arXiv subjects

H. Eisaki

Publications and source records attributed to H. Eisaki.

At least 73 records · Page 4Linked to original sources

arXiv2014

Electronic structure of BaNi$_2$P$_2$ observed by angle-resolved photoemission spectroscopy

We have performed an angle-resolved photoemission spectroscopy (ARPES) study of BaNi$_2$P$_2$ which shows a superconducting transition at $T_c$ $\sim$ 2.5 K. We observed hole and electron Fermi surfaces (FSs) around the Brillouin zone center and corner, respectively, and the shapes of the hole FSs dramatically changed with photon energy, indicating strong three-dimensionality. The observed FSs are consistent with band-structure calculation and de Haas-van Alphen measurements. The mass enhancement factors estimated in the normal state were $m^*$/$m_b$ $\leq$ 2, indicating weak electron correlation compared to typical iron-pnictide superconductors. An electron-like Fermi surface around the Z point was observed in contrast with BaNi$_2$As$_2$ and may be related to the higher $T_c$ of BaNi$_2$P$_2$.

cond-mat.supr-con↗

arXiv2014

Simultaneous Transitions in Cuprate Momentum-Space Topology and Electronic Symmetry Breaking

The existence of electronic symmetry breaking in the underdoped cuprates, and its disappearance with increased hole-density $p$, are now widely reported. However, the relationship between this transition and the momentum space ($\vec{k}$-space) electronic structure underpinning the superconductivity has not been established. Here we visualize the $\vec{Q}$=0 (intra-unit-cell) and $\vec{Q}\neq$0 (density wave) broken-symmetry states simultaneously with the coherent $\vec{k}$-space topology, for Bi$_2$Sr$_2$CaCu$_2$O$_{8+d}$ samples spanning the phase diagram 0.06$\leq p \leq$0.23. We show that the electronic symmetry breaking tendencies weaken with increasing $p$ and disappear close to $p_c$=0.19. Concomitantly, the coherent $\vec{k}$-space topology undergoes an abrupt transition, from arcs to closed contours, at the same $p_c$. These data reveal that the $\vec{k}$-space topology transformation in cuprates is linked intimately with the disappearance of the electronic symmetry breaking at a concealed critical point.

cond-mat.supr-con↗

arXiv2014

Evidence of a universal relation between electron-mode coupling and Tc in Ba1-xKxFe2As2 superconductor from Laser ARPES

We performed a Laser angle-resolved photoemission spectroscopy (ARPES) study on a wide doping range of Ba1-xKxFe2As2 (BaK) iron-based superconductor. We observed a robust low-binding energy (BE) kink structure in the dispersion which is doping dependent where its energy peaks at the optimally-doped (OP) level (x~0.4) and decreases towards the underdoped (UD) and overdoped (OD) sides. It is also temperature-dependent and survives up to ~90K. We attribute this kink to electron-mode coupling in good agreement with the inelastic neutron scattering (INS) and scanning tunneling microscopy (STM) results on the same compound which observed a similar bosonic mode associated with spin excitations. The relation between the mode energy (Ω) and the SC transition temperature (Tc) deduced from our Laser ARPES data follow the universal relation deduced from INS and STM. In addition, we could resolve another kink at higher BE showing less doping and temperature dependence and may thus be of different origin.

cond-mat.supr-con↗

arXiv2014

Evidence for exclusion of the possibility of $d$-wave superconducting-gap symmetry in Ba-doped KFe$_2$As$_2$

We have investigated the superconducting(SC)-gap anisotropy for several Ba-doped KFe$_2$As$_2$ samples using laser-based angle-resolved photoemission spectroscopy. We show that the SC-gap anisotropy and node positions drastically change with a small amount of Ba doping. Our results totally exclude a possibility of $d$-wave symmetry and strongly suggest that both spin and orbital fluctuations are important for the paring interaction in the Ba-doped K122.

cond-mat.supr-con↗

arXiv2014

Charge order driven by Fermi-arc instability in Bi2201

The understanding of the origin of superconductivity in cuprates has been hindered by the apparent diversity of intertwining electronic orders in these materials. We combined resonant x-ray scattering (REXS), scanning-tunneling microscopy (STM), and angle-resolved photoemission spectroscopy (ARPES) to observe a charge order that appears consistently in surface and bulk, and in momentum and real space within one cuprate family, Bi2201. The observed wave vectors rule out simple antinodal nesting in the single-particle limit but match well with a phenomenological model of a many-body instability of the Fermi arcs. Combined with earlier observations of electronic order in other cuprate families, these findings suggest the existence of a generic charge-ordered state in underdoped cuprates and uncover its intimate connection to the pseudogap regime.

