Searcharxiv⌕ Search

arXiv subjects

Gervasi Herranz

Publications and source records attributed to Gervasi Herranz.

13 recordsLinked to original sources

Interacting quantum geometry from dressed parametric vertices

Quantum geometry has emerged as a powerful framework for understanding topological, optical and transport phenomena, revealing connections between the quantum geometric tensor (QGT) and linear response functions. Building on these developments, recent works formulate quantum geometry so that the parameter space is extended from the Brillouin zone to the space of external perturbing fields that modify the ground state. Here we develop a self-consistent diagrammatric route to determine the QGT for generic parameter spaces, including collective fluctuations or structural distortions. With this in view, we generalize previous approaches to build the geometric tensor from interacting vertex correlations that provide the spectral metric and curvature. The formalism presented here extends the interaction-dressed vertex approach (previously applied to electromagnetic responses in momentum space) to collective electronic and structural deformation fields, complementing ongoing efforts to quantify many-body contributions to quantum geometry.

cond-mat.str-el↗

Geometric curvature driven by many-body collective fluctuations

Quantum geometry characterizes the variation of wavefunctions in momentum space through their overlaps and relative phases, providing a general framework for understanding many transport and optical properties. It is generally formulated in terms of interband matrix elements, which, entering the response functions, allow obtaining experimental access to the quantum geometric tensor. Recently, it has been emphasized that quantum geometry can also be interpreted in terms of quantum dipole fluctuations in the ground state driven by interband mixing. Here, we extend this picture to include contributions from many-body collective fluctuations, in which propagators and response vertices are dressed dynamically by the interaction with collective modes. Focusing on the Berry curvature, we show that contributions from collective fluctuations can be experimentally distinguished from bare band-geometric contributions, via specific antisymmetric channels in inelastic scattering spectra. We further identify the non-commutative properties of transverse quantum fluctuations as well as non-local-time interactions as the generators of this dynamical curvature in the susceptibility response.

cond-mat.str-el↗

Obstructed Atomic Limit Topological Protection in C4-Symmetric Photonic Crystals for Optical Communications

Recent developments in photonic topological phases have revealed that protected edge modes can emerge not only from global topological invariants, but also from symmetry-enforced polarization mismatches between distinct bulk phases. In this work, we investigate the capabilities and limitations of a square-lattice ($C_4$-symmetric) photonic crystal composed of a single dielectric material that supports interface-localized modes at the boundary between regions characterized by distinct obstructed atomic limits (OALs). These modes are confined to a common band gap and exhibit high transmission, even in the presence of structural perturbations. Our analysis reveals that the interface modes are stabilized by a mismatch in the position of Wannier centers between the two adjoining crystals. We demonstrate nearly lossless transmission around sharp turns and through localized defects, though the robustness depends asymmetrically on the side of perturbation, reflecting the partial nature of the protection. We also show that increasing the number of photonic crystal periods surrounding the interface enhances both modal confinement and spectral stability. These findings establish polarization mismatch between OALs as a practical and fabrication-compatible mechanism for engineering robust photonic transport in \(C_4\)-symmetric systems.

physics.optics↗

Methodology for Topological Interface Engineering in 2D Photonic Crystals

Topological photonics provides a robust and flexible platform for controlling light, enabling functionalities such as backscattering-immune edge transport and slow-light propagation. In this work, we design and characterize photonic topological interfaces in two-dimensional photonic crystals. We introduce an iterative band connection algorithm that preserves mode symmetry and present a general framework for band symmetry recognition, essential for identifying Z2 topological phases. Design strategies for unit cell geometries are developed to achieve targeted band inversions, overlapping bandgaps, and tailored dispersions. Furthermore, the approach can be readily adapted to specific material platforms and operating wavelengths, including the telecommunication range, by appropriately scaling the lattice parameter as long as absorption remains low. We investigate the trade-off between bandgap size and band flatness, identifying exceptions governed by lattice geometry. Additionally, we demonstrate how photonic crystal periodicity influences the stability of topological modes and enhances unidirectional energy transport.

physics.optics↗

Stoichiometric control of electron mobility and 2D superconductivity at LaAlO$_3$-SrTiO$_3$ interfaces

