arXiv subjects

Guodong Zhu

Publications and source records attributed to Guodong Zhu.

14 recordsLinked to original sources

arXiv2025

Engineering thermal emission with enhanced emissivity and quality factor using bound states in the continuum and electromagnetically-induced absorption

Metal-based thermal metasurfaces exhibit stable spectral characteristics under temperature fluctuations, in contrast to more traditional gray- and near black-bodies, as well as some dielectric metasurfaces, whose emission spectra shift with changing temperatures. However, they often suffer from limited quality (Q) factors due to significant non-radiative ohmic losses. In this study, we address the challenge of achieving high emissivity and Q-factors in metal-based thermal emitters. By leveraging the coupling between a magnetic dipole resonance and two bound-state-in-continuum (BIC) resonances to achieve electromagnetically induced absorption (EIA) in an asymmetric metallic ring structure, we design a metal-based thermal metasurface with a near-unity emissivity (0.96) and a Q factor as high as 320 per simulations. Experimental validation yields an emissivity of 0.82 and a Q factor of 202, representing an approximately five-fold improvement in the experimentally measured Q factor compared to the state-of-the-art metal-based thermal metasurfaces. Our work offers a promising approach for developing efficient, narrow-band, directional thermal emitters with stable emission spectra across a wide temperature range.

physics.optics↗

arXiv2024

Rapid Trapping and Label-free Characterization of Single Nanoscale Extracellular Vesicles and Nanoparticles in Solution

Achieving high-throughput, comprehensive analysis of single nanoparticles to determine their size, shape, and composition is essential for understanding particle heterogeneity with applications ranging from drug delivery to environmental monitoring. Existing techniques are hindered by low throughput, lengthy trapping times, irreversible particle adsorption, or limited characterization capabilities. Here, we introduce Interferometric Electrohydrodynamic Tweezers (IET), an integrated platform that rapidly traps single nanoparticles in parallel within three seconds. IET enables label-free characterization of particle size and shape via interferometric imaging and identifies molecular composition through Raman spectroscopy, all without the need for fluorescent labeling. We demonstrate the platform's capabilities by trapping and imaging colloidal polymer beads, nanoscale extracellular vesicles (EVs), and newly discovered extracellular nanoparticles known as supermeres. By monitoring their interferometric contrast images while trapped, we accurately determine the sizes of EVs and supermeres. Our IET represents a powerful optofluidics platform for comprehensive characterization of nanoscale objects, opening new avenues in nanomedicine, environmental monitoring, and beyond.

physics.optics↗

arXiv2024

Recent Advances in Nanophotonics for Optofluidics

Optofluidics is dedicated to achieving integrated control of particle and fluid motion, particularly on the micrometer scale, by utilizing light to direct fluid flow and particle motion. The field has seen significant growth recently, driven by the concerted efforts of researchers across various scientific disciplines, notably for its successful applications in biomedical science. In this review, we explore a range of optofluidic architectures developed over the past decade, with a primary focus on mechanisms for precise control of micro and nanoscale biological objects and their applications in sensing. Regarding nanoparticle manipulation, we delve into mechanisms based on optical nanotweezers using nanolocalized light fields and light-based hybrid effects with dramatically improved performance and capabilities. In the context of sensing, we emphasize those works that used optofluidics to aggregate molecules or particles to promote sensing and detection. Additionally, we highlight emerging research directions, encompassing both fundamental principles and practical applications in the field.

physics.optics↗

arXiv2023

Chiral topological whispering gallery modes formed by gyromagnetic photonic crystals

We explore a hexagonal cavity that supports chiral topological whispering gallery (CTWG) modes, formed by a gyromagnetic photonic crystal. This mode is a special type of topologically protected optical mode that can propagate in photonic crystals with chiral direction. Finite element method simulations show that discrete edge states exist in the topological band gap due to the coupling of chiral edge states and WG modes. Since the cavity only supports edge state modes with group velocity in only one direction, it can purely generate traveling modes and be immune to interference modes. In addition, we introduced defects and disorder to test the robustness of the cavity, demonstrating that the CTWG modes can be effectively maintained under all types of perturbations. Our topological cavity platform offers useful prototype of robust topological photonic devices. The existence of this mode can have important implications for the design and application of optical devices.

physics.optics↗

arXiv2023

Merging toroidal dipole bound states in the continuum without up-down symmetry in Lieb lattice metasurfaces

