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Guzhi Bao

Publications and source records attributed to Guzhi Bao.

14 recordsLinked to original sources

Quantum-Enhanced Atomic Sensor via Spin Nonequilibrium Criticality

The sensitivity of quantum sensors is fundamentally constrained by the standard quantum limit (SQL) arising from intrinsic quantum fluctuations. While non-classical resources like squeezing or entanglement can surpass this limit, their utility is often restricted by the extreme fragility of entangled states and the complexity of their preparation. Quantum criticality offers a compelling alternative by harnessing divergent susceptibility to amplify signals without requiring fragile non-classical resources. However, the practical benefit of this approach has remained controversial due to the potential for the simultaneous amplification of quantum noise. Here, we demonstrate a universal protocol for noiseless critical sensing by engineering a light-driven atomic ensemble near a dynamical critical point. Analogous to a Kapitza pendulum near its inverted orientation, the spin system enters a non-equilibrium regime where the signal susceptibility diverges while the quantum noise periodically recedes to its coherent baseline. We exploit this ``noise ebbing'' to create a built-in noiseless amplifier, demonstrating a 3.3 dB metrological gain over the SQL in an atomic magnetometer. Our implementation exhibits intrinsic robustness against common experimental imperfections such as detection losses, establishing non-equilibrium critical dynamics as a practical and versatile paradigm for surpassing the fundamental limits of quantum sensing.

quant-ph

Quantum-elevated Chiral Discrimination for Bio-molecules

Chiral discrimination of enantiomeric biomolecules is vital in chemistry, biology, and medicine. Conventional methods, relying on circularly polarized light, face weak chiroptical signals and potential photodamage. Despite extensive efforts to improve sensitivity under low-photon exposure, classical chiral probes remain fundamentally bounded by the shot-noise limit due to quantum fluctuations. To beat these limitations, we demonstrate quantum-elevated chiral discrimination using continuous-variable polarization-entangled states as moderate-photon-flux, high-sensitivity, quantum-noise-squeezed chiral probes. We achieve a 5 dB improvement beyond the SNL in distinguishing L- and D-amino acids in liquid phase. This non-destructive, biocompatible protocol enables high-sensitivity chiral analysis, with broad implications for drug development, biochemical research, environmental monitoring, and asymmetric synthesis.

quant-ph

Quantum Metrology with Higher-order Exceptional Points in Atom-cavity Magnonics

Exceptional points (EPs), which arose early from non-Hermitian physics, significantly amplify the system's response to minor perturbations, and they act as a useful concept to enhance measurement in metrology. In particular, such a metrological enhancement grows dramatically with the EP's order. However, the Langevin noises intrinsically existing in the non-Hermitian systems diminish this enhancement. In this study, we propose a protocol for quantum metrology with the construction of higher-order EPs (HOEPs) in an atom-cavity system through Hermitian magnon-photon interaction. The construction of HOEPs utilizes the atom-cavity non-Hermitian-like dynamical behavior but avoids the external Langevin noises via the Hermitian interaction. A general analysis is exhibited for the construction of arbitrary -order EP (EPn). As a demonstration of the superiority of these HOEPs in quantum metrology, we work out an EP3/4-based atomic sensor with sensitivity being orders of magnitude higher than that achievable in an EP2-based atomic sensor. We further unveil the mechanism behind the sensitivity enhancement from HOEPs. The experimental establishment for this proposal is suggested with potential candidates. This EP-based atomic sensor, taking advantage of the atom-light interface, offers new insight into quantum metrology with HOEPs.

quant-ph

Frequency Range Boosted Magnetometry Beyond the Spin Coherence Limit via Compressive Sensing

Free induction decay (FID) of spin precession serves as an essential tool for quantum sensing across diverse platforms. While extending spin coherence time remains critical for sensitivity enhancement, the requisite long single-shot acquisitions narrow the resolvable frequency range, establishing a fundamental ``spin coherence limit (SCL)'', according to the Nyquist Sampling Theorem. Besides, conventional spectral analysis for FID measurement suffers from frequency alias, causing signal attenuation and positional errors that compromise the measurement validity. Here, we demonstrate a general frequency-range-extended technique that overcomes SCL by leveraging compressive sensing. By applying this method to the FID magnetometer, we expand the resolvable frequency range significantly from the Nyquist-limited range of 251\,Hz to 3000\,Hz, effectively avoiding frequency alias. Our work paves the way for implementing long-coherence-time spin systems in high-sensitivity, broad-bandwidth, and alias-free magnetic field sensing.

