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Gerhard Berth

Publications and source records attributed to Gerhard Berth.

2 recordsLinked to original sources

Second harmonic study of thermally oxidized mono- and few-layer 2H-MoS2

A comprehensive study of second harmonic generation on thermally oxidized MoS2 flakes with thickness ranging from monolayer up to seven layers is presented. Observing the fundamental nonlinear behavior for non-treated and oxidized MoS2 reveals that oxidation causes significant changes in the second harmonic (SH) response for all investigated structures. Excitation power dependent measurements to analyze the nonlinear behavior with respect to the oxidation time show progressive oxidation within the maximum oxidation time of six hours, under the considered oxidation conditions. Here, polarization dependent measurements reveal the structural changes due to oxidation. Additionally, it is found that the oxidation depth is restricted to the top most layer and the oxidation behavior exhibits a layer dependency. These findings are supported by theoretical band structure calculations. The results demonstrate that the thermal oxidation progress of two dimensional MoS2 can be monitored with non-resonant and non-invasive SH microscopy, by following distinct fingerprints of structural modification in the nonlinear response.

cond-mat.mtrl-sci

Evidence of nonlinear diffusion in KTP waveguides

Integrated $χ^{(2)}$ devices are a widespread tool for the generation and manipulation of light fields, since they exhibit high efficiency, small footprint and the ability to interface them with fibre networks. Surprisingly many things are not fully understood until now, in particular the fabrication of structures in potassium titanyl phosphate (KTP). A thorough understanding of the fabrication process and analysis of spatial properties is crucial for the realization and the engineering of high efficiency devices for quantum applications. In this paper we present our studies on rubidium-exchanged waveguides fabricated in KTP. Employing energy dispersive X-ray spectroscopy (EDX), we analysed a set of waveguides fabricated with different production parameters in terms of time and temperature. We find that the waveguide depth is dependent on their widths by reconstructing the waveguide depth profiles. Narrower waveguides are deeper, contrary to the theoretical model usually employed. Moreover, we found that the variation of the penetration depth with the waveguide width is stronger at higher temperatures and times. We attribute this behaviour to stress-induced variation in the diffusion process.

physics.app-ph