cond-mat.supr-con↗

arXiv2013

Muon spin spectroscopy in multiferroic (Cu,Zn)$_{3}$Mo$_{2}$O$_{9}$

We present the muon spin relaxation/rotation spectra in the multiferroic compound (Cu,Zn)$_{3}$Mo$_{2}$O$_{9}$. The parent material Cu$_{3}$Mo$_{2}$O$_{9}$ has a multiferroic phase below $T_{\rm N}$ = 8.0 K, where the canted antiferromagnetism and the ferroelectricity coexist. The asymmetry time spectra taken at RIKEN-RAL pulsed muon facility show a drastic change at $T_{\rm N}$. At low temperatures the weakly beating oscillation caused by the static internal magnetic fields in the antiferromagnetic phase was observed in Cu$_{3}$Mo$_{2}$O$_{9}$ and the lightly ($0.5\%$) Zn-doped sample. From the fitting of the oscillating term, we obtain the order parameter in these samples: ferromagnetic moment in two sublattices of antiferromagnet. In the heavily ($5.0\%$) Zn-doped sample, the muon-spin oscillation is rapidly damped. The frequency-domain spectrum of this sample suggests a formation of magnetic superstructure.

cond-mat.str-el↗

arXiv2013

Large momentum-dependence of the main dispersion "kink" in the high-Tc superconductor Bi2Sr2CaCu2O8+δ

Ultrahigh resolution angle-resolved photoemission spectroscopy with low-energy photons is used to study the detailed momentum dependence of the well-known nodal "kink" dispersion anomaly of Bi2Sr2CaCu2O8+δ. We find that the kink's location transitions smoothly from a maximum binding energy of about 65 meV at the node of the d-wave superconducting gap to 55 meV roughly one-third of the way to the antinode. Meanwhile, the self-energy spectrum corresponding to the kink dramatically sharpens and intensifies beyond a critical point in momentum space. We discuss the possible bosonic spectrum in energy and momentum space that can couple to the k-space dispersion of the electronic kinks.

cond-mat.supr-con↗

arXiv2013

Magnetic and Dielectric Properties in Multiferroic Cu3Mo2O9 under High Magnetic Fields

The magnetic and dielectric properties under high magnetic fields are studied in the single crystal of Cu3Mo2O9. This multiferroic compound has distorted tetrahedral spin chains. The effects of the quasi-one dimensionality and the geometrical spin frustration are expected to appear simultaneously. We measure the magnetoelectric current and the differential magnetization under the pulsed magnetic field up to 74 T. We also measure the electric polarization versus the electric field curve/loop under the static field up to 23 T. Dielectric properties change at the magnetic fields where the magnetization jumps are observed in the magnetization curve. Moreover, the magnetization plateaus are found at high magnetic fields.

cond-mat.str-el↗

arXiv2013

Universal inhomogeneous magnetic-field response in the normal state of cuprate high-Tc superconductors

We report the results of a muon spin rotation (muSR) study of the bulk of Bi{2+x}Sr{2-x}CaCu2O{8+δ}, as well as pure and Ca-doped YBa2Cu3Oy, which together with prior measurements reveal a universal inhomogeneous magnetic-field response of hole-doped cuprates extending to temperatures far above the critical temperature (Tc). The primary features of our data are incompatible with the spatially inhomogeneous response being dominated by known charge density wave (CDW) and spin density wave (SDW) orders. Instead the normal-state inhomogeneous line broadening is found to scale with the maximum value Tc^max for each cuprate family, indicating it is controlled by the same energy scale as Tc. Since the degree of chemical disorder varies widely among the cuprates we have measured, the observed scaling constitutes evidence for an intrinsic electronic tendency toward inhomogeneity above Tc.

cond-mat.supr-con↗

arXiv2013

Strange Inter-layer Properties of $Ba(Fe_{1-x}Co_x)2As_2$ Appearing in Ultrasonic Measurements

