arXiv subjects

H. Amitsuka

Publications and source records attributed to H. Amitsuka.

33 records · Page 2Linked to original sources

arXiv2006

Evolution of Heterogeneous Antiferromagnetic State in URu2Si2: Study of Hydrostatic-Pressure, Uniaxial-Stress and Rh-Dope Effects

We have investigated the nature of the competition between hidden order and antiferromagnetic (AF) order in URu_2Si_2 by performing the neutron scattering experiments under hydrostatic-pressure P, uniaxial-stress sigma, and Rh-substitution conditions. Hidden order observed at ambient pressure in pure URu_2Si_2 is found to be replaced by the AF order by applying P, sigma along the tetragonal basal plane, and by doping Rh. We discuss these experimental results on the basis of the crystalline strain calculations, and suggest that this phase transition is generated by the 0.1% increase of the tetragonal c/a ratio. We have also found that the magnetic excitation observed in the hidden order phase vanishes in the AF phase. We show that this variation can be qualitatively explained by assuming the hidden order parameter to be quadrupole.

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arXiv2006

Pressure-temperature phase diagram of the heavy-electron superconductor URu2Si2

The pressure-temperature phase diagram of the heavy-electron superconductor URu2Si2 has been reinvestigated by ac-susceptibility and elastic neutron-scattering (NS) measurements performed on a small single-crystalline rod (2 mm in diameter, 6 mm in length) in a Cu-Be clamp-type high-pressure cell (P < 1.1 GPa). At ambient pressure, this sample shows the weakest antiferromagnetic (AF) Bragg reflections reported so far, corresponding to the volume-averaged staggered moment of mord ~ 0.011 mB/U. Under applied pressure, the AF scattering intensity exhibits a sharp increase at P ~ 0.7 GPa at low temperatures. The saturation value of the AF scattering intensity above 0.7 GPa corresponds to mord ~ 0.41 mB/U, which is in good agreement with that (~ 0.39 mB/U) observed above 1.5 GPa in our previous NS measurements. The superconductivity is dramatically suppressed by the evolution of AF phase, indicating that the superconducting state coexists only with the hidden order phase. The presence of parasitic ferro- and/or antiferromagnetic phases with transition temperatures T1star =120(5) K, T2star = 36(3) K and T3star = 16.5(5) K and their relationship to the low-T ordered phases are also discussed.

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arXiv2006

New Magnetic State in Incommensurate Magnetic Phase of Heavy-Fermion Superconductor CeRh0.6Co0.4In5

We performed elastic neutron scattering experiments on solid solution CeRh1-xCoxIn5 with x=0.4 to clarify the nature of the antiferromagnetic (AF) phase in the vicinity of the quantum critical point. We observed the incommensurate AF order below T_Nh=3.5 K. The structure of the incommensurate AF order is basically unchanged from that for pure CeRhIn5. We further found the evolution of a new commensurate AF order with the modulation of q_c=(1/2,1/2,1/2) below T_Nc=2.9 K. The volume-averaged moments for the incommensurate and commensurate AF phases are 0.38 mu_B/Ce and 0.21 mu_B/Ce, respectively, which are reduced from the incommensurate AF moment (0.75 mu_B/Ce) for pure CeRhIn5. We suggest from these results that the commensurate magnetic correlation may be tightly coupled with the superconductivity observed below T_c=1.4 K.

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arXiv2005

Competition between hidden order and antiferromagnetism in URu_2Si_2 under uniaxial stress studied by neutron scattering

We have performed elastic neutron scattering experiments under uniaxial stress sigma applied along the tetragonal [100], [110] and [001] directions for the heavy electron compound URu2Si2. We found that antiferromagnetic (AF) order with large moment is developed with sigma along the [100] and [110] directions. If the order is assumed to be homogeneous, the staggered ordered moment mu_o continuously increases from 0.02 mu_B (sigma=0) to 0.22 mu_B (0.25 GPa). The rate of increase partial mu_o/partial sigma is ~ 1.0 mu_B/GPa, which is four times larger than that for the hydrostatic pressure (partial mu_o/partial P sim 0.25 mu_B/GPa). Above 0.25 GPa, mu_o shows a tendency to saturate, similar to the hydrostatic pressure behavior. For sigma||[001], mu_o shows only a slight increase to 0.028 mu_B (sigma = 0.46 GPa) with a rate of ~ 0.02 mu_B/GPa, indicating that the development of the AF state highly depends on the direction of sigma. We have also found a clear hysteresis loop in the isothermal mu_o(sigma) curve obtained for sigma||[110] under the zero-stress-cooled condition at 1.4 K. This strongly suggests that the sigma-induced AF phase is metastable, and separated from the "hidden order" phase by a first-order phase transition. We discuss these experimental results on the basis of crystalline strain effects and elastic energy calculations, and show that the c/a ratio plays a key role in the competition between these two phases.

