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Galien Grosjean

Publications and source records attributed to Galien Grosjean.

14 recordsLinked to original sources

Asymmetries in triboelectric charging: generalizing mosaic models to different-material samples and sliding contacts

Nominally identical materials exchange net electric charge during contact through a mechanism that is still debated. `Mosaic models', in which surfaces are presumed to consist of a random patchwork of microscopic donor/acceptor sites, offer an appealing explanation for this phenomenon. However, recent experiments have shown that global differences persist even between same-material samples, which the standard mosaic framework does not account for. Here, we expand the mosaic framework by incorporating global differences in the densities of donor/acceptor sites. We develop an analytical model, backed by numerical simulations, that smoothly connects the global and deterministic charge transfer of different materials to the local and stochastic mosaic picture normally associated with identical materials. Going further, we extend our model to explain the effect of contact asymmetries during sliding, providing a plausible explanation for reversal of charging sign that has been observed experimentally.

cond-mat.soft

Single-collision statistics reveal a global mechanism driven by sample history for contact electrification in granular media

Models for same-material contact electrification in granular media often rely on a local charge-driving parameter whose spatial variations lead to a stochastic origin for charge exchange. Measuring the charge transfer from individual granular spheres after contacts with substrates of the same material, we find that the charge-driving parameter is global, not local. Cleaning and baking samples fully resets their charging behavior, which indicates the underlying global parameter is not intrinsic to the material, but acquired from its history. Charging behavior is randomly and irreversibly affected by changes in relative humidity, pointing to a mechanism where adsorbates, in particular water, are fundamental to the charge-transfer process.

cond-mat.soft

Magnetically powered metachronal waves induce locomotion in self-assemblies

When tiny soft ferromagnetic particles are placed along a liquid interface and exposed to a vertical magnetic field, the balance between capillary attraction and magnetic repulsion leads to self-organization into well-defined patterns. Here, we demonstrate experimentally that precessing magnetic fields induce metachronal waves on the periphery of these assemblies, similar to the ones observed in ciliates and some arthropods. The outermost layer of particles behaves like an array of cilia or legs whose sequential movement causes a net and controllable locomotion. This bioinspired many-particle swimming strategy is effective even at low Reynolds number, using only spatially uniform fields to generate the waves.

cond-mat.soft

Regimes of motion of magnetocapillary swimmers

The dynamics of a triangular magnetocapillary swimmer is studied using the lattice Boltzmann method. Performing extensive numerical simulations taking into account the coupled dynamics of the fluid-fluid interface and of magnetic particles floating on it and driven by external magnetic fields we identify several regimes of the swimmer motion. In the regime of high frequencies the swimmer's maximum velocity is centered around the particle's inverse coasting time. Modifying the ratio of surface tension and magnetic forces allows to study the swimmer propagation in the regime of significantly lower frequencies mainly defined by the strength of the magnetocapillary potential. Finally, introducing a constant magnetic contribution in each of the particles in addition to their magnetic moment induced by external fields leads to another regime characterised by strong in-plane swimmer reorientations that resemble experimental observations.

cond-mat.soft

Quantitatively consistent, scale-spanning model for same-material tribocharging

By rigorously accounting for mesoscale spatial correlations in donor/acceptor surface properties, we develop a scale-spanning model for same-material tribocharging. We find that mesoscale correlations affect not only the magnitude of charge transfer but also the fluctuations-suppressing otherwise overwhelming charge-transfer variability that is not observed experimentally. We furthermore propose a generic theoretical mechanism by which the mesoscale features might emerge, which is qualitatively consistent with other proposals in the literature.

cond-mat.soft

Capillary assemblies in a rotating magnetic field

Small objects floating on a fluid have a tendency to aggregate due to capillary forces. This effect has been used, with the help of a magnetic induction field, to assemble submillimeter metallic spheres into a variety of structures, whose shape and size can be tuned. Under time-varying fields, these assemblies can propel themselves due to a breaking of time reversal symmetry in their adopted shapes. In this article, we study the influence of an in-plane rotation of the magnetic field on these structures. Various rotational modes have been observed with different underlying mechanisms. The magnetic properties of the particles cause them to rotate individually. Dipole-dipole interactions in the assembly can cause the whole structure to align with the field. Finally, non-reciprocal deformations can power the rotation of the assembly. Symmetry plays an important role in the dynamics, as well as the frequency and amplitude of the applied field. Understanding the interplay of these effects is essential, both to explain previous observations and to develop new functions for these assemblies.

cond-mat.soft

Wave turbulence on the surface of a fluid in a high-gravity environment

We report on the observation of gravity-capillary wave turbulence on the surface of a fluid in a high-gravity environment. By using a large-diameter centrifuge, the effective gravity acceleration is tuned up to 20 times the Earth gravity. The transition frequency between the gravity and capillary regimes is thus increased up to one decade as predicted theoretically. A frequency power-law wave spectrum is observed in each regime and is found to be independent of the gravity level and of the wave steepness. While the timescale separation required by weak turbulence is well verified experimentally regardless of the gravity level, the nonlinear and dissipation timescales are found to be independent of the scale, as a result of the finite size effects of the system (large-scale container modes) that are not taken currently into account theoretically.

