arXiv subjects

Gisela Schütz

Publications and source records attributed to Gisela Schütz.

At least 19 recordsLinked to original sources

arXiv2026

Direct observation of propagating spin waves in a spin-Hall nano-oscillator

Constriction-based spin Hall nano-oscillators (SHNOs) show great promise for application as highly tunable microwave sources with straightforward scalability toward large coupled networks. However, details of the magnetization dynamics within SHNOs have thus far not been addressed experimentally, due to the minute time and length scales involved. In this work, we present direct imaging of the magnetization dynamics within a single CoFeB-based SHNO using time-resolved scanning transmission X-ray microscopy (STXM). Our measurements reveal that the magnon amplitude is the strongest at the two constriction edges, with a pronounced assymetry favoring one edge, and that emitted spin waves exhibit strongly anisotropic propagation. Micromagnetic simulations suggest that grain boundaries and the Dzyaloshinskii-Moriya interaction (DMI) play a key role in both effects. Furthermore, the magnetodynamics changed during the measurement, indicating that the CoFeB/MgO interface may be more susceptible to X-ray induced modifications than previously recognized, challenging its presumed radiation hardness.

cond-mat.mes-hall↗

arXiv2024

Direct determination of the spin-polarization at buried interfaces using voltage dependent MOKE signals

Here, we report a novel and conceptually straightforward technique to detect the spin-polarization directly, with laser spot spatial resolution, at buried ferromagnet/insulator interfaces in ambient settings. This has been accomplished by monitoring the voltage-induced change of the longitudinal MOKE signal as a function of the applied magnetic field and applying an AC voltage across the interface. For the case where the spin polarization enters the VMOKE signal, a simple quantitative model is proposed. A distinct positive majority spin polarization has been found for Fe and Co, whereas Ni exhibits a negative minority spin polarization.

physics.app-ph↗

arXiv2023

Pump--probe x-ray microscopy of photo-induced magnetization dynamics at MHz repetition rates

We present time-resolved scanning x-ray microscopy measurements with picosecond photo-excitation via a tailored infrared pump laser at a scanning transmission x-ray microscope. Specifically, we image the laser-induced demagnetization and remagnetization of thin ferrimagnetic GdFe films proceeding on a few nanoseconds time scale. Controlling the heat load on the sample via additional reflector and heat-sink layers allows us to conduct destruction-free measurements at a repetition rate of \SI{50}{\mega\hertz}. Near-field enhancement of the photo-excitation and controlled annealing effects lead to laterally heterogeneous magnetization dynamics which we trace with \SI{30}{\nano\meter} spatial resolution. Our work opens new opportunities to study photo-induced dynamics on the nanometer scale, with access to picosecond to nanosecond timescales, which is of technological relevance, especially in the field of magnetism.

cond-mat.mtrl-sci↗

arXiv2022

Role of substrate clamping on anisotropy and domain structure in the canted antiferromagnet $α$-Fe$_2$O$_3$

Antiferromagnets have recently been propelled to the forefront of spintronics by their high potential for revolutionizing memory technologies. For this, understanding the formation and driving mechanisms of the domain structure is paramount. In this work, we investigate the domain structure in a thin-film canted antiferromagnet $α$-Fe$_2$O$_3$. We find that the internal destressing fields driving the formation of domains do not follow the crystal symmetry of $α$-Fe$_2$O$_3$, but fluctuate due to substrate clamping. This leads to an overall isotropic distribution of the Néel order with locally varying effective anisotropy in antiferromagnetic thin films. Furthermore, we show that the weak ferromagnetic nature of $α$-Fe$_2$O$_3$ leads to a qualitatively different dependence on magnetic field compared to collinear antiferromagnets such as NiO. The insights gained from our work serve as a foundation for further studies of electrical and optical manipulation of the domain structure of antiferromagnetic thin films.

cond-mat.mes-hall↗

arXiv2022

Observation of a possible diluted ferromagnetism above room temperature in cobalt-substituted LaTa(O,N)3-d

Since 2000, the intensive effort in materials research to develop a diluted magnetic semiconductor exhibiting high-temperature (HT) ferromagnetism above room temperature was not successful. Here, the possible first bulk diluted HT-ferromagnetic non-metallic materials, based on the perovskite-type oxynitrides LaTa1-xCox(O,N)3-d (x = 0.01, 0.03, 0.05) are realized. The Curie temperature of the synthesized powders exceeds 600 K and the sample magnetizations are large enough to be directly attracted by permanent magnets. Cobalt clusters as a possible source for the observed HT-ferromagnetism can be excluded, since all applied characterization methods verify phase purity. Applied conventional and element-specific magnetometry imply ferromagnetic intermediate spin (IS) Co3+ which is included in a ferromagnetic host matrix. This indicates a complex magnetic interplay between the existing crystal structure, the observed anionic vacancies, and the introduced cobalt ions. These results lay the foundation for the experimental investigation and design of further diluted HT-ferromagnetic semiconductors.