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arXiv2005

Phonon Thermal Transport of URu2Si2: Broken Translational Symmetry and Strong-Coupling of the Hidden Order to the Lattice

A dramatic increase in the total thermal conductivity (k) is observed in the Hidden Order (HO) state of single crystal URu2Si2. Through measurements of the thermal Hall conductivity, we explicitly show that the electronic contribution to k is extremely small, so that this large increase in k is dominated by phonon conduction. An itinerant BCS/mean-field model describes this behavior well: the increase in kappa is associated with the opening of a large energy gap at the Fermi Surface, thereby decreasing electron-phonon scattering. Our analysis implies that the Hidden Order parameter is strongly coupled to the lattice, suggestive of a broken symmetry involving charge degrees of freedom.

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arXiv2005

Irreversible dynamics of the phase boundary in U(Ru0.9)Rh0.04)2Si2 and implications for ordering

We report measurements and analysis of the specific heat and magnetocaloric effect at the phase boundary into the single magnetic field-induced phase (phase II) of U(Ru{0.96}Rh{0.04})2Si2, which yield striking similarities to the valence transition of Yb{1-x}YxInCu4. To explain these similarities, we propose a bootstrap mechanism by which a structural distortion causes an electric quadrupolar order parameter within phase II to become coupled to the 5f-electron hybridization, giving rise to a valence change at the transition.

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arXiv2005

Gamma5 quasiparticles and avoided quantum criticality in U(Ru,Rh)2Si2

We discuss recent specific heat data in high magnetic fields on URu2Si2 and 4% Rh-doped URu2Si2 as well as previously published de Haas-van Alphen data at lower magnetic fields in pure URu2Si2; both of which are consistent with quasiparticle bands formed from a hybridization between 5f-electron Gamma5 doublets and regular conduction electrons. The system exhibits itinerant electron metamagnetism that gives rise to a putative quantum critical point at \~ 34 -37 T (depending on the % of Rh) that is subsequently unstable to field-induced phases

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arXiv2005

Quantum critical 5f-electrons avoid singularities in U(Ru,Rh)2Si2

We present specific heat measurements of 4% Rh-doped U(Ru,Rh)2Si2 at magnetic fields above the proposed metamagnetic transition field Hm~34 T, revealing striking similarities to the isotructural Ce analog CeRu2Si2, suggesting that strongly renormalized hybridized band models apply equally well to both systems. The vanishing bandwidths as H --> Hm are consistent with a putative quantum critical point close to Hm. The existence of a phase transition into an ordered phase in the vicinity of Hm for 4% Rh-doped U(Ru,Rh)2Si2, but not for CeRu2Si2, is consistent with a stronger super-exchange in the case of the U 5-f system, with irreversible processes at the transition revealing a strong coupling of the 5f orbitals to the lattice, most suggestive of orbital or electric quadrupolar order.

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arXiv2004

Resistivity and magnetization of U(Ru$_{1-x}$Rh$_x$)$_2$Si$_2$, $x=$ 2, 2.5, 3 and 4 % in magnetic fields of up to 45 T

This posting contains raw data used for extracting features of the phase diagram and quantum criticality versus magnetic field $B$, temperature $T$ and Rh-doping $x$ that will soon appear in Physical Review Letters, 2004. All of the raw resistivity data is shown while only a selection of the magnetization data is shown for which a sample-out background subtraction was made.

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arXiv2004

Magnetic Excitations in U(Ru_{1-x}Rh_x)_2Si_2 (x<=0.03)

We have investigated magnetic excitations for a mixed phase of hidden order (HO) and the antiferromagnetic (AF) order in U(Ru_{1-x}Rh_x)_2Si_2 (x <= 0.03) by means of inelastic neutron scattering. The inelastic peaks observed at Q=(1,0,0) and (1,0.4,0) in the HO phase for x=0 and 0.015 at 1.4 K are found to be strongly reduced in the AF dominant compositions of x=0.02 and 0.03. Similar behavior is observed as the HO is replaced by the AF order upon cooling for x=0.02. The x-T region in which the strong reduction of inelastic peaks is observed corresponds to the AF-rich region, indicating that the magnetic excitations typical for the HO-phase vanish in the AF phase.

