arXiv subjects

Gwynn J. Elfring

Publications and source records attributed to Gwynn J. Elfring.

At least 19 recordsLinked to original sources

arXiv2026

Dissipation and microstructure in sheared active suspensions of squirmers

We study the energy expenditure and structural correlations in semi-dilute to concentrated suspensions of squirmers using active fast Stokesian dynamics simulations. Specifically, we simulate apolar active suspensions of squirmers, or 'shakers,' and show that shear enhances the total dissipation but reduces the relative viscosity for both puller- and pusher-type shakers. At low shear rates where activity dominates, pushers dissipate more energy than pullers, and more so at higher volume fractions, in contrast to bacterial suspensions displaying a 'superfluid' transition. At high shear rates where shear dominates, pullers and pushers behave effectively as passive spheres, generating negative normal stress differences due to shear-induced collision. Remarkably, the rate-dependent rheological responses are accompanied by unusual microstructural signatures of an enhanced nematic order and anisotropic pair correlation, both of which contribute to a higher viscosity under shear. Further simulations of self-propelled, neutral squirmers exhibit similar but weaker shear-thinning, highlighting the importance of activity over motility, underpinned by hydrodynamic interactions. Overall, our results elucidate the interplay of internal activity and external flow on the dissipation and microstructure in sheared active suspensions of squirmers.

cond-mat.soft↗

arXiv2025

Nonmonotonic diffusion in sheared active suspensions of squirmers

We investigate how shear influences the dynamics of active particles in dilute to concentrated suspensions. Using apolar active suspensions of squirmers as model systems, we show how their long-time diffusive dynamics can surprisingly slow down and vary nonmonotonically with the shear rate arising from an interplay between the activity-induced persistent motion and shear-induced reorientation and diffusion. Further simulations of self-propelled particles with tunable persistence exhibit richer dynamics and confirm the observed coupling, suggesting that nonmonotonic diffusion may be a general feature of fluids endowed with an underlying microstructure and large persistence. Our results reveal a nonlinear effect of shear on diffusion in active suspensions, elucidate how internal and external forcing interact, and provide new possibilities to modulate transport in active fluids.

cond-mat.soft↗

arXiv2025

Mixing by squirmers in stratified fluids

We find the mixing induced by a small swimming organism in a density stratified fluid. We model the swimmer as a spherical squirmer and quantify mixing through a mixing efficiency that is the ratio of rate of change of potential energy of fluid to the total work done by the swimmer. Assessing mixing in the near field and far field of the swimmer separately, we find that the near-field mixing aligns with past work, but the overall mixing is much larger than that caused by a point-sized swimmer (like force-dipole), although still small in weak stratification. Equivalent results are also obtained for a homogeneous dilute suspension of non-interacting swimmers. Our study highlights the impact of swimmer size on mixing, revealing that small-sized swimmers cannot induce substantial mixing. However, we propose few (unexplored) pathways through which small swimmers could induce significant mixing, ultimately contributing towards oceanic mixing.

cond-mat.soft↗

arXiv2024

Durotaxis in viscoelastic fluids

Organisms often swim through fluids that are spatially inhomogeneous. If the fluids are polymeric, gradients in polymer concentration may lead to gradients in both fluid viscosity and elasticity. In this letter, we present theoretical results for the dynamics of active particles, biological or otherwise, swimming through spatially inhomogeneous viscoelastic fluids. We model the active particles using the squirmer model, and show that spatial variations in fluid relaxation time lead to a novel mechanism for reorientation and taxis in viscoelastic fluids, which we refer to as a form of durotaxis in fluids.

