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Guido Burkard

Publications and source records attributed to Guido Burkard.

At least 127 records · Page 7Linked to original sources

Spectra of ultrabroadband squeezed pulses and the finite-time Unruh-Davies effect

We study spectral properties of quantum radiation of ultimately short duration. In particular, we introduce a continuous multimode squeezing operator for the description of subcycle pulses of entangled photons generated by a coherent-field driving in a thin nonlinear crystal with second order susceptibility. We find the ultrabroadband spectra of the emitted quantum radiation perturbatively in the strength of the driving field. These spectra can be related to the spectra expected in an Unruh-Davies experiment with a finite time of acceleration. In the time domain, we describe the corresponding behavior of the normally ordered electric field variance.

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Subcycle squeezing of light from a time flow perspective

Light as a carrier of information and energy plays a fundamental role in both general relativity and quantum physics, linking these areas that are still not fully compliant with each other. Its quantum nature and spatio-temporal structure are exploited in many intriguing applications ranging from novel spectroscopy methods of complex many-body phenomena to quantum information processing and subwavelength lithography. Recent access to subcycle quantum features of electromagnetic radiation promises a new class of time-dependent quantum states of light. Paralleled with the developments in attosecond science, these advances motivate an urgent need for a theoretical framework that treats arbitrary wave packets of quantum light intrinsically in the time domain. Here, we formulate a consistent time domain theory of the generation and sampling of few-cycle and subcycle pulsed squeezed states, allowing for a relativistic interpretation in terms of induced changes in the local flow of time. Our theory enables the use of such states as a resource for novel ultrafast applications in quantum optics and quantum information.

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A quadrupolar exchange-only spin qubit

We propose a quadrupolar exchange-only spin (QUEX) qubit that is highly robust against charge noise and nuclear spin dephasing, the dominant decoherence mechanisms in quantum dots. The qubit consists of four electrons trapped in three quantum dots, and operates in a decoherence-free subspace to mitigate dephasing due to nuclear spins. To reduce sensitivity to charge noise, the qubit can be completely operated at an extended charge noise sweet spot that is first-order insensitive to electrical fluctuations. Due to on-site exchange mediated by the Coulomb interaction, the qubit energy splitting is electrically controllable and can amount to several GHz even in the ``off" configuration, making it compatible with conventional microwave cavities.

cond-mat.mes-hall↗

Tunable Berry curvature, valley and spin Hall effect in Bilayer MoS$_2$

The chirality of electronic Bloch bands is responsible for many intriguing properties of layered two-dimensional materials. We show that in bilayers of transition metal dichalcogenides (TMDCs), unlike in few-layer graphene and monolayer TMDCs, both intra-layer and inter-layer couplings give important contributions to the Berry-curvature in the $K$ and $-K$ valleys of the Brillouin zone. The inter-layer contribution leads to the stacking dependence of the Berry curvature and we point out the differences between the commonly available 3R type and 2H type bilayers. Due to the inter-layer contribution the Berry curvature becomes highly tunable in double gated devices. We study the dependence of the valley Hall and spin Hall effects on the stacking type and external electric field. Although the valley and spin Hall conductivities are not quantized, in MoS$_2$ 2H bilayers they may change sign as a function of the external electric field which is reminiscent of the behaviour of lattice Chern insulators.

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Spin-Degenerate Regimes for Single Quantum Dots in Transition Metal Dichalcogenide Monolayers

Strong spin-orbit coupling in transition metal dichalcogenide (TMDC) monolayers results in spin resolvable band structures about the $K$ and $K'$ valleys such that the eigenbasis of a 2D quantum dot (QD) in a TMDC monolayer in zero field is described by the Kramers pairs $|0\rangle_-=|K'\uparrow\rangle$, $|1\rangle_-=|K\downarrow\rangle$ and $|0\rangle_+=|K\uparrow\rangle$, $|1\rangle_+=|K'\downarrow\rangle$. The strong spin-orbit coupling limits the usefulness of single TMDC QDs as spin qubits. Possible regimes of spin-degenerate states, overcoming the spin-orbit coupling in monolayer TMDC QDs are investigated in both zero field, where the spin and valley degrees of freedom become fourfold degenerate, and twofold degeneracy in some magnetic field, localised to a given valley. Such regimes are shown to be achievable in MoS$_{2}$, where the spin orbit coupling is sufficiently low and of the right sign such that the spin resolved conduction bands intersect at points about the $K$ and $K'$ valleys and as such may be exploited by selecting suitable critical dot radii.

