SearcharxivSearch

arXiv subjects

Gergely Nemeth

Publications and source records attributed to Gergely Nemeth.

3 recordsLinked to original sources

Step-scan interferometry for high-fidelity hyperspectral nanoscopy

Fourier transform infrared nanospectroscopy (nano-FTIR) is a novel, increasingly adopted characterization method that leverages decades of established knowledge in infrared spectroscopy at the nanoscale. It opens up new possibilities in the characterization of composite materials and nanophotonic systems. Besides the rapid adoption and new possibilities, the nanoscale nature of these measurements poses new challenges for infrared spectroscopy. The current implementations of hyperspectral image acquisition at high spatial resolution suffer from significant artifacts due to thermal instabilities, which heavily affect positioning. As a result, the spatial and spectral fidelity of the measurements can be unreliable for long acquisitions. Here, we propose a new nano-FTIR measurement methodology based on step-scan interferometry and image registration. We demonstrate that the method provides superior spatial fidelity for photonics research and enables the collection of larger datasets, paving the way for bringing machine learning to characterize nanoscale heterogeneity.

physics.optics

Polaritonic Enhancement of Near-field Scattering of Small Molecules Encapsulated in Boron Nitride Nanotubes

Near-field spectroscopy has been extensively applied recently to analyze collective optical properties of materials at the nanoscale. However, vibrations of small molecules were only recognizable in close proximity to a metallic resonator. We show that encapsulation in boron nitride nanotubes (BNNT) enhances the near-field vibrational spectra of C$_{60}$ fullerene, reaching a sensitivity limit of a few hundred molecules. Furthermore, products of chemical reactions inside the tubes can be identified, so long as their vibrational signatures lie in the polariton gap of the BNNT.

physics.app-ph