arXiv subjects

H. H. Hsieh

Publications and source records attributed to H. H. Hsieh.

At least 19 recordsLinked to original sources

arXiv2024

Activity of main-belt comet 324P/La Sagra

We study the activity evolution of the main-belt comet 324P/La Sagra over time and the properties of its emitted dust. We performed aperture photometry on images taken by a wide range of telescopes at optical and thermal infrared wavelengths between 2010 and 2021. We derived the combined scattering cross section of the nucleus and dust (when present) as a function of time, and we derived the thermal emission properties. Fitting an IAU H-G phase function to the data obtained when 324P was likely inactive, we derived an absolute nucleus magnitude $H_R = (18.4 \pm 0.5)$ mag using $G = 0.15 \pm 0.12$. The activity of 324P/La Sagra during the 2015 perihelion passage has significantly decreased compared to the previous perihelion passage in 2010, and it decreased even further during the 2021 perihelion passage. This decrease in activity may be attributed to mantling or to the depletion of volatile substances. The $Afρ$ profile analysis of the coma of the main-belt comet suggests a near-perihelion transition from a lower-activity pre-perihelion to a higher-activity post-perihelion steady state. We calculate a dust geometric albedo in the range of (2 - 45)%, which prevents us from constraining the spectral type of 324P/La Sagra, but we found an indication of dust superheating at 4.5 micrometers.

astro-ph.EP↗

arXiv2019

Comet 66P/du Toit: not a near Earth main belt comet

Main belt comets (MBCs) are a peculiar class of volatile-containing objects with comet-like morphology and asteroid-like orbits. However, MBCs are challenging targets to study remotely due to their small sizes and the relatively large distance they are from the Sun and the Earth. Recently, a number of weakly active short-period comets have been identified that might originate in the asteroid main belt. Among all of the known candidates, comet 66P/du Toit has been suggested to have one of the highest probabilities of coming from the main belt. We obtained medium and high-resolution spectra of 66P from 300-2500 nm with the X-shooter/VLT and the UVES/VLT instruments in July 2018. We also obtained a series of narrow-band images of 66P to monitor the gas and dust activity between May and July 2018 with TRAPPIST-South. In addition, we applied a dust model to characterize the dust coma of 66P and performed dynamical simulations to study the orbital evolution of 66P. We derive the OPR of ammonia (NH$_3$) in 66P to be 1.08$\pm$0.06, which corresponds to a nuclear spin temperature of $\sim$34 K. We computed the production rates of OH, NH, CN, C$_3,$ and C$_2$ radicals and measured the dust proxy, Af$ρ$. The dust analysis reveals that the coma can be best-fit with an anisotropic model and the peak dust production rate is about 55 kg s$^{-1}$ at the perihelion distance of 1.29 au. Dynamical simulations show that 66P is moderately asteroidal with the capture time, t$_{cap} \sim 10^4$ yr. Our observations demonstrate that the measured physical properties of 66P are consistent with other typical short-period comets and differ significantly from other MBCs. Therefore, 66P is unlikely to have a main belt origin.

astro-ph.EP↗

arXiv2018

Solar system science with the Wide-Field InfraRed Survey Telescope (WFIRST)

We present a community-led assessment of the solar system investigations achievable with NASA's next-generation space telescope, the Wide Field InfraRed Survey Telescope (WFIRST). WFIRST will provide imaging, spectroscopic, and coronagraphic capabilities from 0.43-2.0 $μ$m and will be a potential contemporary and eventual successor to JWST. Surveys of irregular satellites and minor bodies are where WFIRST will excel with its 0.28 deg$^2$ field of view Wide Field Instrument (WFI). Potential ground-breaking discoveries from WFIRST could include detection of the first minor bodies orbiting in the Inner Oort Cloud, identification of additional Earth Trojan asteroids, and the discovery and characterization of asteroid binary systems similar to Ida/Dactyl. Additional investigations into asteroids, giant planet satellites, Trojan asteroids, Centaurs, Kuiper Belt Objects, and comets are presented. Previous use of astrophysics assets for solar system science and synergies between WFIRST, LSST, JWST, and the proposed NEOCam mission are discussed. We also present the case for implementation of moving target tracking, a feature that will benefit from the heritage of JWST and enable a broader range of solar system observations.

astro-ph.EP↗

arXiv2017

Electronic signature of the vacancy ordering in NbO (Nb3O3)

We investigated the electronic structure of the vacancy-ordered 4d-transition metal monoxide NbO (Nb3O3) using angle-integrated soft- and hard-x-ray photoelectron spectroscopy as well as ultra-violet angle-resolved photoelectron spectroscopy. We found that density-functional-based band structure calculations can describe the spectral features accurately provided that self-interaction effects are taken into account. In the angle-resolved spectra we were able to identify the so-called vacancy band that characterizes the ordering of the vacancies. This together with the band structure results indicates the important role of the very large inter-Nb-4d hybridization for the formation of the ordered vacancies and the high thermal stability of the ordered structure of niobium monoxide.

