arXiv subjects

Graeme Bart

Publications and source records attributed to Graeme Bart.

6 recordsLinked to original sources

arXiv2025

Quantum Dial for High-Harmonic Generation

High-harmonic generation (HHG) is a highly nonlinear optical process that typically requires an intense laser to trigger emissions at integer multiples of the driving field frequency. However, the strong fields required for conventional HHG inevitably perturb the system, limiting its use as a nondestructive spectroscopic probe. Recent advances in bright squeezed vacuum (BSV) sources have created opportunities to drive HHG with quantum fields alone. In this work, we demonstrate a regime in which the light-matter interactions can be controlled and tuned using a weak classical field, whose pulse energy is two orders of magnitude lower than that in standard HHG-perturbed by an even weaker quantum field such as BSV. This approach opens new avenues for nonlinear spectroscopy of materials while substantially suppressing strong laser-induced damage, distortions, and heating. We show that a BSV pulse containing less than 5% of the classical driving energy can act as an 'optical dial', allowing tuning of the nonlinear emission spectrum, emission angular dependence, and ionization.

physics.optics↗

arXiv2025

A unified perspective of high-harmonic generation in gases and solids

We present a quantum optical generalization of the quantum-matter Lewenstein model of high-harmonic generation (HHG) in gases that contains two channels corresponding to the inter- and intraband HHG in solids. Both channels can be presented as a semiclassical current multiplied by the vacuum field strength, resulting in a quantitative correction and a faster roll-off of the harmonic power with order than in previous theories. In gases, like in solids, intraband HHG dominates at low orders; the switchover harmonic corresponds to a specific photon energy, independent of pump wavelength.

physics.atom-ph↗

arXiv2025

Quantum engineering of high harmonic generation

In quantum sideband high harmonic generation (QSHHG), high harmonic generation is perturbed by a bright quantum field resulting in harmonic sidebands, with the intent to transfer non-classical properties from the quantum perturbation to the harmonic sidebands. So far, non-classical features have not been found in QSHHG yet. The closed form theory of QSHHG in atoms and solids developed here answers the question under which conditions non-classical features can be realized. QSHHG results in a multi-mode entanglement between harmonic sideband modes and perturbative quantum mode. A projective measurement on either creates a variety of non-classical states commonly used in quantum information science. This opens a pathway towards quantum engineering high harmonic generation as a short wavelength source for quantum information science.

quant-ph↗

arXiv2025

Strong field physics in open quantum systems

Dephasing is the loss of phase coherence due to the interaction of an electron with the environment. The most common approach to model dephasing in light-matter interaction is the relaxation time approximation. Surprisingly, its use in intense laser physics results in a pronounced failure, because ionization {is highly overestimated.} Here, this shortcoming is corrected by developing a strong field model in which the many-body environment is represented by a heat bath. Our model reveals that ionization enhancement and suppression by several orders of magnitude are still possible, however only in more extreme parameter regimes. Our approach allows the integration of many-body physics into intense laser dynamics with minimal computational and mathematical complexity, thus facilitating the identification of novel effects in strong-field physics and attosecond {science}.

physics.optics↗

arXiv2017

Explicit formulation of second and third order optical nonlinearity in the FDTD framework

The finite-difference time-domain (FDTD) method is a flexible and powerful technique for rigorously solving Maxwell's equations. However, three-dimensional optical nonlinearity in current commercial and research FDTD softwares requires solving iteratively an implicit form of Maxwell's equations over the entire numerical space and at each time step. Reaching numerical convergence demands significant computational resources and practical implementation often requires major modifications to the core FDTD engine. In this paper, we present an explicit method to include second and third order optical nonlinearity in the FDTD framework based on a nonlinear generalization of the Lorentz dispersion model. A formal derivation of the nonlinear Lorentz dispersion equation is equally provided, starting from the quantum mechanical equations describing nonlinear optics in the two-level approximation. With the proposed approach, numerical integration of optical nonlinearity and dispersion in FDTD is intuitive, transparent, and fully explicit. A strong-field formulation is also proposed, which opens an interesting avenue for FDTD-based modelling of the extreme nonlinear optics phenomena involved in laser filamentation and femtosecond micromachining of dielectrics.

physics.optics↗

arXiv2015

Saturable Lorentz model for fully explicit three-dimensional modeling of nonlinear optics

Inclusion of the instantaneous Kerr nonlinearity in the FDTD framework leads to implicit equations that have to be solved iteratively. In principle, explicit integration can be achieved with the use of anharmonic oscillator equations, but it tends to be unstable and inappropriate for studying strong-field phenomena like laser filamentation. In this paper, we show that nonlinear susceptibility can be provided instead by a harmonic oscillator driven by a nonlinear force, chosen in a way to reproduce the polarization obtained from the solution of the quantum mechanical two level equations. The resulting saturable, nonlinearly-driven, harmonic oscillator model reproduces quantitatively the quantum mechanical solutions of harmonic generation in the under-resonant limit, up to the 9th harmonic. Finally, we demonstrate that fully explicit leapfrog integration of the saturable harmonic oscillator is stable, even for the intense laser fields that characterize laser filamentation and high harmonic generation.

physics.optics↗