arXiv subjects

Gang Su

Publications and source records attributed to Gang Su.

At least 37 records · Page 2Linked to original sources

arXiv2025

Diameter-Controlled High-Order Vortex States and Magnon Hybridization in VSe2 Nanotubes

Curved magnets offer a rich phase diagram and hold great promise for next-generation spintronic technologies. This study establishes the paramount significance of high-order vortex states (e.g., 3$φ$ with winding number $n$ > 1) in VSe2 nanotubes, which uniquely enable magnonic functionalities fundamentally inaccessible to conventional magnetic systems. These states arise from diameter-dependent competition between the nearest-neighbor ferromagnetic ($J_1$) and longer-range antiferromagnetic ($J_2$/$J_3$) couplings, as rigorously validated through density-functional theory calculations and Heisenberg modeling of phase diagrams. Critically, by the Landau-Lifshitz-Gilbert equation, we find that high-order vortex configurations unlock an intrinsic hybridization mechanism governed by strict orbital angular momentum (OAM) selection rules ($Δl = \pm 2(n-1)$) -- a process strictly forbidden in fundamental vortices ($n$ = 1) -- generating complex high-OAM magnons with measurable topological charge. This is vividly demonstrated in the 3$φ$ state, where hybridization between $l$ = -4, 0 and 4 modes produces eight-petal magnon density patterns. Such states provide an essential platform-free solution for generating high-OAM magnons, wchich is crucial for spin-wave-based information transport. These findings establish a predictive theoretical framework for controlling high-order vortex states in curved magnets and highlight VSe2 nanotubes as a promising platform for exploring complex magnetism and developing future magnonic and spintronic devices.

cond-mat.mtrl-sci↗

arXiv2025

Kitaev-derived Gapless Spin Liquid in the $K$-$J$-$Γ$-$Γ'$ Quantum Magnet Na$_2$Co$_2$TeO$_6$

The realization of quantum spin liquids (QSLs) in Kitaev magnets represents an intriguing topic in frustrated quantum magnetism. Despite prediction in the pure Kitaev honeycomb model, realization of QSLs in realistic systems and materials remain scarce. The recent discovery of cobalt-based compound Na$_2$Co$_2$TeO$_6$ has raised significant research interest. By establishing a realistic $K$-$J$-$Γ$-$Γ'$ model for Na$_2$Co$_2$TeO$_6$ -- with a dominant antiferromagnetic (AFM) Kitaev interaction ($K>0$) that quantitatively explains its thermodynamics measurements -- we reveal an intermediate gapless QSL phase under [111] magnetic fields with tensor-network calculations. We confirm the QSL nature of this phase by demonstrating its adiabatic connection to the intensively studied intermediate QSL of the pure AFM Kitaev model under out-of-plane fields. Our results show excellent agreement with recent high-field experiments, thereby explaining the intermediate-field phase in Na$_2$Co$_2$TeO$_6$. These findings bridge the gap between theoretical proposals for a Kitaev-derived QSL and experimental realization, opening new avenues for exploring exotic quantum states of matter in realistic Kitaev materials.

cond-mat.str-el↗

arXiv2025

Fishing for Answers: Exploring One-shot vs. Iterative Retrieval Strategies for Retrieval Augmented Generation

Retrieval-Augmented Generation (RAG) based on Large Language Models (LLMs) is a powerful solution to understand and query the industry's closed-source documents. However, basic RAG often struggles with complex QA tasks in legal and regulatory domains, particularly when dealing with numerous government documents. The top-$k$ strategy frequently misses golden chunks, leading to incomplete or inaccurate answers. To address these retrieval bottlenecks, we explore two strategies to improve evidence coverage and answer quality. The first is a One-SHOT retrieval method that adaptively selects chunks based on a token budget, allowing as much relevant content as possible to be included within the model's context window. Additionally, we design modules to further filter and refine the chunks. The second is an iterative retrieval strategy built on a Reasoning Agentic RAG framework, where a reasoning LLM dynamically issues search queries, evaluates retrieved results, and progressively refines the context over multiple turns. We identify query drift and retrieval laziness issues and further design two modules to tackle them. Through extensive experiments on a dataset of government documents, we aim to offer practical insights and guidance for real-world applications in legal and regulatory domains.

