arXiv subjects

H. -Q. Lin

Publications and source records attributed to H. -Q. Lin.

4 recordsLinked to original sources

arXiv2025

Evolution of correlated electronic states of La2NiO4 under hydrostatic pressure

We elucidate the electronic structure and quantum many-body instabilities of the monolayer nickelate La2NiO4 under hydrostatic pressure using a combination of density functional theory, dynamical mean-field theory (DFT+DMFT), and random phase approximation (RPA). Our DFT+DMFT calculations reveal non-Fermi-liquid behavior and coherence loss near the Fermi level at low pressures, driven by strong electron correlations within the Ni-e_g orbital manifold, which is analogous to the low-energy electronic properties observed in La3Ni2O7. However, multi-orbital spin susceptibility analysis demonstrates an exceptionally suppressed critical Stoner parameter U_c (about 0.4~0.7 eV), indicating robust magnetic order that dominates the ground state and precludes superconductivity in the pristine system. Below U_c, superconducting instabilities exhibit a pressure-driven symmetry transition: the d_(x2-y2)-wave pairing prevails at ambient and low pressure, while the s+g-wave symmetry occurs above 75 GPa. This transition is attributed to pressure-induced self-doping effect. The high-angular-momentum g-wave component incurs significant energetic penalties, rendering high-Tc superconductivity unlikely. We conclude that the absence of superconductivity in La2NiO4 arises from its robust intrinsic magnetism and the unfavorable pairing symmetry under pressure, suggesting that alternative routes-such as chemical doping or epitaxial strain-are necessary to suppress magnetism and unlock superconducting states.

cond-mat.str-el↗

arXiv2025

Pressure and doping control of magnetic order and metallization in Ruddlesden-Popper La2NiO4

The discovery of superconductivity in multilayer nickelates under pressure has intensified interest in understanding the magnetic and electronic properties of Ruddlesden-Popper nickelates. Using density functional theory with Hubbard corrections, we investigate the magnetic ground state, electronic structure evolution under pressure, and Sr-doping effects in La$_2$NiO$_4$. We find that at ambient pressure, tetragonal La$_2$NiO$_4$ exhibits G-type antiferromagnetic order with negligible interlayer magnetic coupling. Under hydrostatic pressure, the system undergoes a continuous insulator-metal transition at ~50 GPa while maintaining robust magnetic order up to 75 GPa, contrasting sharply with the rapid magnetic suppression in La$_3$Ni$_2$O$_7$. Sr doping induces a systematic evolution from G-type to A-type, to striped antiferromagnetic orders, and eventually to ferromagnetic order, accompanied by metallization. Furthermore, LaSrNiO$_4$ displays weak charge and orbital orders. These results reveal the unique pressure and doping effects of single-layer nickelates and provide insights into the magnetic mechanisms underlying nickelate superconductivity.

cond-mat.supr-con↗

arXiv2022

Quantum dynamics of Gaudin magnets

Quantum dynamics of many-body systems is a fascinating and significant subject for both theory and experiment. The question of how an isolated many-body system evolves to its steady state after a sudden perturbation or quench still remains challenging. In this paper, using the Bethe ansatz wave function, we study the quantum dynamics of an inhomogeneous Gaudin magnet. We derive explicit analytical expressions for various local dynamic quantities with an arbitrary number of flipped bath spins, such as: the spin distribution function, the spin-spin correlation function, and the Loschmidt echo. We also numerically study the relaxation behavior of these dynamic properties, gaining considerable insight into coherence and entanglement between the central spin and the bath. In particular, we find that the spin-spin correlations relax to their steady value via a nearly logarithmic scaling, whereas the Loschmidt echo shows an exponential relaxation to its steady value. Our results advance the understanding of relaxation dynamics and quantum correlations of long-range interacting models of Gaudin type.

cond-mat.str-el↗

arXiv2014

Orbital density wave order and electronic correlation driven insulating 1T-TaS2 monolayer

We present the orbital resolved electronic properties of structurally distorted 1T-TaS2 monolayers. After optimizing the crystal structures, we obtain the lattice parameters and atomic positions in the star-of-David structure, and show the low-temperature band structures of distorted bulk are consistent with recent angle resolved photoemission spectroscopy (ARPES) data. We further clearly demonstrate that $5d$ electrons of Ta form ordered orbital-density-wave (ODW) state with dominant $5d_{3{z}^2-{r}^2}$ character in central Ta, driving the one-dimensional metallic state in paramagnetic bulk and half-filled insulator in monolayer. Meanwhile, the star-of-David distortion in monolayers favors charge density wave and the flat band stabilizes ferromagnetic density wave of Ta spins with the same wavevector of ODW 4/13 b_1+1/13 b2. We propose that $1$T-TaS$_{2}$ monolayer may pave a new way to study the exciton physics, exciton-polaron coupling, and potential applications for its exciton luminescence.

cond-mat.str-el↗