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Theory of Strain-Induced Confinement in Transition Metal Dichalcogenide Monolayers

Recent experimental studies of out-of-plane straining geometries of transition metal dichalchogenide (TMD) monolayers have demonstrated sufficient band gap renormalisation for device application such as single photon emitters. Here, a simple continuum-mechanical plate-theory approach is used to estimate the topography of TMD monolayers layered atop nanopillar arrays. From such geometries, the induced conduction band potential and band gap renormalisation is given, demonstrating a curvature of the potential that is independent of the height of the deforming nanopillar. Additionally, with a semi-classical WKB approximation, the expected escape rate of electrons in the strain potential may be calculated as a function of the height of the deforming nanopillar. This approach is in accordance with experiment, supporting recent findings suggesting that increasing nanopillar height decreases the linewidth of the single photon emitters observed at the tip of the pillar, and predicting the shift in photon energy with nanopillar height for systems with consistent topography.

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Effective theory of monolayer TMDC double quantum dots

Monolayer Transition Metal Dichalcogenides (TMDCs) are promising candidates for quantum technologies, such as quantum dots, because they are truly two-dimensional semiconductors with a direct band gap. In this work, we analyse theoretically the behaviour of a double quantum dot (DQD) system created in the conduction band of these materials, with two electrons in the (1,1) charge configuration. Motivated by recent experimental progress, we consider several scenarios, including different spin-orbit splittings in the two dots and including the case when the valley degeneracy is lifted due to an insulating ferromagnetic substrate. Finally, we discuss in which cases it is possible to reduce the low energy subspace to the lowest Kramers pairs. We find that in this case the low energy model is formally identical to the Heisenberg exchange Hamiltonian.

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Spin-strain interaction in nitrogen-vacancy centers in diamond

The interaction of solid-state electronic spins with deformations of their host crystal is an important ingredient in many experiments realizing quantum information processing schemes. Here, we theoretically characterize that interaction for a nitrogen-vacancy (NV) center in diamond. We derive the symmetry-allowed Hamiltonian describing the interaction between the ground-state spin-triplet electronic configuration and the local strain. We numerically calculate the six coupling-strength parameters of the Hamiltonian using density functional theory, and propose an experimental setup for measuring those coupling strengths. The importance of this interaction is highlighted by the fact that it enables to drive spin transitions, both magnetically allowed and forbidden, via mechanically or electrically driven spin resonance. This means that the ac magnetic field routinely used in a wide range of spin-resonance experiments with NV centers could in principle be replaced by ac strain or ac electric field, potentially offering lower power requirements, simplified device layouts, faster spin control, and local addressability of electronic spin qubits.

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High-fidelity quantum gates in Si/SiGe double quantum dots

Motivated by recent experiments of Zajac et al. [arXiv:1708.03530], we theoretically describe high-fidelity two-qubit gates using the exchange interaction between the spins in neighboring quantum dots subject to a magnetic field gradient. We use a combination of analytical calculations and numerical simulations to provide the optimal pulse sequences and parameter settings for the gate operation. We present a novel synchronization method which avoids detrimental spin flips during the gate operation and provide details about phase mismatches accumulated during the two-qubit gates which occur due to residual exchange interaction, non-adiabatic pulses, and off-resonant driving. By adjusting the gate times, synchronizing the resonant and off-resonant transitions, and compensating these phase mismatches by phase control, the overall gate fidelity can be increased significantly.