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arXiv2004

Weak magnetism phenomena in heavy-fermion superconductors: selected $μ$SR studies

The behavior of the so-called weak moment antiferromagnetic states, observed in the heavy-fermion superconductors UPt$_3$ and URu$_2$Si$_2$, is discussed in view of recent $μ$SR results obtained as function of control parameters like chemical substitution and external pressure. In UPt$_3$, the Pd substitution for Pt reveals the dynamical character of the weak moment order. On the other hand, $μ$SR measurements performed on samples in which Th substitutes U suggest that crystallographic disorder on the magnetic sites deeply affects the fluctuation timescale. In URu$_2$Si$_2$, a phase separation between the so-called hidden order state, present at ambient pressure, and an antiferromagnetic state, occurring under pressure, is observed. In view of the pressure-temperature phase diagram obtained by $μ$SR, it is deduced that the respective order parameters have different symmetries.

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arXiv2003

Neutron Scattering Study on Competition between Hidden Order and Antiferromagnetism in U(Ru_{1-x}Rh_x)_2Si_2 (x <= 0.05)

We have performed elastic and inelastic neutron scattering experiments on the solid solutions U(Ru_{1-x}Rh_x)_2Si_2 for the Ru rich concentrations: x=0, 0.01, 0.02, 0.025, 0.03, 0.04 and 0.05. Hidden order is suppressed with increasing x, and correspondingly the onset temperature T_m (~ 17.5 K at x=0) of weak antiferromagnetic (AF) Bragg reflection decreases. For x=0.04 and 0.05, no magnetic order is detected in the investigated temperature range down to 1.4 K. In the middle range, 0.02 <= x <= 0.03, we found that the AF Bragg reflection is strongly enhanced. At x=0.02, this takes place at ~ 7.7 K (=T_M), which is significantly lower than T_m (~ 13.7 K). T_M increases with increasing x, and seems to merge with T_m at x=0.03. If the AF state is assumed to be homogeneous, the staggered moment μ_o estimated at 1.4 K increases from 0.02(2) μ_B/U (x=0) to 0.24(1) μ_B/U (x=0.02). The behavior is similar to that observed under hydrostatic pressure (μ_o increases to ~ 0.25 μ_B/U at 1.0 GPa), suggesting that the AF evolution induced by Rh doping is due to an increase in the AF volume fraction. We also found that the magnetic excitation observed at Q=(1,0,0) below T_m disappears as T is lowered below T_M.

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arXiv2002

Nonequilibrium Antiferromagnetic State in the Heavy Electron Compound URu_2Si_2

We have investigated the nature of the antiferromagnetic (AF) phase induced by uniaxial stress sigma in URu2Si2, by performing elastic neutron scattering measurements up to 0.4 GPa. We have found that the AF Bragg-peak intensity shows a clear hysteresis loop with sigma under the zero-stress cooling condition. The result strongly suggests that the sigma-induced AF phase is metastable and separated from the coexisting "hidden ordered" phase by a first-order phase transition. We also present the analyses of the crystalline strain effects, and suggest that the c/a ratio plays an important role in the competition between these two phases.

cond-mat.str-el↗

arXiv2002

Effects of Uniaxial Stress on Antiferromagnetic Moment in the Heavy Electron Compound URu_2Si_2

We have performed the elastic neutron scattering experiments under uniaxial stress σalong the tetragonal [100], [110] and [001] directions for URu2Si2. For σ// [100] and [110], the antiferromagnetic moment μ_o is strongly enhanced from 0.02 μ_B (σ=0) to 0.22 μ_B (σ=2.5 kbar) at 1.5 K. The rate of increase dμ_o/dσis roughly estimated to be ~ 0.1 μ_B/kbar, which is much larger than that for the hydrostatic pressure (~ 0.025 μ_B/kbar). Above 2.5 kbar, μ_o shows a tendency to saturate similar to the behavior in the hydrostatic pressure. For σ// [001], on the other hand, μ_o shows only a slight increase to 0.028 μ_B (σ= 4.6 kbar) with a rate of ~ 0.002 μ_B/kbar. The observed anisotropy suggests that the competition between the hidden order and the antiferromagnetic state in URu2Si2 is strongly coupled with the tetragonal four-fold symmetry and the c/a ratio, or both.

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arXiv1999

Effect of Pressure on Tiny Antiferromagnetic Moment in the Heavy-Electron Compound URu_2Si_2

We have performed elastic neutron-scattering experiments on the heavy-electron compound URu_2Si_2 for pressure P up to 2.8 GPa. We have found that the antiferrmagnetic (100) Bragg reflection below T_m ~ 17.5 K is strongly enhanced by applying pressure. For P < 1.1 GPa, the staggered moment mu_o at 1.4 K increases linearly from ~ 0.017(3) mu_B to ~ 0.25(2) mu_B, while T_m increases slightly at a rate ~ 1 K/GPa, roughly following the transition temperature T_o determined from macroscopic anomalies. We have also observed a sharp phase transition at P_c ~ 1.5 GPa, above which a 3D-Ising type of antiferromagnetic phase (mu_o ~ 0.4 mu_B) appears with a slightly reduced lattice constant.

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