature.

cond-mat.mtrl-sci↗

arXiv2009

X-ray imaging of the dynamic magnetic vortex core deformation

Magnetic platelets with a vortex configuration are attracting considerable attention. The discovery that excitation with small in-plane magnetic fields or spin polarised currents can switch the polarisation of the vortex core did not only open the possibility of using such systems in magnetic memories, but also initiated the fundamental investigation of the core switching mechanism itself. Micromagnetic models predict that the switching is mediated by a vortex-antivortex pair, nucleated in a dynamically induced vortex core deformation. In the same theoretical framework, a critical core velocity is predicted, above which switching occurs. Although these models are extensively studied and generally accepted, experimental support has been lacking until now. In this work, we have used high-resolution time-resolved X-ray microscopy to study the detailed dynamics in vortex structures. We could reveal the dynamic vortex core deformation preceding the core switching. Also, the threshold velocity could be measured, giving quantitative comparison with micromagnetic models.

cond-mat.other↗

arXiv2008

Polarisation selective magnetic vortex dynamics and core reversal in rotating magnetic fields

A magnetic vortex occurs as an equilibrium configuration in thin ferromagnetic platelets of micron and sub-micron size and is characterised by an in-plane curling magnetisation. At the centre, a magnetic singularity is avoided by an out-of-plane magnetisation core. This core has a gyrotropic excitation mode, which corresponds to a circular motion of the vortex around its equilibrium position, where the rotation sense is determined by the direction of the vortex core magnetisation, its polarisation. Unlike linear fields or spin polarised currents, which excite both polarisation states, an in-plane rotating field can selectively excite one of the polarisation states. Here we report the observation of vortex dynamics in response to rotating magnetic fields, imaged with time-resolved scanning X-ray microscopy. We demonstrate that the rotating field only excites the gyrotropic mode if the rotation sense of the field coincides with the vortex gyration sense and that such a field can selectively reverse the vortex polarisation.

cond-mat.other↗