cs.IR↗

arXiv2025

Intercalation-Induced Near Room-Temperature Ferromagnetism in CrI3 via Synergistic Exchange Pathways

The development of room-temperature magnetic semiconductors is critical for advancing spintronic technologies, yet van der Waals magnets like CrI3 exhibit intrinsically low Curie temperatures (Tc = 45 K). This study employs first-principles calculations to demonstrate that atom intercalation, particularly lithium (Li), dramatically enhances magnetic exchange couplings in CrI3, achieving near room-temperature ferromagnetism with a predicted Tc of 286 K-aligning with experimental reports of 420 K. The underlying mechanism involves synergistic superexchange and double-exchange interactions: intercalation reduces the |Ep-Ed| energy difference between iodine p-orbitals and chromium d-orbitals, strengthening superexchange pathways, while charge transfer induces valence mixing (e.g., Cr3+ to Cr2+, as confirmed by experimental X-ray photoelectron spectrometry data), promoting double-exchange. Theoretical predictions extend to other intercalants including Cu and Na, with Cu0.25CrI3 and Na0.25CrI3 exhibiting Tc of 267 K and 247 K, respectively, establishing a versatile strategy for designing high-Tc magnetic semiconductors. This work bridges theoretical insights with experimental validation, offering a transferable framework for intercalation-driven material design and accelerating practical spintronic device realization.

cond-mat.mtrl-sci↗

arXiv2025

Universal Magnetocaloric Effect near Quantum Critical Point of Magnon Bose-Einstein Condensation

Bose-Einstein condensation (BEC), a macroscopic quantum phenomenon arising from phase coherence and bosonic statistics, has been realized in quantum magnets. Here, we report the observation of a universal magnetocaloric effect (MCE) near a BEC quantum critical point (QCP) in copper sulfate crystal ($CuSO_4 \cdot 5H_2O$). By conducting magnetocaloric and nuclear magnetic resonance measurements, we uncover a field-driven BEC QCP, evidenced by the universal scaling law $T_c \propto (B_c - B)^{2/3}$ and the perfect data collapse of the magnetic Grüneisen ratio. Thermal excitation triggers a dimensional crossover to a 1D quantum-critical regime, where the MCE scaling strictly matches the universality class of 1D Fermi gases. Notably, the quantum-critical MCE enables cooling down to 12.8 mK without helium-3, with very fast thermal relaxation rate that is critical for high cooling power. This work demonstrates the universal MCE in magnon BEC systems, using a common copper sulfate compound as a paradigmatic example, and paves the way for next-generation sub-Kelvin cooling.

cond-mat.str-el↗

arXiv2025

Hund's Rule, Interorbital Hybridization, and High-$T_c$ Superconductivity in the Bilayer Nickelate

Understanding the pairing mechanism in bilayer nickelate superconductors constitutes a fascinating quest. Here we investigate the intriguing interplay between Hund's rule coupling and interorbital hybridization in a two-orbital model for bilayer nickelates, using a comprehensive tensor network approach: density matrix renormalization group for finite-size systems, infinite projected entangled-pair states in the thermodynamic limit, and thermal tensor networks for finite-temperature properties. We explain the pressure-dependent high-$T_c$ superconductivity observed in experiment, by identifying three distinct superconductive (SC) regimes: hybridization dominant, Hund's rule dominant, and the hybrid-Hund synergistic SC regimes. In these SC regimes, both $d_{x^2-y^2}$ and $d_{z^2}$ orbitals exhibit algebraic pairing correlations with similar Luttinger parameters $K_{\mathrm{SC}}$. However, the former exhibits a much stronger amplitude than the latter, with a distinctly higher SC characteristic temperature $T_c^*$, below which the pairing susceptibility diverges as $χ_{\mathrm{SC}}(T) \sim 1/T^{2-K_{\mathrm{SC}}}$. With realistic model parameters, we find the pressurized La$_3$Ni$_2$O$_7$ falls into the Hund's rule dominated SC regime. As hybridization further enhances with pressure, it leads to significant interorbital frustration and in turn suppresses the SC correlations, explaining the rise and fall of high-$T_c$ superconductivity under high pressure. Our results offer a comprehensive understanding of the interlayer pairing in superconducting La$_3$Ni$_2$O$_7$.