cond-mat.mtrl-sci↗

arXiv2022

Terahertz spin-to-charge current conversion in stacks of ferromagnets and the transition-metal dichalcogenide NbSe$_2$

Transition-metal dichalcogenides (TMDCs) are an aspiring class of materials with unique electronic and optical properties and potential applications in spin-based electronics. Here, we use terahertz emission spectroscopy to study spin-to-charge current conversion (S2C) in the TMDC NbSe$_2$ in ultra-high-vacuum-grown F|NbSe$_2$ thin-film stacks, where F is a layer of ferromagnetic Fe or Ni. Ultrafast laser excitation triggers an ultrafast spin current that is converted into an in-plane charge current and, thus, a measurable THz electromagnetic pulse. The THz signal amplitude as a function of the NbSe$_2$ thickness shows that the measured signals are fully consistent with an ultrafast optically driven injection of an in-plane-polarized spin current into NbSe$_2$. Modeling of the spin-current dynamics reveals that a sizable fraction of the total S2C originates from the bulk of NbSe$_2$ with the same, negative, sign as the spin Hall angle of pure Nb. By quantitative comparison of the emitted THz radiation from F|NbSe$_2$ to F|Pt reference samples and the results of ab-initio calculations, we estimate that the spin Hall angle of NbSe$_2$ for an in-plane polarized spin current lies between -0.2% and -1.1%, while the THz spin-current relaxation length is of the order of a few nanometers.

cond-mat.mes-hall↗

arXiv2021

Commensurate vortex core switching in magnetic nanodisks at Gigahertz frequencies

The development of future spintronic applications requires a thorough and fundamental understanding of the magnetisation dynamics. Of particular interest are magnetic nanodisks, in which the vortex state emerges as a stable spin configuration. Here, we focus on how the vortex core polarisation can be reversed periodically by an oscillating magnetic field, applied perpendicularly to the disk's surface. By means of micromagnetic simulations, we demonstrate the presence of several subharmonic switching modes, i.e., the commensurate ratio between the switching frequency of the core and the driving frequency. The underlying mechanism of this periodic behaviour depends on the disk thickness. For thin disks, the core switches periodically due to resonant excitation of radial spin wave modes, while it is due to the breathing mode in the case of thick disks. However, overlap of both modes impedes periodic vortex core switching. For thin disks, the threshold field amplitude required for periodic switching can be lowered to about 30~mT by increasing the disk diameter. For thick disks, in contrast, the minimal field is largely unaffected by the disk diameter, as only the energy density of a central region around the vortex core is relevant to excite the breathing mode. Our results contribute to the understanding of the switching mechanisms in magnetic nanodisks, which are of technological interest due to their potential in non-volatile memory devices.

cond-mat.mes-hall↗

arXiv2021

Reconfigurable sub-micron spin-wave majority gate with electrical transducers

Spin waves are excitations in ferromagnetic media that have been proposed as information carriers in hybrid spintronic devices with much lower operation power than conventional charge-based electronics. Their wave nature can be exploited in majority gates by using interference for computation. However, a scalable spin-wave majority gate that can be co-integrated alongside conventional electronics is still lacking. Here, we demonstrate a sub-micron inline spin-wave majority gate with fan-out. Time-resolved imaging of the magnetization dynamics by scanning transmission x-ray microscopy illustrates the device operation. All-electrical spin-wave spectroscopy further demonstrates majority gates with sub-micron dimensions, reconfigurable input and output ports, and frequency-division multiplexing. Challenges for hybrid spintronic computing systems based on spin-wave majority gates are discussed.

physics.app-ph↗

arXiv2021

Maskless off-axis X-ray Holography

Off-axis X-ray holography is a lensless imaging technique that allows unambiguous retrieval of an object's exit-wave function with high fidelity. It has been used with great success to study nanoscale phenomena and spatio-temporal dynamics in solids, with sensitivity to the phase component of electronic and magnetic textures. However, the method requires patterning a nanostructured holography mask directly onto the sample. This invasive fabrication process is labor-intensive and defines a fixed field of view, limiting the range of applicable samples and diminishing the signal-to-noise ratio at high-resolution. In this work, we propose using wavefront-shaping X-ray diffractive optics to create a spatially structured probe with full control of its phase at the sample plane, obviating the need for a holography mask. We demonstrate in silico that the method can image nanoscale structures and magnetic textures. The proposed holography route can image extended regions of interest, enabling the investigation of a broad range of physical phenomena at the nanoscale including magnetism and electronic phase coexistence in quantum materials. We further envisage applications in phase-contrast imaging of other weakly absorbing objects in the realm of soft and biological matter research.

