arXiv subjects

Georg von Freymann

Publications and source records attributed to Georg von Freymann.

At least 37 records · Page 2Linked to original sources

arXiv2025

Enhancing Vector Network Analysis With a Photonic Frequency Extender Setup

We present a photonic ultra-wideband frequency extension for a commercial Vector Network Analyzer (VNA) to perform free-space measurements in a frequency range from 70 GHz up to 520 GHz with a Hz level resolution. The concept is based on the synchronization of continuous-wave (CW) lasers with highly frequency-stable electronic emitter sources as a reference. The use of CW photomixers with bandwidths up to several terahertz allows for the straightforward expansion of the covered frequency range to 1 THz or even beyond. This can be achieved, for instance, by cascading additional lasers within the synchronization scheme. Consequently, the necessity for additional frequency extender modules, as seen in current state-of-the-art VNAs, is eliminated, thereby reducing the complexity and cost of the system significantly. To showcase the capabilities of the Photonic Vector Network Analyzer (PVNA) extender concept, we conducted S21 transmission measurements of various cross-shaped bandpass filters and waveguide-coupled high-frequency (HF) components. Additionally, the analyzed magnitude and phase data were either compared to electro-magnetic (EM) simulations or referenced against data obtained from commercial electronic frequency extender modules.

physics.optics↗

arXiv2024

Terahertz Quantum Imaging

Quantum imaging with undetected photons spatially transfers amplitude and phase information from one spectral region of physical interest to another spectral region that is easy to detect. The photon energy of the two spectral regions can, in principle, be separated by several orders of magnitude. However, quantum imaging with undetected photons has so far only been demonstrated in spectral regions of similar order of magnitude in frequency (and for which cameras are commercially available). Here, we demonstrate amplitude- and phase-sensitive imaging in the terahertz spectral region (1.5 THz center frequency) by detecting only visible photons (center wavelength 662.2 nm, 452.7 THz center frequency) more than two orders of magnitude apart. As a result, terahertz spectral information can be reliably detected with a standard CMOS camera without cooling, achieving a spatial resolution close to the wavelength. By taking advantage of quantum distillation in a nonlinear interferometer, the influence of ubiquitous thermal terahertz photons can be neglected. Our results are in good agreement with numerical simulations of the imaging process and demonstrate the huge potential of this method to address otherwise challenging spectral regions where cameras do not exist.

quant-ph↗

arXiv2024

Wide-range resistivity characterization of semiconductors with terahertz time-domain spectroscopy

Resistivity is one of the most important characteristics in the semiconductor industry. The most common way to measure resistivity is the four-point probe method, which requires physical contact with the material under test. Terahertz time domain spectroscopy, a fast and non-destructive measurement method, is already well established in the characterization of dielectrics. In this work, we demonstrate the potential of two Drude model-based approaches to extract resistivity values from terahertz time-domain spectroscopy measurements of silicon in a wide range from about 10$^{-3}$ $Ω$cm to 10$^{2}$ $Ω$cm. One method is an analytical approach and the other is an optimization approach. Four-point probe measurements are used as a reference. In addition, the spatial resistivity distribution is imaged by X-Y scanning of the samples to detect inhomogeneities in the doping distribution.

physics.optics↗

arXiv2023

Local temperature control of magnon frequency and direction of supercurrents in a magnon Bose-Einstein condensate

The creation of temperature variations in magnetization, and hence in the frequencies of the magnon spectrum in laser-heated regions of magnetic films, is an important method for studying Bose-Einstein condensation of magnons, magnon supercurrents, Bogoliubov waves, and similar phenomena. In our study, we demonstrate analytically, numerically, and experimentally that, in addition to the magnetization variations, it is necessary to consider the connected variations of the demagnetizing field. In case of a heat induced local minimum of the saturation magnetization, the combination of these two effects results in a local increase in the minimum frequency value of the magnon dispersion at which the Bose-Einstein condensate emerges. As a result, a magnon supercurrent directed away from the hot region is formed.

cond-mat.quant-gas↗

arXiv2023

Broadband mode division multiplexing of OAM-modes by a micro printed waveguide structure

