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Georgia T. Papadakis

Publications and source records attributed to Georgia T. Papadakis.

28 records · Page 2Linked to original sources

Experimental Demonstration of Dynamic Thermal Regulation using Vanadium Dioxide Thin Films

We present an experimental demonstration of passive, dynamic thermal regulation in a solid-state system with temperature-dependent thermal emissivity switching. We achieve this effect using a multilayered device, comprised of a vanadium dioxide (VO2) thin film on a silicon substrate with a gold back reflector. We experimentally characterize the optical properties of the VO2 film and use the results to optimize device design. Using a calibrated, transient calorimetry experiment we directly measure the temperature fluctuations arising from a time-varying heat load. Under laboratory conditions, we find that the device regulates temperature better than a constant emissivity sample. We use the experimental results to validate our thermal model, which can be used to predict device performance under the conditions of outer space. In this limit, thermal fluctuations are halved with reference to a constant-emissivity sample.

physics.app-ph↗

Nonreciprocal metamaterial obeying time-reversal symmetry

We introduce a class of non-Hermitian systems that break electromagnetic reciprocity while preserving time-reversal symmetry, and describe its novel polarization dynamics. We show that this class of systems can be realized using van der Waals heterostructures involving transition-metal dichalcogenides (TMDs). Our work provides a path towards achieving strong optical nonreciprocity and polarization-dependent directional amplification using compact, large-area and magnet-free structures.

physics.optics↗

Nonreciprocal radiative heat transfer between two planar bodies

We develop an analytical framework for nonreciprocal radiative heat transfer in two-body planar systems. Based on our formalism, we identify effects that are uniquely nonreciprocal in near-field heat transfer in planar systems. We further introduce a general thermodynamic constraint that is applicable for both reciprocal and nonreciprocal planar systems, in agreement with the second law of thermodynamics. We numerically demonstrate our findings in an example system consisting of magneto-optical materials. Our formalism applies to both near- and far-field regimes, opening opportunities for exploiting nonreciprocity in two-body radiative heat transfer systems.

physics.optics↗

Broadening near-field emission for performance enhancement in thermophotovoltaics

The conventional notion for achieving high efficiency in thermophotovoltaics (TPVs) is to use a monochromatic emission at a photon energy corresponding to the band gap of the cell. Here, we prove theoretically that such a notion is only accurate under idealized conditions, and further show that when non-radiative recombination is taken into account, efficiency improvement can be achieved by broadening the emission spectrum, due to an enhancement in the open-circuit voltage. Broadening the emission spectrum also improves the electrical power density, by increasing the short-circuit current. To practically illustrate these findings, we focus on surface polariton-mediated near-field TPVs. We propose a versatile design strategy for broadening the emission spectrum via stacking of multiple plasmonic thin film layers. As an example, we consider a realistic ITO/InAs TPV, and predict a conversion efficiency of $50\%$ simultaneously with a power density of nearly $80$ W$/\mathrm{cm}^2$ at a $1300$ K emitter temperature. The performance of our proposed system far exceeds previous works in similar systems using a single plasmonic layer emitter.

physics.optics↗

Experimental demonstration of tunable graphene hyperbolic metamaterial

Tuning the macroscopic dielectric response on demand holds potential for actively tunable metaphotonics and optical devices. In recent years, graphene has been extensively investigated as a tunable element in nanophotonics. Significant theoretical work has been devoted on the tuning the hyperbolic properties of graphene/dielectric heterostructures, however, until now, such a motif has not been demonstrated experimentally. Here we focus on a graphene/polaritonic dielectric metamaterial, with strong optical resonances arising from the polar response of the dielectric, which are, in general, difficult to actively control. By controlling the doping level of graphene via external bias we experimentally demonstrate a wide range of tunability from a Fermi level of EF = 0 eV to EF = 0.5 eV, which yields an effective epsilon-near-zero crossing and tunable dielectric properties, verified through spectroscopic ellipsometry and transmission measurements.