cond-mat.mtrl-sci↗

arXiv2017

The Castalia Mission to Main Belt Comet 133P/Elst-Pizarro

We describe Castalia, a proposed mission to rendezvous with a Main Belt Comet (MBC), 133P/Elst-Pizarro. MBCs are a recently discovered population of apparently icy bodies within the main asteroid belt between Mars and Jupiter, which may represent the remnants of the population which supplied the early Earth with water. Castalia will perform the first exploration of this population by characterising 133P in detail, solving the puzzle of the MBC's activity, and making the first in situ measurements of water in the asteroid belt. In many ways a successor to ESA's highly successful Rosetta mission, Castalia will allow direct comparison between very different classes of comet, including measuring critical isotope ratios, plasma and dust properties. It will also feature the first radar system to visit a minor body, mapping the ice in the interior. Castalia was proposed, in slightly different versions, to the ESA M4 and M5 calls within the Cosmic Vision programme. We describe the science motivation for the mission, the measurements required to achieve the scientific goals, and the proposed instrument payload and spacecraft to achieve these.

astro-ph.EP↗

arXiv2017

Rotation of Cometary Nuclei: New Lightcurves and an Update of the Ensemble Properties of Jupiter-Family Comets

We report new lightcurves and phase functions for nine Jupiter-family comets (JFCs). They were observed in the period 2004-2015 with various ground telescopes as part of the Survey of Ensemble Physical Properties of Cometary Nuclei (SEPPCoN) as well as during devoted observing campaigns. We add to this a review of the properties of 35 JFCs with previously published rotation properties. The photometric time-series were obtained in Bessel R, Harris R and SDSS r' filters and were absolutely calibrated using stars from the Pan-STARRS survey. This specially-developed method allowed us to combine data sets taken at different epochs and instruments with absolute-calibration uncertainty down to 0.02 mag. We used the resulting time series to improve the rotation periods for comets 14P/Wolf, 47P/Ashbrook-Jackson, 94P/Russell, and 110P/Hartley 3 and to determine the rotation rates of comets 93P/Lovas and 162P/Siding-Spring for the first time. In addition to this, we determined the phase functions for seven of the examined comets and derived geometric albedos for eight of them. We confirm the known cut-off in bulk densities at $\sim$0.6 g $\mathrm{cm^{-3}}$ if JFCs are strengthless. Using the model of Davidsson (2001) for prolate ellipsoids with typical density and elongations, we conclude that none of the known JFCs require tensile strength larger than 10-25 Pa to remain stable against rotational instabilities. We find evidence for an increasing linear phase function coefficient with increasing geometric albedo. The median linear phase function coefficient for JFCs is 0.046 mag/deg and the median geometric albedo is 4.2 per cent.

astro-ph.EP↗

arXiv2016

Dynamic atomic reconstruction: how Fe3O4 thin films evade polar catastrophe for epitaxy

Polar catastrophe at the interface of oxide materials with strongly correlated electrons has triggered a flurry of new research activities. The expectations are that the design of such advanced interfaces will become a powerful route to engineer devices with novel functionalities. Here we investigate the initial stages of growth and the electronic structure of the spintronic Fe3O4/MgO (001) interface. Using soft x-ray absorption spectroscopy we have discovered that the so-called A-sites are completely missing in the first Fe3O4 monolayer. This allows us to develop an unexpected but elegant growth principle in which during deposition the Fe atoms are constantly on the move to solve the divergent electrostatic potential problem, thereby ensuring epitaxy and stoichiometry at the same time. This growth principle provides a new perspective for the design of interfaces.

cond-mat.mtrl-sci↗

arXiv2012

Local correlations, non-local screening, multiplets, and band formation in NiO

We report on a comparative study of the valence band electronic structure of NiO as bulk material and of NiO as impurity in MgO. From the impurity we have been able to determine reliably the parameters which describe the local correlations, thereby establishing the compensated-spin character of the first ionization state or the state created by hole doping. Using bulk-sensitive x-ray photoemission we identify pronounced satellite features in the valence band of bulk NiO which cannot be explained by single-site many body approaches nor by mean field calculations. We infer the presence of screening processes involving local quasi-core states in the valence band and non-local coherent many body states. These processes are strong and the propagation of an extra hole in the valence band of NiO will therefore be accompanied by a range of high energy excitations. This in turn will make the observation of the dispersion relations in the Ni 3d bands difficult, also because the effective band width is no more than 0.25 eV as estimated from multi-site calculations.

cond-mat.str-el↗

arXiv2010

Local electronic structure of Fe$^{2+}$ impurities in MgO thin films: Temperature-dependent soft x-ray absorption spectroscopy study