A light beam carrying orbital angular momentum (OAM) is characterized by a helical phase-front that winds around the center of the beam. These beams have unique properties that have found numerous applications. In the field of data transmission, they represent a degree of freedom that could potentially increase capacity by a factor of several distinct OAM modes. While an efficient method for (de)composing beams based on their OAM exists for free-space optics, a device capable of performing this (de)composition in an integrated, compact fiber application without the use of external active optical elements and for multiple OAM modes simultaneously has not been reported. In this study, a waveguide structure is presented that can serve as a broadband OAM (de)multiplexer. The structure design is based on the adiabatic principle used in photonic lanterns for highly efficient conversion of spatially separated single modes into eigenmodes of a few-mode fiber. In addition, an artificial magnetic field is introduced by twisting the structure during the adiabatic evolution, which removes the degeneracy between modes having the same absolute OAM. This structure can simplify, stabilize, and miniaturize the creation or decomposition of OAM beams, making them useful for various applications.

physics.optics↗

arXiv2023

Coherent and incoherent magnons induced by strong ultrafast demagnetization in thin permalloy films

Understanding spin dynamics on femto- and picosecond timescales offers new opportunities for faster and more efficient spintronic devices. Here, we experimentally investigate the coherent spin dynamics after ultrashort laser excitation by time-resolved magneto optical Kerr effect (TR-MOKE) in thin Ni80Fe20 films. We provide a detailed study of the magnetic field and pump fluence dependence of the coherent precessional dynamics. We show that the coherent precession lifetime increases with the applied external magnetic field which cannot be understood by viscous Gilbert damping of the coherent magnons. Instead, it can be explained by nonlinear magnon interactions and by the change in the fraction of incoherent magnons. This interpretation is in agreement with the observed trends of the coherent magnon amplitude and lifetime as a function of the exciting laser fluence. Our results provide a new insight into the magnetization relaxation processes in ferromagnetic thin films, which is of great importance for further spintronic applications.

cond-mat.mes-hall↗

arXiv2023

Mixing Rule for Calculating the Effective Refractive Index Beyond the Limit of Small Particles

Considering light transport in disordered media, the medium is often treated as an effective medium requiring accurate evaluation of an effective refractive index. Because of its simplicity, the Maxwell-Garnett (MG) mixing rule is widely used, although its restriction to particles much smaller than the wavelength is rarely satisfied. Using 3D finite-difference time-domain simulations, we show that the MG theory indeed fails for large particles. Systematic investigation of size effects reveals that the effective refractive index can be instead approximated by a quadratic polynomial whose coefficients are given by an empirical formula. Hence, a simple mixing rule is derived which clearly outperforms established mixing rules for composite media containing large particles, a common condition in natural disordered media.

physics.optics↗

arXiv2023

Rapid-prototyping of microscopic thermal landscapes in Brillouin light scattering spectroscopy

Since temperature and its spatial and temporal variations affect a wide range of physical properties of material systems, they can be used to create reconfigurable spatial structures of various types in physical and biological objects. This paper presents an experimental optical setup for creating tunable two-dimensional temperature patterns on a micrometer scale. As an example of its practical application, we have produced temperature-induced magnetization landscapes in ferrimagnetic yttrium iron garnet films and investigated them using micro-focused Brillouin light scattering spectroscopy. It is shown that, due to the temperature dependence of the magnon spectrum, temperature changes can be visualized even for microscale thermal patterns.

cond-mat.quant-gas↗

arXiv2023

Coherent magnetization dynamics in strongly quenched Ni thin films

The remagnetization process after ultrafast demagnetization can be described by relaxation mechanisms between the spin, electron, and lattice reservoirs. Thereby, collective spin excitations in form of spin waves and their angular momentum transfer play an important role on the longer timescales. In this work, we address the question whether the strength of demagnetization affects the coherency and the phase of the excited spin waves. We present a study of coherent magnetization dynamics in thin nickel films after ultrafast demagnetization using the all-optical, time-resolved magneto-optical Kerr-effect (tr-MOKE) technique. The largest coherent oscillation amplitude was observed for strongly quenched systems, showing the conservation of coherency for demagnetizations of up to 90%. Moreover, the phase of the excited spin-waves increases with pump power, indicating a delayed start of the precession during the remagnetization.

