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George Toh

Publications and source records attributed to George Toh.

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Tripartite entanglement of remote atomic qubits

Distributed entanglement across multi-node quantum networks is essential for a wide range of quantum technologies, including modular quantum computers, distributed sensing and metrology, and multi-party secure communication protocols. Such large-scale quantum networks will require photonic interconnects to generate and sustain entangled states across localized nodes. Previously, three-node distributed Greenberger-Horne-Zeilinger (GHZ) states have been generated between solid-state qubits and atomic ensembles, but not yet in the platform of individual atomic qubits, which can be replicated, detected, and individually controlled with high fidelity. Here we report the first fully-distributed GHZ state of qubits across a three-node quantum network of single atomic memories, using photonic interconnects. We achieve a bounded fidelity of $0.841(17) \leq \mathcal{F} \leq 0.881(17)$ at an entanglement generation rate of 0.095(5)/sec and measure a clear violation of Mermin's inequality while closing the detection loophole for the first time in a fully-distributed multipartite entangled state.

quant-ph

Photonic Networking of Quantum Memories in High-Dimensions

Quantum networking enables the exchange of quantum information between physically separated quantum systems, which has applications ranging from quantum computing to unconditionally secure communication. Such quantum information is generally represented by two-level quantum systems or qubits. Here, we demonstrate a quantum network of high-dimensional (HD) quantum memories or ``qudits" stored in individual atoms. The interference and detection of HD time-bin encoded single photons emitted from atomic qudit memories heralds maximally-entangled Bell states across pairs of atomic qudit levels. This approach expands the quantum information capacity of a quantum network while improving the entanglement success fraction beyond the standard 50\% limit of qubit-based measurement protocols.

quant-ph

Non-invasive mid-circuit measurement and reset on atomic qubits

Mid-circuit measurement and reset of subsets of qubits is a crucial ingredient of quantum error correction and many quantum information applications. Measurement of atomic qubits is accomplished through resonant fluorescence, which typically disturbs neighboring atoms due to photon scattering. We propose and prototype a new scheme for measurement that provides both spatial and spectral isolation by using tightly-focused individual laser beams and narrow atomic transitions. The unique advantage of this scheme is that all operations are applied exclusively to the read-out qubit, with negligible disturbance to the other qubits of the same species and little overhead. In this letter, we pave the way for non-invasive and high fidelity mid-circuit measurement and demonstrate all key building blocks on a single trapped barium ion.

quant-ph

Entanglement fidelity limits of photonically-networked atomic qubits from recoil and timing

The remote entanglement of two atomic quantum memories through photonic interactions is accompanied by atomic momentum recoil. When the interactions occur at different times, such as from the random emission over the lifetime of the atomic excited state, the difference in recoil timing can expose ``which-path'' information and ultimately lead to decoherence. Time-bin encoded photonic qubits can be particularly sensitive to asynchronous recoil timing. In this paper we study the limits of entanglement fidelity in atomic systems due to recoil and other timing imbalances and show how these effects can be suppressed or even eliminated through proper experimental design.

quant-ph

High-fidelity remote entanglement of trapped atoms mediated by time-bin photons

Photonic interconnects between quantum processing nodes are likely the only way to achieve large-scale quantum computers and networks. The bottleneck in such an architecture is the interface between well-isolated quantum memories and flying photons. We establish high-fidelity entanglement between remotely separated trapped atomic qubit memories, mediated by photonic qubits stored in the timing of their pulses. Such time-bin encoding removes sensitivity to polarization errors, enables long-distance quantum communication, and is extensible to quantum memories with more than two states. Using a measurement-based error detection process and suppressing a fundamental source of error due to atomic recoil, we achieve an entanglement fidelity of 97% and show that fidelities beyond 99.9% are feasible.

quant-ph

Fast photon-mediated entanglement of continuously-cooled trapped ions for quantum networking