cond-mat.str-el↗

arXiv2025

Electro-optic Kerr Effect Induced by Nonlinear Transport in monolayer WTe2

The nonlinear Hall effect (NLHE) can induce optical anisotropy by modifying a material's dielectric tensor, presenting opportunities for novel characterization and device applications. While the magneto-optical Kerr effect (MOKE) probes the linear Hall effect (LHE) in magnetic materials, an analogous optical probe for NLHE in non-magnetic, time-reversal symmetric systems remains highly desirable. Here, we theoretically propose and investigate an NLHE-induced Electro-optic Kerr Effect (EOKE) as such a probe. Focusing on monolayer (ML) WTe$_2$, a prototypical NLHE material, our analysis considers contributions from Berry curvature dipole (BCD), Drude, injection, and shift mechanisms. We demonstrate that the EOKE signal in WTe$_2$ is predominantly governed by the BCD. Furthermore, the Kerr angle exhibits temporal oscillations at different optical frequencies, suggesting EOKE as a promising route for the time-resolved detection of NLHE and the dynamic investigation of material topology.

cond-mat.other↗

arXiv2025

Reasoning RAG via System 1 or System 2: A Survey on Reasoning Agentic Retrieval-Augmented Generation for Industry Challenges

Retrieval-Augmented Generation (RAG) has emerged as a powerful framework to overcome the knowledge limitations of Large Language Models (LLMs) by integrating external retrieval with language generation. While early RAG systems based on static pipelines have shown effectiveness in well-structured tasks, they struggle in real-world scenarios requiring complex reasoning, dynamic retrieval, and multi-modal integration. To address these challenges, the field has shifted toward Reasoning Agentic RAG, a paradigm that embeds decision-making and adaptive tool use directly into the retrieval process. In this paper, we present a comprehensive review of Reasoning Agentic RAG methods, categorizing them into two primary systems: predefined reasoning, which follows fixed modular pipelines to boost reasoning, and agentic reasoning, where the model autonomously orchestrates tool interaction during inference. We analyze representative techniques under both paradigms, covering architectural design, reasoning strategies, and tool coordination. Finally, we discuss key research challenges and propose future directions to advance the flexibility, robustness, and applicability of reasoning agentic RAG systems. Our collection of the relevant research has been organized into a https://github.com/ByebyeMonica/Reasoning-Agentic-RAG.

cs.AI↗

arXiv2025

Ferroelectric control of bipolar magnetic semiconductor with room Curie temperature

The development of room-temperature tunable magnetic semiconductors is crucial for the advancement of low-power, high-performance information technologies. Using density functional theory calculations, we propose a series of two-dimensional magnetic semiconductors with critical temperature above room temperature, including three ferromagnetic and two antiferromagnetic semiconductors.Their stability is confirmed through phonon spectra, molecular dynamics simulations, and formation energy calculations. In particular, we demonstrate a ferromagnetic bipolar magnetic semiconductor (BMS), Cr2NiSe4, formed via Ni intercalation into bilayer CrSe2, which exhibits a 0.40 eV band gap and a Curie temperature of 352 K. Nonvolatile carrier spin polarization control in Cr2NiSe4 is achieved by switching the ferroelectric polarization of an Al2Se3 substrate. Switching the ferroelectric state of monolayer Al2Se3 induces a BMS-to-half-metal transition. Reversing the polarization of bilayer Al2Se3 yields a half-metallic Cr2NiSe4 with fully opposite carrier spin polarization. Furthermore, we propose a multiferroic nonvolatile memory design: write operations are controlled by the ferroelectric polarization state of bilayer Al2Se3, while read operations rely on detecting the distinct carrier spin polarizations of Cr2NiSe4. Our work reports a two dimensional BMS with Curie temperature above room temperature and presents a feasible strategy for its nonvolatile electrical control.

cond-mat.mtrl-sci↗

arXiv2025

Enhancement of temperature of quantum anomalous Hall effect in two-dimensional germanene/magnetic semiconductor heterostructures

