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Giancarlo Ruocco

Publications and source records attributed to Giancarlo Ruocco.

At least 91 records · Page 5Linked to original sources

Self-Starting Micromotors in a Bacterial Bath

Micromotors pushed by biological entities, like motile bacteria, constitute a fascinating way to convert chemical energy into mechanical work at the micrometer scale. Here we show, by using numerical simulations, that a properly designed asymmetric object can be spontaneously set into the desired motion when immersed in a chaotic bacterial bath. Our findings open the way to conceive new hybrid microdevices exploiting the mechanical power production of bacterial organisms. Moreover, the system provides an example of how, in contrast with equilibrium thermal baths, the irreversible chaotic motion of active particles can be rectified by asymmetric environments.

cond-mat.soft↗

Ultrashort pulse propagation and the Anderson localization

We investigate the dynamics of a 10 fs light pulse propagating in a random medium by the direct solution of the 3D Maxwell equations. Our approach employs molecular dynamics to generate a distribution of spherical scatterers and a parallel finite-difference time-domain code for the vectorial wave propagation. We calculate the disorder-averaged energy velocity and the decay time of the transmitted pulse Versus the localization length for an increasing refractive index.

physics.optics↗

Observation of a gradient catastrophe generating solitons

We investigate the propagation of a dark beam in a defocusing medium in the strong nonlinear regime. We observe for the first time a shock fan filled with non-interacting one-dimensional grey solitons that emanates from a gradient catastrophe developing around a null of the optical intensity. Remarkably this scenario turns out to be very robust, persisting also when the material nonlocal response averages the nonlinearity over dimensions much larger than the emerging soliton filaments.

physics.optics↗

Condensation in disordered lasers: theory, 3D+1 simulations and experiments

The complex processes underlying the generation of a coherent-like emission from the multiple-scattering of photons and wave-localization in the presence of structural disorder are still mostly un-explored. Here we show that a single nonlinear Schroedinger equation, playing the role of the Schawlow-Townes law for standard lasers, quantitatively reproduces experimental results and three-dimensional time-domain parallel simulations of a colloidal laser system.

physics.optics↗

Free-energy transition in a gas of non-interacting nonlinear wave-particles

We investigate the dynamics of a gas of non-interacting particle-like soliton waves, demonstrating that phase transitions originate from their collective behavior. This is predicted by solving exactly the nonlinear equations and by employing methods of the statistical mechanics of chaos. In particular, we show that a suitable free energy undergoes a metamorphosis as the input excitation is increased, thereby developing a first order phase transition whose measurable manifestation is the formation of shock waves. This demonstrates that even the simplest phase-space dynamics, involving independent (uncoupled) degrees of freedom, can sustain critical phenomena.

nlin.PS↗

Crossover between hydrodynamic and kinetic modes in binary liquid alloys

Inelastic x-ray scattering (IXS) measurements of the dynamic structure factor in liquid Na57K43, sensitive to the atomic-scale coarse graining, reveal a sound velocity value exceeding the long wavelength, continuum value and indicate the coexistence of two phonon-like modes. Applying Generalized Collective Mode (GCM) analysis scheme, we show that the positive dispersion of the sound velocity occurs in a wavelength region below the crossover from hydrodynamic to atom-type excitations and, therefore, it can not be explained as sound propagation over the light specie (Na) network. The present result experimentally proves the existence of positive dispersion in a binary mixture due to a relaxation process, as opposed to fast sound phenomena.

cond-mat.dis-nn↗

Dynamically correlated regions and configurational entropy in supercooled liquids

When a liquid is cooled below its melting temperature, if crystallization is avoided, it forms a glass. This phenomenon, called glass transition, is characterized by a marked increase of viscosity, about 14 orders of magnitude, in a narrow temperature interval. The microscopic mechanism behind the glass transition is still poorly understood. However, recently, great advances have been made in the identification of cooperative rearranging regions, or dynamical heterogeneities, i.e. domains of the liquid whose relaxation is highly correlated. The growth of the size of these domains is now believed to be the driving mechanism for the increase of the viscosity. Recently a tool to quantify the size of these domains has been proposed. We apply this tool to a wide class of materials to investigate the correlation between the size of the heterogeneities and their configurational entropy, i.e. the number of states accessible to a correlated domain. We find that the relaxation time of a given system, apart from a material dependent pre-factor, is a universal function of the configurational entropy of a correlated domain. As a consequence, we find that at the glass transition temperature, the size of the domains and the configurational entropy per unit volume are anti-correlated, as originally predicted by the Adam-Gibbs theory. Finally, we use our data to extract some exponents defined in the framework of the Random First Order Theory, a recent quantitative theory of the glass transition.