physics.flu-dyn↗

arXiv2024

Equilibrium states of a liquid bridge between flexible sheets

We study equilibrium states of a drop between flexible sheets clamped on both ends. Revisiting first the case of parallel sheets, we find multiple equilibria which we classify in a parameter space. In solution branching diagrams we identify hysteresis cycles and folds indicating abrupt transitions, yet not necessarily leading to channel collapse. Between nonparallel sheets, a drop can stay in equilibrium away from the ends even when the liquid is totally wetting, which is impossible between nonparallel rigid plates. We also show that nonparallel sheets can delay or prevent collapse in comparison to straight channels, suggesting thus a mechanism that protects slender structures inside micro-devices from damage by surface tension.

cond-mat.soft↗

arXiv2024

Hydrodynamic diffusion in apolar active suspensions

Active suspensions encompass a wide range of complex fluids containing microscale energy-injecting particles, such as cells, bacteria or artificially powered active colloids. Because they are intrinsically non-equilibrium, active suspensions can display a number of fascinating phenomena, including turbulent-like large-scale coherent motion and enhanced diffusion. Here, using a recently developed active Fast Stokesian Dynamics method, we present a detailed numerical study on the hydrodynamic diffusion in apolar active suspensions. Specifically, we simulate suspensions of active but non-self-propelling spherical squirmers, of either puller- or pusher-type, at volume fractions from 0.5% to 55%. Our results show little difference between pullers and pushers in their instantaneous and long-time dynamics, where the translational dynamics vary non-monotonically with the volume fraction, with a peak diffusivity at around 10% to 20%, in stark contrast to suspensions of self-propelling particles. On the other hand, the rotational dynamics tend to increase with the volume fraction as is the case for self-propelling particles. To explain these dynamics, we provide detailed scaling and statistical analyses based on the activity-induced hydrodynamic interactions and the observed microstructural correlations, which display a weak local order. Overall, these results elucidate and highlight the different effects of particle activity on the collective dynamics and transport phenomena in active fluids.

cond-mat.soft↗

arXiv2024

Adaptive design of experiments methodology for noise resistance with unreplicated experiments

A new gradient-based adaptive sampling method is proposed for design of experiments applications which balances space filling, local refinement, and error minimization objectives while reducing reliance on delicate tuning parameters. High order local maximum entropy approximants are used for metamodelling, which take advantage of boundary-corrected kernel density estimation to increase accuracy and robustness on highly clumped datasets, as well as conferring the resulting metamodel with some robustness against data noise in the common case of unreplicated experiments. Two-dimensional test cases are analyzed against full factorial and latin hypercube designs and compare favourably. The proposed method is then applied in a unique manner to the problem of adaptive spatial resolution in time-varying non-linear functions, opening up the possibility to adapt the method to solve partial differential equations.

stat.ME↗

arXiv2024

Swimming efficiency in viscosity gradients

In this note, we study the effect of viscosity gradients on the energy dissipated by the motion of microswimmers and the associated efficiency of that motion. Using spheroidal squirmer model swimmers in weak linearly varying viscosity fields, we find that efficiency depends on whether they generate propulsion from the back (pushers) or the front (pullers). Pushers are faster and more efficient when moving down gradients but slower and less efficient moving up viscosity gradients, and the opposite is true for pullers. However, both pushers and pullers display negative viscotaxis, therefore pushers dynamically tend to the most efficient orientation while pullers the least. We also evaluate the effect of shape on power expenditure and efficiency when swimming in viscosity gradients and find that in general the change in both due to gradients monotonically decreases with increasing slenderness. This work shows how shape and gait play an important role in determining dynamics and efficiency in inhomogeneous environments, and demonstrating that both efficiency minimizing and maximizing stable dynamical states are possible.

