arXiv subjects

Georg M. Bruun

Publications and source records attributed to Georg M. Bruun.

At least 19 recordsLinked to original sources

arXiv2026

Exciton interacting with the phonons of an electronic Wigner crystal

With the advent of atomically thin and tunable van der Waals materials, a two-dimensional electronic Wigner crystal has recently been observed. The smoking gun signal was the appearance of an umklapp branch in optical exciton spectroscopy coming from the periodic potential generated by the Wigner crystal assumed to be static. Vibrations of the Wigner crystal however leads to a gapless phonon spectrum, which may affect the exciton spectrum. To explore this, we develop a field theoretical description of an exciton interacting with electrons forming a Wigner crystal including the coupling to the phonons. We show that importance of the exciton-phonon coupling scales with the exciton-electron interaction strength relative to the typical phonon energy squared. The motion of the exciton leads to two kinds of scattering processes, where the exciton emits a phonon either staying within the same Bloch band (intraband scattering) or changing its band (interband scattering). Using a non-perturbative self-consistent Born approximation, we demonstrate that these scattering processes lead to the formation of quasiparticles (polarons) consisting of the exciton in Bloch states dressed by Wigner crystal phonons. The energy shift and damping of these polarons depend on the electron density in a non-trivial way since it affects both the exciton-phonon interaction strength, as well as the phonon and exciton spectra. In particular, the damping is strongly affected by whether the polaron energy is inside the gapless phonon scattering continuum or not. Using these results, we finally analyse their effects on the observed spectral properties of the exciton.

cond-mat.str-el↗

arXiv2026

Scale invariance of the polaron energy at the Mott-superfluid critical point

Continuous quantum phase transitions are characterized by an order parameter and correlation functions that are often challenging to access experimentally or in direct numerical simulations. The energy of an added impurity can on the other hand be probed by established polaron spectroscopy, or numerically with Monte Carlo methods. We provide evidence from ground-state quantum Monte Carlo calculations that the energy of a mobile impurity interacting weakly with a surrounding lattice Bose gas provides access to the critical behavior of the Mott insulator-superfluid phase transition. Finite-size scaling of the energy reveals that its value is scale invariant at the critical point of the quantum phase transition, and we extract a scaling exponent that is currently unexplained by theory. For a small lattice we further observe a flattening of the impurity-boson density-density correlations at the critical point, which hints at a divergence of a corresponding length scale in the thermodynamic limit. Our results suggest that impurity spectroscopy represents a useful way to probe the critical properties of quantum phase transitions in general.

cond-mat.quant-gas↗

arXiv2026

Hole and spin dynamics in an anti-ferromagnet close to half filling

The interplay between charge and spin dynamics is at the heart of strongly correlated materials. Inspired by recent quantum simulation experiments, we develop a conserving diagrammatic method to describe the Fermi-Hubbard model for strong repulsion and small hole doping away from the half-filled anti-ferromagnetic ground state. We show that doping leads to four hole pockets in the Brillouin zone formed by magnetic polarons, which become increasingly damped with hole concentration. Likewise, the magnon spectrum of the anti-ferromagnet softens and dampens with doping due to hole-induced magnetic frustration. This gives rise to a suppression of the anti-ferromagnetic correlations in agreement with recent experiments. We then calculate the response of the system to a lattice modulation and recover the qualitative difference between in-phase and out-of-phase modulations seen in experiments, which was interpreted as signs of pseudogap physics. Our results indicate that the complex competition between spin and charge degrees of freedom and the emergence of the pseudogap phase may be usefully analyzed for small dopings, where systematic theories can be developed.

cond-mat.quant-gas↗

arXiv2026

Phenomenological model of decaying Bose polarons

Cold atom experiments show that a mobile impurity particle immersed in a Bose-Einstein condensate forms a well-defined quasiparticle (Bose polaron) for weak to moderate impurity-boson interaction strengths, whereas a significant line broadening is consistently observed for strong interactions. Motivated by this, we introduce a phenomenological theory based on the assumption that the most relevant states are characterized by the impurity correlated with at most one boson, since they have the largest overlap with the uncorrelated states to which the most common experimental probes couple. These experimentally relevant states can however decay to lower energy states characterised by correlations involving multiple bosons, and we model this using a minimal variational wave function combined with a complex impurity-boson interaction strength. We first motivate this approach by comparing to a more elaborate theory that includes correlations with up to two bosons. Our phenomenological model is shown to recover the main results of two recent experiments probing both the spectral and the non-equilibrium properties of the Bose polaron. Our work offers an intuitive framework for analyzing experimental data and highlights the importance of understanding the complicated problem of the Bose polaron decay in a many-body setting.

