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Guangyu Fan

Publications and source records attributed to Guangyu Fan.

8 recordsLinked to original sources

Engineering High-Order Harmonic Generation through Gas Confinement at Sub-Millimeter Lengths

Attosecond light sources based on high-order harmonic generation (HHG) constitute to date the only table-top solution for producing coherent broadband radiation covering the spectral range from the extreme ultraviolet to the soft X-rays. The so-called emission cutoff can be extended towards higher photon energies by increasing the driving wavelength at the expense of conversion efficiency. An alternative route is to overdrive the process by using higher laser intensities, with the challenging requirement of interacting with higher plasma densities over short propagation distances. Here, we address this challenge by using a differentially pumped glass chip designed for optimal gas confinement over sub-mm lengths. By driving HHG with multicycle pulses at either 800 nm or 1500 nm, we demonstrate a cutoff extension by a factor of two compared to conventional phase matching approaches and surpassing the present record using multicycle fields. Our three-dimensional propagation simulations, in excellent agreement with the experiment, confirm that gas confinement is crucial since efficient phase matching of cutoff harmonics occurs only for short propagation lengths. Additionally, we show that the high photon energy component is not only temporally confined to the leading edge of the driving pulse, but also spatially confined in the near-field to an off-axis contribution due to reshaping of the driving field along propagation inside the medium. Our findings contribute to the fundamental understanding of HHG across different regimes.

physics.optics

Spatiotemporal Topological Combs for Robust High-Dimensional Information Transmission

Sculpting light across its independent degrees of freedom-from orbital angular momentum to the discrete wavelengths of optical frequency combs-has unlocked vast communication bandwidth by enabling massively parallel information channels. However, the Shannon-Hartley theorem sets a hard limit by tying channel capacity to the trade-off between SNR and rate, a central challenge in communication. Inspired by lock-in amplification in electronics, we encode data on THz optical burst carriers so the signal resides beyond the conventional noise band, yielding exceptional robustness. By leveraging a programmable all-degree-of-freedom (All-DoF) modulator, we generate a spatiotemporal topological comb (ST-Comb) that structures light into a vast, highentropy state space for high-dimensional information encoding. Crucially, we find that the associated topological winding number is preserved under diverse perturbations, ensuring stable information encoding and retrieval. This paradigm illustrates how structured light can simultaneously expand channel dimensionality and maintain robustness, charting a pathway to chip-scale, reconfigurable photonic platforms for the PHz era, while also opening previously inaccessible regimes of light-matter interaction.

physics.optics

Resolving Rydberg-Electron Recapture Dynamics via Laser-driven Frustrated Tunneling Ionization

By employing two-color counter-rotating circularly polarized laser fields, we investigate the dynamics of electron recapture into Rydberg states under strong, ultrashort laser pulses, probed via coherent extreme-ultraviolet free-induction decay (XFID). Our study reveals significant distinctions between XFID and above-threshold high-order harmonic generation in terms of their ellipticity dependence on the driving-laser waveforms, yield variations with the laser-intensity ratios, and sensitivity to the driving-laser ellipticity. All these differences arise from the fundamentally distinct electron trajectories underlying the two processes. More importantly, our findings provide compelling evidence that Rydberg-electron recapture predominantly occurs at the end of the driving laser field, offering the first direct experimental confirmation of this long-proposed mechanism.

physics.optics

Transfer Learning in Vocal Education: Technical Evaluation of Limited Samples Describing Mezzo-soprano

Vocal education in the music field is difficult to quantify due to the individual differences in singers' voices and the different quantitative criteria of singing techniques. Deep learning has great potential to be applied in music education due to its efficiency to handle complex data and perform quantitative analysis. However, accurate evaluations with limited samples over rare vocal types, such as Mezzo-soprano, requires extensive well-annotated data support using deep learning models. In order to attain the objective, we perform transfer learning by employing deep learning models pre-trained on the ImageNet and Urbansound8k datasets for the improvement on the precision of vocal technique evaluation. Furthermore, we tackle the problem of the lack of samples by constructing a dedicated dataset, the Mezzo-soprano Vocal Set (MVS), for vocal technique assessment. Our experimental results indicate that transfer learning increases the overall accuracy (OAcc) of all models by an average of 8.3%, with the highest accuracy at 94.2%. We not only provide a novel approach to evaluating Mezzo-soprano vocal techniques but also introduce a new quantitative assessment method for music education.

eess.AS

Extension of the bright high-harmonic photon energy range via nonadiabatic critical phase matching

