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Gabriel Molina-Terriza

Publications and source records attributed to Gabriel Molina-Terriza.

At least 19 recordsLinked to original sources

Upper bound to optical forces through the multipolar control of optical beams

Optical tweezers enable the manipulation of microscopic objects using light, yet the fundamental limits to the optical forces that can be exerted on matter remain unknown. Here we derive a general upper bound to the maximum optical force that can be applied to a particle, based on an expansion of electromagnetic fields into well-defined helicity multipolar modes. This method finds the optimal force for any kind of fields external to the particle, including evanescent fields. We apply the method to homogeneous spherical particles in a stable trap and identify the field distributions that saturate this bound for the trapping stiffness. We further provide experimentally accessible strategies to approach these optimal conditions, including configurations using counterpropagating and single-beam traps. Experiments demonstrate a threefold enhancement of trapping forces relative to conventional designs, while theoretical predictions indicate that order-of-magnitude improvements are achievable for larger particles and high angular momentum beams. Our results establish fundamental design principles for maximizing optical forces and define the ultimate limits of optical manipulation.

physics.optics↗

Controlling the centre of mass motion of levitated particles using structured wavefronts

Optically levitated particles have great potential to form the basis of novel quantum- enhanced sensors. These systems are very well suited for inertial sensing, as the particles are isolated from the environment when they are levitated at low pressures. However, there are many challenges in the experimental realization that may affect the performance of these systems. For example, optical aberrations in the wavefront of the trapping laser which arise from optical elements or misalignment have a great impact on the trapping potential. The detrimental effect of optical aberrations has not been thoroughly studied, and usually they are iteratively corrected, giving some conflicting results depending on the figures of merit that are used. In this work, we present a thorough study of the effects of structuring the wavefront of the trapping beams. We observe that clean beams, i.e. highly focused beams with unaberrated wavefronts, may be used to optimize the longitudinal frequencies, at the cost of the transversal ones. Our work is based in a combination of experimental studies using a complete basis of orthogonal polynomials (Zernike polynomials) to control the wavefront and a set of numerical calculations, which allow us to compare the impact of structured wavefronts on the quality of traps for optically levitated particles in vacuum. This will have direct applications in quantum sensing and fundamental studies of quantum mechanics, as it allows the reduction of optical backaction and thermal decoherence of the particles.

physics.optics↗

Unconditional full vector magnetometry using spin selectivity in Nitrogen Vacancy centers in diamond

Quantum sensors based on nitrogen vacancy (NV) centers in diamond have been a central topic in the sensing community for more than a decade. The extraordinary properties at room temperature of the spin system in diamond have made it one of the most prominent quantum platforms for the development of commercial quantum sensors. In particular, the sensitivity of the electronic spin in NV centers has made diamond-based magnetic sensors of special interest for their potential application in medical, industrial or navigation solutions. However, the use of these sensors for universal vector magnetometry was constrained by the need for previous knowledge on the field being measured to fully exploit their benefits. In this work, we show a method to perform unconditional vector magnetometry without the need of external information on the magnetic field, based only on the spatial arrangement of the diamond and the microwave antenna combination. While previous NV-based vector magnetometry methods require partial knowledge of the magnetic field (e.g. a calibrated bias field), we exploit the possibilities of selecting particular directions of the spins in the diamond with elliptically polarized microwave fields. We prove that our method allows to estimate both magnitude and direction of external magnetic fields without further assumptions or constraints.

quant-ph↗

Squeezing-Enhanced Rotational Doppler Metrology

A rotating surface can induce a frequency shift in incident light by changing its angular momentum, a phenomenon known as the rotational Doppler effect. This effect provides a means to estimate the angular velocity of the rotating surface. In this work, we develop a continuous-variable quantum protocol for estimating the angular velocity of a rotating surface via the rotational Doppler effect. Our approach exploits squeezed and displaced Laguerre-Gaussian modes as quantum resources, which interact with a rotating metallic disc with surface roughness. The frequency shift induced by the rotational Doppler effect is then measured using a homodyne detection scheme. By analyzing the Fisher information, we demonstrate that the proposed squeezing-enhanced protocol achieves Heisenberg scaling in the ideal noiseless regime. Furthermore, we investigate the influence of noise and consider different surface models to assess their impact on the protocol's performance. While Heisenberg scaling is degraded in the presence of noise, we show that optimizing the energy allocation ratio between displacement and squeezing of the probe ensures that the quantum strategy consistently outperforms its classical counterpart.