cond-mat.mtrl-sci↗

arXiv2022

General simulation method for quantum-sensing systems

Quantum sensing encompasses highly promising techniques with diverse applications including noise-reduced imaging, super-resolution microscopy as well as imaging and spectroscopy in challenging spectral ranges. These detection schemes use biphoton correlations to surpass classical limits or transfer information to different spectral ranges. Theoretical analysis is mostly confined to idealized conditions. Therefore, theoretical predictions and experimental results for the performance of quantum-sensing systems often diverge. Here we present a general simulation method that includes experimental imperfections to bridge the gap between theory and experiment. We develop a theoretical approach and demonstrate the capabilities with the simulation of aligned and misaligned quantum-imaging experiments. The results recreate the characteristics of experimental data. We further use the simulation results to improve the obtained images in post-processing. As simulation method for general quantum-sensing systems, this work provides a first step towards powerful simulation tools for interactively exploring the design space and optimizing the experiment's characteristics.

quant-ph↗

arXiv2022

Utilizing the sensitization effect for direct laser writing in a novel photoresist based on the chitin monomer N-acetyl-D-glucosamine

The great flexibility of direct laser writing arises from the possibility to fabricate precise three-dimensional structures on very small scales as well as the broad range of applicable materials. However, there is still a vast number of promising materials which are currently inaccessible requiring the continuous development of novel photoresists. Here, a new bio-sourced resist is reported which relies on the monomeric unit of chitin, N-acetyl-D-glucosamine, expanding the existing plant-based biopolymer resists by a bio-based monomer from the animal kingdom. In addition it is shown that combined use of two photoinitiators is advantageous over the use of a single one. In our approach, the first photoinitator is a good two-photon absorber at the applied wavelength, while the second photoinitiator exhibits poor two-photon absorbtion abilities, but is better suited for crosslinking of the monomer. The first photoinitiator absorbs the light acting as a sensitizer and transfers the energy to the second initiator, which subsequently forms a radical and initializes the polymerization. This sensitization effect enables a new route to utilize reactive photointiators with a small two-photon absorption cross-section for direct laser writing without changing their chemical structure.

physics.optics↗

arXiv2022

Initiator-free photo-crosslinkable cellulose-based resists for fabricating submicron patterns via direct laser writing

Novel bifunctional cellulose diacetate derivatives were synthesized in order to achieve bio-based photoresists, which can be structured by two-photon absorption via direct laser writing (DLW) without the need to use a photoinitiator. Therefore, cellulose diacetate is functionalized with thiol moieties and olefinic or methacrylic side groups enabling thiol-conjugated crosslinking. These cellulose derivatives are also photo-crosslinkable via UV irradiation ($λ$ = 254 nm and 365 nm) without using an initiator.

physics.optics↗

arXiv2022

General simulation method for spontaneous parametric down- and parametric up-conversion experiments

Spontaneous parametric down-conversion (SPDC) sources are an important technology for quantum sensing and imaging. We demonstrate a general simulation method, based on modeling from first principles, reproducing the spectrally and spatially resolved absolute counts of a SPDC experiment. By simulating additional processes and effects we accomplish good agreement with the experimental results. This method is broadly applicable and allows for the separation of contributing processes, virtual characterization of SPDC sources, and enables the simulation of many quantum based applications.

quant-ph↗

arXiv2022

Confinement of Bose-Einstein magnon condensates in adjustable complex magnetization landscapes

Coherent wave states such as Bose-Einstein condensates (BECs), which spontaneously form in an overpopulated magnon gas even at room temperature, have considerable potential for wave-based computing and information processing at microwave frequencies. The ability to control the transport properties of magnon BECs plays an essential role for their practical use. Here, we demonstrate spatio-temporal control of the BEC density distribution through the excitation of magnon supercurrents in an inhomogeneously magnetized yttrium iron garnet film. The BEC is created by microwave parametric pumping and probed by Brillouin light scattering spectroscopy. The desired magnetization profile is prepared by heating the film with optical patterns projected onto its surface using a phase-based wavefront modulation technique. Specifically, we observe a pronounced spatially localized magnon accumulation caused by magnon supercurrents flowing toward each other originating in two heated regions. This accumulation effect increases the BEC lifetime due to the constant influx of condensed magnons into the confinement region. The shown approach to manipulate coherent waves provides an opportunity to extend the lifetime of freely evolving magnon BECs, create dynamic magnon textures, and study the interaction of magnon condensates formed in different regions of the sample.

