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Golrokh Akhgar

Publications and source records attributed to Golrokh Akhgar.

7 recordsLinked to original sources

Ferroelectric--Superconducting Interaction in Epitaxial YBa2Cu3O7-δ/BaTiO3 Films

Microscopic theories predict that the critical temperature of a superconducting layer can be strongly modified in proximity to a ferroelectric; however, experimental evidence is lacking. We report on BaTiO3 (BTO)/YBa2Cu3O7-δ (YBCO) heterostructures grown on SrTiO3 (001) substrates using pulsed laser deposition (PLD), with precise control of growth conditions and oxygen stoichiometry. Piezoresponse force microscopy confirms ferroelectric switching within both single-layer and heterostructured films. Neutron reflectometry measurements show low roughness parameters for the buried interfaces, which is critical for mediating the interfacial coupling between superconductivity and ferroelectric polarization. The superconducting transition temperature ($T_{\mathrm{C}}^{R}$) measured from the $R(T)$ curve of the single-layer YBCO was approximately 86 K, and a transition temperature ($T_{\mathrm{C}}^{M}$) of approximately 80-85 K was observed from the $M(T)$ curve. For the heterostructure film (YBCO/BTO/YBCO) grown under the same conditions, both resistivity and magnetization measurements indicate lower transition temperatures of approximately 75 K and approximately 55 K, respectively, as well as a lower overall susceptibility. These findings highlight the need to combine multiple techniques to characterize BTO/YBCO heterostructures and identify subtle features of the ferroelectric--superconducting coupling. This establishes BTO/YBCO heterostructures as promising systems for tunable oxide electronics and reconfigurable superconducting devices.

cond-mat.supr-con

High-field Magnetotransport Studies of Surface Conducting Diamonds

The observation of strong and tunable spin-orbit interaction (SOI) in surface conducting diamond opens up a new avenue for building diamond-based spintronics. Herein we provide a comprehensive method to analyze the magnetotransport behavior of surface conducting hydrogen-terminated diamond (H-diamond) Hall bar devices and Al/Al2O3/V2O5/H-diamond MOSFETs, respectively. By adopting a significantly improved theoretical magneto transport model, the reduced magnetoconductance can be accurately explained both within and outside the quantum diffusive regime. The model is valid for all doping strategies of surface conducting diamond tested. From this analysis, we find that the orbital magnetoresistance, a classical effect distinct from the SOI, dominates the magnetotransport in surface conducting diamond at high magnetic fields. Furthermore, local hole mobilities as high as 1000 ~ 3000 cm2/Vs have been observed in this work, indicating the possibility of diamond-based electronics with ultra-high hole mobilities at cryogenic temperatures.

cond-mat.mtrl-sci

Increased Phase Coherence Length in a Porous Topological Insulator

The surface area of Bi2Te3 thin films was increased by introducing nanoscale porosity. Temperature dependent resistivity and magnetotransport measurements were conducted both on as-grown and porous samples (23 and 70 nm). The longitudinal resistivity of the porous samples became more metallic, indicating the increased surface area resulted in transport that was more surface-like. Weak antilocalization (WAL) was present in all samples, and remarkably the phase coherence length doubled in the porous samples. This increase is likely due to the large Fermi velocity of the Dirac surface states. Our results show that the introduction of nanoporosity does not destroy the topological surface states but rather enhances them, making these nanostructured materials promising for low energy electronics, spintronics and thermoelectrics.

cond-mat.mtrl-sci

Formation of a stable surface oxide in MnBi$_2$Te$_4$ thin films

Understanding the air-stability of MnBi$_2$Te$_4$ thin films is crucial for the development and long-term operation of electronic devices based around magnetic topological insulators. In the present work, we study MnBi$_2$Te$_4$ thin films upon exposure to atmosphere using a combination of synchrotron-based photoelectron spectroscopy, room temperature electrical transport and atomic force microscopy to determine the oxidation process. After 2 days air exposure a 2 nm thick oxide passivates the surface, corresponding to oxidation of only the top two surface layers, with the underlying layers preserved. This protective oxide layer results in samples that still exhibit metallic conduction even after several days air exposure. Furthermore, the work function decreases from 4.4 eV for pristine MnBi$_2$Te$_4$ to 4.0 eV after the formation of the oxide, along with only a small shift in the core levels indicating minimal doping as a result of air exposure. With the oxide confined to the top surface layers, and the underlying layers preserved, it may be possible to explore new avenues in how to handle, prepare and passivate future MnBi$_2$Te$_4$ devices.

