arXiv subjects

Gregory A. Fiete

Publications and source records attributed to Gregory A. Fiete.

At least 73 records · Page 4Linked to original sources

arXiv2018

Topological Magnon Bands and Unconventional Superconductivity in Pyrochlore Iridate Thin Films

We theoretically study the magnetic properties of pyrochlore iridate bilayer and trilayer thin films grown along the $[111]$ direction using a strong coupling approach. We find the ground state magnetic configurations on a mean field level and carry out a spin-wave analysis about them. In the trilayer case the ground state is found to be the all-in-all-out (AIAO) state, whereas the bilayer has a deformed AIAO state. For all parameters of the spin-orbit coupled Hamiltonian we study, the lowest magnon band in the trilayer case has a nonzero Chern number. In the bilayer case we also find a parameter range with nonzero Chern numbers. We calculate the magnon Hall response for both geometries, finding a striking sign change as function of temperature. Using a slave-boson mean-field theory we study the doping of the trilayer system and discover an unconventional time-reversal symmetry broken $d+id$ superconducting state. Our study complements prior work in the weak coupling limit and suggests that the $[111]$ grown thin film pyrochlore iridates are a promising candidate for topological properties and unconventional orders.

cond-mat.str-el↗

arXiv2018

Magnon thermal Hall effect in kagome antiferromagnets with Dzyaloshinskii-Moriya interactions

We theoretically study magnetic and topological properties of antiferromagnetic kagome spin systems in the presence of both in- and out-of-plane Dzyaloshinskii-Moriya interactions. In materials such as the iron jarosites, the in-plane interactions stabilize a canted noncollinear "umbrella" magnetic configuration with finite scalar spin chirality. We derive expressions for the canting angle, and use the resulting order as a starting point for a spin-wave analysis. We find topological magnon bands, characterized by non-zero Chern numbers. We calculate the magnon thermal Hall conductivity, and propose the iron jarosites as a promising candidate system for observing the magnon thermal Hall effect in a noncollinear spin configuration. We also show that the thermal conductivity can be tuned by varying an applied magnetic field, or the in-plane Dzyaloshinskii-Moriya strength. In contrast with previous studies of topological magnon bands, the effect is found to be large even in the limit of small canting.

cond-mat.str-el↗

arXiv2018

Floquet Hofstadter Butterfly on the Kagome and Triangular Lattices

In this work we use Floquet theory to theoretically study the influence of monochromatic circularly and linearly polarized light on the Hofstadter butterfly---induced by a uniform perpendicular magnetic field--for both the kagome and triangular lattices. In the absence of the laser light, the butterfly has fractal structure with inversion symmetry about magnetic flux $ϕ=1/4$, and reflection symmetry about $ϕ=1/2$. As the system is exposed to an external laser, we find circularly polarized light deforms the butterfly by breaking the mirror symmetry at flux $ϕ=1/2$. By contrast, linearly polarized light deforms the original butterfly while preserving the mirror symmetry at flux $ϕ=1/2$. We find the inversion symmetry is always preserved for both linear and circular polarized light. For linearly polarized light, the Hofstadter butterfly depends on the polarization direction. Further, we study the effect of the laser on the Chern number of lowest band in the off-resonance regime (laser frequency is larger than the bandwidth). For circularly polarized light, we find that low laser intensity will not change the Chern number, but beyond a critical intensity the Chern number will change. For linearly polarized light, the Chern number depends on the polarization direction. Our work highlights the generic features expected for the periodically driven Hofstadter problem on different lattices.