physics.flu-dyn

Optimal motion of triangular magnetocapillary swimmers

A system of ferromagnetic particles trapped at a liquid-liquid interface and subjected to a set of magnetic fields (magnetocapillary swimmers) is studied numerically using a hybrid method combining the pseudopotential lattice Boltzmann method and the discrete element method. After investigating the equilibrium properties of a single, two and three particles at the interface, we demonstrate a controlled motion of the swimmer formed by three particles. It shows a sharp dependence of the average center-of-mass speed on the frequency of the time-dependent external magnetic field. Inspired by experiments on magnetocapillary microswimmers, we interpret the obtained maxima of the swimmer speed by the optimal frequency centered around the characteristic relaxation time of a spherical particle. It is also shown that the frequency corresponding to the maximum speed grows and the maximum average speed decreases with increasing inter-particle distances at moderate swimmer sizes. The findings of our lattice Boltzmann simulations are supported by bead-spring model calculations.

cond-mat.soft

Surface microswimmers, harnessing the interface to self-propel

In the study of microscopic flows, self-propulsion has been particularly topical in recent years, with the rise of miniature artificial swimmers as a new tool for flow control, low Reynolds number mixing, micromanipulation or even drug delivery. It is possible to take advantage of interfacial physics to propel these micro-robots, as demonstrated by recent experiments using the proximity of an interface, or the interface itself, to generate propulsion at low Reynolds number. This paper discusses how a nearby interface can provide the symmetry breaking necessary for propulsion. An overview of recent experiments illustrates how forces at the interface can be used to generate locomotion. This paper then presents original results concerning two systems. The first is composed of floating ferromagnetic spheres that assemble through capillarity into swimming structures. The second system, also powered by a magnetic field, is a centimeter-sized piece that swims similarly to water striders.

physics.flu-dyn

Magnetocapillary self-assemblies: locomotion and micromanipulation along a liquid interface

This paper presents an overview and discussion of magnetocapillary self-assemblies. New results are presented, in particular concerning the possible development of future applications. These self-organizing structures possess the notable ability to move along an interface when powered by an oscillatory, uniform magnetic field. The system is constructed as follows. Soft magnetic particles are placed on a liquid interface, and submitted to a magnetic induction field. An attractive force due to the curvature of the interface around the particles competes with an interaction between magnetic dipoles. Ordered structures can spontaneously emerge from these conditions. Furthermore, time-dependent magnetic fields can produce a wide range of dynamic behaviours, including non-time-reversible deformation sequences that produce translational motion at low Reynolds number. In other words, due to a spontaneous breaking of time-reversal symmetry, the assembly can turn into a surface microswimmer. Trajectories have been shown to be precisely controllable. As a consequence, this system offers a way to produce microrobots able to perform different tasks. This is illustrated in this paper by the capture, transport and release of a floating cargo, and the controlled mixing of fluids at low Reynolds number.

physics.flu-dyn

Realization of the Najafi-Golestanian microswimmer

A paradigmatic microswimmer is the three-linked-spheres model, which follows a minimalist approach for propulsion by shape shifting. As such, it has been the subject of numerous analytical and numerical studies. In this Rapid Communication, an experimental three-linked-spheres swimmer is created by self-assembling ferromagnetic particles at an air-water interface. It is powered by a uniform oscillating magnetic field. A model, using two harmonic oscillators, reproduces the experimental findings. Because the model remains general, the same approach could be used to design a variety of efficient microswimmers.

cond-mat.soft

Statics and dynamics of magnetocapillary bonds

When ferromagnetic particles are suspended at an interface under magnetic fields, dipole-dipole interactions compete with capillary attraction. This combination of forces has recently given promising results towards controllable self-assemblies, as well as low Reynolds swimming systems. The elementary unit of these assemblies is a pair of particles. Although equilibrium properties of this interaction are well described, dynamics remain unclear. In this letter, the properties of magnetocapillary bonds are determined by probing them with magnetic perturbations. Two deformation modes are evidenced and discussed. These modes exhibit resonances whose frequencies can be detuned to generate non-reciprocal motion. A model is proposed which can become the basis for elaborate collective behaviours.

cond-mat.soft

Remote control of self-assembled microswimmers

Physics governing the locomotion of microorganisms and other microsystems is dominated by viscous damping. An effective swimming strategy involves the non-reciprocal and periodic deformations of the considered body. Here, we show that a magnetocapillary-driven self-assembly, composed of three soft ferromagnetic beads, is able to swim along a liquid-air interface when powered by an external magnetic field. More importantly, we demonstrate that trajectories can be fully controlled, opening ways to explore low Reynolds number swimming. This magnetocapillary system spontaneously forms by self-assembly, allowing miniaturization and other possible applications such as cargo transport or solvent flows.

physics.flu-dyn

Magnetocapillary Swimmers

We present an experiment where three mesoscopic soft ferromagnetic beads are placed onto a liquid surface and submitted to the influence of magnetic fields. A vertical magnetic field creates a repulsion which counterbalances the capillary attraction. We show that the competition with a second, oscillating field, deforms the structure in a non reciprocal way. As a consequence, the structure is able to swim. This experiment is fully described in a fluid dynamics video attached to this submission.

physics.flu-dyn