We have investigated the elastic constant C33 of Ba(Fe1-xCox)2As2 with eight different Co concentrations by ultrasonic measurement. We found remarkable elastic anomalies near the quantum critical point. We have studied them by measuring the electrical resistivity, heat capacity, and ultrasonic attenuation in addition to the elastic constant. These results have revealed that the inter-layer three-dimensional properties appearing in C33 to be possibly originated from the magnetic character of these materials. Our data about the elastic constant C33 highlight the importance of controlling the c-axis length in the emergence of superconductivity in iron-based superconductors.

cond-mat.supr-con↗

arXiv2013

Universality of dispersive spin-resonance mode in superconducting BaFe2As2

Spin fluctuations in superconducting BaFe2(As1-xPx)2 (x=0.34, Tc = 29.5 K) are studied using inelastic neutron scattering. Well-defined commensurate magnetic signals are observed at (π,0), which is consistent with the nesting vector of the Fermi surface. Antiferromagnetic (AFM) spin fluctuations in the normal state exhibit a three-dimensional character reminiscent of the AFM order in nondoped BaFe2As2. A clear spin gap is observed in the superconducting phase forming a peak whose energy is significantly dispersed along the c-axis. The bandwidth of dispersion becomes larger with approaching the AFM ordered phase universally in all superconducting BaFe2As2, indicating that the dispersive feature is attributed to three-dimensional AFM correlations. The results suggest a strong relationship between the magnetism and superconductivity.

cond-mat.supr-con↗

arXiv2013

Pseudogap formation above the superconducting dome in iron-pnictides

The nature of the pseudogap in high transition temperature (high-Tc) superconducting cuprates has been a major issue in condensed matter physics. It is still unclear whether the high-Tc superconductivity can be universally associated with the pseudogap formation. Here we provide direct evidence of the existence of the pseudogap phase via angle-resolved photoemission spectroscopy in another family of high-Tc superconductor, iron-pnictides. Our results reveal a composition dependent pseudogap formation in the multi-band electronic structure of BaFe2(As1-xPx)2. The pseudogap develops well above the magnetostructural transition for low x, persists above the nonmagnetic superconducting dome for optimal x and is destroyed for x ~ 0.6, thus showing a notable similarity with cuprates. In addition, the pseudogap formation is accompanied by inequivalent energy shifts in xz/yz orbitals of iron atoms, indicative of a peculiar iron orbital ordering which breaks the four-fold rotational symmetry.

cond-mat.supr-con↗

arXiv2013

Normal-state charge dynamics in doped BaFe2As2: Roles of doping and necessary ingredients for superconductivity

We carried out a comparative study of the in-plane resistivity and optical spectrum of doped BaFe2As2 and investigated the doping evolution of the charge dynamics. For BaFe2As2, charge dynamics is incoherent at high temperatures. Electron (Co) and isovalent (P) doping into BaFe2As2 increase coherence of the system and transform the incoherent charge dynamics into highly coherent one. On the other hand, charge dynamics remains incoherent for hole (K) doping. It is found in common with any type of doping that superconductivity with high transition temperature emerges when the normal-state charge dynamics maintains incoherence and when the resistivity associated with the coherent channel exhibits dominant temperature-linear dependence.

cond-mat.supr-con↗

arXiv2013

Strong electronic correlations in iron pnictides: Comparison of the optical spectra for BaFe2As2-related compounds

We carried out combined transport and optical measurements for BaFe2As2 and five isostructural transition-metal (TM) pnictides. The low-energy optical conductivity spectra of these compounds are, to a good approximation, decomposed into a narrow Drude (coherent) component and an incoherent component. The iron arsenides, BaFe2As2 and KFe2As2, are distinct from other pnictides in their highly incoherent charge dynamics or bad metallic behavior with the coherent Drude component occupying a tiny fraction of the low-energy spectral weight. The fraction of the coherent spectral weight or the degree of coherence is shown to be well correlated with the TM-pnictogen bond angle and the electron filling of TM 3d orbitals, which are measures of the strength of electronic correlations. The iron arsenides are thus strongly correlated systems, and the doping into BaFe2As2 controls the strength of electronic correlations. This naturally explains a remarkable asymmetry in the charge dynamics of electron- and hole-doped systems, and the unconventional superconductivity appears to emerge when the correlations are fairly strong.