cond-mat.mes-hall↗

arXiv2018

Floquet topological transitions in extended Kane-Mele models with disorder

In this work we use Floquet theory to theoretically study the influence of circularly polarized light on disordered two-dimensional models exhibiting topological transitions. We find circularly polarized light can induce a topological transition in extended Kane-Mele models that include additional hopping terms and on-site disorder. The topological transitions are understood from the Floquet-Bloch band structure of the clean system at high symmetry points in the first Brillouin zone. The light modifies the equilibrium band structure of the clean system in such a way that the smallest gap in the Brillouin zone can be shifted from the $M$ points to the $K(K')$ points, the $Γ$ point, or even other lower symmetry points. The movement of the minimal gap point through the Brillouin zone as a function of laser parameters is explained in the high frequency regime through the Magnus expansion. In the disordered model, we compute the Bott index to reveal topological phases and transitions. The disorder can induce transitions from topologically non-trivial states to trivial states or vice versa, both examples of Floquet topological Anderson transitions. As a result of the movement of the minimal gap point through the Brillouin zone as a function of laser parameters, the nature of the topological phases and transitions is laser-parameter dependent--a contrasting behavior to the Kane-Mele model.

cond-mat.mes-hall↗

arXiv2017

Dynamical recovery of SU(2) symmetry in the mass-quenched Hubbard model

We use non-equilibrium dynamical mean-field theory with iterative perturbation theory as an impurity solver to study the recovery of $SU(2)$ symmetry in real-time following a hopping integral parameter quench from a mass-imbalanced to a mass-balanced single-band Hubbard model at half-filling. A dynamical order parameter $γ(t)$ is defined to characterize the evolution of the system towards $SU(2)$ symmetry. By comparing the momentum dependent occupation from an equilibrium calculation (with the $SU(2)$ symmetric Hamiltonian after the quench at an effective temperature) with the data from our non-equilibrium calculation, we conclude that the $SU(2)$ symmetry recovered state is a thermalized state. Further evidence from the evolution of the density of states supports this conclusion. At the same time, we find the order parameter in the weak Coulomb interaction regime undergoes an approximate exponential decay. We numerically investigate the interplay of the relevant parameters (initial temperature, Coulomb interaction strength, initial mass-imbalance ratio) and their combined effect on the thermalization behavior. Finally, we study evolution of the order parameter as the hopping parameter is changed with either a linear ramp or a pulse. Our results can be useful in strategies to engineer the relaxation behavior of interacting, quantum many-particle systems.

cond-mat.str-el↗

arXiv2017

Orbital-selective thermalization plateau in the mass imbalanced Hubbard model

We use time-dependent non-equilibrium dynamical mean-field theory with weak-coupling auxiliary-field continuous time quantum Monte Carlo as an impurity solver to study the thermalization behavior of the mass-imbalanced single-band Hubbard model after a quench of the Coulomb interaction from the non-interacting limit to a finite positive value. By contrast, when the Coulomb interaction in our model is increased under equilibrium conditions, the quasi-particle weight for spin-up and spin-down (the mass imbalance) electrons approach zero simultaneously, indicating the absence of an orbital selective Mott transition. Our out-of-equilibrium study suggests that there exists a time window where an orbital selective dynamical phase transition occurs. The dynamical phase transition is characterized by the relaxation behavior of energy (kinetic and Coulomb interaction) and the spin-resolved momentum-dependent occupation. To make connection with possible experiments, we calculate the spin-resolved two-time optical conductivity, which confirms the orbital-selective thermalization plateau. We find the time window for the orbital selective dynamical phase transition grows as the mass imbalance increases.

cond-mat.str-el↗

arXiv2017

Floquet band structure of a semi-Dirac system

In this work we use Floquet-Bloch theory to study the influence of circularly and linearly polarized light on two-dimensional band structures with semi-Dirac band touching points, taking the anisotropic nearest neighbor hopping model on the honeycomb lattice as an example. We find circularly polarized light opens a gap and induces a band inversion to create a finite Chern number in the two-band model. By contrast, linearly polarized light can either open up a gap (polarized in the quadratically dispersing direction) or split the semi-Dirac band touching point into two Dirac points (polarized in the linearly dispersing direction) by an amount that depends on the amplitude of the light. Motivated by recent pump-probe experiments, we investigated the non-equilibrium spectral properties and momentum-dependent spin-texture of our model in the Floquet state following a quench in absence of phonons, and in the presence of phonon dissipation that leads to a steady-state independent of the pump protocol. Finally, we make connections to optical measurements by computing the frequency dependence of the longitudinal and transverse optical conductivity for this two-band model. We analyze the various contributions from inter-band transitions and different Floquet modes. Our results suggest strategies for optically controlling band structures and experimentally measuring topological Floquet systems.