cond-mat.quant-gas↗

arXiv2025

Spin-charge bound states and emerging fermions in a quantum spin liquid

The complex interplay between charge and spin dynamics lies at the heart of strongly correlated quantum materials, and it is a fundamental topic in basic research with far reaching technological perspectives. We explore in this paper the dynamics of holes in a single band extended $t-J$ model where the background spins form a $\mathbb{Z}_{2}$ quantum spin liquid (QSL). Using a field theory approach based on a parton construction, we show that while the electrons for most momenta fractionalize into uncorrelated charge carrying holons and spin carrying spinons as generally expected for a QSL, the spinon-holon scattering cross-section diverges for certain momenta signalling strong correlations. By deriving an effective low-energy Hamiltonian describing this dynamics, we demonstrate that these divergencies are due to the formation of long lived spinon-holon bound states. We then show that quantum gas microscopy with atoms in optical lattices provides an excellent platform for verifying and probing the internal spatial structure of these emergent fermions. The fermions will furthermore show up as clear quasiparticle peaks in angle-resolved photoemission spectroscopy with an intensity determined by their internal structure. For a non-zero hole concentration, the fermions form hole pockets with qualitatively the same location, shape, and intensity variation in the Brillouin zone as the so-called Fermi arcs observed in the pseudogap phase. Such agreement is remarkable since the Fermi arcs arise from the delicate interplay between the symmetry of the QSL and the internal structure of the emerging fermions in a minimal single band model with no extra degrees of freedom added. Our results, therefore, provide a microscopic mechanism for the conjectured fractionalized Fermi liquid and open up new pathways for exploring the pseudogap phase and high temperature superconductivity as arising from a QSL.

cond-mat.str-el↗

arXiv2025

Polarons in atomic gases and two-dimensional semiconductors

In this work we provide a comprehensive review of theoretical and experimental studies of the properties of polarons formed by mobile impurities strongly interacting with quantum many-body systems. We present a unified perspective on the universal concepts and theoretical techniques used to characterize polarons in two distinct platforms, ultracold atomic gases and atomically-thin transition metal dichalcogenides, which are linked by many deep parallels. We review polarons in both fermionic and bosonic environments, highlighting their similarities and differences including the intricate interplay between few- and many-body physics. Various kinds of polarons with long-range interactions or in magnetic backgrounds are discussed, and the theoretical and experimental progress towards understanding interactions between polarons is described. We outline how polaron physics, regarded as the low density limit of quantum mixtures, provides fundamental insights regarding the phase diagram of complex condensed matter systems. Furthermore, we describe how polarons may serve as quantum sensors of many-body physics in complex environments. Our work highlights the open problems, identifies new research directions and provides a comprehensive framework for this rapidly evolving research field.

cond-mat.quant-gas↗

arXiv2024

Green's function approach to interacting lattice polaritons and optical nonlinearities in subwavelength arrays of quantum emitters

Sub-wavelength arrays of quantum emitters offer an efficient free-space approach to coherent light-matter interfacing, using ultracold atoms or two-dimensional solid-state quantum materials. The combination of collectively suppressed photon-losses and emerging optical nonlinearities due to strong photon-coupling to mesoscopic numbers of emitters holds promise for generating nonclassical light and engineering effective interactions between freely propagating photons. While most studies have thus far relied on numerical simulations, we describe here a diagrammatic Green's function approach that permits analytical investigations of nonlinear processes. We illustrate the method by deriving a simple expression for the scattering matrix that describes photon-photon interactions in an extended two-dimensional array of quantum emitters, and reproduces the results of numerical simulations of coherently driven arrays. The approach yields intuitive insights into the nonlinear response of the system and offers a promising framework for a systematic development of a theory for interacting photons and many-body effects on collective radiance in two-dimensional arrays of quantum emitters.

