arXiv subjects

Giacomo Bighin

Publications and source records attributed to Giacomo Bighin.

15 recordsLinked to original sources

arXiv2026

Crossing the Rotational Sound Barrier in a Quantum Solvent

Molecules embedded in superfluids provide an experimentally controllable platform for investigating impurity physics. Here, we investigate a driven molecule rotating in a superfluid environment, including helium and Bose--Einstein condensates, at rotation frequencies similar to the bath dynamics. Within the experimentally relevant platform of an optical centrifuge, we show that the rotor remains localized up to a characteristic harmonic frequency that can realistically exceed the excitation energies of the bath, enabling access to ultrafast rotating impurities. In the co-rotating frame, the bath excitations experience a rotational Doppler shift, generating angular-momentum-resolved resonances absent in equilibrium angulon theory. We identify a dissipative rotational sound barrier at which the molecule resonantly emits bath excitations and undergoes strong angular momentum exchange with the surrounding medium. Overall, we establish the dynamical phase diagram of the driven rotor in a quantum solvent and introduce a generic platform for investigating fast driven rotating impurities in quantum many-body systems.

cond-mat.quant-gas↗

arXiv2026

Optical centrifuge as a probe of strong dissipative coupling between a molecular rotor and superfluid helium

A macroscopic manifestation of superfluidity is that objects moving through liquid helium experience negligible friction below the Landau critical velocity. How this frictionless motion breaks down at the nanoscale remains an open question. Molecules embedded in helium nanodroplets represent a well-controlled system for studying this breakdown, yet none has reached the regime of strong dissipative coupling, when energy transfer from the molecule to the superfluid dominates the observed dynamics. Molecular rotation, induced by short laser pulses, offer a suitable probe to reach rotational energies in the range of the roton gap, where superfluid helium supports a large number of elementary excitations. However, the solvation shell around a rotating molecule caps the energy reachable by a free rotor after impulsive excitation well below the roton excitation energy. Here we show that continuous driving with an ultraslow optical centrifuge overcomes this limitation: the strong field dresses the molecule into pendular states whose energies fall within the spectrum of the collective excitations of the superfluid, placing the system in the strong-dissipation regime. The resulting rapid thermalization locks the molecule to the rotating field until the rotation-induced level splittings overtake the thermalization rate, beyond which the molecular alignment is progressively lost. Our approach offers a direct measurement of the molecule-bath coupling in a quantum fluid.

quant-ph↗

arXiv2025

Resonantly enhanced superconductivity mediated by spinor condensates

Achieving strong interactions in fermionic many-body systems is a major theme of research in condensed matter physics. It is well-known that interactions between fermions can be mediated through a bosonic medium, such as a phonon bath or Bose-Einstein condensate (BEC). Here we show that such induced attraction can be resonantly enhanced when the bosonic medium is a two-component spinor BEC. The strongest interaction is achieved by tuning the boson-boson scattering to the quantum critical spinodal point of the BEC where the sound velocity vanishes. The fermion pairing gap and the superconducting critical temperature can thus be dramatically enhanced. We propose two experimental realizations of this scenario, with exciton-polariton systems in two-dimensional semiconductors and ultracold atomic Bose-Fermi mixtures.

cond-mat.quant-gas↗

arXiv2025

Environment-limited transfer of angular momentum in Bose liquids

Impurity motion in a many-body environment has been a central issue in the field of low-temperature physics for decades. In bosonic quantum fluids, the onset of a drag force experienced by point-like objects is due to collective environment excitations, driven by the exchange of linear momentum between the impurity and the many-body bath. In this work we consider a rotating impurity, with the aim of exploring how angular momentum is exchanged with the surrounding bosonic environment. In order to elucidate this issues, we employ a quasiparticle approach based on the angulon theory, which allows us to effectively deal with the non-trivial algebra of quantized angular momentum in presence of a many-body environment. We uncover how impurity dressing by environmental excitations can establish an exchange channel, whose effectiveness crucially depends on the initial state of the impurity. Remarkably, we find that there is a critical value of initial angular momentum, above which this channel effectively freezes.

cond-mat.quant-gas↗

arXiv2024

Universal scaling in real dimension

The concept of universality has shaped our understanding of many-body physics, but is mostly limited to homogenous systems. Here, we present a study of universality on a non-homogeneous graph, the long-range diluted graph (LRDG). Its scaling theory is controlled by a single parameter, the spectral dimension $d_{s}$, which plays the role of the relevant parameter on complex geometries. The graph under consideration allows us to tune the value of the spectral dimension continuously also to noninteger values and to find the universal exponents as continuous functions of the dimension. By means of extensive numerical simulations, we probe the scaling exponents of a simple instance of $O(\mathcal{N})$ symmetric models on the LRDG showing quantitative agreement with the theoretical prediction of universal scaling in real dimensions.