physics.flu-dyn↗

arXiv2023

Active spheroids in viscosity gradients

In this paper, we explore the hydrodynamics of spheroidal active particles in viscosity gradients. This work provides a more accurate modeling approach, in comparison to spherical particles, for anisotropic organisms like Paramecium swimming through inhomogeneous environments, but more fundamentally examines the influence of particle shape on viscotaxis. We find that spheroidal squirmers generally exhibit dynamics consistent with their spherical analogs, irrespective of the classification of swimmers as pushers, pullers, or neutral swimmers. However, the slenderness of the spheroids tends to reduce the impact of viscosity gradients on their dynamics; when swimmers become more slender, the viscosity difference across their body is reduced, which leads to slower reorientation. We also derive the mobility tensor for passive spheroids in viscosity gradients generalizing previous results for spheres and slender bodies. This work enhances our understanding of how shape factors into the dynamics of passive and active particles in viscosity gradients, and offers new perspectives that could aid the control of both natural and synthetic swimmers in complex fluid environments.

physics.flu-dyn↗

arXiv2023

Capillary imbibition in a diverging flexible channel

We study the imbibition of a wetting liquid between flexible sheets that are fixed on both ends. Assuming a narrow gap between the sheets, we solve the lubrication equation coupled with slender body deformation. When the sheets are parallel, we find that the deformation initially speeds up the flow, as shown in previous studies, but only up to the middle of the channel. As the channel contracts, the hydrodynamic resistance increases and ultimately slows down the filling process. Below a threshold stiffness, the channel collapses and imbibition stops. We propose a scaling of the filling duration near this threshold. Next we show that if the sheets are initially tilted with a minimal angle, the channel avoids collapse. The liquid front pulls the diverging sheets and spreads in a nearly parallel portion, which maintains the capillary propulsion and enhances the wicking. Therefore, while it is established that diverging rigid plates imbibe liquids slower than parallel ones, we show that elasticity reverses this principle: diverging flexible sheets imbibe liquids faster than parallel ones. We find an optimal tilt angle that gives the shortest filling time.

physics.flu-dyn↗

arXiv2023

Densitaxis: Active particle motion in density gradients

Organisms often swim through density stratified fluids. In this Letter, we investigate the dynamics of small active particles swimming in density gradients and report theoretical evidence of taxis as a result of density stratification ($\textit{densitaxis}$). Specifically, we calculate the effect of density stratification on the dynamics of a force-free spherical squirmer and show that density stratification induces reorientation that tends to align swimming either parallel or normal to the gradient depending on the swimming gait. In particular, particles that propel by generating thrust in the front (pullers) rotate to swim parallel to gradients and hence display (positive or negative) densitaxis, while particles that propel by generating thrust in the back (pushers) rotate to swim normal to the gradients. This work could be useful to understand the motion of marine organisms in ocean, or be leveraged to sort or organize a suspension of active particles by modulating density gradients.

cond-mat.soft↗

arXiv2023

Energetics of Cytoskeletal Gel Contraction

Cytoskeletal gels are prototyped to reproduce the mechanical contraction of the cytoskeleton in-vitro. They are composed of a polymer network (backbone), swollen by the presence of a liquid solvent, and active molecules (molecular motors, MMs) that transduce chemical energy into the mechanical work of contraction. These motors attach to the polymer chains to shorten them and/or act as dynamic crosslinks, thereby constraining the thermal fluctuation of the chains. We describe both mechanisms thermodynamically as a microstructural reconfiguration, where the backbone stiffens to motivate solvent (out)flow and accommodate contraction. Via simple steady-state energetic analysis, under the simplest case of isotropic contraction, we quantify the mechanical energy required to achieve contraction as a function of polymer chain density and molecular motor density. We identify two limit cases, (fm) fast MM activation for which MMs provide all the available mechanical energy instantaneously and leave the polymer in a stiffened state, i.e. their activity occurs at a time scale that is much smaller than solvent diffusion, and (sm) slow MM activation for which the MM activation timescale is much longer. To achieve the same final contracted state, fm requires the largest amount of work per unit reference volume, while sm requires the least. For all intermediate cases where the timescale of MM activation is comparable with that of solvent flow, the required work ranges between the two cases. We provide all these quantities as a function of chain density and MM density. Finally, we compare our results with experiments and observe good agreement.