cond-mat.dis-nn↗

On the origin of the $λ$-transition in liquid Sulphur

Developing a novel experimental technique, we applied photon correlation spectroscopy using infrared radiation in liquid Sulphur around $T_λ$, i.e. in the temperature range where an abrupt increase in viscosity by four orders of magnitude is observed upon heating within few degrees. This allowed us - overcoming photo-induced and absorption effects at visible wavelengths - to reveal a chain relaxation process with characteristic time in the ms range. These results do rehabilitate the validity of the Maxwell relation in Sulphur from an apparent failure, allowing rationalizing the mechanical and thermodynamic behavior of this system within a viscoelastic scenario.

cond-mat.dis-nn↗

Shocks in nonlocal media

We investigate the formation of collisionless shocks along the spatial profile of a gaussian laser beam propagating in nonlocal nonlinear media. For defocusing nonlinearity the shock survives the smoothing effect of the nonlocal response, though its dynamics is qualitatively affected by the latter, whereas for focusing nonlinearity it dominates over filamentation. The patterns observed in a thermal defocusing medium are interpreted in the framework of our theory.

physics.optics↗

Light diffusion and localization in 3D nonlinear disordered media

Using a 3D Finite-Difference Time-Domain parallel code, we report on the linear and nonlinear propagation of light pulses in a disordered assembly of scatterers, whose spatial distribution is generated by a Molecular Dynamics code; refractive index dispersion is also taken into account. We calculate the static and dynamical diffusion constant of light, while considering a pulsed excitation. Our results are in quantitative agreement with reported experiments, also furnishing evidence of a non-exponential decay of the transmitted pulse in the linear regime and in the presence of localized modes. By using an high power excitation, we numerically demonstrate the ``modulational instability random laser'': at high peak input powers energy is transferred to localized states from the input pulse, via third-order nonlinearity and optical parametric amplification, and this process is signed by a power-dependent non-exponential time-decay of the transmitted pulse.

cond-mat.dis-nn↗

Liquid-like behavior of supercritical fluids

The high frequency dynamics of fluid oxygen have been investigated by Inelastic X-ray Scattering. In spite of the markedly supercritical conditions ($T\approx 2 T_c$, $P>10^2 P_c$), the sound velocity exceeds the hydrodynamic value of about 20%, a feature which is the fingerprint of liquid-like dynamics. The comparison of the present results with literature data obtained in several fluids allow us to identify the extrapolation of the liquid vapor-coexistence line in the ($P/P_c$, $T/T_c$) plane as the relevant edge between liquid- and gas-like dynamics. More interestingly, this extrapolation is very close to the non metal-metal transition in hot dense fluids, at pressure and temperature values as obtained by shock wave experiments. This result points to the existence of a connection between structural modifications and transport properties in dense fluids.

cond-mat.dis-nn↗

Aging of the Nonlinear Optical Susceptibility of colloidal solutions

Using Z-scan and dynamic light scattering measurements we investigate the nonlinear optics response of a colloidal solution undergoing dynamics slowing down with age. We study the high optical nonlinearity of an organic dye (Rhodamine B) dispersed in a water-clay (Laponite) solution, at different clay concentrations (2.0 wt% - 2.6 wt%), experiencing the gelation process. We determine the clay platelets self diffusion coefficient and, by its comparison with the structural relaxation time, we conclude that the gelation process proceeds through the structuring of interconnecting clay platelets network rather than through clusters growth and aggregation.

cond-mat.soft↗

Laser beam filamentation in fractal aggregates

We investigate filamentation of a cw laser beam in soft matter such as colloidal suspensions and fractal gels. The process, driven by electrostriction, is strongly affected by material properties, which are taken into account via the static structure factor, and have impact on the statistics of the light filaments.