physics.atom-ph

Near-perfect broadband quantum memory enabled by intelligent spinwave compaction

Quantum memory, a pivotal hub in quantum information processing, is expected to achieve high-performance storage and coherent manipulation of quantum states, with memory efficiency exceeding 90% and quantum fidelity surpassing the non-cloning limit. However, the current performance falls short of these requirements due to the inherent trade-off between memory efficiency enhancement and noise amplification, which not only imposes significant demands on quantum purification but also fundamentally impedes continuous-variable quantum information processing. In this paper, we break through these constraints, enabling high-performance quantum memory and unlocking new possibilities for quantum technologies. We unveil a Hankel-transform spatiotemporal mapping for light-spinwave conversion in quantum memory, and propose an intelligent light-manipulated strategy for adaptive spinwave compaction, which can maximize the conversion efficiency and simultaneously suppress the excess noise. This strategy is experimentally demonstrated for a Raman quantum memory in warm 87Rb atomic vapor with an efficiency up to 94.6% and a low noise level of only 0.026 photons/pulse. The unconditional fidelity reaches 98.91% with an average of 1.0 photons/pulse for a 17-ns input signal. Our results successfully demonstrate a practical benchmark for broadband quantum memory, which may facilitate advancements in high-speed quantum networks, quantum state manipulation, and scalable quantum computation.

quant-ph

Quantum Twin Interferometers

Quantum-correlated interferometer is a newly emerging tool in quantum technology that offers classical-limit-breaking phase sensitivity. But to date, there exists a configurational bottleneck for its practicability due to the low phase-sensitive photon numbers limited by the current detection strategies. Here we establish an innovative development termed as ``quantum twin interferometer'' with dual pairs of entangled twin beams arranged in the parallel configuration, allowing fully exploits the quantum resource through the new configuration of entangled detection. We observe the distributed phase sensing with 3 dB quantum noise reduction in phase-sensing power at the level of milliwatts, which advances the record of signal-to-noise ratio so far achieved in photon-correlated interferometers by three orders of magnitude. The developed techniques in this work can be used to revolutionize a diversity of quantum devices requiring phase measurement.

physics.atom-ph

Quantum Locking of Intrinsic Spin Squeezed State in Earth-field-range Magnetometry

In the Earth-field range, the nonlinear Zeeman (NLZ) effect has been a bottleneck limiting the sensitivity and accuracy of atomic magnetometry from physical mechanism. To break this bottleneck, various techniques are introduced to suppress the NLZ effect. Here we revisit the spin dynamics in the Earth-field-range magnetometry and identify the existence of the intrinsic spin squeezed state (SSS) generated from the geomagnetically induced NLZ effect with the oscillating squeezing degree and squeezing axis. Such oscillating features of the SSS prevent its direct observation and as well, accessibility to magnetic sensing. To exploit quantum advantage of the intrinsic SSS in the Earth-field-range magnetometry, it's essential to lock the oscillating SSS to a persistent one. Hence, we develop a quantum locking technique to achieve a persistent SSS, benefiting from which the sensitivity of the Earth-field-range magnetometer is quantum-enhanced. This work presents an innovative way turning the drawback of NLZ effect into the quantum advantage and opens a new access to quantum-enhanced magnetometry in the Earth-field range.

physics.atom-ph

Quantum-enhanced Electrometer based on Microwave-dressed Rydberg Atoms

Rydberg atoms have been shown remarkable performance in sensing microwave field. The sensitivity of such an electrometer based on optical readout of atomic ensemble has been demonstrated to approach the photon-shot-noise limit. However, the sensitivity can not be promoted infinitely by increasing the power of probe light due to the increased collision rates and power broadening. Compared with classical light, the use of quantum light may lead to a better sensitivity with lower number of photons. In this paper, we exploit entanglement in a microwave-dressed Rydberg electrometer to suppress the fluctuation of noise. The results show a sensitivity enhancement beating the shot noise limit in both cold and hot atom schemes. Through optimizing the transmission of optical readout, our quantum advantage can be maintained with different absorptive index of atomic vapor, which makes it possible to apply quantum light source in the absorptive electrometer.

quant-ph

Sensing performance enhancement via asymmetric gain optimization in the atom-light hybrid interferometer

The SU (1,1)-type atom-light hybrid interferometer (SALHI) is a kind of interferometer that is sensitive to both the optical phase and atomic phase. However, the loss has been an unavoidable problem in practical applications and greatly limits the use of interferometers. Visibility is an important parameter to evaluate the sensing performance of interferometers. Here, we experimentally demonstrate the mitigating effect of the loss on visibility of the SALHI via asymmetric gain optimization, where the maximum threshold of loss to visibility close to $100\%$ is increased. Furthermore, we theoretically find that the optimal condition for the largest visibility is the same as that for the enhancement of signal-to-noise ratio (SNR) to the best value in the presence of losses using the intensity detection, indicating that the visibility can act as an experimental operational criterion for SNR improvement in practical applications. Improvement of the interference visibility means achievement of SNR enhancement. Our results provide a significant foundation for practical application of the SALHI in radar and ranging measurements.