Quantum anomalous Hall effect (QAHE) is significant for future low-power electronics devices, where a main challenge is realizing QAHE at high temperatures. In this work, based on experimentally reported two-dimensional (2D) germanene and magnetic semiconductors Cr$_2$Ge$_2$Te$_6$ and Cr$_2$Si$_2$Te$_6$, and the first principle calculations, germanene/magnetic semiconductor heterostructures are investigated. Topologically nontrivial edge states and quantized anomalous Hall conductance are demonstrated. It is shown that the QAHE temperature can be enhanced to approximately 62 K in germanene/monolayer (ML) Cr$_2$Ge$_2$Te$_6$ with 2.1\% tensile strain, 64 K in germanene/bilayer (BL) Cr$_2$Ge$_2$Te$_6$ with 1.4\% tensile strain, and 50 K in germanene/ML Cr$_2$Si$_2$Te$_6$ with 1.3\% tensile strain. With increasing tensile strain of these heterostructures, the band gap decreases and the Curie temperature rises, and the highest temperature of QAHE is obtained. Since these 2D materials were discovered in recent experiments, our results provide promising materials for achieving high-temperature QAHE.

cond-mat.mes-hall↗

arXiv2025

Unifying Strain-driven and Pressure-driven Superconductivity in La$_{3}$Ni$_{2}$O$_{7}$: Suppressed charge/spin density waves and enhanced interlayer coupling

Recent strain-stabilized superconductivity at ambient pressure in La$_3$Ni$_2$O$_{7}$ films opens new avenues for nickelates research, in parallel with its pressure-induced counterpart. Using density functional theory calculations, we elucidate the critical factors bridging strain- and pressure-driven superconductivity in La$_3$Ni$_2$O$_{7}$ by comprehensively analyzing structural, electronic, magnetic, and density wave characteristics. Consistent with recent scanning transmission electron microscopy observations, we find an $I4/mmm$ structural transition at $-0.9\%$ strain, preceding superconductivity onset. Electronic analysis shows compressive strain lowers Ni-$d_{z^2}$ orbital energy levels, while interfacial Sr diffusion effectively reconstructs the $d_{z^2}$ pockets, quantitatively matching angle-resolved photoemission spectroscopy experiments. The interlayer antiferromagnetic coupling $J_\perp$ under pressure or strain closely tracks experimental superconducting $T_c$ variation. The dome-shaped pressure dependence and monotonic strain dependence of $J_\perp$ mainly arise from modulations in the apical oxygen $p_z$ energy levels. Moreover, compressive strain suppresses both charge density waves (CDW) and spin density waves (SDW) instabilities analogous to pressure effects, with SDW vanishing concurrently with the structural transition and CDW disappearing at $\sim-3.3\%$ strain. Our results indicate that suppressed density waves and enhanced $J_\perp$ are crucial for both strain- and pressure-driven superconductivity. Accordingly, we propose several candidate substrates capable of achieving greater compressive strain, thereby potentially increasing $T_c$.

cond-mat.supr-con↗

arXiv2025

Inter-Layer Correlation of Loop Current Charge Density Wave on the Bilayer Kagomé Lattice

Loop current order has been suggested as a promising candidate for the spontaneous time-reversal symmetry breaking $2a_0 \times 2a_0$ charge density wave (CDW) revealed in vanadium-based kagomé metals \avs\ ($A$ = K, Rb, Cs) near van Hove filling $n_\text{vH} = 5/12$. Weak-coupling analyses and mean field calculations have demonstrated that nearest-neighbor Coulomb repulsion $V_1$ and next-nearest-neighbor Coulomb repulsion $V_2$ drives, respectively, real and imaginary bond-ordered CDW, with the latter corresponding to time-reversal symmetry breaking loop current CDW. It is important to understand the inter-layer correlation of these bond-ordered CDWs and its consequences in the bulk kagomé materials. To provide physical insights, we investigate in this paper the $c$-axis stacking of them, loop current CDW in particular, on the minimal bilayer kagomé lattice. The bare susceptibilities for stacking of real and imaginary bond orders are calculated for the free electrons on the bilayer kagomé lattice with inter-layer coupling $t_\perp=0.2t$, which splits the van Hove filling to $n_{+\text{vH}}=4.64/12$ and $n_{-\text{vH}}=5.44/12$. While real and imaginary bond-ordered CDWs are still favored, respectively, by $V_1$ and $V_2$, their inter-layer coupling is sensitive to band filling $n$. They tend to stack symmetrically near $n_{\pm\text{vH}}$ with identical bond orders in the two layers and give rise to a $2a_0 \times 2a_0 \times 1c_0$ CDW. On the other hand, they prefer to stack antisymmetrically around $n_\text{vH}$ with opposite bond orders in the two layers and lead to a $2a_0 \times 2a_0 \times 2c_0$ CDW. The concrete bilayer $t$-$t_\perp$-$V_1$-V$_2$ model is then studied. We obtain the mean-field ground states and determine the inter-layer coupling as a function of band filling at various interactions. The nontrivial topological properties of loop current CDWs are studied ...