cond-mat.dis-nn↗

Glassy behavior of light in random lasers

A theoretical analysis [Angelani et al., Phys. Rev. Lett. 96, 065702 (2006)] predicts glassy behaviour of light in a nonlinear random medium. This implies slow dynamics related to the presence of many metastable states. We consider very general equations (that also apply to other systems, like Bose-Condensed gases) describing light in a disordered non-linear medium and through some approximations we relate them to a mean-field spin-glass-like model. The model is solved by the replica method, and replica-symmetry breaking phase transition is predicted. The transition describes a mode-locking process in which the phases of the modes are locked to random (history and sample-dependent) values. The results are based on very general theory, and embrace a variety of physical phenomena.

cond-mat.dis-nn↗

Optical spatial solitons in soft-matter: mode coupling theory approach

We predict that spatial self-trapping of light can occur in soft matter encompassing a wide class of new materials such as colloids, foams, gels, fractal aggregates etc. We develop a general nonlocal theory that allows to relate the properties of the trapped state of Maxwell equations to the measurable static structure factor of the specific material. We give numerical evidence for stable trapping in fractal aggregates and suggest also the possibility of soliton spectroscopy of soft-matter.

physics.optics↗

Microscopic dynamics in liquid metals: the experimental point of view

The experimental results relevant for the understanding of the microscopic dynamics in liquid metals are reviewed, with special regards to the ones achieved in the last two decades. Inelastic Neutron Scattering played a major role since the development of neutron facilities in the sixties. The last ten years, however, saw the development of third generation radiation sources, which opened the possibility of performing Inelastic Scattering with X rays, thus disclosing previously unaccessible energy-momentum regions. The purely coherent response of X rays, moreover, combined with the mixed coherent/incoherent response typical of neutron scattering, provides enormous potentialities to disentangle aspects related to the collectivity of motion from the single particle dynamics. If the last twenty years saw major experimental developments, on the theoretical side fresh ideas came up to the side of the most traditional and established theories. Beside the raw experimental results, therefore, we review models and theoretical approaches for the description of microscopic dynamics over different length-scales, from the hydrodynamic region down to the single particle regime, walking the perilous and sometimes uncharted path of the generalized hydrodynamics extension. Approaches peculiar of conductive systems, based on the ionic plasma theory, are also considered, as well as kinetic and mode coupling theory applied to hard sphere systems, which turn out to mimic with remarkable detail the atomic dynamics of liquid metals. Finally, cutting edges issues and open problems, such as the ultimate origin of the anomalous acoustic dispersion or the relevance of transport properties of a conductive systems in ruling the ionic dynamic structure factor are discussed.

cond-mat.dis-nn↗

Topology and phase transitions: from an exactly solvable model to a relation between topology and thermodynamics

The elsewhere surmised topological origin of phase transitions is given here new important evidence through the analytic study of an exactly solvable model for which both topology and thermodynamics are worked out. The model is a mean-field one with a k-body interaction. It undergoes a second order phase transition for k=2 and a first order one for k>2. This opens a completely new perspective for the understanding of the deep origin of first and second order phase transitions, respectively. In particular, a remarkable theoretical result consists of a new mathematical characterization of first order transitions. Moreover, we show that a "reduced" configuration space can be defined in terms of collective variables, such that the correspondence between phase transitions and topology changes becomes one-to-one, for this model. Finally, an unusual relationship is worked out between the microscopic description of a classical N-body system and its macroscopic thermodynamic behaviour. This consists of a functional dependence of thermodynamic entropy upon the Morse indexes of the critical points (saddles) of the constant energy hypersurfaces of the microscopic 2N-dimensional phase space. Thus phase space (and configuration space) topology is directly related to thermodynamics.

cond-mat.stat-mech↗

Comment on "Collective dynamics in liquid lithium, sodium, and aluminum"

In a recent paper, S. Singh and K. Tankeshwar (ST), [Phys. Rev. E \textbf{67}, 012201 (2003)], proposed a new interpretation of the collective dynamics in liquid metals, and, in particular, of the relaxation mechanisms ruling the density fluctuations propagation. At variance with both the predictions of the current literature and the results of recent Inelastic X-ray Scattering (IXS) experiments, ST associate the quasielastic component of the $S(Q,ω)$ to the thermal relaxation, as it holds in an ordinary adiabatic hydrodynamics valid for non-conductive liquids and in the $Q \to 0$ limit. We show here that this interpretation leads to a non-physical behaviour of different thermodynamic and transport parameters.

cond-mat.dis-nn↗