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Gerhard G Paulus

Publications and source records attributed to Gerhard G Paulus.

2 recordsLinked to original sources

Laser-driven high-flux source of coherent quasi-monochromatic extreme ultraviolet radiation for coincidence spectroscopy

We present a source of coherent extreme ultraviolet (XUV) radiation with a flux of 10$^{13}$ photons per second at 26.5 eV. The source is based on high-harmonic generation (HHG) in argon and pumped by a frequency-doubled 100 kHz repetition rate fiber laser providing 30 fs pulses centered at 515 nm. We report on the characterization of the source and the generated XUV radiation using optical imaging and photoelectron spectroscopy. The generated radiation is quasi-monochromatized using a suitably coated XUV mirror and used for coincidence spectroscopy of ions and electrons generated from a cold gas target. The high intensity of the focused XUV pulses is confirmed by the observation of two-photon double ionization in argon. Moreover, we demonstrate the capability to perform pump-probe experiments using XUV and visible laser pulses.

physics.atom-ph

Coincidence measurement of two-photon double ionization of argon through an autoionizing resonance

We present coincidence measurements of two-photon double-ionization (TPDI) of argon driven by femtosecond pulses tunable around 26.5 eV photon energy, which are obtained from a high-harmonic generation source. The measured photoelectron spectra are interpreted with regard to three TPDI mechanisms. Theoretical predictions are obtained by an approximate model for direct TPDI and atomic structure calculations, which are implemented into a Monte Carlo simulation. The prevailing mechanism involves the excitation and prompt photoionization of an autoionizing resonance in neutral argon. We provide evidence for pronounced electron-electron interaction in this ultrafast ionization process. Furthermore, we show that the dominant TPDI mechanism can be altered by slight tuning of the photon energy. The present work paves the way for scrutinizing and controlling non-linear photoionization in the extreme ultraviolet using table-top sources.

physics.atom-ph