cond-mat.quant-gas↗

arXiv2022

Phase-quadrature quantum imaging with undetected photons

Sensing with undetected photons allows access to spectral regions with simultaneous detection of photons of another region and is based on nonlinear interferometry. To obtain the full information of a sample, the corresponding interferogram has to be analyzed in terms of amplitude and phase, which has been realized so far by multiple measurements followed by phase variation. Here, we present a polarization-optics-based phase-quadrature implementation in a nonlinear interferometer for imaging with undetected photons in the infrared region. This allows us to obtain phase and visibility with a single image acquisition without the need of varying optical paths or phases, thus enabling the detection of dynamic processes. We demonstrate the usefullness of our method on a static phase mask opaque to the detected photons as well as on dynamic measurement tasks as the drying of an isopropanol film and the stretching of an adhesive tape.

quant-ph↗

arXiv2022

Electronic Phase Detection with sub-10 fs Timing Jitter for Terahertz Time-Domain Spectroscopy Systems

Terahertz time-domain spectroscopy systems based on resonator-internal repetition-rate modulation, such as SLAPCOPS [12] and ECOPS [11], rely on electronic phase detectors which are typically prone to exhibit both a non-negligible random and systematic timing error. This limits the quality of the recorded information significantly. Here, we present the results of our recent attempt to reduce these errors in our own electronic phase detection systems. A more than six-fold timing-jitter reduction from 59.0 fs to 8.6 fs led to a significant increase in both exploitable terahertz bandwidth and signal-to-noise ratio. Additionally, utilizing our interferometrically monitored delay line as a calibration standard, the systematic error could be removed almost entirely and thus, excellent resolution of spectral absorption lines be accomplished. These improvements increased the accuracy of our multi-layer thickness measurements based on electronic phase detection by more than a factor of five, pushing the overall performance well into the sub-μm regime.

physics.optics↗

arXiv2022

Towards efficient structure prediction and pre-compensation in multi-photon lithography

Microscale 3D printing technologies have been of increasing interest in industry and research for several years. Unfortunately, the fabricated structures always deviate from the respective expectations, often caused by the physico-chemical properties during and after the printing process. Here, we show first steps towards a simple, fast and easy to implement algorithm to predict the final structure topography for multi-photon lithography - also known as Direct Laser Writing (DLW). The three main steps of DLW, (i) exposure of a photo resin, (ii) cross-linking of the resin, and (iii) subsequent shrinkage are approximated by mathematical operations, showing promising results in coincidence with experimental observations. E.g., the root-mean-square error (rmse) between the unmodified 3D print of a radial-symmetrically chirped topography and our predicted topography is only 0.46 $μ$m, whereas the rmse between this 3D print and its target is 1.49 $μ$m. Thus, our robust predictions can be used prior to the printing process to minimize undesired deviations between the target structure and the final 3D printed structure. Using a Downhill-Simplex algorithm for identifying the optimal prediction parameters, we were able to reduce the rmse from 4.04 $μ$m to 0.33 $μ$m by only two correction loops in our best-case scenario (rmse = 0.72 $μ$m after one loop). Consequently, this approach can eliminate the need for many structural optimization loops to produce highly conformal and high quality micro structures in the future.

physics.optics↗

arXiv2022

Fiber-tip endoscope for optical and microwave control

We present a robust, fiber based endoscope with a silver direct-laser-written (DLW) structure for radio frequency (RF) emission next to the optical fiber facet. Thereby, we are able to excite and probe a sample, such as nitrogen vacancy (NV) centers in diamond, with RF and optical signals simultaneously and specifically measure the fluorescence of the sample fully through the fiber. At our targeted frequency-range around 2.9 GHz the facet of the fiber-core is in the near-field of the RF-guiding silver-structure, which comes with the advantage of an optimal RF-intensity decreasing rapidly with the distance. By creating a silver structure on the cladding of the optical fiber we achieve the minimal possible distance between an optically excited and detected sample and an antenna structure without affecting the optical performance of the fiber. This allows us realizing a high RF-amplitude at the sample's position when considering an endoscope solution with integrated optical and RF access. The capabilities of the endoscope are quantified by optically detected magnetic resonance (ODMR) measurements of a NV-doped microdiamond that we probe as a practical use case. We demonstrate a magnetic sensitivity of our device of 17.8 nT/$\sqrt{\mathrm{Hz}}$ per when measuring the ODMR exclusively through our fiber and compare the sensitivity to a measurement using a confocal microscope. Moreover, such an endoscope could be used as a powerful tool for measuring a variety of fluorescent particles that can otherwise only be measured with bulky and large optical setups. Furthermore, our endoscope points toward precise distance measurements based on Rabi oscillations.

physics.ins-det↗