cond-mat.mes-hall↗

arXiv2017

Floquet states in (LaNiO$_3$)$_2$/(LaAlO$_3$)$_N$ heterostructures grown along the (111) direction

Using Floquet-Bloch theory we study the effect of circularly and linearly polarized light on the electronic structure of (LaNiO$_3$)$_2$/(LaAlO$_3$)$_N$ heterostructure grown along the (111) direction. In equilibrium, a tight-binding fit to the first principles band structure shows that nearest-neighbor hopping plays a dominant role while second-neighbor hopping breaks the particle-hole symmetry and determines the finer band features. The four bands of the LaNiO$_3$ bilayer exhibit both quadratic band touching points and Dirac points. By varying the amplitude of the incident light, one can independently tune the first and second-neighbor hopping for fixed frequency, which leads to considerable control over the Floquet band structure. We investigate this control in detail, and study how the quadratic and Dirac band touchings are influenced by the polarization and intensity of the light. We derive effective 2-band Hamiltonians (for both quadratic and Dirac band touching points) that accurately captures these results. We further study an extended model which explicitly includes oxygen $p$-orbitals and compare the results to the effective model that contains only the nickel $d$-orbitals. We conclude with a computation of the frequency dependent optical Hall conductivity using the full four band model and analyze the various inter-band contributions of the Floquet modes.

cond-mat.mes-hall↗

arXiv2016

Thermal conductivity of local moment models with strong spin-orbit coupling

We study the magnetic and lattice contributions to the thermal conductivity of electrically insulating strongly spin-orbit coupled magnetically ordered phases on a two-dimensional honeycomb lattice using the Kitaev-Heisenberg model. Depending on model parameters, such as the relative strength of the spin-orbit induced anisotropic coupling, a number of magnetically ordered phases are possible. In this work, we study two distinct regimes of thermal transport depending on whether the characteristic energy of the phonons or the magnons dominates, and focus on two different relaxation mechanisms, boundary scattering and magnon-phonon scattering. For spatially anisotropic magnetic phases, the thermal conductivity tensor can be highly anisotropic when the magnetic energy scale dominates, since the magnetic degrees of freedom dominate the thermal transport for temperatures well below the magnetic transition temperature. In the opposite limit in which the phonon energy scale dominates, the thermal conductivity will be nearly isotropic, reflecting the isotropic (at low temperatures) phonon dispersion assumed for the honeycomb lattice. We further discuss the extent to which thermal transport properties are influenced by strong spin-orbit induced anisotropic coupling in the local moment regime of insulating magnetic phases. The developed methodology can be applied to any 2D magnon-phonon system, and more importantly to systems where an analytical Bogoliubov transformation cannot be found and magnon bands are not necessarily isotropic.

cond-mat.mes-hall↗

arXiv2016

Quadratic band touching points and flat bands in two-dimensional topological Floquet systems

In this work we theoretically study, using Floquet-Bloch theory, the influence of circularly and linearly polarized light on two-dimensional band structures with Dirac and quadratic band touching points, and flat bands, taking the nearest neighbor hopping model on the kagome lattice as an example. We find circularly polarized light can invert the ordering of this three band model, while leaving the flat-band dispersionless. We find a small gap is also opened at the quadratic band touching point by 2-photon and higher order processes. By contrast, linearly polarized light splits the quadratic band touching point (into two Dirac points) by an amount that depends only on the amplitude and polarization direction of the light, independent of the frequency, and generally renders dispersion to the flat band. The splitting is perpendicular to the direction of the polarization of the light. We derive an effective low-energy theory that captures these key results. Finally, we compute the frequency dependence of the optical conductivity for this 3-band model and analyze the various interband contributions of the Floquet modes. Our results suggest strategies for optically controlling band structure and interaction strength in real systems.

