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Gusthavo M. S. Brizolla

Publications and source records attributed to Gusthavo M. S. Brizolla.

3 recordsLinked to original sources

Anatomy of Spin--Orbit Torques in Monolayer Fe$_3$GeTe$_2$ and Fe$_3$GaTe$_2$: Insights from atomistic and momentum-space decompositions

We present a systematic first-principles study of the spin-orbit torques in the ferromagnetic monolayers Fe$_3$GeTe$_2$ (FGT) and Fe$_3$GaTe$_2$ (FGaT). Despite sharing the same crystal structure (point group $D_{3h}$) and predominantly Fe~$3d$ spin-polarized bands, the two materials exhibit markedly different current-induced torques. We reveal these differences by computing the full angular dependence of the torkance---the torque per unit applied electric field---using linear-response theory with symmetry-adapted spin--orbit-coupled Wannier functions. FGaT may be viewed as a hole-doped analogue of FGT, since Ga contributes one valence electron fewer than Ge. Although the work functions differ by only about $28$~meV, the band filling near $K$ and $K'$ changes substantially: the density of states at $\varepsilon_F$ is reduced by a factor of three and its spin polarization reverses from minority in FGT to majority in FGaT. These electronic changes are reflected in the torques resolved by time-reversal parity, sublattice, and momentum. In particular, we identify pronounced hidden torques in FGaT and relate the suppression of its fourth-harmonic Fermi-sea component to the evolution of momentum-space pockets. Finally, we discuss the emergence of such self-torques, which are not captured by the conventional picture of current-induced spin accumulation, within a symmetry-based phenomenological framework. Our results provide microscopic insight into current-induced torques in two-dimensional ferromagnets and offer guidance for defect and van der Waals engineering of layered magnetic materials.

cond-mat.mtrl-sci↗

Electric-current control of anomalous Hall effect

We demonstrate robust and reversible electric-current control of the anomalous Hall effect (AHE) in a two-dimensional WTe2/Fe3GeTe2 (FGT) stack. Applying a current through Td-WTe2 leads to a giant modulation of the AHE of the adjacent FGT layer, with the relative change of the AHE conductivity exceeding 180%. Control experiments show that i) the observed effect is absent in pure FGT, ii) the modulation weakens in thicker FGT films, confirming its interfacial origin, and iii) the modulation peaks for bilayer WTe2, indicating that the Berry-curvature dipole (BCD) plays the dominant role in the modulation. We propose that the charge current I generates an out-of-plane magnetization Mz via BCD in WTe2 and Mz modifies the exchange splitting of FGT via the inverse magnetic proximity effect, thereby altering its Berry curvature and nontrivially influencing the AHE. The demonstrated method of AHE control offers new possibilities for magnetism control, i.e., for the study of AHE-transistors as well as electric-current control of quantum magnets, especially magnetic insulators.

cond-mat.mes-hall↗

Ferroelectric-controllable spin-orbit torque in two-dimensional multiferroic heterostructure

Spin-orbit torque (SOT), which enables electrical control of magnetization, plays a crucial role in the development of next-generation spintronic devices. Realizing SOT in two-dimensional van der Waals systems, together with achieving efficient nonvolatile manipulation via ferroelectricity, would be highly beneficial for the implementation of tunable logic devices with enhanced storage density. In this work, based on first-principles calculation and using a multiferroic Fe$_{3}$GeTe$_{2}$/In$_{2}$Se$_{3}$ heterostructure as a representative example, we demonstrate that switching the ferroelectric polarization of the In$_{2}$Se$_{3}$ layer induces a pronounced modification in the magnetization-dependent distribution of torkance within the heterostructure. Specifically, when the magnetization is in the plane, where the torque is maximal, reversing the polarization of In$_{2}$Se$_{3}$ from upward to downward enhances the total torkance to more than 150% of its original value. This substantial variation primarily originates from the polarization-induced modulation of the $z$ component of the time-reversal-odd torkance, which is mainly associated with an approximately 233% change in the atomic-resolved torque contributed from the middle Fe layer in Fe$_{3}$GeTe$_{2}$ layer. Further analysis reveals that the electronic states near $Γ$ on the Fermi surface undergo significant reconstruction upon polarization switching, which is responsible for the observed variation in the time-reversal-odd torque. Our results not only provide new insights into the functional potential of van der Waals multiferroic heterostructures, but also offer a viable strategy for achieving electrically tunable SOT, paving the way for future programmable spintronic devices.

cond-mat.mes-hall↗