cond-mat.quant-gas↗

arXiv2024

Lattice Bose polarons at strong coupling and quantum criticality

We develop a new theoretical framework for exploring a mobile impurity interacting strongly with a highly correlated bath of bosons in the quantum critical regime of a Mott insulator (MI) to superfluid (SF) quantum phase transition. Our framework is based on a powerful quantum Gutzwiller (QGW) description of the bosonic bath combined with diagrammatic field theory for the impurity-bath interactions. By resumming a selected class of diagrams to infinite order, a rich picture emerges where the impurity is dressed by the fundamental modes of the bath, which change character from gapped particle-hole excitations in the MI to Higgs and gapless Goldstone modes in the SF. This gives rise to the existence of several quasiparticle (polaron) branches with properties reflecting the strongly correlated environment. In particular, one polaron branch exhibits a sharp cusp in its energy, while a new ground-state polaron emerges at the $O(2)$ quantum phase transition point for integer filling, which reflects the nonanalytic behavior at the transition and the appearance of the Goldstone mode in the SF phase. Smooth versions of these features are inherited in the polaron spectrum away from integer filling because of the varying ``Mottness" of the bosonic bath. We furthermore compare our diagrammatic results with quantum Monte Carlo calculations, obtaining excellent agreement. This accuracy is quite remarkable for such a highly non-trivial case of strong interactions between the impurity and bosons in a maximally correlated quantum critical regime, and it establishes the utility of our framework. Finally, our results show how impurities can be used as quantum sensors and highlight fundamental differences between experiments performed at a fixed particle number or a fixed chemical potential.

cond-mat.quant-gas↗

arXiv2024

Microscopic theory of polariton-polariton interactions

We develop a comprehensive theoretical model for the interaction strength between a pair of exciton-polaritons in microcavity devices. Ab initio numerical calculations for dipolar polaritons in one dimension are used as a starting point to build a Born-Oppenheimer theory that generally applies to generic -- dipolar or non-dipolar polaritons -- in both one and two dimensions. This theory anticipates that the strong coupling to the cavity mode leads to a drastic enhancement of the polariton interactions as compared to bare excitons, and predicts unexpected scaling laws in the interaction strength as a function of system parameters. Comparisons with available experimental data are drawn, and specific suggestions to validate it with new experiments are made. Promising strategies towards the observation of a strong polariton blockade regime are finally sketched.

cond-mat.mes-hall↗

arXiv2024

Exciton interacting with a moiré lattice: Polarons, strings, and optical probing of spin correlations

We develop a general theory for how an exciton in an atomically thin transition metal dichacogenide (TMD) monolayer couples to spin and charge correlations in an adjacent moire lattice created by a TMD bi-layer. Virtual tunneling of charge carriers, assumed for concreteness to be holes, between the moire lattice and the monolayer combined with the presence of bound hole-exciton states, i.e. trions, give rise to an effective interaction between the moire holes and the exciton. In addition to the Umklapp scattering, we show that this interaction is spin-dependent and therefore couples the exciton to the spin correlations of the moire holes, which may be in- as well as out-of-plane. We then use our theory to examine two specific examples where the moire holes form in-plane ferromagnetic or anti-ferromagnetic order. In both cases, the exciton creates spin waves in the moire lattice, which we analyse by using a self-consistent Born approximation that includes such processes to infinite order. We show that the competition between magnetic order and exciton motion leads to the formation of a well-defined quasiparticle consisting of the exciton surrounded by a cloud of magnetic frustration in the moire lattice sites below. For the anti-ferromagnet, we furthermore demonstrate the presence of the elusive geometric string excitations and discuss how they can be observed via their smoking gun energy dependence on the spin-spin coupling, which can be tuned by varying the twist angle of the moire bi-layer. All these phenomena have clear signatures in the exciton spectrum, and as such our results illustrate that excitons are promising probes providing optical access to the spin correlations of new quantum phases predicted to exist in TMD materials.

cond-mat.mes-hall↗

arXiv2024

Chiral polaron formation on the edge of topological quantum matter

Immersing a mobile impurity in a quantum many-body environment can reveal fundamental properties of the background medium, hence providing a powerful probe of quantum matter. This approach is particularly intriguing when considering media with exotic properties, such as strongly-correlated phases and topological states of matter. In this work, we study the dressing of a mobile impurity interacting with a chiral mode, as provided by the edge of topological quantum matter. The resulting ''chiral polaron'' is characterized by an asymmetric spectral function, which reflects the chirality and group velocity of the topological edge mode and the drag experienced by the mobile impurity. We first build our theoretical understanding from an effective one-dimensional chiral model, which captures the hallmark signatures of the chiral polaron. We then demonstrate how this simple picture extends to realistic models of integer and fractional Chern insulator states, by adapting tensor-network methods to polaron spectroscopy. Injecting mobile impurities on the edge of topological quantum matter is shown to be a powerful tool to probe exotic edge properties, particularly suitable for cold-atom experiments.