cond-mat.str-el↗

arXiv2025

High Curie temperature in diluted magnetic semiconductors (B, Mn)X (X = N, P, As, Sb)

Doping nonmagnetic semiconductors with magnetic impurities is a feasible way to obtain diluted magnetic semiconductors (DMSs). It is generally accepted that for the most extensively studied DMS, (Ga, Mn)As, its highest Curie temperature T$_{\text{C}}$ was achieved at 200 K with a Mn concentration of approximately 16\% in experiments. A recent experiment reported record-breaking high electron and hole mobilities in the semiconductor BAs [\href{https://www.science.org/doi/10.1126/science.abn4290}{Science 377, 437 (2022)}]. Since BAs shares the same zinc-blende structure with GaAs, here we predict four DMSs (B, Mn)X (X $=$ N, P, As, Sb) by density functional theory calculations. Using a rescaling method to diminish the overestimation of Curie temperature, our results indicate that a significantly higher T$_{\text{C}}$ in the range of 467 K to 485 K for (B, Mn)As with a Mn concentration of around 15.6\% and even higher T$_{\text{C}}$ values above the room temperature for (B, Mn)P with a Mn concentration exceeding 9.4\%. Furthermore, using the method of Ab initio Scattering and Transport (AMSET) with first-principles material parameters, we have predicted a hole mobility of 48.9 cm$^{\text{2}}$V$^{\text{-1}}$s$^{\text{-1}}$ at 300 K for (B, Mn)As with the hole concentration of about n$_{\text{h}}$ $=$ 4.2 $\times$ 10$^{\text{19}}$ cm$^{\text{-3}}$, which is about two times larger than the hole mobility at 300 K in the calculations for (Ga, Mn)As. The hole mobility of (B, Mn)As can be enhanced faster than that of (Ga, Mn)As when the hole concentration is decreased. Our findings predict the emergence of a new family of DMS, (B, Mn)X, and are expected to stimulate both experimental and theoretical studies of the DMS with possible high T$_{\text{C}}$.

cond-mat.mtrl-sci↗

arXiv2025

Giant Magnetocaloric Effect in Spin Supersolid Candidate Na$_2$BaCo(PO$_4$)$_2$

Supersolid, an exotic quantum state of matter that consists of particles forming an incompressible solid structure while simultaneously showing superfluidity of zero viscosity [1], is one of the long-standing pursuits in fundamental research [2, 3]. Although the initial report of $^4$He supersolid turned out to be an artifact [4], this intriguing quantum matter has inspired enthusiastic investigations into ultracold quantum gases [5-8]. Nevertheless, the realization of supersolidity in condensed matter remains elusive. Here we find evidence for a quantum magnetic analogue of supersolid -- the spin supersolid -- in the recently synthesized triangular-lattice antiferromagnet Na$_2$BaCo(PO$_4$)$_2$ [9]. Notably, a giant magnetocaloric effect related to the spin supersolidity is observed in the demagnetization cooling process, manifesting itself as two prominent valley-like regimes, with the lowest temperature attaining below 100 mK. Not only is there an experimentally determined series of critical fields but the demagnetization cooling profile also shows excellent agreement with the theoretical simulations with an easy-axis Heisenberg model. Neutron diffractions also successfully locate the proposed spin supersolid phases by revealing the coexistence of three-sublattice spin solid order and interlayer incommensurability indicative of the spin superfluidity. Thus, our results indicate a strong entropic effect of the spin supersolid phase in a frustrated quantum magnet and open up a viable and promising avenue for applications in sub-Kelvin refrigeration, especially in the context of persistent concerns about helium shortages [10, 11].