SrTiO$_3$-based conducting interfaces, which exhibit coexistence of gate-tunable 2D superconductivity and strong Rashba spin-orbit coupling (RSOC), are candidates to host topological superconductive phases. Yet, superconductivity is usually in the dirty limit, which tends to suppress nonconventional pairing and therefore challenges these expectations. Here we report on LaAlO$_3$/SrTiO$_3$ (LAO/STO) interfaces with remarkably large mobility and mean free paths comparable to the superconducting coherence length, approaching the clean limit for superconductivity. We further show that the carrier density, mobility, and formation of the superconducting condensate are controlled by the fine-tuning of La/Al chemical ratio in the LAO film. Interestingly, we find a region in the superconducting phase diagram where the critical temperature is not suppressed below the Lifshitz transition, at odds with previous experimental investigations. These findings point out the relevance of achieving a clean-limit regime to enhance the observation of unconventional pairing mechanisms in these systems

cond-mat.supr-con↗

Jahn-Teller states mixed by spin-orbit coupling in an electromagnetic field

Spin-orbit coupling plays a pivotal role in condensed matter physics. For instance, spin-orbit interactions affect the magnetization and transport dynamics in solids, while spins and momenta are locked in topological matter. Alternatively, spin-orbit entanglement may play an important role in exotic phenomena, like quantum spin liquids in 4d and 5d systems. An interesting question is how electronic states mixed by spin orbit coupling interact with electromagnetic fields, which may hold potential to tune their properties and reveal interesting physics. Motivated by our recent discovery of large gyrotropic signals in some Jahn-Teller manganites, here we explore the interaction of light with spin-mixed states in a d4 transition metal. We show that spin-orbit mixing enables electronic transitions that are sensitive to circularly polarized light, giving rise to a gyrotropic response that increases with spin-orbit coupling. Interestingly, photoexcited transitions that involve spin reversal are behind such gyrotropic resonances. Additionally, we find that the interaction with the electromagnetic field depends strongly on the relative orientation of the propagation of light with respect to Jahn-Teller distortions and spin quantization. We suggest that such interactions offer the opportunity to use electromagnetic waves at optical wavelengths to entangle orbital and spin degrees of freedom. Our approach, which includes a group-theoretical treatment of spin-orbit coupling, has wide applicability and provides a versatile tool to explore the interaction of electromagnetic fields with electronic states in transition metals with arbitrary spin-orbit coupling strength and pointgroup symmetries.

cond-mat.str-el↗

Dynamic control of octahedral rotation in perovskites by defect engineering

Engineering oxygen octahedra rotation patterns in $ABO_3$ perovskites is a powerful route to design functional materials. Here we propose a strategy that exploits point defects that create local electric dipoles and couple to the oxygen sublattice, enabling direct actuation on the rotational degrees of freedom. This approach, which relies on substituting an $A$ site with a smaller ion, paves a way to couple dynamically octahedra rotations to external electric fields. A common antisite defect, $\mathrm{Al_{La}}$ in rhombohedral LaAlO$_3$ is taken as a prototype to validate the idea, with atomistic density functional theory calculations supported with an effective lattice model to simulate the dynamics of switching of the local rotational degrees of freedom to long distances. Our simulations provide an insight of the main parameters that govern the operation of the proposed mechanism, and allow to define guidelines for screening other systems where this approach could be used for tuning the properties of the host material.

cond-mat.mtrl-sci↗

Non-collinear and strongly asymmetric polar moments at back-gated SrTiO3 interfaces

The highly mobile electrons at the interface of SrTiO3 with other oxide insulators, such as LaAlO3 or AlOx, are of great current interest. A vertical gate voltage allows controlling a metal/superconductor-to-insulator transition, as well as electrical modulation of the spin-orbit Rashba coupling for spin-charge conversion. These findings raise important questions about the origin of the confined electrons as well as the mechanisms that govern the interfacial electric field. Here we use infrared ellipsometry and confocal Raman spectroscopy to show that an anomalous polar moment is induced at the interface that is non-collinear, highly asymmetric and hysteretic with respect to the vertical gate electric field. Our data indicate that an important role is played by the electromigration of oxygen vacancies and their clustering at the antiferrodistortive domain boundaries of SrTiO3, which generates local electric and possibly also flexoelectric fields and subsequent polar moments with a large lateral component. Our results open new perspectives for the defect engineering of lateral devices with strongly enhanced and hysteretic local electric fields that can be manipulated with various other parameters, like strain, temperature, or photons.