cond-mat.mes-hall↗

arXiv2016

Disorder effects in correlated topological insulators

Using exact diagonalization and quantum Monte Carlo calculations we investigate the effects of disorder on the phase diagram of both non-interacting and interacting models of two-dimensional topological insulators. In the fermion sign problem-free interacting models we study, electron-electron interactions are described by an on-site repulsive Hubbard interaction and disorder is included via the one-body hopping operators. In both the non-interacting and interacting models we make use of recent advances in highly accurate real-space numerical evaluation of topological invariants to compute phase boundaries, and in the non-interacting models determine critical exponents of the transitions. We find different models exhibit distinct stability conditions of the topological phase with respect to interactions and disorder. We provide a general analytical theory that accurately predicts these trends.

cond-mat.str-el↗

arXiv2016

Thermoelectric transport in double-Weyl semimetals

We study the thermoelectric properties of a double-Weyl fermion system, possibly realized in $\mathrm{HgCr_2Se_4}$ and $\mathrm{SrSi_2}$, by a semi-classical Boltzmann transport theory. We investigate different relaxation processes including short-range disorder and electron-electron interaction on the thermoelectric transport coefficients. It is found that the anisotropy of the band dispersion for in-plane and out-of-plane momentum directions affects the relaxation time for transport in different directions. The transport also exhibits an interesting directional dependence on the chemical potential and model parameters, differing from a simple isotropic quadratic or linearly dispersing electron gas. By applying a static magnetic field along the linearly dispersing direction, the longitudinal and transverse electrical and thermal magnetoconductivity show a similar dependence on the in-plane cyclotron frequency to the linear dispersing Weyl nodes. By including internode scattering, we find that the chiral anomaly contribution to the thermoelectric coefficients doubles that of a linearly dispersing Weyl node in both the semi-classical and quantum regimes. A magnetic field applied along the quadratically dispersing direction will split the double Weyl point into two single Weyl points with the same chirality.

cond-mat.str-el↗

arXiv2015

Universal entanglement spectra in critical spin chains

We advocate that in critical spin chains, and possibly in a larger class of 1D critical models, a gap in the momentum-space entanglement spectrum separates the universal part of the spectrum, which is determined by the associated conformal field theory, from the non-universal part, which is specific to the model. To this end, we provide affirmative evidence from multicritical spin chains with low energy sectors described by the SU(2)$_2$ or the SU(3)$_1$ Wess-Zumino-Witten model.

cond-mat.str-el↗

arXiv2015

Fractionalized Topological Insulators

Topological insulators have emerged as a major topic of condensed matter physics research with several novel applications proposed. Although there are now a number of established experimental examples of materials in this class, all of them can be described by theories based on electronic band structure, which implies that they do not possess electronic correlations strong enough to fundamentally change this theoretical description. Here, we review recent theoretical progress in the description of a class of strongly correlated topological insulators - fractionalized topological insulators - where band theory fails dramatically due to the fractionalization of the electron into other degrees of freedom.

cond-mat.str-el↗

arXiv2015

Electronic Cooling in Weyl and Dirac Semimetals

Energy transfer from electrons to phonons is an important consideration in any Weyl or Dirac semimetal based application. In this work, we analytically calculate the cooling power of acoustic phonons, i.e. the energy relaxation rate of electrons which are interacting with acoustic phonons, for Weyl and Dirac semimetals in a variety of different situations. For cold Weyl or Dirac semimetals with the Fermi energy at the nodal points, we find the electronic temperature, $T_e$, decays in time as a power law. In the heavily doped regime, $T_e$ decays linearly in time far away from equilibrium. In a heavily doped system with short-range disorder we predict the cooling power of acoustic phonons is drastically increased because of an enhanced energy transfer between electrons and phonons. When an external magnetic field is applied to an undoped system, the cooling power is linear in magnetic field strength and $T_e$ has square root decay in time, independent of magnetic field strength over a range of values.