quant-ph↗

Detection of Hybrid Optical Anapoles in Dielectric Microspheres

Nonradiating optical anapoles are special configurations of charge_current distributions that do not radiate. It was theoretically predicted that, for microspheres, electric and magnetic dipolar coefficients can simultaneously vanish by engineering the incident light, leading to the excitation of nonradiating hybrid optical anapoles. In this work, the experimental detection of hybrid optical anapoles in dielectric microspheres (TiO2) is reported using dual detection optical spectroscopy, developed to enable sequential measurement of forward and backward scattering under tightly_focused Gaussian beam (TFGB) illumination. The results show that the excitation of TiO2 microspheres (diameter, d approx. 1 um) under TFGB illumination leads to the appearance of scattering minima in both the forward and backward directions within specific wavelength ranges. These scattering minima are found to be due to vanishing electric and magnetic dipolar coefficients associated with hybrid optical anapoles. The ability to confine electromagnetic fields associated with hybrid optical anapoles can give rise to several novel optical phenomena and applications.

physics.optics↗

Characterizing the Backscattered Spectrum of Mie Spheres

This study describes both experimentally and theoretically an important hitherto undiscovered feature of the scattering of micron_sized spherical objects when illuminated with highly focused circularly polarized light. This is a regime of high experimental relevance which has not been described in full detail. The experiments are complemented with the analytical formulas explaining the field scattered directed toward the backward hemispace. In particular, it is proven that this field shows a very regular oscillatory dependency with the optical size. This phenomenon is typically hidden in the total scattered field, as the field is scattered much less toward the backward hemisphere than toward the forward one. These regular oscillations are measured experimentally. It is proven that, by analyzing them, it is possible to determine the index of refraction of isolated micron_sized particles, opening new paths for applications in sensing and metrology.

physics.optics↗

Optical forces, helicity, angular momentum and how they are all intertwined

The theoretical description of optical forces and torques on micron_sized particles is a crucial area of research and has formed the foundation for advancements in optical trapping and manipulation technologies. In this study, we derive analytical expressions for optical forces and torques on micron_sized spherical particles illuminated by focused Laguerre_Gaussian (LG) beams, employing the well_defined helicity multipolar decomposition of electromagnetic fields and Mie theory. We developed a multifunctional program, Multipolar Optical Forces Toolbox, based on this theoretical framework. The program, available on GitHub, was used to generate optical trapping stability maps. These maps predict trap stability across a wide range of system parameters and serve as a practical tool for designing advanced optical trapping experiments. Our analysis reveals the important role of helicity p and orbital angular momentum l on the dynamics of particles trapped off_axis in LG beams and demonstrates the unique nature of the tangential torque. Our findings also highlight notable differences in longitudinal optical forces resulting from pure helicity modifications in Gaussian beams. Furthermore, we showcase the ability of LG beams to isolate Mie resonances, offering a novel approach to locate the spectral positions of the resonances of high multipolar modes. These insights deepen the understanding of helicity in LG optical traps and pave the way for the development of more advanced optical manipulation techniques.

physics.optics↗

On-Axis Optical Trapping with Vortex Beams: The Role of the Multipolar Decomposition

Optical trapping is a well_established, decades old technology with applications in several fields of research. The most common scenario deals with particles that tend to be centered on the brightest part of the optical trap. Consequently, the optical forces keep the particle away from the dark zones of the beam. However, this is not the case when a focused doughnut_shaped beam generates on_axis trapping. In this system, the particle is centered on the intensity minima of the laser beam and the bright annular part lies on the periphery of the particle. Researchers have shown great interest in this phenomenon due to its advantage of reducing light interaction with trapped particles and the intriguing increase in the trapping strength. This work presents experimental and theoretical results that extend the analysis of on_axis trapping with light vortex beams. Specifically, in our experiments, we trap micron_sized spherical silica (SiO2) particles in water and we measure, through the power spectrum density method, the trap stiffness constant \k{appa} generated by vortex beams with different topological charge orders. The optical forces are calculated from the exact solutions of the electromagnetic fields provided by the generalized Lorentz_Mie theory. We show a remarkable agreement between the theoretical prediction and the experimental measurements of \k{appa}. Moreover, our numerical model gives us information about the electromagnetic fields inside the particle, offering valuable insights into the influence of the electromagnetic fields present in the vortex beam trapping scenario.

physics.optics↗

Lorentz invariant materials and metamaterials

We show that electromagnetic constitutive relations of materials, defined by a scalar permittivity, $\varepsilon$, and permeability, $μ$, are the same for all inertial observers provided that $\varepsilonμ= 1$ is satisfied. To highlight the practical power of our general result, we discuss schemes in which this property plays a significant role, such as Fresnel-Fizeau optical drag or modified Snell's law for moving dielectrics. We also proof that such a particular behavior can be extended to systems like uniaxial anisotropic media or negative refractive index metamaterials.

