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Giovanni De Ninno

Publications and source records attributed to Giovanni De Ninno.

32 records · Page 2Linked to original sources

Hidden phase in parent Fe-pnictide superconductors

We investigate the origin of exoticity in Fe-based systems via studying the Fermiology of CaFe2As2 employing Angle Resolved Photoemission spectroscopy (ARPES). While the Fermi surfaces (FSs) at 200 K and 31 K are observed to exhibit two dimensional (2D) and three dimensional (3D) topology, respectively, the FSs at intermediate temperatures reveal emergence of the 3D topology at much lower temperature than the structural & magnetic phase transition temperature (170 K, for the sample under scrutiny). This leads to the conclusion that the evolution of FS topology is not directly driven by the structural transition. In addition, we discover the existence in ambient conditions of energy bands related to the collapsed tetragonal (cT) phase. These bands are distinctly resolved in the high-photon energy spectra exhibiting strong Fe 3d character. They gradually move to higher binding energies due to thermal compression with cooling, leading to the emergence of 3D topology in the Fermi surface. These results reveal the so-far hidden existence of a cT phase in ambient conditions, which is argued to lead to quantum fluctuations responsible for the exotic electronic properties in Fe-pnictide superconductors.

cond-mat.supr-con↗

Absence of thermalization for systems with long-range interactions coupled to a thermal bath

We investigate the dynamics of a small long-range interacting system, in contact with a large long-range thermal bath. Our analysis reveals the existence of striking anomalies in the energy flux between the bath and the system. In particular, we find that the evolution of the system is not influenced by the kinetic temperature of the bath, as opposed to what happens for short-range collisional systems. As a consequence, the system may get hotter also when its initial temperature is larger than the bath temperature. This observation is explained quantitatively in the framework of the collisionless Vlasov description of toy models with long-range interactions and shown to be valid whenever the Vlasov picture applies, from cosmology to plasma physics.

cond-mat.stat-mech↗

Spectro-temporal shaping of seeded free-electron laser pulses

We demonstrate the ability to control and shape the spectro-temporal content of extreme-ultraviolet (XUV) pulses produced by a seeded free-electron laser (FEL). The control over the spectro-temporal properties of XUV light was achieved by precisely manipulating the linear frequency chirp of the seed laser. Our results agree with existing theory, which allows retrieving the temporal properties (amplitude and phase) of the FEL pulse from measurements of the spectra as a function of the FEL operating parameters. Furthermore, we show the first direct evidence of the full temporal coherence of FEL light and generate Fourier limited pulses by fine-tuning the FEL temporal phase. The possibility to tailor the spectro-temporal content of intense short-wavelength pulses represents the first step towards efficient nonlinear optics in the XUV to X-ray spectral region and will enable precise manipulation of core-electron excitations using the methods of coherent quantum control.

physics.optics↗

Spectral-phase interferometry for direct electric-field reconstruction applied to seeded extreme-ultraviolet free-electron lasers

We present a setup for complete characterization of femtosecond pulses generated by seeded free-electron lasers (FEL's) in the extreme-ultraviolet spectral region. Two delayed and spectrally shifted replicas are produced and used for spectral phase interferometry for direct electric field reconstruction (SPIDER). We show that it can be achieved by a simple arrangement of the seed laser. Temporal shape and phase obtained in FEL simulations are well retrieved by the SPIDER reconstruction, allowing to foresee the implementation of this diagnostic on existing and future sources. This will be a significant step towards an experimental investigation and control of FEL spectral phase.

physics.optics↗

Generation of Coherent Extreme-Ultraviolet Radiation Carrying Orbital Angular Momentum

We propose an effective scheme for the generation of intense coherent extreme ultraviolet light beams carrying orbital angular momentum (OAM). The light is produced by a high-gain harmonic-generation free-electron laser (FEL), seeded using a laser pulse with a transverse staircase-like phase pattern. During amplification, diffraction and mode selection drive the radiation profile towards a dominant OAM mode at saturation. With a seed laser at 260 nm, gigawatt power levels are obtained at wavelengths approaching those of soft x-rays. Compared to other proposed schemes to generate OAM with FELs, our approach is robust, easier to implement, and can be integrated into already existing FEL facilities without extensive modifications of the machine layout.

physics.optics↗

Direct Spectro-Temporal Characterization of Femtosecond Extreme-Ultraviolet Pulses

We propose a method for a straightforward characterization of the temporal shape of femtosecond pulses in the extreme-ultraviolet/soft X-ray spectral region. The approach is based on the presence of a significant linear frequency chirp in the pulse. This allows to establish an homothetic relation between the pulse spectrum and its temporal profile. The theoretical approach is reminiscent of the one employed by Fraunhofer for describing far-field diffraction. As an application, we consider the case of a seeded free-electron laser (FEL). Theory is successfully benchmarked with numerical simulations and with experimental data collected on the FERMI@Elettra FEL. The proposed method provides FEL users with an on-line, shot-to-shot spectro-temporal diagnostic for time-resolved experiments.

physics.optics↗

Chirped seeded free-electron lasers: self-standing light sources for two-colour pump-probe experiments

We demonstrate the possibility to run a single-pass free-electron laser in a new dynamical regime, which can be exploited to perform two-colour pump-probe experiments in the VUV/X-ray domain, using the free-electron laser emission both as a pump and as a probe. The studied regime is induced by triggering the free-electron laser process with a powerful laser pulse, carrying a significant and adjustable frequency chirp. As a result, the emitted light is eventually split in two sub-pulses, whose spectral and temporal separations can be independently controlled. We provide a theoretical description of this phenomenon, which is found in good agreement with experiments performed on the FERMI@Elettra free-electron laser.