cond-mat.soft↗

arXiv2022

Rheology of periodically sheared suspensions undergoing reversible-irreversible transition

The rheology of non-colloidal suspensions under cyclic shear is studied numerically. The main findings are a strain amplitude ($γ_0$) dependent response in the shear stress and second normal stress difference ($N_2$). Specifically, we find a reduced viscosity, an enhanced intracycle shear thinning, the onset of a finite $N_2$ and its frequency doubling, all near a critical strain amplitude $γ_c$ that scales with the volume fraction $ϕ$ as $γ_c \sim ϕ^{-2}$. These rheological changes also signify a reversible-irreversible transition (RIT), dividing stroboscopic particle dynamics into a reversible absorbing phase (for $γ_0<γ_c$) and a persistently diffusing phase (for $γ_0>γ_c$). We explain the results based on two flow-induced mechanisms and elucidate their connection in the context of RIT through the underlying microstructure, which tends towards hyperuniformity near $γ_0=γ_c$. Overall, we expect this correspondence between rheology and emergent dynamics to hold in a wide range of settings where structural organizations are dominated by volume exclusions.

cond-mat.soft↗

arXiv2022

Statistics and spectral analysis of turbulent duct flows with flexible and rigid polymer solutions

We present an experimental investigation of turbulent drag reduction with flexible and rigid polymer solutions. The flexible polymer is partially hydrolyzed polyacrylamide (HPAM) and the rigid polymer is xanthan gum (XG). The experiments are carried out at low drag reduction ($\%DR < 40$), high drag reduction ($\%DR > 40$) and maximum drag reduction (where the velocity profile $U^+$ roughly matches Virk's asymptote). We compare velocity profiles, streamwise and wall-normal Reynolds stresses and power spectra of streamwise velocity fluctuations measured by Laser Doppler Anemometry (LDA). Our results show that the effects of both XG and HPAM polymers on turbulence are similar, provided that the Reynolds numbers and $\%DR$ are also similar. At high levels of $\%DR$, the power spectral densities of streamwise velocity fluctuations of both XG and HPAM flows show a power-law decay near $-3$ instead of $-5/3$ in the inertial range. A slope of the power spectra of $-3$ was recently interpreted as evidence of elasto-inertial turbulence (EIT) in polymer jets. At relatively low concentrations, we observe that flexible polymer solutions are more effective at reducing drag, while XG only reaches MDR at very high concentrations. Thus, we hypothesize that the formation of polymer aggregates with higher concentrations contributes to increase viscoelasticity, and thus $\%DR$, with XG and other rigid polymer solutions.

physics.flu-dyn↗

arXiv2022

Confined active matter in external fields

We analyze a dilute suspension of active particles confined between walls and subjected to fields that can modulate particle speed as well as orientation. Generally, the particle distribution is different in the bulk compared to near the walls. In the bulk, particles tend to accumulate in the regions of low speed, but in the presence of an orienting field, particles rotate to align with the field and accumulate downstream in the field direction. At the walls, particles tend to accumulate pointing into the walls and thereby exert pressure on walls. But the presence of strong orienting fields can cause the particles to reorient away from the walls, and hence shows a possible mechanism for preventing contamination of surfaces. The pressure at the walls depends on the wall separation and the field strengths. This work demonstrates how multiple fields with different functionalities can be used to control active matter under confinement.

cond-mat.soft↗

arXiv2022

Active particles crossing sharp viscosity gradients

Active particles (living or synthetic) often move through inhomogeneous environments, such as gradients in light, heat or nutrient concentration, that can lead to directed motion (or taxis). Recent research has explored inhomogeneity in the rheological properties of a suspending fluid, in particular viscosity, as a mechanical (rather than biological) mechanism for taxis. Theoretical and experimental studies have shown that gradients in viscosity can lead to reorientation due to asymmetric viscous forces. In particular, recent experiments with Chlamydomonas reinhardtii algae swimming across sharp viscosity gradients have observed that the microorganisms are redirected and scattered due to the viscosity change. Here we develop a simple theoretical model to explain these experiments. We model the swimmers as spherical squirmers and focus on small, but sharp, viscosity changes. We derive a law, analogous to Snell's law of refraction, that governs the orientation of active particles in the presence of a viscosity interface. Theoretical predictions show good agreement with experiments and provide a mechanistic understanding of the observed reorientation process.