physics.optics↗

Quantum-inspired clustering with light

This article introduces a novel approach to perform the simulation of a single qubit quantum algorithm using laser beams. Leveraging the polarization states of photonic qubits, and inspired by variational quantum eigensolvers, we develop a variational quantum algorithm implementing a clustering procedure following the approach proposed by some of us in SciRep 13, 13284 (2023). A key aspect of our research involves the utilization of non-orthogonal states within the photonic domain, harnessing the potential of polarization schemes to reproduce unitary circuits. By mapping these non-orthogonal states into polarization states, we achieve an efficient and versatile quantum information processing unit which serves as a clustering device for a diverse set of datasets.

quant-ph↗

Versatile quadrature antenna for precise control of large electron spin ensembles in diamond

We present an easily reproducible inexpensive microwave antenna that can generate a strong and homogeneous magnetic field of arbitrary polarization, which enables fast and coherent control of electron spins over a large volume. Unlike preceding works, we present a resonant antenna that maintains its resonant behaviour regardless of the proximity of other experimental hardware components. This robustness is crucial as it enables, amongst others, using microscope objectives with short working distances to perform wide field imaging/sensing with bulk diamonds. The antenna generates a magnetic field strength of 22.3 A/m for 1 W total driving power, which doubles the power efficiency compared with previously reported patch antenna designs. The magnetic field homogeneity in a volume of $0.3 \text{mm}^3$, $0.5 \text{mm}^3$ and $1 \text{mm}^3$ is within 6\%, 8\% and 13\%, respectively. The antenna has a full width at half maximum bandwidth of $\sim$160 MHz and its resonant frequency can be tuned over a 400 MHz range via four capacitors or varactors. The antenna has been tested and found to remain within safe handling temperatures during continuous-wave operation at 8 W. The files required to reproduce this antenna, which can be built on a standard and affordable double sided PCB, are provided open-source. This work facilitates a robust and versatile piece of instrumentation, being particularly appealing for applications such as high sensitivity magnetometry and wide field imaging/sensing with Nitrogen Vacancy centers.

physics.ins-det↗

Towards a realistic setup for a dynamical measurement of deviations from Newton's $1/r^2$ law: the impact of air viscosity

A novel experimental setup to measure deviations from the $1/r^2$ distance dependence of Newtonian gravity was proposed in arXiv:1609.05654. The underlying theoretical idea was to study the orbits of a microscopically-sized planetary system composed of a ``Satellite'', with mass $m_{\rm S} \sim {\cal O}(10^{-9})$ g, and a ``Planet'', with mass $M_{\rm P} \sim {\cal O} (10^{-5}) $ g at an initial distance of hundreds of microns. The detection of precession of the orbit in this system would be an unambiguous indication of a central potential with terms that scale with the distance differently from $1/r$. This is a huge advantage with respect to the measurement of the absolute strength of the attraction between two bodies, as most electrically-induced background potentials do indeed scale as $1/r$. Detection of orbit precession is unaffected by these effects, allowing for better sensitivities. In arXiv:2106.08611, the impact of other subleading backgrounds that may induce orbit precession, such as, {\em e.g.}, the electrical Casimir force or general relativity, was studied in detail. It was found that the proposed setup could test Yukawa-like corrections, $α\times \exp(-r/λ)$, to the $1/r$ potential with couplings as low as $α\sim 10^{-2}$ for distances as small as $λ\sim 10$ $μ$m, improving by roughly an order of magnitude present bounds. In this paper, we start to move from a theoretical study of the proposal to a more realistic implementation of the experimental setup. As a first step, we study the impact of air viscosity on the proposed setup and see how the setup should be modified in order to preserve the theoretical sensitivity achieved in our previous works.

hep-ph↗

On the origin of the Kerker phenomena

We provide an insight into the origin of the phenomena reported 40 years ago by Kerker, Wang and Giles (Journal of the Optical Society of America, 73, 6, pp. 765-767, (1983)). We show that the impedance and refractive index matching conditions, discussed in Sections II and IV of the seminal paper, are intimately related with space-time symmetries. We derive our results starting from the theory of representations of the Poincaré group, as it is the theory on which one of the most elemental descriptions of electromagnetic waves is based. We show that fundamental features of electromagnetic waves in material environments can be derived from group theoretical arguments. In particular, we identify the Casimir invariants of $P_{\scriptscriptstyle{3,1}}$ subgroup as the magnitudes which describe the nature of monochromatic electromagnetic waves propagating in matter. Finally, we show that the emergence of the Kerker phenomena is associated with the conservation of such Casimir invariants in piecewise homogeneous media.