cond-mat.str-el↗

arXiv2025

The second-order intrinsic Wiedemann-Franz law

In recent years, the nonlinear anomalous thermal Hall effect has attracted substantial attention. In this paper, we carry out a theoretical exploration of the intrinsic anomalous thermal Hall and Nernst effect that is induced by the thermal Berry connection polarizability. This effect is independent of the relaxation time and can be present in antiferromagnets possessing PT symmetry. Additionally, we put forward a second-order intrinsic Wiedemann-Franz law, which represents the ratio of the second-order intrinsic thermal conductivity coefficient to the second-order intrinsic electrical conductivity coefficient . When analyzed within a four-band PT symmetric Dirac model, we observe that the second-order intrinsic thermal conductivity coefficient is linearly proportional to the second-order intrinsic electrical conductivity coefficient , and the second-order intrinsic Wiedemann-Franz law is characterized by the chemical potential $μ$ in the low-temperature regime. These findings provide significant implications for experimental verification.

cond-mat.mes-hall↗

arXiv2025

Ferromagnetic Semiconductor Nanotubes with Room Curie Temperatures

Realizing ferromagnetic semiconductors with room Curie temperature $T\rm_C$ remains a challenge in spintronics. Inspired by the recent experimental progress on the nanotubes based on 2D van der Waals non-magnetic transition-metal dichalcogenides, magnetic nanotubes based on monolayer ferromagnetic materials are highly possible. Here, we proposed a way how to obtain high $T\rm_C$ ferromagnetic semiconductor nanotubes. Some high $T\rm_C$ ferromagnetic semiconductors are predicted in the MX$_2$ nanotubes (M = V, Cr, Mn, Fe, Co, Ni; X = S, Se, Te), including CrS$_2$ and CrTe$_2$ zigzag nanotubes with the diameter of 18 unit cells showing $T\rm_C$ above 300 K. In addition, due to the strain gradient in walls of nanotubes, an electrical polarization at level of $0.1$ eV/Å~inward of the radial direction is obtained. Our results not only present novel ferromagnetic semiconductor nanotubes with room Curie temperature but also be indicative of how to obtain such nanotubes based on experimentally obtained 2D high $T\rm_C$ ferromagnetic metals.

cond-mat.mtrl-sci↗

arXiv2024

Magnon Landau-Zener tunnelling and spin current generation by electric field

To control the magnon transport in magnetic systems is of great interest in magnonics. Due to the feasibility of electric field, how to generate and manipulate magnon with pure electrical method is one of the most desired goals. Here we propose that the magnon spin current is generated by applying time-dependent electric field, where the coupling between the magnon and electric field is invoked via Aharonov-Casher effect. In particular, the magnon spin current is dominated by electric field component which perpendicular to the magnetization direction. We apply our theory to 1D ferromagnetic SSH model and show that the generated magnon spin current is closely related to the band geometry. Our findings expands the horizons of magnonics and electric-control-magnon mechanisms.

cond-mat.mes-hall↗

arXiv2024

Double Magnon-Roton Excitations in the Triangular-Lattice Spin Supersolid

Supersolid is an exotic quantum state of matter that spontaneously hosts the features of both solid and superfluid, which breaks the translation and U(1) gauge symmetries. Here we study the spin dynamics in the triangular-lattice compound Na$_2$BaCo(PO$_4$)$_2$, which is revealed in [Xiang et al., Nature 625, 270-275 (2024)] as a quantum magnetic analog of supersolid. We simulate the easy-axis Heisenberg model with tensor network approach and uncover unique dynamic traits. These features are manifested in two branches of excitations that can be associated with the spin solidity and superfluidity, respectively. One branch contains the U(1) Goldstone and roton modes, while the other comprises pseudo-Goldstone and roton modes. The gapless Goldstone modes of the in-plane superfluid order are confirmed by our inelastic neutron scattering measurements. Together with the evident out-of-plane solid order indicated by the magnetic Bragg peaks, our findings provide spectroscopic evidence for spin supersolidity in this easy-axis antiferromagnet. Akin to the role of phonon-roton modes -- Landau elementary excitations -- in shaping the helium superfluid thermodynamics, the intriguing double magnon-roton dispersion here determines the low-temperature thermodynamics of spin supersolid down to sub-Kelvin regime, explaining the recently observed giant magnetocaloric effect in Na$_2$BaCo(PO$_4$)$_2$.

cond-mat.str-el↗