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H. Ahmadi

Publications and source records attributed to H. Ahmadi.

10 recordsLinked to original sources

Role of intermediate resonances in attosecond photoelectron interferometry in neon

Attosecond photoelectron interferometry based on the combination of an attosecond pulse train and a synchronized infrared field is a fundamental technique for the temporal characterization of attosecond waveforms and for the investigation of electron dynamics in the photoionization process. In this approach, the comb of extreme ultraviolet harmonics typically lies above the ionization threshold of the target under investigation, thus releasing a photoelectron by single-photon absorption. The interaction of the outgoing photoelectron with the infrared pulse results in the absorption or emission of infrared photons, thereby creating additional peaks in the photoelectron spectrum, referred to as sidebands. While, in the absence of resonances in the first ionization step, the phases imparted on the photoionization process evolve smoothly with the photon energy, the presence of intermediate resonances imprints a large additional phase on the outgoing photoelectron wave packet. In this work, using a comb of harmonics below and above the ionization threshold of neon, we investigate the effect of intermediate bound excited states on attosecond photoelectron interferometry. We show that the phase of the oscillations of the sidebands and their angular distributions are strongly affected by such resonances. By slightly tuning the photon energies of the extreme ultraviolet harmonics, we show how the contributions of selected resonances can be enhanced or suppressed.

physics.atom-ph

Joint Network Lifetime Maximization and Relay Selection Design in Underwater Acoustic Sensor Networks

The paper proposes a new approach to minimize the number of relays while maximizing the lifetime of underwater acoustic sensor networks (UASNs). This involves formulating the relay node placement (RNP) problem as a multi-objective optimization problem and employing the multi-objective lexico-graphic method (MOLM) to solve it. To achieve the optimal solution, the MOLM consists of two steps. First, the problem of lifetime maximization is tackled to find RNP solutions. This transforms the RNP into a non-convex optimization problem which is then converted into a convex programming equivalent. The proposed method has the same computational complexity as previous relay-node adjustment (RA) and difference convex algorithm (DCA) methods. The second step introduces a novel relay node selection to reach the optimal number of relays. Simulation results demonstrate that it has superior network lifetime and efficiency compared to RA and DCA.

cs.NI

On the analysis of inexact augmented Lagrangian schemes for misspecified conic convex programs

We consider the misspecified optimization problem of minimizing a convex function $f(x;θ^*)$ in $x$ over a conic constraint set represented by $h(x;θ^*) \in \mathcal{K}$, where $θ^*$ is an unknown (or misspecified) vector of parameters, $\mathcal{K}$ is a closed convex cone and $h$ is affine in $x$. Suppose $θ^*$ is unavailable but may be learnt by a separate process that generates a sequence of estimators $θ_k$, each of which is an increasingly accurate approximation of $θ^*$. We develop a first-order inexact augmented Lagrangian (AL) scheme for computing an optimal solution $x^*$ corresponding to $θ^*$ while simultaneously learning $θ^*$. In particular, we derive rate statements for such schemes when the penalty parameter sequence is either constant or increasing, and derive bounds on the overall complexity in terms of proximal-gradient steps when AL subproblems are inexactly solved via an accelerated proximal-gradient scheme. Numerical results for a portfolio optimization problem with a misspecified covariance matrix suggest that these schemes perform well in practice while naive sequential schemes may perform poorly in comparison.

math.OC

Vectorial optical field reconstruction by attosecond spectral interferometry

An electrical pulse E(t) is completely defined by its time-dependent amplitude and polarisation direction. For optical pulses the manipulation and characterisation of the light polarisation state is fundamental due to its relevance in several scientific and technological fields. In this work we demonstrate the complete temporal reconstruction of the electric field of few-cycle pulses with a complex time-dependent polarisation. Our experimental approach is based on extreme ultraviolet interferometry with isolated attosecond pulses and on the demonstration that the motion of an attosecond electron wave packet is sensitive to perturbing fields only along the direction of its motion. By exploiting the sensitivity of interferometric techniques and by controlling the emission and acceleration direction of the wave packet, pulses with energies as low as few hundreds of nanojoules can be reconstructed. Our approach opens the possibility to completely characterise the electric field of the pulses typically used in visible pump-probe spectroscopy.