We entangle two co-trapped atomic barium ion qubits by collecting single visible photons from each ion through in-vacuo 0.8 NA objectives, interfering them through an integrated fiber-beamsplitter and detecting them in coincidence. This projects the qubits into an entangled Bell state with an observed fidelity lower bound of F > 94%. We also introduce an ytterbium ion for sympathetic cooling to remove the need for recooling interruptions and achieve a continuous entanglement rate of 250 1/s.

quant-ph

Ion Trap with In-Vacuum High Numerical Aperture Imaging for a Dual-Species Modular Quantum Computer

Photonic interconnects between quantum systems will play a central role in both scalable quantum computing and quantum networking. Entanglement of remote qubits via photons has been demonstrated in many platforms; however, improving the rate of entanglement generation will be instrumental for integrating photonic links into modular quantum computers. We present an ion trap system that has the highest reported free-space photon collection efficiency for quantum networking. We use a pair of in-vacuum aspheric lenses, each with a numerical aperture of 0.8, to couple 10% of the 493 nm photons emitted from a $^{138}$Ba$^+$ ion into single-mode fibers. We also demonstrate that proximal effects of the lenses on the ion position and motion can be mitigated.

quant-ph

Determination of the scalar and vector polarizabilities of the cesium $6s \ ^2S_{1/2} \rightarrow 7s \ ^2S_{1/2}$ transition and implications for atomic parity non-conservation

Using recent high-precision measurements of electric dipole matrix elements of atomic cesium, we make an improved determination of the scalar ($α$) and vector ($β$) polarizabilities of the cesium $6s \ ^2S_{1/2} \rightarrow 7s \ ^2S_{1/2} $ transition calculated through a sum-over-states method. We report values of $α= -268.82 \ (30) \ a_0^3$ and $β= 27.139 \ (42) \ a_0^3$ with the highest precision to date. We find a discrepancy between our value of $β$ and the past preferred value, resulting in a significant shift in the value of the weak charge $Q_w$ of the cesium nucleus. Future work to resolve the differences in the polarizability will be critical for interpretation of parity non-conservation measurements in cesium, which have implications for physics beyond the Standard Model.

physics.atom-ph

Measurement of the radial matrix elements for the $6s ^2S_{1/2} \rightarrow 7p ^2P_J$ transitions in cesium

We report measurements of the electric dipole matrix elements of the $^{133}$Cs $\ $ $6s\,^2S_{1/2} \rightarrow 7p\,^2P_{1/2}$ and $6s\,^2S_{1/2} \rightarrow 7p\,^2P_{3/2}$ transitions. Each of these determinations is based on direct, precise comparisons of the absorption coefficients between two absorption lines. For the $\langle 6s\,^2S_{1/2}||r|| 7p\,^2P_{3/2} \rangle$ matrix element, we measure the ratio of the absorption coefficient on this line with that of the D$_1$ transition, $6s\,^2S_{1/2} \rightarrow 6p\,^2P_{1/2}$. The matrix element of the D$_1$ line has been determined with high precision previously by many groups. For the $\langle 6s\,^2S_{1/2}||r|| 7p\,^2P_{1/2} \rangle$ matrix element, we measure the ratio of the absorption coefficient on this line with that of the $6s\,^2S_{1/2} \rightarrow 7p\,^2P_{3/2}$ transition. Our results for these matrix elements are $\langle 6s\,^2S_{1/2}||r|| 7p\,^2P_{3/2} \rangle = 0.57417 \: (57)~a_0$ and $\langle 6s\,^2S_{1/2}||r|| 7p\,^2P_{1/2} \rangle = 0.27810 \: (45)~a_0$. These measurements have implications for the interpretation of parity nonconservation in atoms.

physics.atom-ph

Measurement of the lifetime of the $7s^2S_{1/2} $ state in atomic cesium using asynchronous gated detection