physics.optics↗

arXiv2021

Freezing and thawing magnetic droplet solitons

Magnetic droplets are non-topological magnetodynamical solitons displaying a wide range of complex dynamic phenomena with potential for microwave signal generation. Bubbles, on the other hand, are internally static cylindrical magnetic domains, stabilized by external fields and magnetostatic interactions. In its original theory, the droplet was described as an imminently collapsing bubble stabilized by spin transfer torque and, in its zero-frequency limit, as equivalent to a bubble. Without nanoscale lateral confinement, pinning, or an external applied field, such a nanobubble is unstable, and should collapse. Here, we show that we can freeze dynamic droplets into static nanobubbles by decreasing the magnetic field. While the bubble has virtually the same resistance as the droplet, all signs of low-frequency microwave noise disappear. The transition is fully reversible and the bubble can be thawed back into a droplet if the magnetic field is increased under current. Whereas the droplet collapses without a sustaining current, the bubble is highly stable and remains intact for days without external drive. Electrical measurements are complemented by direct observation using scanning transmission x-ray microscopy, which corroborates the analysis and confirms that the bubble is stabilized by pinning.

cond-mat.mes-hall↗

arXiv2019

Real space observation of magnon interaction with driven space-time crystals

The concept of Space-Time Crystals (STC), i.e. translational symmetry breaking in time and space, was recently proposed and experimentally demonstrated for quantum systems. Here, we transfer this concept to magnons and experimentally demonstrate a driven STC at room temperature. The STC is realized by strong homogeneous micro-wave pumping of a micron-sized permalloy (Py) stripe and is directly imaged by Scanning Transmission X-ray Microscopy (STXM). For a fundamental understanding of the formation of the STC, micromagnetic simulations are carefully adapted to model the experimental findings. Beyond the mere generation of a STC, we observe the formation of a magnonic band structure due to back folding of modes at the STC's Brillouin zone boundaries. We show interactions of magnons with the STC that appear as lattice scattering. This results in the generation of ultra short spin waves down to 100 nm wavelength that cannot be described by classical dispersion relations for linear spin wave excitations. We expect that room temperature STCs will be a useful tool to investigate non-linear wave physics, as they can be easily generated and manipulated to control their spatial and temporal band structure.

cond-mat.mes-hall↗

arXiv2019

Magnons in a Quasicrystal: Propagation, Localization and Extinction of Spin Waves in Fibonacci Structures

Magnonic quasicrystals exceed the possibilities of spin wave (SW) manipulation offered by regular magnonic crystals, because of their more complex SW spectra with fractal characteristics. Here, we report the direct x-ray microscopic observation of propagating SWs in a magnonic quasicrystal, consisting of dipolarly coupled permalloy nanowires arranged in a one-dimensional Fibonacci sequence. SWs from the first and second band as well as evanescent waves from the band gap between them are imaged. Moreover, additional mini-band gaps in the spectrum are demonstrated, directly indicating an influence of the quasiperiodicity of the system. The experimental results are interpreted using numerical calculations and we deduce a simple model to estimate the frequency position of the magnonic gaps in quasiperiodic structures. The demonstrated features of SW spectra in one-dimensional magnonic quasicrystals allows utilizing this class of metamaterials for magnonics and makes them an ideal basis for future applications.

cond-mat.mes-hall↗

arXiv2017

X-Ray Microscopy of Spin Wave Focusing using a Fresnel Zone Plate

Magnonics, i.e. the artificial manipulation of spin waves, is a flourishing field of research with many potential uses in data processing within reach. Apart from the technological applications the possibility to directly influence and observe these types of waves is of great interest for fundamental research. Guidance and steering of spin waves has been previously shown and lateral spin wave confinement has been achieved. However, true spin wave focusing with both lateral confinement and increase in amplitude has not been shown before. Here, we show for the first time spin wave focusing by realizing a Fresnel zone plate type lens. Using x-ray microscopy we are able to directly image the propagation of spin waves into the nanometer sized focal spot. Furthermore, we observe that the focal spot can be freely moved in a large area by small variations of the bias field. Thus, this type of lens provides a steerable intense nanometer sized spin wave source. Potentially, this could be used to selectively illuminate magnonic devices like nano oscillators with a steerable spin wave beam.

cond-mat.mes-hall↗

arXiv2017

Direct observation of magnetic droplet solitons in all-perpendicular spin torque nano-oscillators