quant-ph

Coherence Protection of Electron Spin in Earth-field Range by All-optical Dynamic Decoupling

In recent years, unshielded atomic systems have been attracting researchers' attention, in which decoherence is one of the major problems, especially for high precision measurements. The nonlinear Zeeman effect and magnetic field gradient are the main decoherence sources of atomic electron spin in Earth-field range. Here, we propose a method to cancel out the two dominant broadening effects simultaneously by an all-optical dynamic decoupling approach based on Raman scattering in the 87Rb Zeeman sublevels. By adjusting the parameters of the Raman lasers, we realize spin control along an arbitrary direction. We analyze the state evolution of atomic spin under the Raman light control sequence in detail. The results show that both the nonlinear Zeeman effect and magnetic field gradient can be significantly suppressed.

physics.atom-ph

Evidence for degenerate mirrorless lasing in alkali metal vapor: forward beam magneto-optical experiment

We report an experimental observation of degenerate mirrorless lasing in forward direction under excitation of a dilute atomic Rb vapor with a single linearly polarized cw laser light resonant with cycling Fe > Fg atomic D2 transitions. Light polarized orthogonally to the laser light is generated for the input light intensity exceeding a threshold value of about 3 mW/cm^2. Application of a transverse magnetic field directed along the input light polarization reveals a sharp about 20 mG wide magnetic resonance centered at B = 0. Increasing the incident light intensity from 3 to 300 mW/cm^2, the generated light undergoes rapid amplitude increase followed by a decline and resonance broadening. Such nonlinear behavior of the observed magnetic resonance is attributed to the population inversion on optical transitions between magnetic sublevels established under linearly polarized excitation. We present observations that indicate that a combination of nonlinear-optical effects occurs in this system, including degenerate mirrorless lasing and four-wave mixing.

physics.atom-ph

All-Optical Spin Locking in Alkali-Vapor Magnetometers

The nonlinear Zeeman effect can induce splittings and asymmetries of magnetic-resonance lines in the geophysical magnetic-field range. We demonstrate a scheme to suppress the nonlinear Zeeman effect all optically based on spin locking. Spin locking is achieved with an effective oscillating magnetic field provided by the AC Stark-shift of an intensity-modulated and polarization-modulated laser beam. This results in the collapse of the multi-component asymmetric magnetic-resonance line with about 100 Hz width in the Earth-field range into a peak with a central component width of 25Hz. The technique is expected to be broadly applicable in practical magnetometry, potentially boosting the sensitivity and accuracy of Earth-surveying magnetometers by increasing the magnetic-resonance amplitude and decreasing its width. Advantage of an all-optical approach is the absence of cross-talk between nearby sensors when these are used in a gradiometric or in an array arrangement.

physics.atom-ph

Suppression of nonlinear Zeeman effect and heading error in earth-field-range alkali-vapor magnetometers

The nonlinear Zeeman effect can induce splitting and asymmetries of magnetic-resonance lines in the geophysical magnetic field range. This is a major source of "heading error" for scalar atomic magnetometers. We demonstrate a method to suppress the nonlinear Zeeman effect and heading error based on spin locking. In an all-optical synchronously pumped magnetometer with separate pump and probe beams, we apply a radio-frequency field which is in-phase with the precessing magnetization. In an earth-range field, a multi-component asymmetric magnetic-resonance line with ? 60 Hz width collapses into a single peak with a width of 22 Hz, whose position is largely independent of the orientation of the sensor. The technique is expected to be broadly applicable in practical magnetometry, potentially boosting the sensitivity and accuracy of earth-surveying magnetometers by increasing the magnetic resonance amplitude, decreasing its width and removing the important and limiting heading-error systematic.

physics.atom-ph

A compact 3.5-dB squeezed light source with atomic ensembles

We reported a compact squeezed light source consisting of an diode laser near resonant on 87Rb optical D1 transition and an warm Rubidium vapor cell. The -4dB vacuum squeezing at 795 nm via nonlinear magneto-optical rotation was observed when applying the magnetic field orthogonal to the propagation direction of the light beam. This compact squeezed light source can be potentially utilized in the quantum information protocols such as quantum repeater and memory, and quantum metrology such as atomic magnetometer.

quant-ph