We report a measurement of the lifetime of the cesium $7s\,^2S_{1/2}$ state using time-correlated single-photon counting spectroscopy in a vapor cell. We excite the atoms using a Doppler-free two-photon transition from the $6s\,^2S_{1/2}$ ground state, and detect the 1.47$μ$m photons from the spontaneous decay of the $7s\,^2S_{1/2}$ to the $6p\,^2P_{3/2}$ state. We use a gated single photon detector in an asynchronous mode, allowing us to capture the fluorescence profile for a window much larger than the detector gate length. Analysis of the exponential decay of the photon count yields a $7s\,^2S_{1/2}$ lifetime of 48.28$\pm$0.07ns, an uncertainty of 0.14%. These measurements provide sensitive tests of theoretical models of the Cs atom, which play a central role in parity violation measurements.

physics.atom-ph

Measurement of the Stark shift of the $6s^2S_{1/2} \rightarrow 7p^2P_{J} $ transitions in atomic cesium

We report measurements of the Stark shift of the cesium $6s \: ^2S_{3/2} \rightarrow 7p \: ^2P_{3/2} $ and the $6s \: ^2S_{1/2} \rightarrow 7p \: ^2P_{1/2} $ transitions at $λ= 456$ nm and 459 nm, respectively, in an atomic beam. From these, we determine the static scalar polarizability for both 7P states, and the tensor polarizability for the 7P$_{3/2}$ state. The fractional uncertainty of the scalar polarizabilites is $\sim$0.18\%, while that of the tensor term is 0.66\%. These measurements provide sensitive tests of theoretical models of the Cs atom, which has played a central role in parity nonconservation measurements.

physics.atom-ph

Electric dipole matrix elements for the $6p\ ^2P_J \rightarrow 7s\ ^2S_{1/2}$ transition in atomic cesium

We report a measurement of the ratio of electric dipole transition matrix elements of cesium for the $6p\,^2P_{1/2} \rightarrow 7s\,^2S_{1/2}$ and $6p\,^2P_{3/2} \rightarrow 7s\,^2S_{1/2}$ transitions. We determine this ratio of matrix elements through comparisons of two-color, two-photon excitation rates of the $7s\,^2S_{1/2}$ state using laser beams with polarizations parallel to one another vs.\ perpendicular to one another. Our result of $R \equiv \langle 7s\ ^2S_{1/2} || r || 6p\ ^2P_{3/2} \rangle / \langle 7s\ ^2S_{1/2} || r || 6p\ ^2P_{1/2} \rangle = 1.5272 \ (17)$ is in excellent agreement with a theoretical prediction of $R=1.5270 \ (27)$. Moreover, the accuracy of the experimental ratio is sufficiently high to differentiate between various theoretical approaches. To our knowledge, there are no prior experimental measurements of $R$. Combined with our recent determination of the lifetime of the $7s\,^2S_{1/2}$ state, we determine reduced matrix elements for these two transitions, $\langle 7s\ ^2S_{1/2} || r || 6p\ ^2P_{3/2} \rangle = -6.489 \ (5) \ a_0$ and $\langle 7s\ ^2S_{1/2} || r || 6p\ ^2P_{1/2} \rangle = -4.249 \ (4) \ a_0$. These matrix elements are also in excellent agreement with theoretical calculations. These measurements improve knowledge of Cs properties needed for parity violation studies and provide benchmarks for tests of high-precision theory.

physics.atom-ph

Gain measurement scheme for precise determination of atomic parity violation through two-pathway coherent control

Precision measurements of parity non-conserving (PNC) interactions in atoms, molecules and ions can lead to the discovery of new physics beyond the standard model and understanding of weak-force induced interactions in the nucleus. In this paper, we propose and analyze a novel atomic parity violation measurement scheme for a forbidden transition where we combine a two-pathway coherent control mechanism with probe gain techniques. We detail a feasible experimental geometry for $6S_{1/2}\rightarrow 7S_{1/2}$ transitions in a cesium vapor cell, and consider the statistical noise of such a measurement under reasonable laboratory conditions. We estimate the signal-to-noise ratio to be approaching $\sim2.3/\sqrt{Hz}$. This scheme, with low expected systematic errors, would allow for precise measurements in cesium and other heavy metal systems.

physics.atom-ph