Extending the photon energy range of bright high-harmonic generation to cover the entire soft X-ray region is important for many applications in science and technology. The concept of critical ionization fraction has been essential, because it dictates the maximum driving laser intensity that can be used while preserving bright harmonic emission. In this work, we reveal a second, nonadiabatic critical ionization fraction that substantially extends the maximum phase-matched high-harmonic photon energy, that arises due to strong reshaping of the intense driving laser field. We validate this understanding through a systematic comparison between experiment and theory, for a wide range of pulse durations and driving laser wavelengths. In particular, high harmonics driven by intense few-cycle pulses experience the most pronounced spectral reshaping, significantly extending the bright photon energy range. We also present an analytical model that predicts the spectral extension that can be achieved for different driving lasers. This reveals an increasing role of nonadiabatic critical phase matching when driven by few-cycle mid-infrared lasers. These findings are important for the development of high-brightness soft X-ray sources for applications in spectroscopy and imaging.

physics.optics

Spatially homogeneous few-cycle compression of Yb lasers via all-solid-state free-space soliton management

The high power and variable repetition rate of Yb femtosecond lasers make them very attractive for ultrafast science. However, for capturing sub-200 fs dynamics, efficient, high-fidelity, and high-stability pulse compression techniques are essential. Spectral broadening using an all-solid-state free-space geometry is particularly attractive, as it is simple, robust, and low-cost. However, spatial and temporal losses caused by spatio-spectral inhomogeneities have been a major challenge to date, due to coupled space-time dynamics associated with unguided nonlinear propagation. In this work, we use all-solid-state free-space compressors to demonstrate compression of 170 fs pulses at a wavelength of 1030nm from a Yb:KGW laser to ~9.2 fs, with a highly spatially homogeneous mode. This is achieved by ensuring that the nonlinear beam propagation in periodic layered Kerr media occurs in soliton modes and confining the nonlinear phase through each material layer to less than 1.0 rad. A remarkable spatio-spectral homogeneity of ~0.87 can be realized, which yields a high efficiency of >50% for few-cycle compression. The universality of the method is demonstrated by implementing high-quality pulse compression under a wide range of laser conditions. The high spatiotemporal quality and the exceptional stability of the compressed pulses are further verified by high-harmonic generation. This work represents the highest efficiency and the best spatio-spectral quality ever achieved by an all-solid-state free-space pulse compressor for few-cycle-pulse generation.

physics.optics

Solitary beam propagation in a nonlinear optical resonator enables high-efficiency pulse compression and mode self-cleaning

Generating intense ultrashort pulses with high-quality spatial modes is crucial for ultrafast and strong-field science. This can be accomplished by controlling propagation of femtosecond pulses under the influence of Kerr nonlinearity and achieving stable propagation with high intensity. In this work, we propose that the generation of spatial solitons in periodic layered Kerr media can provide an optimum condition for supercontinuum generation and pulse compression using multiple thin plates. With both the experimental and theoretical investigations, we successfully identify these solitary modes and reveal a universal relationship between the beam size and the critical nonlinear phase. Space-time coupling is shown to strongly influence the spectral, spatial and temporal profiles of femtosecond pulses. Taking advantage of the unique characters of these solitary modes, we demonstrate single-stage supercontinuum generation and compression of femtosecond pulses from initially 170 fs down to 22 fs with an efficiency ~90%. We also provide evidence of efficient mode self-cleaning which suggests rich spatial-temporal self-organization processes of laser beams in a nonlinear resonator.

physics.optics

Enhanced multi-colour gating for the generation of high-power isolated attosecond pulses

Isolated attosecond pulses (IAP) generated by high-order harmonic generation are valuable tools that enable dynamics to be studied on the attosecond time scale. The applicability of these IAP would be widened drastically by increasing their energy. Here we analyze the potential of using multi-colour driving pulses for temporally gating the attosecond pulse generation process. We devise how this approach can enable the generation of IAP with the available high-energy kHz-repetition-rate Ytterbium-based laser amplifiers (delivering 180-fs, 1030-nm pulses). We show theoretically that this requires a three-colour field composed of the fundamental and its second harmonic as well as a lower-frequency auxiliary component. We present pulse characterization measurements of such auxiliary pulses generated directly by white-light seeded OPA with the required significantly shorter pulse duration than the that of the fundamental. This, combined with our recent experimental results on three-colour waveform synthesis [Phys. Rev. X 4, 021028 (2014)], proves that the theoretically considered multi-colour drivers for IAP generation can be realized with existing high-power laser technology. The high-energy driver pulses, combined with the strongly enhanced single-atom-level conversion efficiency we observe in our calculations, thus make multi-colour drivers prime candidates for the development of unprecedented high-energy IAP sources in the near future.

physics.atom-ph