physics.app-ph↗

Gate-tunable near-field heat transfer

Active control over the flow of heat in the near-field holds promise for nanoscale thermal management, with applications in refrigeration, thermophotovoltaics, and thermal circuitry. Analogously to its electronic counterpart, the metal-oxide-semiconductor (MOS) capacitor, we propose a thermal switching mechanism based on accumulation and depletion of charge carriers in an ultra-thin plasmonic film, via application of external bias. In our proposed configuration, the plasmonic film is placed on top of a polaritonic dielectric material that provides a surface phonon polariton (SPhP) thermal channel, while also ensuring electrical insulation for application of large electric fields. The variation of carrier density in the plasmonic film enables the control of the surface plasmon polariton (SPP) thermal channel. We show that the interaction of the SPP with the SPhP significantly enhances the net heat transfer. We study SiC as the oxide and explore three classes of gate-tunable plasmonic materials: transparent conductive oxides, doped semiconductors, and graphene, and theoretically predict contrast ratios as high as 225%.

physics.app-ph↗

Ultra-light Å-scale Optimal Optical Reflectors

High-reflectance in many state-of-the-art optical devices is achieved with noble metals. However, metals are limited by losses, and for certain applications, by their high mass density. Using a combination of ab initio and optical transfer matrix calculations, we evaluate the behavior of graphene-based Å-scale metamaterials and find that they could act as nearly-perfect reflectors in the mid-long wave infrared (IR) range. The low density of states for electron-phonon scattering and interband excitations leads to unprecedented optical properties for graphene heterostructures, especially alternating atomic layers of graphene and hexagonal boron nitride, at wavelengths greater than $10~μ$m. At these wavelengths, these materials exhibit reflectivities exceeding 99.7% at a fraction of the weight of noble metals, as well as plasmonic mode confinement and quality factors that are greater by an order of magnitude compared to noble metals. These findings hold promise for ultra-compact optical components and waveguides for mid-IR applications. Moreover, unlike metals, the photonic properties of these heterostructures could be actively tuned via chemical and/or electrostatic doping, providing exciting possibilities for tunable devices.

cond-mat.mes-hall↗

Optical Magnetism in Planar Metamaterial Heterostructures

Harnessing artificial optical magnetism requires rather complex two- and three-dimensional structures, examples include split-ring and fishnet metamaterials and nanoparticles with non-trivial magnetic properties. By contrast, dielectric properties can be tailored even in planar and pattern-free, one-dimensional (1D) arrangements, for example metal/dielectric multilayer metamaterials. These systems are extensively investigated due to their hyperbolic and plasmonic response, which, however, is considered to be limited to TM polarization, based on the general consensus that they do not possess interesting magnetic properties. In this work, we tackle these two seemingly unrelated issues simultaneously, by proposing conceptually and demonstrating experimentally a mechanism for artificial magnetism in planar, 1D metamaterials. We show experimentally that the magnetic response of metal/high-index dielectric hyperbolic metamaterials can be anisotropic, leading to frequency regimes of magnetic hyperbolic dispersion. We investigate the implications of our results for TE polarization and show that such systems can support TE interface-bound states, analogous to their TM counterparts, surface plasmon polaritons. Our results simplify the structural complexity for tailoring artificial magnetism in lithography-free systems and generalize the concept of plasmonic and hyperbolic properties to encompass both TE and TM polarizations at optical frequencies.

physics.optics↗

Field-effect induced tunability in planar hyperbolic metamaterials

We demonstrate that use of the field effect to tune the effective optical parameters of a layered hyperbolic metamaterial leads to topological transitions in its dispersion characteristics in the optical regime. Field effect gating electrically modulates the permittivity in transparent conductive oxides via changes in the carrier density. These permittivity changes lead to active extreme modulation of ~200% of the effective electromagnetic parameters along with active control of the anisotropic dispersion surface of hyperbolic metamaterials and enable the opening and closing of photonic band gaps.

physics.optics↗

Retrieval of material parameters for uniaxial metamaterials

We present a general method for retrieving the effective tensorial permittivity of any uniaxially anisotropic metamaterial. By relaxing the usually imposed condition of non-magnetic metal/dielectric metamaterials, we also retrieve the permeability tensor and show that hyperbolic metamaterials exhibit a strong diamagnetic response in the visible regime. We obtain global material parameters, directly measurable with spectroscopic ellipsometry and distinguishable from mere wave parameters, by using the generalized dispersion equation for uniaxial crystals along with existing homogenization methods. Our method is analytically and experimentally verified for Ag/SiO2 planar metamaterials with varying number of layers and compared to the effective medium theory. We also propose an experimental method for retrieving material parameters using methods other than ellipsometry.

cond-mat.mes-hall↗