The significance of bound states in the continuum (BICs) lies in their potential for theoretically infinite quality factors. However, their actual quality factors are limited by imperfections in fabrication, which lead to coupling with the radiation continuum. In this study, we present a novel approach to address this issue by introducing a merging BIC regime based on a Lieb lattice. By utilizing this approach, we effectively suppress the out-of-plane scattering loss, thereby enhancing the robustness of the structure against fabrication artifacts. Notably, unlike previous merging systems, our design does not rely on the up-down symmetry of metasurfaces. This characteristic grants more flexibility in applications that involve substrates and superstrates with different optical properties, such as microfluidic devices. Furthermore, we incorporate a lateral band gap mirror into the design to encapsulate the BIC structure. This mirror serves to suppress the in-plane radiation resulting from finite-size effects, leading to a remarkable ten-fold improvement in the quality factor. Consequently, our merged BIC metasurface, enclosed by the Lieb lattice photonic crystal mirror, achieves an exceptionally high-quality factor of 105 while maintaining a small footprint of 26.6X26.6 um. Our findings establish an appealing platform that capitalizes on the topological nature of BICs within compact structures. This platform holds great promise for various applications, including optical trapping, optofluidics, and high-sensitivity biodetection, opening up new possibilities in these fields.

physics.optics↗

arXiv2022

Molecular Plasmon Hybridizition in Olefin Chains

With the continuous emergence of molecular and cluster devices or systems, the relationship between the plasmonic properties of multiple clusters and molecular interactions and the properties of the original single cluster or molecule becomes more and more important. Similar to plasmonic nanoparticle hybridization, there is also a hybrid phenomenon between two molecules with plasmon excitation modes. Using linear response time-dependent density functional theory (LR-TDDFT) and real-time propagation time-dependent density functional theory (RT-TDDFT) and combining the plasmonicity index (PI) and the transition contribution maps (TCM) methods we identify the plasmon excitation mode in the small molecular olefin chains with -OH and -NH2 groups and analyze the hybridization characteristics using charge transitions. The results show that for the plasmons in molecules, there are also plasmon hybridization mechanism exist when the two molecules coupling together. The TCM analysis shows that the plasmon modes and hybridization is a result of coexist of collective and single particle excitation. When there is extra charge depose in the molecules, as the electrons can moving in the whole molecules, the plasmon mode becomes stronger and the individual properties of the molecules maintains in the coupling. The study paves a way for molecule plasmon and the physics picture when the molecules are coupled together.

cond-mat.mes-hall↗

arXiv2021

Analytical Model for Gaussian Disorder Traps in Organic Thin-Film Transistor

Structural defects and chemical impurities exist in organic semiconductors acting as trap centers for the excited states. This work presents a novel analytical model to calculate the trapping and detrapping rates between two Gaussian density of states. Miller-Abrahams rate and Fermi-Dirac statistics are employed in this model. The introduction of effective filled and empty sites for correlated bands greatly simplifies the expression of recombination rate. A technology computer-aided design simulator was used to simulate the donor-like traps in an organic semiconductor DPP-DTT based thin-film transistor, showing good agreement with the measured transfer characteristic.

physics.app-ph↗

arXiv2021

Ring gap resonant modes on disk/film coupling system caused by strong interaction

Peculiar ring gap modes on the surface of disk close to the metallic thin film are excited in the visible light regime. We apply plasmon hybridization method to illustrate the ring gap modes arising from the interaction between localized disk plasmons and continuum surface plasmons, which cannot be easily excited by the plane wave with polarization parallel to the film interface. In the coupled system, the hybrid modes energy and the surface charge distribution of nanoparticle are investigated both in simulation and hybridization method, showing consistence with each other. The excitation of ring gap modes provides further insight into strong coupling of the plasmon and the design of novel nanostructures.

physics.optics↗

arXiv2020

Strong Interaction between Surface Plasmons and Chiral Molecules

In plasmonic chirality, the phenomenon of circular dichroism for achiral nanoparitcles caused by Coulomb interaction between metal nanoparticles (NPs) and chiral molecules have been studied. At the same time, under the resonance condition, the dye molecules and metal NPs will produce huge Rabi splitting due to strong coupling. If the chiral molecules are at the resonance of the plasmon, what will happen for the strong interaction between the plasmon and molecules with chirality introduced? In this paper, we investigate a spherical core-shell model and analyze its spectral phenomena under the excitation of circularly polarized light (CPL). Based on Coulomb interaction between NPs and chiral molecules, we will show how the various factors affect the strong coupling. We have obtained three mechanisms for the interaction between plasmons and chiral molecules: strong coupling (Rabi splitting up to 243mev), enhanced absorption and induced transparency. The interaction between CPL and chiral molecules with the opposite chirality to CPL is stronger than that of the same chirality, and the line width of the two peaks is closer than that of the same chirality, which shows that for the Rabi splitting with chirality, there are deeper mechanisms for the interaction. This result will be helpful for further research on the interaction between plasmon and molecules with chirality.

cond-mat.mes-hall↗

arXiv2020

Quantization of electromagnetic modes and angular momentum on plasmonic nanowires

Quantum theory of surface plasmons is very important for studying the interactions between light and different metal nanostructures in nanoplasmonics. In this work, using the canonical quantization method, the SPPs on nanowires and their orbital and spin angular momentum are investigated. The results show that the SPPs on nanowire carry both orbital and spin momentum during propagation. Later, the result is applied on the plasmonic nanowire waveguide to show the agreement of the theory. The study is helpful for the nano wire based plasmonic interactions and the quantum information based optical circuit in the future.