cond-mat.mtrl-sci

Crossover from 2D ferromagnetic insulator to wide bandgap quantum anomalous Hall insulator in ultra-thin MnBi2Te4

Intrinsic magnetic topological insulators offer low disorder and large magnetic bandgaps for robust magnetic topological phases operating at higher temperatures. By controlling the layer thickness, emergent phenomena such as the Quantum Anomalous Hall (QAH) effect and axion insulator phases have been realised. These observations occur at temperatures significantly lower than the Neel temperature of bulk MnBi2Te4, and measurement of the magnetic energy gap at the Dirac point in ultra-thin MnBi2Te4 has yet to be achieved. Critical to achieving the promise of this system is a direct measurement of the layer-dependent energy gap and verifying whether the gap is magnetic in the QAH phase. Here we utilise temperature dependent angle-resolved photoemission spectroscopy to study epitaxial ultra-thin MnBi2Te4. We directly observe a layer dependent crossover from a 2D ferromagnetic insulator with a bandgap greater than 780 meV in one septuple layer (1 SL) to a QAH insulator with a large energy gap (>100 meV) at 8 K in 3 and 5 SL MnBi2Te4. The QAH gap is confirmed to be magnetic in origin, as it abruptly diminishes with increasing temperature above 8 K. The direct observation of a large magnetic energy gap in the QAH phase of few-SL MnBi2Te4 is promising for further increasing the operating temperature of QAH materials.

cond-mat.mtrl-sci

Recent Progress in Proximity Coupling of Magnetism to Topological Insulators

Inducing long-range magnetic order in three-dimensional topological insulators can gap the Diraclike metallic surface states, leading to exotic new phases such as the quantum anomalous Hall effect or the axion insulator state. These magnetic topological phases can host robust, dissipationless charge and spin currents or unique magnetoelectric behavior, which can be exploited in low-energy electronics and spintronics applications. Although several different strategies have been successfully implemented to realize these states, to date these phenomena have been confined to temperatures below a few Kelvin. In this review, we focus on one strategy, inducing magnetic order in topological insulators by proximity of magnetic materials, which has the capability for room temperature operation, unlocking the potential of magnetic topological phases for applications. We discuss the unique advantages of this strategy, the important physical mechanisms facilitating magnetic proximity effect, and the recent progress to achieve, understand, and harness proximity-coupled magnetic order in topological insulators. We also highlight some emerging new phenomena and applications enabled by proximity coupling of magnetism and topological materials, such as skyrmions and the topological Hall effect, and we conclude with an outlook on remaining challenges and opportunities in the field.

cond-mat.mes-hall

Quantum Transport in Air-stable Na3Bi Thin Films

Na3Bi has attracted significant interest in both bulk form as a three-dimensional topological Dirac semimetal and in ultra-thin form as a wide-bandgap two-dimensional topological insulator. Its extreme air sensitivity has limited experimental efforts on thin- and ultra-thin films grown via molecular beam epitaxy to ultra-high vacuum environments. Here we demonstrate air-stable Na3Bi thin films passivated with magnesium difluoride (MgF2) or silicon (Si) capping layers. Electrical measurements show that deposition of MgF2 or Si has minimal impact on the transport properties of Na3Bi whilst in ultra-high vacuum. Importantly, the MgF2-passivated Na3Bi films are air-stable and remain metallic for over 100 hours after exposure to air, as compared to near instantaneous degradation when they are unpassivated. Air stability enables transfer of films to a conventional high-magnetic field cryostat, enabling quantum transport measurements which verify that the Dirac semimetal character of Na3Bi films is retained after air exposure.

cond-mat.mtrl-sci