cond-mat.mtrl-sci↗

Giant topological Hall effect in correlated oxide thin films

Strong electronic correlations can produce remarkable phenomena such as metal-insulator transitions and greatly enhance superconductivity, thermoelectricity, or optical non-linearity. In correlated systems, spatially varying charge textures also amplify magnetoelectric effects or electroresistance in mesostructures. However, how spatially varying spin textures may influence electron transport in the presence of correlations remains unclear. Here we demonstrate a very large topological Hall effect (THE) in thin films of a lightly electron-doped charge-transfer insulator, (Ca, Ce)MnO3. Magnetic force microscopy reveals the presence of magnetic bubbles, whose density vs. magnetic field peaks near the THE maximum, as is expected to occur in skyrmion systems. The THE critically depends on carrier concentration and diverges at low doping, near the metal-insulator transition. We discuss the strong amplification of the THE by correlation effects and give perspectives for its non-volatile control by electric fields.

cond-mat.mtrl-sci↗

Giant Optical Polarization Rotation Induced by Spin-Orbit Coupling in Polarons

We have uncovered a giant gyrotropic magneto-optical response for doped ferromagnetic manganite La2/3Ca1/3MnO3 around the near room-temperature paramagnetic-to-ferromagnetic transition. At odds with current wisdom, where this response is usually assumed to be fundamentally fixed by the electronic band structure, we point to the presence of small polarons as the driving force for this unexpected phenomenon. We explain the observed properties by the intricate interplay of mobility, Jahn-Teller effect and spin-orbit coupling of small polarons. As magnetic polarons are ubiquitously inherent to many strongly correlated systems, our results provide an original, general pathway towards the generation of gigantic gyrotropic responses that can be harnessed for nonreciprocal devices that exploit the polarization of light.

cond-mat.str-el↗

Conducting interfaces between amorphous oxide layers and SrTiO3(110) and SrTiO3(111)

Interfaces between (110) and (111)SrTiO3 (STO) single crystalline substrates and amorphous oxide layers, LaAlO3 (a-LAO), Y:ZrO2 (a-YSZ), and SrTiO3 (a-STO) become conducting above a critical thickness tc. Here we show that tc for a-LAO is not depending on the substrate orientation, i.e. tc (a-LAO/(110)STO) ~ tc(a-LAO/(111)STO) interfaces, whereas it strongly depends on the composition of the amorphous oxide: tc(a-LAO/(110)STO) < tc(a-YSZ/(110)STO) < tc(a-STO/(110)STO). It is concluded that the formation of oxygen vacancies in amorphous-type interfaces is mainly determined by the oxygen affinity of the deposited metal ions, rather than orientational-dependent enthalpy vacancy formation and diffusion. Scanning transmission microscopy characterization of amorphous and crystalline LAO/STO(110) interfaces shows much higher amount of oxygen vacancies in the former, providing experimental evidence of the distinct mechanism of conduction in these interfaces.

cond-mat.mtrl-sci↗

High mobility conduction at (110) and (111) LaAlO3/SrTiO3 interfaces

In recent years, striking discoveries have revealed that two-dimensional electron liquids (2DEL) confined at the interface between oxide band-insulators can be engineered to display a high mobility transport. The recognition that only few interfaces appear to suit hosting 2DEL is intriguing and challenges the understanding of these emerging properties not existing in bulk. Indeed, only the neutral TiO2 surface of (001)SrTiO3 has been shown to sustain 2DEL. We show that this restriction can be surpassed: (110) and (111) surfaces of SrTiO3 interfaced with epitaxial LaAlO3 layers, above a critical thickness, display 2DEL transport with mobilities similar to those of (001)SrTiO3. Moreover we show that epitaxial interfaces are not a prerequisite: conducting (110) interfaces with amorphous LaAlO3 and other oxides can also be prepared. These findings open a new perspective both for materials research and for elucidating the ultimate microscopic mechanism of carrier doping.

cond-mat.mtrl-sci↗

Electron energy loss spectroscopy determination of Ti oxidation state at the (001) LaAlO3/SrTiO3 interface as a function of LaAlO3 growth conditions

At the (001) interface between the two band-insulators LaAlO3 and SrTiO3, a high-mobility electron gas may appear, which has been the object of numerous works over the last four years. Its origin is a subject of debate between the interface polarity and unintended doping. Here we use electron energy loss 'spectrum images', recorded in cross-section in a scanning transmission electron microscope, to analyse the Ti3+ ratio, characteristic of extra electrons. We find an interface concentration of Ti3+ that depends on growth conditions.

cond-mat.mtrl-sci↗