physics.optics

Attosecond electronic recollision as field detector

We demonstrate the complete reconstruction of the electric field of visible-infrared pulses with energy as low as a few tens of nanojoules. The technique allows for the reconstruction of the instantaneous electric field vector direction and magnitude, thus giving access to the characterisation of pulses with an arbitrary time-dependent polarisation state. The technique combines extreme ultraviolet interferometry with the generation of isolated attosecond pulses.

physics.optics

Observation and Control of Laser-Enabled Auger Decay

Single photon laser enabled Auger decay (spLEAD) has been redicted theoretically [Phys. Rev. Lett. 111, 083004 (2013)] and here we report its first experimental observation in neon. Using coherent, bichromatic free-electron laser pulses, we have detected the process and coherently controlled the angular distribution of the emitted electrons by varying the phase difference between the two laser fields. Since spLEAD is highly sensitive to electron correlation, this is a promising method for probing both correlation and ultrafast hole migration in more complex systems.

physics.atom-ph

Identifying spatially asymmetric high-order harmonic emission during the falling edge of an intense laser pulse

Two different induced effects of a laser falling edge on high-order harmonic generation are resolved by solving numerically full-dimensional electronic time-dependent Schrödinger equation beyond the Born-Oppenheimer approximation. The harmonic spectrum of H$_2^+$ and T$_2^+$ isotopes are compared to see the effects of a 4-cycle falling edge of a 800 nm, 15-cycle trapezoidal laser pulse of $I=$3 $\times 10^{14}$ Wcm$^{-2}$ intensity on harmonic emission spectrum. The harmonic emission at the laser falling part is negligible for H$_2^+$ due to ionization suppression, but considerable for T$_2^+$. The falling edge of the laser pulse induces two effects on the HHG in T$_2^+$. The first well-known effect is non-adiabatic frequency redshift of generated odd-order harmonics. The second unknown one is spatially asymmetric harmonic emission which appears as even harmonic orders. In order to clarify this new effect, spatial distribution of HHG and resolving HHG into different components are demonstrated. The asymmetric emission would appear for both atoms and molecules as long as harmonic emission of either rising or falling edge of an intense trapezoidal or non-trapezoidal laser pulse is dominant.

physics.atom-ph

Understanding molecular harmonic emission at relatively long intense laser pulses: Beyond the Born-Oppenheimer approximation

The underlying physics behind the molecular harmonic emission in relatively long sin$^2$-like laser pulses is investigated. We numerically solved the full-dimensional electronic time-dependent Schrödinger equation beyond the Born-Oppenheimer approximation for simple molecular ion H$_2^+$. The occurrence and the effect of electron localization, non-adiabatic redshift and spatially asymmetric emission are evaluated to understand better complex patterns appearing in the high-order harmonic generation (HHG) spectrum. Results show that the complex patterns in the HHG spectrum originate mainly from a non-adiabatic response of the molecule to the rapidly changing laser field and also from a spatially asymmetric emission along the polarization direction. The effect of electron localization on the HHG spectrum was not observed as opposed to what is reported in the literature.

physics.atom-ph

On the rate analysis of inexact augmented Lagrangian schemes for convex optimization problems with misspecified constraints

We consider a misspecified optimization problem that requires minimizing of a convex function $f(x;θ^*)$ in x over a constraint set represented by $h(x;θ^*)\leq 0$, where $θ^*$ is an unknown (or misspecified) vector of parameters. Suppose $θ^*$ can be learnt by a distinct process that generates a sequence of estimators $θ_k$, each of which is an increasingly accurate approximation of $θ^*$. We develop a first-order augmented Lagrangian scheme for computing an optimal solution $x^*$ while simultaneously learning $θ^*$.

math.OC

Complicated high-order harmonic generation due to the falling edge of a trapezoidal laser pulse

High-order harmonic generation (HHG) is investigated for H$_2^+$ and its isotopomers under seven- and ten-cycle trapezoidal laser pulses at 800 nm wavelength and $I$=4$\times 10^{14}$ W$/$cm$^2$ intensity. We solved numerically full-dimensional electronic time-dependent Schrödinger equation with and without the Born-Oppenheimer approximation. We show that the HHG at the falling edge of a trapezoidal laser pulse can result in redshift and complexity on the total HHG spectrum which can be removed by considering different laser pulse duration and nuclear motion not possible for sin$^2$ and Gaussian laser pulses. We resolve the redshifts and complexities of the HHG spectra into different electronic and vibrational states and their interferences.

physics.atom-ph