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A Coherent Spin-Photon Interface in Silicon

Electron spins in silicon quantum dots are attractive systems for quantum computing due to their long coherence times and the promise of rapid scaling using semiconductor fabrication techniques. While nearest neighbor exchange coupling of two spins has been demonstrated, the interaction of spins via microwave frequency photons could enable long distance spin-spin coupling and "all-to-all" qubit connectivity. Here we demonstrate strong-coupling between a single spin in silicon and a microwave frequency photon with spin-photon coupling rates g_s/(2π) > 10 MHz. The mechanism enabling coherent spin-photon interactions is based on spin-charge hybridization in the presence of a magnetic field gradient. In addition to spin-photon coupling, we demonstrate coherent control of a single spin in the device and quantum non-demolition spin state readout using cavity photons. These results open a direct path toward entangling single spins using microwave frequency photons.

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Input-output theory for spin-photon coupling in Si double quantum dots

The interaction of qubits via microwave frequency photons enables long-distance qubit-qubit coupling and facilitates the realization of a large-scale quantum processor. However, qubits based on electron spins in semiconductor quantum dots have proven challenging to couple to microwave photons. In this theoretical work we show that a sizable coupling for a single electron spin is possible via spin-charge hybridization using a magnetic field gradient in a silicon double quantum dot. Based on parameters already shown in recent experiments, we predict optimal working points to achieve a coherent spin-photon coupling, an essential ingredient for the generation of long-range entanglement. Furthermore, we employ input-output theory to identify observable signatures of spin-photon coupling in the cavity output field, which may provide guidance to the experimental search for strong coupling in such spin-photon systems and opens the way to cavity-based readout of the spin qubit.

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Holonomic Quantum Control by Coherent Optical Excitation in Diamond

Although geometric phases in quantum evolution were historically overlooked, their active control now stimulates strategies for constructing robust quantum technologies. Here, we demonstrate arbitrary single-qubit holonomic gates from a single cycle of non-adiabatic evolution, eliminating the need to concatenate two separate cycles. Our method varies the amplitude, phase, and detuning of a two-tone optical field to control the non-Abelian geometric phase acquired by a nitrogen-vacancy center in diamond over a coherent excitation cycle. We demonstrate the enhanced robustness of detuned gates to excited-state decoherence and provide insights for optimizing fast holonomic control in dissipative quantum systems.

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Hyperfine-induced dephasing in three-electron spin qubits

We calculate the pure dephasing time of three-electron exchange-only qubits due to interaction with the nuclear hyperfine field. Within the $S=S_z=1/2$ spin subspace, we derive formulas for the dephasing time in the $(1,1,1)$ charge region and in the neighboring charge sectors coupled by tunneling. The nuclear field and the tunneling are taken into account in a second order approximation. The analytical solutions accurately reproduce the numerical evaluation of the full problem, and in comparison with existing experimental data, we find that the dephasing times are longer but on the same timescale as for single spins. Our analysis also applies to the resonant exchange (RX), always-on exchange-only (AEON) and hybrid qubits.

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Low-Error Operation of Spin Qubits with Superexchange Coupling

In this theoretical work we investigate superexchange, as a means of indirect exchange interaction between two single electron spin qubits, each embedded in a single semiconductor quantum dot (QD). The exchange interaction is mediated by an intermediate, empty QD. Our findings suggest the existence of first order "super sweet spots", in which the qubit operations implemented by superexchange interaction are simultaneously insensitive to charge noise and errors due to spin-orbit interaction. We also find that the sign of the superexchange can be changed by varying the energy detunings between the QDs.

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High Resolution Valley Spectroscopy of Si Quantum Dots

We study an accumulation mode Si/SiGe double quantum dot (DQD) containing a single electron that is dipole coupled to microwave photons in a superconducting cavity. Measurements of the cavity transmission reveal dispersive features due to the DQD valley states in Si. The occupation of the valley states can be increased by raising temperature or applying a finite source-drain bias across the DQD, resulting in an increased signal. Using cavity input-output theory and a four-level model of the DQD, it is possible to efficiently extract valley splittings and the inter- and intra-valley tunnel couplings.