cond-mat.quant-gas↗

arXiv2023

Wave function and spatial structure of polarons in an antiferromagnetic bilayer

Adding a dopant to an antiferromagnetic spin background disturbs the magnetic order and leads to the formation of a quasiparticle coined the magnetic polaron, which plays a central role in understanding strongly correlated materials. Recently, remarkably detailed insights into the spatial properties of such polarons have been obtained using atoms in optical lattices. Motivated by this we develop a nonperturbative scheme for calculating the wave function of the magnetic polaron in a bilayer antiferromagnet using the self-consistent Born approximation. The scheme includes an infinite number of spin waves, which is crucial for an accurate description of the most interesting regime of strong correlations. Utilizing the developed wave function, we explore the spatial structure of the polaron dressing cloud consisting of magnetically frustrated spins surrounding the hole. Mimicking the nonmonotonic behavior of the antiferromagnetic order, we find that the dressing cloud first decreases and then increases in size with increasing interlayer hopping. The increase reflects the decrease in the magnetic order as a quantum phase transition to a disordered state is approached for large interlayer hopping. We, furthermore, find that the symmetry of the ground state dressing cloud changes as the interlayer coupling increases. Our results should be experimentally accessible using quantum simulation with optical lattices.

cond-mat.str-el↗

arXiv2023

Strongly interacting Bose-Fermi mixture: mediated interaction, phase diagram and sound propagation

Motivated by recent surprising experimental findings, we develop a strong-coupling theory for Bose-Fermi mixtures capable of treating resonant inter-species interactions while satisfying the compressibility sum rule. We show that the mixture can be stable at large interaction strengths close to resonance, in agreement with the experiment but at odds with the widely used perturbation theory. We also calculate the sound velocity of the Bose gas in the $^{133}$Cs-$^6$Li mixture, again finding good agreement with the experimental observations both at weak and strong interactions. A central ingredient of our theory is the generalization of a fermion mediated interaction to strong Bose-Fermi scatterings and to finite frequencies. This further leads to a predicted hybridization of the sound modes of the Bose and Fermi gases, which can be directly observed using Bragg spectroscopy.

cond-mat.quant-gas↗

arXiv2023

Polarons and bipolarons in a two-dimensional square lattice

Quasiparticles and their interactions are a key part of our understanding of quantum many-body systems. Quantum simulation experiments with cold atoms have in recent years advanced our understanding of isolated quasiparticles, but so far they have provided limited information regarding their interactions and possible bound states. Here, we show how exploring mobile impurities immersed in a Bose-Einstein condensate (BEC) in a two-dimensional lattice can address this problem. First, the spectral properties of individual impurities are examined, and in addition to the attractive and repulsive polarons known from continuum gases, we identify a new kind of quasiparticle stable for repulsive boson-impurity interactions. The spatial properties of polarons are calculated showing that there is an increased density of bosons at the site of the impurity both for repulsive and attractive interactions. We then derive an effective Schrödinger equation describing two polarons interacting via the exchange of density oscillations in the BEC, which takes into account strong impurity-boson two-body correlations. Using this, we show that the attractive nature of the effective interaction between two polarons combined with the two-dimensionality of the lattice leads to the formation of bound states -- i.e. bipolarons. The wave functions of the bipolarons are examined showing that the ground state is symmetric under particle exchange and therefore relevant for bosonic impurities, whereas the first excited state is doubly degenerate and odd under particle exchange making it relevant for fermionic impurities. Our results show that quantum gas microscopy in optical lattices is a promising platform to explore the spatial properties of polarons as well as to finally observe the elusive bipolarons.

