arXiv subjects

H. C. Chang

Publications and source records attributed to H. C. Chang.

4 recordsLinked to original sources

arXiv2019

Probing plasmon-NV$^0$ coupling at the nanometer scale with photons and fast electrons

The local density of optical states governs an emitters lifetime and quantum yield through the Purcell effect. It can be modified by a surface plasmon electromagnetic field, but such a field has a spatial extension limited to a few hundreds of nanometers, which complicates the use of optical methods to spatially probe the emitter-plasmon coupling. Here we show that a combination of electron-based imaging, spectroscopies and photon-based correlation spectroscopy enables measurement of the Purcell effect with nanometer and nanosecond spatio-temporal resolutions. Due to the large variability of radiative lifetimes of emitters embedded in nanoparticles with inhomogeneous sizes we relied on a statistical approach to unambiguously probe the coupling between nitrogen-vacancy centers (NV^0) in nanodiamonds and surface plasmons in silver nanocubes. We quantified the Purcell effect by measuring the NV^0 excited state lifetimes in a large number of either isolated nanodiamonds or nanodiamond-nanocube dimers and demonstrated a statistically significant lifetime reduction for dimers.

cond-mat.mes-hall↗

arXiv2015

Ambient Pressure Structural Quantum Critical Point in the Phase Diagram of (Ca$_x$Sr$_{1-x}$)$_3$Rh$_4$Sn$_{13}$

The quasi-skutterudite superconductor Sr$_3$Rh$_4$Sn$_{13}$ features a pronounced anomaly in electrical resistivity at $T^*\sim$138 K. We show that the anomaly is caused by a second-order structural transition, which can be tuned to 0 K by applying physical pressure and chemical pressure via the substitution of Ca for Sr. A broad superconducting dome is centred around the structural quantum critical point. Detailed analysis of the tuning parameter dependence of $T^*$ as well as insights from lattice dynamics calculations strongly support the existence of a structural quantum critical point at ambient pressure when the fraction of Ca is 0.9 (i.e., $x_c=0.9$). This establishes (Ca$_x$Sr$_{1-x}$)$_3$Rh$_4$Sn$_{13}$ series as an important system for exploring the physics of structural quantum criticality without the need of applying high pressures.

cond-mat.supr-con↗

arXiv2014

Reestablishing Kepler_s first two laws for planets from the non_stationary Earth

The Earth itself is not stationary but keeps revolving, and its motion further satisfies the law of equal area according to the heliocentric doctrine. That satisfaction can be used to construct the mathematical relationships between the planet_Sun and Earth_Sun distances. The law of equal area for planets can hence be reestablished naturally from the moving Earth using the observed angular speed of a planet over the Sun. Furthermore, for the periodicity of a planet to the Sun, the distance from each planet to the Sun may be expressed as an angular periodic function. By coordinating with the observed data, this periodic distance function depicts an exact elliptical path. Here, we apply relatively simple mathematical skills to illustrate the invariant forms of planetary motions and indicate the key factors used to analyze the motions in complicated planetary systems.

physics.class-ph↗

arXiv2014

Anomalous Pressure Dependence of the Superconducting Transition Temperature in TlNi$_2$Se$_{2-x}$S$_x$

We report the pressure dependence of the superconducting transition temperature, $T_c$, in TlNi$_2$Se$_{2-x}$S$_x$ detected via the AC susceptibility method. The pressure-temperature phase diagram constructed for TlNi$_{2}$Se$_{2}$, TlNi$_{2}$S$_{2}$ and TlNi$_{2}$SeS exhibits two unexpected features: (a) a sudden collapse of the superconducting state at moderate pressure for all three compositions and (b) a dome-shaped pressure dependence of $T_c$ for TlNi$_{2}$SeS. These results point to the nontrivial role of S substitution and its subtle interplay with applied pressure, as well as novel superconducting properties of the TlNi$_2$Se$_{2-x}$S$_x$ system.

cond-mat.supr-con↗