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Guangkai Zhang

Publications and source records attributed to Guangkai Zhang.

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$d$-wave altermagnetism revealed by resonant inelastic X-ray scattering

Altermagnetism defines a third fundamental class of collinear magnetic order, featuring compensated magnetic moments with antiparallel spin alignment, yet lifted Kramers degeneracy without the need for relativistic spin-orbit coupling. Its ability to host spin-polarized electronic bands and unconventional chiral magnons makes it a promising platform for functional materials. However, experimental verification has proven challenging; while circular dichroism in resonant inelastic X-ray scattering (RIXS) has been suggested as a signature of chiral magnons, it remains controversial whether this effect is an intrinsic property of altermagnetism or an artifact of experimental geometry. In this work, we resolve this debate and provide unambiguous experimental evidence of $d$-wave altermagnetism in the strongly correlated Lieb-lattice magnet La$_2$O$_3$Mn$_2$Se$_2$. The RIXS spectra exhibit a $d$-wave-symmetry circular dichroism in the magnetic excitations that vanishes in the paramagnetic phase. Through RIXS-operator symmetry analysis and exact-diagonalization calculations, we prove that the observed dichroism is a direct consequence of altermagnetic symmetry constraints, independent of magnon branch splitting. Our results provide definitive evidence for the experimental realization of $d$-wave altermagnetism in La$_2$O$_3$Mn$_2$Se$_2$ and establish circularly polarized RIXS as a highly symmetry-sensitive spectroscopic framework for detecting magnetic phases that evade conventional probes.

cond-mat.str-el

Long-range magnetic order with disordered spin orientations in a high-entropy antiferromagnet

Disorder in magnetic systems typically suppresses long-range order, promoting short-range states such as spin glasses and magnetic clusters. This is particularly prominent in high-entropy materials, characterized by the random distributions of local magnetic entities and exchange interactions. However, in rare exceptions, long-range magnetic order can persist in high-entropy systems, while the microscopic characters and underlying mechanisms remain elusive, especially the magnetic behaviors of individual elements. Here, combining neutron diffraction and resonant soft x-ray scattering, we have conducted an element-specific investigation into the magnetic order of a high-entropy honeycomb-lattice van der Waals material (Mn1/4Fe1/4Co1/4Ni1/4)PS3. Despite significant atomic disorder, long-range zigzag antiferromagnetic order is observed below 72 K, with all four transition-metal elements participating in a unified phase transition. However, the spin orientations of various elements are distinct, attributed to the competition between single-ion anisotropies and exchange interactions. Our findings showcase a novel form of long-range magnetic order with disordered spin orientations, which is synergically stabilized by distinct magnetic elements in a high entropy magnet, offering a new paradigm for understanding complex magnetic systems.

cond-mat.str-el