cond-mat.quant-gas↗

arXiv2022

Life and death of the Bose polaron

Spectroscopic and interferometric measurements complement each other in extracting the fundamental properties of quantum many-body systems. While spectroscopy provides precise measurements of equilibrated energies, interferometry can elucidate the dynamical evolution of the system. For an impurity immersed in a bosonic medium, both are equally important for understanding the quasiparticle physics of the Bose polaron. Here, we compare the interferometric and spectroscopic timescales to the underlying dynamical regimes of the impurity dynamics and the polaron lifetime, highlighting the capability of the interferometric approach to clearly resolve polaron dynamics. In particular, interferometric measurements of the coherence amplitude at strong interactions reveal faster quantum dynamics at large repulsive interaction strengths than at unitarity. These observations are in excellent agreement with a short-time theoretical prediction including both the continuum and the attractive polaron branch. For longer times, qualitative agreement with a many-body theoretical prediction which includes both branches is obtained. Moreover, the polaron energy is extracted from interferometric measurements of the observed phase velocity in agreement with previous spectroscopic results from weak to strong attractive interactions. Finally, the phase evolution allows for the measurement of an energetic equilibration timescale, describing the initial approach of the phase velocity to the polaron energy. Theoretically, this is shown to lie within the regime of universal dynamics revealing a fast initial evolution towards the formation of polarons. Our results give a comprehensive picture of the many-body physics governing the Bose polaron and thus validates the quasiparticle framework for further studies.

cond-mat.quant-gas↗

arXiv2022

Light-induced topological superconductivity in transition metal dichalcogenide monolayers

Monolayer transition metal dichalcogenides (TMDs) host deeply bound excitons interacting with itinerant electrons, and as such they represent an exciting new quantum many-body Bose-Fermi mixture. Here, we demonstrate that electrons interacting with a Bose-Einstein condensate (BEC) of exciton-polaritons can realise a two-dimensional topological $p_x+ip_y$ superconductor. Using strong coupling Eliashberg theory, we show that this is caused by an attractive interaction mediated by the BEC, which overcompensates the repulsive Coulomb interaction between the electrons. The hybrid light-matter nature of the BEC is crucial for achieving this, since it can be used to reduce retardation effects and increase the mediated interaction in regimes important for pairing. We finally show how the great flexibility of TMDs allows one to tune the critical temperature of the topological superconducting phase to be within experimental reach.

cond-mat.supr-con↗

arXiv2022

Holes and magnetic polarons in a triangular lattice antiferromagnet

The intricate interplay between charge motion and magnetic order in geometrically frustrated lattices is central for the properties of many two-dimensional quantum materials. The triangular lattice antiferromagnet is a canonical example of a frustrated system, and here we analyse the dynamics of a hole in such a lattice focusing on observables that have become accessible in a new generation of experiments. Using the $t$-$J$ model, we solve the problem exactly within linear spin wave theory in the limit of strong magnetic interactions, showing that the ground state is described by a coherent state of spin waves. The derivation highlights the crucial role played by the interaction between a static hole and the neighboring spins, which originates in the geometric frustration and has often been omitted in earlier works. Furthermore, we show that the non-equilibrium dynamics after a hole has abruptly been inserted at a lattice site is given exactly by a coherent state with time-dependent oscillatory coefficients. Physically, this describes a burst of magnetic frustration propagating through only two-thirds of the lattice sites, since a destructive interference of spin waves leaves spins parallel to that removed by the hole unperturbed. After the wave has propagated through the lattice, the magnetization relaxes to that of the ground state. We then use our analytical solution to benchmark the widely used self-consistent Born approximation (SCBA), showing that it is very accurate also for a triangular lattice. The magnetic polaron spectrum is analysed for general magnetic interactions using the SCBA, and we compare our results with those for a square lattice.

cond-mat.quant-gas↗

arXiv2022

Strong photon interactions from weakly interacting particles

The hybridization of light and matter excitations in the form of polaritons has enabled major advances in understanding and controlling optical nonlinearities. Entering the quantum regime of strong interactions between individual photons has however remained challenging since the strength of achievable polariton interactions is typically limited by the available interactions in the material. Here, we investigate collisions between dark-state polaritons in three-level systems and discover a resonant process that yields effective interactions, which are much larger than the underlying interaction between their matter constituents. We systematically investigate the underlying mechanism and demonstrate a substantial enhancement of polariton interactions by several orders of magnitude. This suggests a promising approach to quantum nonlinear optics in a range of physical settings, from atomic gases to excitons in semiconductors and two-dimensional bilayer materials.

cond-mat.quant-gas↗