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Electron Spin Relaxation in a Transition-Metal Dichalcogenide Quantum Dot

We study the relaxation of a single electron spin in a circular quantum dot in a transition-metal dichalcogenide monolayer defined by electrostatic gating. Transition-metal dichalcogenides provide an interesting and promising arena for quantum dot nano-structures due to the combination of a band gap, spin-valley physics and strong spin-orbit coupling. First we will discuss which bound state solutions in different B-field regimes can be used as the basis for qubits states. We find that at low B-fields combined spin-valley Kramers qubits to be suitable, while at large magnetic fields pure spin or valley qubits can be envisioned. Then we present a discussion of the relaxation of a single electron spin mediated by electron-phonon interaction via various different relaxation channels. In the low B-field regime we consider the spin-valley Kramers qubits and include impurity mediated valley mixing which will arise in disordered quantum dots. Rashba spin-orbit admixture mechanisms allows for relaxation by in-plane phonons either via the deformation potential or by piezoelectric coupling, additionally direct spin-phonon mechanisms involving out-of-plane phonons give rise to relaxation. We find that the relaxation rates scale as $\propto B^6$ for both in-plane phonons coupling via deformation potential and the piezoelectric effect, while relaxation due to the direct spin-phonon coupling scales independant to B-field to lowest order but scales strongly on device mechanical tension. We will also discuss the relaxation mechanisms for pure spin or valley qubits formed in the large B-field regime.

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A cavity-mediated quantum CPHASE gate between NV spin qubits in diamond

While long spin coherence times and efficient single-qubit quantum control have been implemented successfully in nitrogen-vacancy (NV) centers in diamond, the controlled coupling of remote NV spin qubits remains challenging. Here, we propose and analyze a controlled-phase (CPHASE) gate for the spins of two NV centers embedded in a common optical cavity and driven by two off-resonant lasers. In combination with previously demonstrated single-qubit gates, CPHASE allows for arbitrary quantum computations. The coupling of the NV spin to the cavity mode is based upon Raman transitions via the NV excited states and can be controlled with the laser intensities and relative phase. We find characteristic laser frequencies at which the scattering amplitude of a laser photon into the cavity mode is strongly dependent on the NV center spin. A scattered photon can be reabsorbed by another selectively driven NV center and generate a conditional phase (CPHASE) gate. Gate times around 200 ns are within reach, nearly three orders of magnitude shorter than typical NV spin coherence times of around 10 microseconds. The separation between the two interacting NV centers is only limited by the extension of the cavity.

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Three-electron spin qubits

The goal of this article is to review the progress of three-electron spin qubits from their inception to the state of the art. We direct the main focus towards the resonant exchange (RX) qubit and the exchange-only qubit, but we also discuss other qubit implementations using three electron spins. For each three-spin qubit we describe the qubit model, the physical realization, the implementations of single-qubit operations, as well as the read-out and initialization schemes. Two-qubit gates and decoherence properties are discussed for the RX qubit and the exchange-only qubit, thereby, completing the list of requirements for a viable candidate qubit implementation for quantum computation. We start with describing the full system of three electrons in a triple quantum dot, then discuss the charge-stability diagram and restrict ourselves to the relevant subsystem, introduce the qubit states, and discuss important transitions to other charge states. Introducing the various qubit implementations, we begin with the exchange-only qubit, followed by the spin-charge qubit, the hybrid qubit, and the RX qubit, discussing for each the single-qubit operations, read-out, and initialization methods, whereas the main focus will be on the RX qubit, whose single-qubit operations are realized by driving the qubit at its resonant frequency in the microwave range similar to electron spin resonance. Two different types of two-qubit operations are presented for the exchange-only and the RX qubit which can be divided into short-ranged and long-ranged interactions. Both of these interaction types can be expected to be necessary in a large-scale quantum computer. We also take into account the decoherence of the qubit through the influence of magnetic noise as well as dephasing due to charge noise.

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