physics.optics↗

Vlasov equation for long-range interactions on a lattice

We show that, in the continuum limit, the dynamics of Hamiltonian systems defined on a lattice with long-range couplings is well described by the Vlasov equation. This equation can be linearized around the homogeneous state and a dispersion relation, that depends explicitly on the Fourier modes of the lattice, can be derived. This allows one to compute the stability thresholds of the homogeneous state, which turn out to depend on the mode number. When this state is unstable, the growth rates are also function of the mode number. Explicit calculations are performed for the $α$-HMF model with $0 \leq α<1$, for which the zero mean-field mode is always found to dominate the exponential growth. The theoretical predictions are successfully compared with numerical simulations performed on a finite lattice.

nlin.CD↗

Efficiency of cyclic devices working with non-Boltzmannian fluids: challenging the second principle of thermodynamics

According to classical Boltzmannian thermodynamics, the efficiency of a cyclic machine is strictly lower than one. Such a result is a straightforward consequence of the second principle of thermodynamics. Recent advances in the study of the thermodynamics of long-range interacting system report however on a rather intricate zoology of peculiar behaviors, which are occasionally in contrast with customarily accepted scenarios, dueling with intuition and common sense. In this paper, a thermodynamical cycle is assembled for an ideal device working with non-Boltzmaniann long-range fluid and operating in contact with two thermal reservoirs. The system is analytically shown to violate the second principle of thermodynamics, a phenomenon that ultimately relates to the existence of regions with negative kinetic specific heat, in the canonical ensemble for the system under scrutiny. We argue that the validity of the second principle of thermodynamics can be possibly restored, by revisiting the definition of canonical ensemble, as well as the Fourier law of heat transport, and consequently relaxing the constraint on the maximal efficiency as imposed by the Carnot theorem.

cond-mat.stat-mech↗

Out of equilibrium statistical ensemble inequivalence

We consider a paradigmatic model describing the one-dimensional motion of $N$ rotators coupled through a mean-field interaction, and subject to the perturbation of an external magnetic field. The latter is shown to significantly alter the system behaviour, driving the emergence of ensemble inequivalence in the out-of-equilibrium phase, as signalled by a negative (microcanonical) magnetic susceptibility. The thermodynamic of the system is analytically discussed, building on a maximum entropy scheme justified from first principles. Simulations confirm the adequacy of the theoretical picture. Ensemble inequivalence is shown to rely on a peculiar phenomenon, different from the one observed in previous works. As a result, the existence of a convex intruder in the micro-canonical energy is found to be a necessary but not sufficient condition for inequivalence to be (macroscopically) observed. Negative temperature states are also found to occur. These intriguing phenomena reflect the non-Boltzmanian nature of the scrutinized problem and, as such, bear traits of universality that embraces equilibrium as well out-of-equilibrium regimes.

cond-mat.stat-mech↗

Out-of-equilibrium mean-field dynamics of a model for wave-particle interaction

The out-of-equilibrium mean-field dynamics of a model for wave-particle interaction is investigated. Such a model can be regarded as a general formulation for all those applications where the complex interplay between particles and fields is known to be central, e.g., electrostatic instabilities in plasma physics, particle acceleration and free-electron lasers (FELs). The latter case is here assumed as a paradigmatic example. A transition separating different macroscopic regimes is numerically identified and interpreted by making use of the so-called violent relaxation theory. In the context of free-electron lasers, such a theory is showed to be effective in predicting the saturated regime for energies below the transition. The transition is explained as a dynamical switch between two metastable regimes, and is related to the properties of a stationary point of an entropic functional.

physics.plasm-ph↗

Out of equilibrium phase transitions in mean field Hamiltonian dynamics

Systems with long-range interactions display a short-time relaxation towards Quasi-Stationary States (QSSs), whose lifetime increases with system size. With reference to the Hamiltonian Mean Field (HMF) model, we here review Lynden-Bell's theory of ``violent relaxation''. The latter results in a maximum entropy scheme for a water-bag initial profile which predicts the presence of out-of-equilibrium phase transitions} separating homogeneous (zero magnetization) from inhomogeneous (non-zero magnetization) QSSs. Two different parametric representations of the initial condition are analyzed and the features of the phase diagram are discussed. In both representations we find a second order and a first order line of phase transitions that merge at a tricritical point. Particular attention is payed to the condition of existence and stability of the homogenous phase.

cond-mat.stat-mech↗

Statistical theory of high-gain free-electron laser saturation

We propose a new approach, based on statistical mechanics, to predict the saturated state of a single-pass, high-gain free-electron laser (FEL). In analogy with the violent relaxation process in self-gravitating systems and in the Euler equation of 2D turbulence, the initial relaxation of the laser can be described by the statistical mechanics of an associated Vlasov equation. The Laser field intensity and the electron bunching parameter reach quasi-stationary values that are well fitted by a Vlasov stationary state if the number of electrons $N$ is sufficiently large. Finite $N$ effects (granularity) finally drive the system to Boltzmann-Gibbs statistical equilibrium, but this occurs on times that are unphysical (i.e. excessively long undulators). All theoretical predictions are successfully tested in finite $N$ numerical experiments. Our results may provide important hints to the optimization of the length of the FEL undulator.

cond-mat.stat-mech↗

Controlled Hopf Bifurcation of a storage-ring free-electron laser

Local bifurcation control is a topic of fundamental importance in the field of nonlinear dynamical systems. We discuss an original example within the context of storage-ring free-electron laser physics by presenting a new model that enables analytical insight into the system dynamics. The transition between the stable and the unstable regimes, depending on the temporal overlapping between the light stored in the optical cavity and the electrons circulating into the ring, is found to be a Hopf bifurcation. A feedback procedure is implemented and shown to provide an effective stabilization of the unstable steady state.

physics.optics↗