cond-mat.stat-mech↗

arXiv2023

Non-equilibrium dynamics of dipolar polarons

We study the out-of-equilibrium quantum dynamics of dipolar polarons, i.e., impurities immersed in a dipolar Bose-Einstein condensate, after a quench of the impurity-boson interaction. We show that the dipolar nature of the condensate and of the impurity results in anisotropic relaxation dynamics, in particular, anisotropic dressing of the polaron. More relevantly for cold-atom setups, quench dynamics is strongly affected by the interplay between dipolar anisotropy and trap geometry. Our findings pave the way for simulating impurities in anisotropic media utilizing experiments with dipolar mixtures.

cond-mat.quant-gas↗

arXiv2022

A simple model for high rotational excitations of molecules in a superfluid

We present a simple quantum mechanical model describing excited rotational states of molecules in superfluid helium nanodroplets, as recently studied in non-adiabatic molecular alignment experiments [Cherepanov et al., Phys. Rev. A 104, L061303 (2021)]. We show that a linear molecule immersed in a superfluid can be seen as an effective symmetric top, similar to the rotational structure of radicals, such as OH or NO, but with the angular momentum of the superfluid playing the role of the electronic angular momentum in free molecules. The model allows to evaluate the effective rotational and centrifugal distortion constants for a broad range of species and to explain the crossover between light and heavy molecules in superfluid $^4$He in terms of the many-body wavefunction structure. Most important, the simple theory allows to answer the question as to what happens when the rotational angular momentum of the molecule increases beyond the lowest excited states accessible by infrared spectroscopy. Some of the above mentioned insights can be acquired by analyzing a simple 2x2 matrix.

physics.chem-ph↗

arXiv2021

An impurity in a heteronuclear two-component Bose mixture

We study the fate of an impurity in an ultracold heteronuclear Bose mixture, focusing on the experimentally relevant case of a $^{41}$K-$^{87}$Rb mixture, with the impurity in a $^{41}$K hyperfine state. Our work provides a comprehensive description of an impurity in a BEC mixture with contact interactions across its phase diagram. We present results for the miscible and immiscible regimes, as well as for the impurity in a self-bound quantum droplet. Here, varying the interactions, we find novel, exotic states where the impurity localizes either at the center or at the surface of the droplet.

cond-mat.quant-gas↗

arXiv2021

Excited rotational states of molecules in a superfluid

We combine experimental and theoretical approaches to explore excited rotational states of molecules embedded in helium nanodroplets using CS$_2$ and I$_2$ as examples. Laser-induced nonadiabatic molecular alignment is employed to measure spectral lines for rotational states extending beyond those initially populated at the 0.37 K droplet temperature. We construct a simple quantum mechanical model, based on a linear rotor coupled to a single-mode bosonic bath, to determine the rotational energy structure in its entirety. The calculated and measured spectral lines are in good agreement. We show that the effect of the surrounding superfluid on molecular rotation can be rationalized by a single quantity -- the angular momentum, transferred from the molecule to the droplet.

physics.chem-ph↗

arXiv2020

Rotational coherence spectroscopy of molecules in helium nanodroplets: Reconciling the time and the frequency domains

Alignment of OCS, CS$_2$ and I$_2$ molecules embedded in helium nanodroplets is measured as a function of time following rotational excitation by a non-resonant, comparatively weak ps laser pulse. The distinct peaks in the power spectra, obtained by Fourier analysis, are used to determine the rotational, B, and centrifugal distortion, D, constants. For OCS, B and D match the values known from IR spectroscopy. For CS$_2$ and I$_2$, they are the first experimental results reported. The alignment dynamics calculated from the gas-phase rotational Schrödinger equation, using the experimental in-droplet B and D values, agree in detail with the measurement for all three molecules. The rotational spectroscopy technique for molecules in helium droplets introduced here should apply to a range of molecules and complexes.