cond-mat.soft↗

arXiv2022

Fully turbulent flows of viscoplastic fluids in a rectangular duct

Turbulent flows of viscoplastic fluids at high Reynolds numbers have been investigated recently with direct numerical simulations (DNS) but experimental results have been limited. For this reason, we carry out an experimental study of fully turbulent flows of a yield stress fluid in a rectangular aspect ratio channel with a high-resolution laser doppler velocimetry (LDA) setup. We employ aqueous Carbopol solutions, often considered to be a simple yield stress fluid. We formulate different concentrations to address the effect of the rheology of the fluid on the turbulence statistics at an approximately constant Reynolds number. Additionally, we also perform experiments with a single Carbopol formulation at different Reynolds numbers to study its effect. The flow analysis is performed via rheology measurements, turbulence statistics and power spectral densities of velocity fluctuations. The addition of Carbopol to the flow increases turbulence anisotropy, with an enhancement of streamwise velocity fluctuations and a decrease in wall normal velocity fluctuations in comparison to water at the same mean velocity. This change is reflected on the power spectral densities of streamwise velocity fluctuations, where we observe a large increase in energy of large scale turbulent structures. Conversely, the energy of smaller scales is decreased in comparison to water, where the energy drops with a steeper scale than the Newtonian power law of $k_x^{-5/3}$. As we increase the Reynolds number with a Carbopol solution, the streamwise Reynolds stresses approach Newtonian values in the core, which suggests diminishing effects of shear-thinning. The power spectral densities reveal that the energy content at larger scales decreases slightly with the Reynolds number. However, the shear thinning effects do not disappear even as the Reynolds number approaches 50000.

physics.flu-dyn↗

arXiv2021

Turbulent drag reduction of viscoelastic wormlike micellar gels

Long-chained, viscoelastic surfactant solutions (VES) have been widely employed in the oil and gas industry, particularly in hydraulic fracturing and gravel-packing operations, where turbulence is commonly reached due to high pumping rates. With this motivation, we experimentally investigate the turbulent duct flow of an under-studied class of wormlike micellar solutions that forms a gel at room temperature. The fluid is characterized via rotational rheometry, and the turbulent velocity and Reynolds stress profiles are measured via Laser Doppler Anemometry (LDA). Three surfactant concentrations are investigated at increasing Reynolds numbers. The turbulent flow fields of water, and semi-dilute solutions of partially hydrolyzed polyacrylamide (HPAM) and xanthan gum (XG) are used as comparisons. Our study reveals that the gel-like structure of the wormlike micellar gel is mostly broken down during turbulent flow, especially in the near-wall region where the results indicate the presence of a water layer. Turbulent flow at low concentrations of surfactant show a Newtonian-like flow field throughout most of the duct, where the energy spectra shows a -5/3 power law scale with wavenumber, whereas higher concentrations lead to drag reduction and lower power spectral densities at large wavenumbers. A comparison of the flow of polymeric fluids and the wormlike micellar solutions at maximum drag reduction (MDR) shows comparable drag-reduction effects, with a large decrease in Reynolds shear stresses, and increased turbulence anisotropy in the buffer layer due to the large streamwise fluctuations and near-zero wall-normal fluctuations. Additionally, the MDR regime was bounded by Virk's asymptote for both polymers and the micellar gel, which implies a similar mechanism of drag reduction at MDR.

physics.flu-dyn↗