physics.optics↗

arXiv2020

Orbital angular momentum dichroism caused by the interaction of electric-magnetic dipole moments in chiral metal nanoparticles

Circular dichroism (CD) caused by the response of a chiral object to circularly polarized light has been well established, and the strong CD of plasmonic meta-molecules has also become of interest in recent years; however, their response if the light also has orbital angular momentum is unclear. In this paper, the dichroism of a plasmonic cuboid-protuberance chiral structure under the illumination of a light beam with both orbital and spin angular momentums is numerically investigated. Distinguished spectra are observed under the different momentums. The circular dichroism under the combination of vortex beam and light spin is enhanced. This phenomenon is attributed to the partial spatial excitation of the nanoparticle, and the strong dichroism is simultaneously caused because of the interaction of the induced electric and magnetic modes and other higher-order modes caused by the partial excitation of the vortex beam. This research provides further insight into chiral light-matter interactions and the dichroism of light with orbital angular momentum.

physics.optics↗

arXiv2019

Stochastic and Simulation-based Models for Setting Flow Rates in Collaborative Trajectory Options Program (CTOP)

As a new tool in the NextGen portfolio, the Collaborative Trajectory Options Programs (CTOP) combines multiple features from its forerunners including Ground Delay Program (GDP), Airspace Flow Program (AFP) and reroutes, and can manage multiple Flow Constrained Areas (FCAs) with a single program. A key research question in CTOP is how to set traffic flow rates under traffic demand and airspace capacity uncertainties. In this paper, we first investigate existing CTOP related stochastic optimization models and point out their roles in CTOP flow rate planning, and their advantages and disadvantages in terms of model flexibility, performance, practicality and Collaborative Decision Making (CDM) software compatibility, etc. CTOP FCA rate planning problem has been split into two steps: traffic flow rate optimization given demand estimation, and flow rate adaptation when flight rerouting is considered. Second, we discuss in detail a class of models called FCA-PCA (Potentially Constrained Area) models, which are extended from GDP models to solve the first step of the problem, and were considered promising as they are designed to be consistent with current CTOP software implementation. We will reveal one inherent shortcoming suffered by FCA-PCA models and show that how this deficiency can be addressed by the PCA model family. We will talk about the problems that prevent stochastic programming being optimal in the second step of the problem. Third, we discuss the applicability of simulation-based optimization, combine it with stochastic programming based heuristics and test the resulting new model on a realistic use case. The results are very encouraging. The models and discussions in this work are not only useful in more effectively implementing and analyzing CTOP programs, but are also valuable for the design of future air traffic flow program.

math.OC↗

arXiv2019

A Strong Formulation for Stochastic Multiple Constrained Resources Air Traffic Flow Management with Reroutes

This paper addresses the air traffic flow management research problem of determining reroute, ground delay and air delay for flights using stochastic weather forecast information. The overall goal is to minimize system-wide reroute and delay costs. This problem is a primary concern in United States and especially in its northeastern region, and is also the key in enhancing the performance of the new FAA Traffic Management Initiative called Collaborative Trajectory Options Program (CTOP). In this work we present six stochastic integer programming models, including two two-stage models and four multistage models, which are based on a notable strong deterministic flight-by-flight level traffic flow formulation and an aggregate Eulerian traffic flow formulation. Our preliminary numerical results show that completely integer solutions can be achieved from linear relaxation, for all proposed models and for both no-route and reroute cases.

math.OC↗

arXiv2014

Tunable charge-trap memory based on few-layer MoS2

Charge-trap memory with high-\k dielectric materials is considered to be a promising candidate for next-generation memory devices. Ultrathin layered two-dimensional (2D) materials like graphene and MoS2 have been receiving much attention because of their novel physical properties and potential applications in electronic devices. Here, we report on a dual-gate charge-trap memory device composed of a few-layer MoS2 channel and a three-dimensional (3D) Al2O3/HfO2/Al2O3 charge-trap gate stack. Owing to the extraordinary trapping ability of both electrons and holes in HfO2, the MoS2 memory device exhibits an unprecedented memory window exceeding 20 V. More importantly, with a back gate the window size can be effectively tuned from 15.6 to 21 V; the program/erase current ratio can reach up to 104, far beyond Si-based flash memory, which allows for multi-bit information storage. Furthermore, the device shows a high mobility of 170 cm2V-1s-1, a good endurance of hundreds of cycles and a stable retention of ~28% charge loss after 10 years which is drastically lower than ever reported MoS2 flash memory. The combination of 2D materials with traditional high-\k charge-trap gate stacks opens up an exciting field of novel nonvolatile memory devices.

cond-mat.mtrl-sci↗