cond-mat.supr-con↗

arXiv2013

Superconducting gap with sign reversal between hole pockets in heavily hole-doped Ba1-xKxFe2As2

To gain insight into the unconventional superconductivity of Fe-pnictides with no electron pockets, we measure the thermal conductivity $κ$ and penetration depth $λ$ in the heavily hole-doped regime of Ba$_{1-x}$K$_x$Fe$_2$As$_2$. The residual thermal conductivity $(κ/T)_{T \rightarrow 0\,{\rm K}}$ and $T$-dependence of $λ$ consistently indicate the fully gapped superconductivity at $x=0.76$ and the (line) nodal superconductivity at higher hole concentrations. The magnitudes of $\fracκ{T}\cdot T_c|_{T \rightarrow 0\,{\rm K}}$ and $\frac{dλ}{d(T/T_c)}$ at low temperatures, both of which are determined by the properties of the low-energy excitations, exhibit a highly unusual non-monotonic x-dependence. These results indicate a dramatic change of the nodal characteristics in a narrow doping range, suggesting a doping crossover of the gap function between the s-wave states with and without sign reversal between $Γ$-centered hole pockets.

cond-mat.supr-con↗

arXiv2013

Anisotropy of the in-plane resistivity of underdoped Ba(Fe$_{1-x}$Co$_x$)$_2$As$_2$ superconductors induced by impurity scattering in the antiferromagnetic orthorhombic phase

We investigated the in-plane resistivity anisotropy for underdoped Ba(Fe$_{1-x}$Co$_x$)$_2$As$_2$ single crystals with improved quality. We demonstrate that the anisotropy in resistivity in the magnetostructural ordered phase arises from the anisotropy in the residual component which increases in proportion to the Co concentration $x$. This gives evidence that the anisotropy originates from the impurity scattering by Co atoms substituted for the Fe sites, rather than so far proposed mechanism such as the anisotropy of Fermi velocities of reconstructed Fermi surface pockets. As doping proceeds to the paramagnetic-tetragonal phase, a Co impurity transforms to a weak and isotropic scattering center.

cond-mat.supr-con↗

arXiv2013

Effects of Zn substitution on the electronic structure of BaFe$_2$As$_2$ revealed by angle-resolved photoemission spectroscopy

In Fe-based superconductors, electron doping is often realized by the substitution of transition-metal atoms for Fe. In order to investigate how the electronic structure of the parent compound is influenced by Zn substitution, which supplies nominally four extra electrons per substituted atom but is expected to induce the strongest impurity potential among the transition-metal atoms, we have performed an angle-resolved photoemission spectroscopy measurements on Ba(Fe_{1-x}Zn_x)_2As_2 (Zn-122). In Zn-122, the temperature dependence of the resistivity shows a kink around T~135 K, indicating antiferromagnetic order below the Neel temperature of T_N ~ 135 K. In fact, folded Fermi surfaces (FSs) similar to those of the parent compound have been observed below T_N. The hole and electron FS volumes are, therefore, different from those expected from the rigid-band model. The results can be understood if all the extra electrons occupy the Zn 3d state ~10 eV below the Fermi level and do not participate in the formation of the FSs.

cond-mat.supr-con↗

arXiv2013

Surface-enhanced charge-density-wave instability in underdoped Bi2201

Neutron and x-ray scattering experiments have provided mounting evidence for spin and charge ordering phenomena in underdoped cuprates. These range from early work on stripe correlations in Nd-LSCO to the latest discovery of charge-density-waves in YBCO. Both phenomena are characterized by a pronounced dependence on doping, temperature, and an externally applied magnetic field. Here we show that these electron-lattice instabilities exhibit also a previously unrecognized bulk-surface dichotomy. Surface-sensitive electronic and structural probes uncover a temperature-dependent evolution of the CuO2 plane band dispersion and apparent Fermi pockets in underdoped Bi2201, which is directly associated with an hitherto-undetected strong temperature dependence of the incommensurate superstructure periodicity below 130K. In stark contrast, the structural modulation revealed by bulk-sensitive probes is temperature independent. These findings point to a surface-enhanced incipient charge-density-wave instability, driven by Fermi surface nesting. This discovery is of critical importance in the interpretation of single-particle spectroscopy data and establishes the surface of cuprates and other complex oxides as a rich playground for the study of electronically soft phases.

cond-mat.supr-con↗