cond-mat.str-el↗

arXiv2015

Correlation effects in pyrochlore iridate thin films grown along the $[111]$ direction

Over the past few years bulk pyrochlore iridates of the form $A_2$Ir$_2$O$_7$ (where $A$ is a rare earth element, Ir is iridium, and O is oxygen) have been studied as model systems for investigating the interplay of electronic correlations and strong spin-orbit coupling, particularly with the aim of finding correlation-driven topological phases. In this work, we use cellular dynamical mean field theory (CDMFT) to study effects of electronic correlations beyond Hartree-Fock theory in thin films of pyrochlore irradiates grown along the $[111]$ direction. We focus on the bilayer and trilayer systems, and compute the phase diagrams of these systems as a function of electron-electron interaction strength, which is modeled by an on-site Hubbard interaction. By evaluating the $Z_2$ invariant and Chern number using formulas based on the single-particle Green's function and the quasi-particle effective Hamiltonian, we show that on-site correlations can drive an interaction-induced topological phase transition, turning a time-reversal invariant topological insulator and a nearly flat band metal to a correlated Chern insulator (CI) in bilayer and trilayer systems, respectively. By comparing with the Hartree-Fock results, the CDMFT results show that quantum fluctuations enhance the robustness of the interaction-driven CI phase in the thin films. Furthermore, our numerical analysis of the quasiparticle spectrum reveals that the topological phases we find in our many-body calculations are adiabatically connected to those in the single-particle picture.

cond-mat.str-el↗

arXiv2015

Nanoscale $β$-Nuclear Magnetic Resonance Depth Imaging of Topological Insulators

Considerable evidence suggests that variations in the properties of topological insulators (TIs) at the nanoscale and at interfaces can strongly affect the physics of topological materials. Therefore, a detailed understanding of surface states and interface coupling is crucial to the search for and applications of new topological phases of matter. Currently, no methods can provide depth profiling near surfaces or at interfaces of topologically inequivalent materials. Such a method could advance the study of interactions. Herein we present a non-invasive depth-profiling technique based on $β$-NMR spectroscopy of radioactive $^8$Li$^+$ ions that can provide "one-dimensional imaging" in films of fixed thickness and generates nanoscale views of the electronic wavefunctions and magnetic order at topological surfaces and interfaces. By mapping the $^8$Li nuclear resonance near the surface and 10 nm deep into the bulk of pure and Cr-doped bismuth antimony telluride films, we provide signatures related to the TI properties and their topological non-trivial characteristics that affect the electron-nuclear hyperfine field, the metallic shift and magnetic order. These nanoscale variations in $β$-NMR parameters reflect the unconventional properties of the topological materials under study, and understanding the role of heterogeneities is expected to lead to the discovery of novel phenomena involving quantum materials.

cond-mat.mtrl-sci↗

arXiv2014

Momentum-Space Entanglement Spectrum of Bosons and Fermions with Interactions

We study the momentum space entanglement spectra of bosonic and fermionic formulations of the spin-1/2 XXZ chain with analytical methods and exact diagonalization. We investigate the behavior of the entanglement gaps, present in both partitions, across quantum phase transitions in the XXZ chain. In both cases, finite size scaling reveals that the entanglement gap closure does not occur at the physical transition points. For bosons, we find that the entanglement gap observed in [Thomale et al., Phys. Rev. Lett. 105, 116805 (2010)] depends on the scaling dimension of the conformal field theory as varied by the XXZ anisotropy. For fermions, the infinite entanglement gap present at the XX point persists well past the phase transition at the Heisenberg point. We elaborate on how these shifted transition points in the entanglement spectra may in fact support the numerical study of physical transitions in the momentum space density matrix renormalization group.

cond-mat.str-el↗