physics.optics↗

Characterizing cylindrical particles upon local measurements of two Stokes parameters

Researchers routinely characterize optical samples by computing the scattering cross-section. However, the experimental determination of this magnitude requires the measurement and integration of the components of the scattered field in all directions. Here, we propose a method to determine the scattering cross-section and global polarization state of radiation through measurements of two Stokes parameters at an angle of choice in far-field. The method applies to cylindrically symmetric samples whose optical response is well-described by a single multipolar order j. Moreover, the formalism is applicable for a wide range of different illuminations, and it only requires the use of a single camera and conventional wave plates. Our findings significantly reduce the complexity of routine characterization measurements for cylindrical samples in optical laboratories.

physics.optics↗

Spheres of maximum electromagnetic chirality

The search for objects that yield maximum electromagnetic chirality in their emitted wavefield has garnered significant attention in recent years. However, achieving such maximum chirality is challenging, as it typically requires complex chiral metamaterials. Here we demonstrate that chiral spheres can yield maximum chirality in their emitted wavefield. Specifically, we analytically find the spectral trajectories at which chiral spheres become optically transparent to a given helicity of the incident field, while for its opposite helicity, they behave as dual objects, i.e., on scattering, they preserve helicity. Since chiral spheres behave as dual objects at the first Kerker condition of zero backscattering, we significantly simplify this condition in terms of a Riccati-Bessel function. Importantly, all our results are exact and applicable regardless of the multipolar order, refractive index contrast, optical size, and intrinsic chirality of the chiral sphere. Thus, our exact findings can serve as building blocks for designing novel metasurfaces or metamaterials with maximum electromagnetic chirality properties.

physics.optics↗

Resonant helicity mixing of electromagnetic waves propagating through matter

Dual scatterers preserve the helicity of an incident field, whereas antidual scatterers flip it completely. In this setting of linear electromagnetic scattering theory, we provide a completely general proof on the non-existence of passive antidual scatterers. However, we show that scatterers fulfilling the refractive index matching condition flip the helicity of the fields very efficiently without being in contradiction with the law of energy conservation. Moreover, we find that this condition is paired with the impedance matching condition in several contexts of electromagnetism and, in particular, within Fresnel's and Mie's scattering problems. Finally, we show that index-matched media induce a resonant helicity mixing on the propagating electromagnetic waves. We reach to this conclusion by identifying that the refractive index matching condition leads to the phenomenon of avoided level-crossing. Our contribution not only closes a historical discussion within the Nanophotonics community, but also opens up new possibilities in the fields of Metamaterials and Particle Physics.

physics.optics↗

Capturing near-field circular dichroism enhancements from far-field measurements

Molecular Circular dichroism (CD) spectroscopy faces significant limitations due to the inherent weakness of chiroptical light-matter interactions. In this view, resonant optical antennas constitute a promising solution to this problem since they can be tuned to increase the CD enhancement factor, fCD, a magnitude describing the electromagnetic near-field enhancement of scatterers associated with a given helicity. Here, we derive an exact multipolar expansion of fCD, which is valid to deduce the integrated near-field CD enhancements of chiral molecules in the presence of scatterers of any size and shape under general illumination conditions. Based on our analytical findings, we show that the near-field fCD factor can be related to magnitudes that can be computed in the far-field, i.e., the scattering cross-section and the helicity expectation value. Moreover, we show that in the case of lossless cylindrically symmetric samples, the near-field fCD factor can be inferred experimentally only from two far-field measurements at specific scattering angles. Our contribution paves the way for the experimental characterization of devices capable of enhancing molecular CD spectroscopy.

physics.optics↗

Preservation and destruction of the purity of two-photon states in the interaction with a nanoscatterer

The optical resonances supported by nanostructures offer the possibility to enhance the interaction between matter and the quantum states of light. In this work, we provide a framework to study the scattering of quantum states of light with information encoded in their helicity by a nanostructure. We analyze the purity of the scattered output quantum state, and we find that the purity of the incident state can be lost, when it interacts with the optical resonances of the nanostructure. To explain the loss of quantum purity, we develop a physical picture based on time delays and frequency shifts between the output two-photon modes. The framework and analysis proposed in this work establishes a tool to address the interaction between quantum light and nanoenvironments.

quant-ph↗