Magnetic droplets are non-topological dynamical solitons that can be nucleated and sustained in nano-contact based spin torque nano-oscillators (NC-STNOs) with perpendicular anisotropy free layers. While originally predicted in all-perpendicular NC-STNOs, all experimental demonstrations have so far relied on orthogonal devices with an in-plane polarizing layer that requires a strong magnetic field for droplet nucleation. Here, we instead show the nucleation and sustained operation of magnetic droplets in all-perpendicular NC-STNOs in modest perpendicular fields and over a wide range of nano-contact size. The droplet is observed electrically as an intermediate resistance state accompanied by broadband low-frequency microwave noise. Using canted fields, which introduce a non-zero relative angle between the free and fixed layer, the actual droplet precession frequency can also be determined. Finally, the droplet size, its perimeter width, and its fully reversed core are directly observed underneath a 80 nm diameter nano-contact using scanning transmission x-ray microscopy on both the Ni and Co edges. The droplet diameter is 150 nm, i.e. almost twice the nominal size of the nano-contact, and the droplet has a perimeter width of about 70 nm.

cond-mat.mes-hall↗

arXiv2016

Skyrmion Hall Effect Revealed by Direct Time-Resolved X-Ray Microscopy

Magnetic skyrmions are highly promising candidates for future spintronic applications such as skyrmion racetrack memories and logic devices. They exhibit exotic and complex dynamics governed by topology and are less influenced by defects, such as edge roughness, than conventionally used domain walls. In particular, their finite topological charge leads to a predicted "skyrmion Hall effect", in which current-driven skyrmions acquire a transverse velocity component analogous to charged particles in the conventional Hall effect. Here, we present nanoscale pump-probe imaging that for the first time reveals the real-time dynamics of skyrmions driven by current-induced spin orbit torque (SOT). We find that skyrmions move at a well-defined angle Θ_{SH} that can exceed 30° with respect to the current flow, but in contrast to theoretical expectations, Θ_{SH} increases linearly with velocity up to at least 100 m/s. We explain our observation based on internal mode excitations in combination with a field-like SOT, showing that one must go beyond the usual rigid skyrmion description to unravel the dynamics.

cond-mat.mtrl-sci↗

arXiv2016

Spin wave mediated unidirectional Vortex Core Reversal by Two Orthogonal Monopolar Field Pulses: The Essential Role of Three-dimensional Magnetization Dynamics

Scanning transmission x-ray microscopy is employed to investigate experimentally the reversal of the magnetic vortex core polarity in cylindrical Ni81Fe19 nanodisks triggered by two orthogonal monopolar magnetic field pulses with peak amplitude $B_0$, pulse length $τ$=60 ps and delay time $Δ$t in the range from -400 ps to +400 ps between the two pulses. The two pulses are oriented in-plane in the x- and y-direction. We have experimentally studied vortex core reversal as function of $B_0$ and $Δ$t. The resulting phase diagram shows large regions of unidirectional vortex core switching where the switching threshold is modulated due to resonant amplification of azimuthal spin waves. The switching behavior changes dramatically depending on whether the first pulse is applied in the x- or the y-direction. This asymmetry can be reproduced by three-dimensional micromagnetic simulations but not by two-dimensional simulations. This behavior demonstrates that in contrast to previous experiments on vortex core reversal the three-dimensionality in the dynamics is essential here.

cond-mat.mes-hall↗

arXiv2015

Enhanced Non-Adiabaticity in Vortex Cores due to the Emergent Hall Effect

We present a combined theoretical and experimental study, investigating the origin of the enhanced non-adiabaticity of magnetic vortex cores. Scanning transmission X-ray microscopy is used to image the vortex core gyration dynamically to measure the non-adiabaticity with high precision, including a high confidence upper bound. Using both numerical computations and analytical derivations, we show that the large non-adiabaticity parameter observed experimentally can be explained by the presence of local spin currents arising from a texture-induced emergent Hall effect. This enhanced non-adiabaticity is only present in two- and three-dimensional magnetic textures such as vortices and skyrmions and absent in one-dimensional domain walls, in agreement with experimental observations.

cond-mat.mes-hall↗

arXiv2015

Three-dimensional Character of the Magnetization Dynamics in Magnetic Vortex Structures - Hybridization of Flexure Gyromodes with Spin Waves

Three-dimensional linear spin-wave eigenmodes of a Permalloy disk having finite thickness are studied by micromagnetic simulations based on the Landau-Lifshitz-Gilbert equation. The eigenmodes found in the simulations are interpreted as linear superpositions (hybridizations) of 'approximate' three-dimensional eigenmodes, which are the fundamental gyromode $G_0$, the spin-wave modes and the higher-order gyromodes $G_N$ (flexure modes), the thickness dependence of which is represented by perpendicular standing spin waves. This hybridization leads to new and surprising dependencies of the mode frequencies on the disk thickness. The three-dimensional character of the eigenmodes is essential to explain the recent experimental results on vortex-core reversal observed in relatively thick Permalloy disks.

cond-mat.mes-hall↗