physics.atm-clus↗

arXiv2019

Intermolecular forces and correlations mediated by a phonon bath

Inspired by the possibility to experimentally manipulate and enhance chemical reactivity in helium nanodroplets, we investigate the effective interaction and the resulting correlations between two diatomic molecules immersed in a bath of bosons. By analogy with the bipolaron, we introduce the \emph{biangulon} quasiparticle describing two rotating molecules that align with respect to each other due to the effective attractive interaction mediated by the excitations of the bath. We study this system in different parameter regimes and apply several theoretical approaches to describe its properties. Using a Born-Oppenheimer approximation, we investigate the dependence of the effective intermolecular interaction on the rotational state of the two molecules. In the strong-coupling regime, a product-state ansatz shows that the molecules tend to have a strong alignment in the ground state. To investigate the system in the weak-coupling regime, we apply a one-phonon excitation variational ansatz, which allows us to access the energy spectrum. In comparison to the angulon quasiparticle, the biangulon shows shifted angulon instabilities and an additional spectral instability, where resonant angular momentum transfer between the molecules and the bath takes place. These features are proposed as an experimentally observable signature for the formation of the biangulon quasiparticle. Finally, by using products of single angulon and bare impurity wave functions as basis states, we introduce a diagonalization scheme that allows us to describe the transition from two separated angulons to a biangulon as a function of the distance between the two molecules.

cond-mat.mes-hall↗

arXiv2019

BKT-paired phase in coupled XY models

We study the effect of a linear tunneling coupling between 2D systems, each separately exhibiting the topological Berezinskii-Kosterlitz-Thouless (BKT) transition. In the uncoupled limit, there are two phases: one where the 1-body correlation functions are algebraically decaying and the other with exponential decay. When the linear coupling is turned on, a third BKT-paired phase emerges, in which 1-body correlations are exponentially decaying, while 2-body correlation functions exhibit power-law decay. We perform numerical simulations in the paradigmatic case of two coupled XY models at finite temperature, finding that for any finite value of the interlayer coupling, the BKT-paired phase is present. We provide a picture of the phase diagram using a renormalization group approach.

cond-mat.stat-mech↗

arXiv2019

Far-from-equilibrium dynamics of angular momentum in a quantum many-particle system

We use laser-induced rotation of single molecules embedded in superfluid helium nanodroplets to reveal angular momentum dynamics and transfer in a controlled setting, under far-from-equilibrium conditions. As an unexpected result, we observe pronounced oscillations of time-dependent molecular alignment that have no counterpart in gas-phase molecules. Angulon theory reveals that these oscillations originate from the unique rotational structure of molecules in He droplets and quantum-state-specific transfer of rotational angular momentum to the many-body He environment on picosecond timescales. Our results pave the way to understanding collective effects of macroscopic angular momentum exchange in solid state systems in a bottom-up fashion.

physics.atm-clus↗

arXiv2018

Variational approaches to quantum impurities: from the Fröhlich polaron to the angulon

Problems involving quantum impurities, in which one or a few particles are interacting with a macroscopic environment, represent a pervasive paradigm, spanning across atomic, molecular, and condensed-matter physics. In this paper we introduce new variational approaches to quantum impurities and apply them to the Fröhlich polaron -- a quasiparticle formed out of an electron (or other point-like impurity) in a polar medium, and to the angulon -- a quasiparticle formed out of a rotating molecule in a bosonic bath. We benchmark these approaches against established theories, evaluating their accuracy as a function of the impurity-bath coupling.

cond-mat.mes-hall↗

arXiv2017

Diagrammatic approach to orbital quantum impurities interacting with a many-particle environment

Recently it was shown that an impurity exchanging orbital angular momentum with a surrounding bath can be described in terms of the angulon quasiparticle [Phys. Rev. Lett. 118, 095301 (2017)]. The angulon consists of a quantum rotor dressed by a many-particle field of boson excitations, and can be formed out of, for example, a molecule or a nonspherical atom in superfluid helium, or out of an electron coupled to lattice phonons or a Bose condensate. Here we develop an approach to the angulon based on the path-integral formalism, which sets the ground for a systematic, perturbative treatment of the angulon problem. The resulting perturbation series can be interpreted in terms of Feynman diagrams, from which, in turn, one can derive a set of diagrammatic rules. These rules extend the machinery of the graphical theory of angular momentum - well known from theoretical atomic spectroscopy - to the case where an environment with an infinite number of degrees of freedom is present. In particular, we show that each diagram can be interpreted as a 'skeleton', which enforces angular momentum conservation, dressed by an additional many-body contribution. This connection between the angulon theory and the graphical theory of angular momentum is particularly important as it allows to systematically and substantially simplify the analytical representation of each diagram. In order to exemplify the technique, we calculate the 1- and 2-loop contributions to the angulon self-energy, the spectral function, and the quasiparticle weight. The diagrammatic theory we develop paves the way to investigate next-to-leading order quantities in a more compact way compared to the variational approaches.

cond-mat.quant-gas↗