We report on the local electronic structure of Fe impurities in MgO thin films. Using soft x-ray absorption spectroscopy (XAS) we verified that the Fe impurities are all in the 2+ valence state. The fine details in the line shape of the Fe $L_{2,3}$ edges provide direct evidence for the presence of a dynamical Jahn-Teller distortion. We are able to determine the magnitude of the effective $D_{4h}$ crystal field energies. We also observed a strong temperature dependence in the spectra which we can attribute to the thermal population of low-lying excited states that are present due to the spin-orbit coupling in the Fe 3d. Using this Fe$^{2+}$ impurity system as an example, we show that an accurate measurement of the orbital moment in Fe$_3$O$_4$ will provide a direct estimate for the effective local low-symmetry crystal fields on the Fe$^{2+}$ sites, important for the theoretical modeling of the formation of orbital ordering.

cond-mat.str-el↗

arXiv2010

Local symmetry and magnetic anisotropy in multiferroic MnWO4 and antiferromagnetic CoWO4 studied by soft x-ray absorption spectroscopy

Soft x-ray absorption experiments on the transition metal L2,3 edge of multiferroic MnWO4 and antiferromagnetic CoWO4 are presented. The observed linear polarization dependence, analyzed by full-multiplet calculations, is used to determine the ground state wave function of the magnetic Mn2+ and Co2+ ions. The impact of the local structure and the spin-orbit coupling on the orbital moment is discussed in terms of the single-ion anisotropy. It is shown that the orbital moment in CoWO4 is responsible for the collinear antiferromagnetism, while the small size of spin-orbit coupling effects make spiral magnetic order in MnWO4 possible, enabling the material to be multiferroic.

cond-mat.str-el↗

arXiv2010

Far-infrared measurements of oxygen-doped polycrystalline La2CuO4.0315 superconductor under slow-cooled and fast-cooled conditions

We have studied the far-infrared (far-IR) charge dynamics of an equilibrated pure oxygen doped La2CuO4+0.0315 under slow-cooled and fast-cooled conditions. The superconducting transition temperature (Tc) for the slow-cooled and that for the fast-cooled processes were respectively found to be close to the two intrinsic Tc's: One at 30 K and the other at 15 K. Direct comparison with our previous results and other far-IR and Raman studies on single crystalline La2-xSrxCuO4, we conclude that the topology of the pristine electronic phases that are responsible for the two intrinsic Tc's is holes arranged into two-dimensional (2D) square lattices.

cond-mat.supr-con↗

arXiv2010

Crystal-field and Kondo scale investigation of CeMIn5 (M=Co, Ir and Rh): a combined x-ray absorption and inelastic neutron study

Linear polarized soft-x ray absorption (XAS) and inelastic neutron scattering (INS) experiments have been performed on CeMIn5 with M = Rh, Ir, and Co to determine the crystal-field scheme and characteristic Kondo temperatures T* for the hybridization between 4f and conduction electrons. The ground state wave functions are determined from the polarization dependent soft-XAS data at the cerium M4,5 edge and the crystal-field splittings from INS. The characteristic temperature T* has been determined from the line widths of the neutron scattering data. We find that the quasielastic line widths of the superconducting compounds CeCoIn5 and CeIrIn5 are comparable with the low energy crystal-field splitting.

cond-mat.str-el↗

arXiv2009

Epitaxy, stoichiometry, and magnetic properties of Gd-doped EuO films on YSZ (001)

We have succeeded in preparing high-quality Gd-doped single-crystalline EuO films. Using Eu-distillation-assisted molecular beam epitaxy and a systematic variation in the Gd and oxygen deposition rates, we have been able to observe sustained layer-by-layer epitaxial growth on yttria-stabilized cubic zirconia (001). The presence of Gd helps to stabilize the layer-by-layer growth mode. We used soft x-ray absorption spectroscopy at the Eu and Gd M4,5 edges to confirm the absence of Eu3+ contaminants and to determine the actual Gd concentration. The distillation process ensures the absence of oxygen vacancies in the films. From magnetization measurements we found the Curie temperature to increase smoothly as a function of doping from 70 K up to a maximum of 125 K. A threshold behavior was not observed for concentrations as low as 0.2%.

cond-mat.str-el↗

arXiv2009

Electronic and magnetic properties of the kagome systems YBaCo4O7 and YBaCo3MO7 (M=Al, Fe)

We present a combined experimental and theoretical x-ray absorption spectroscopy (XAS) study of the new class of cobaltates YBaCo4O7 and YBaCo3MO7 (M= Al, Fe). The focus is on the local electronic and magnetic properties of the transition metal ions in these geometrically frustrated kagome compounds. For the mixed valence cobaltate YBaCo4O7, both the Co2+ and Co3+ are found to be in the high spin state. The stability of these high spin states in tetrahedral coordination is compared with those in the more studied case of octahedral coordination. For the new compound YBaCo3FeO7, we find exclusively Co2+ and Fe3+ as charge states.

cond-mat.str-el↗

arXiv2009

Epitaxial and layer-by-layer growth of EuO thin films on yttria-stabilized cubic zirconia (001) using MBE distillation

We have succeeded in growing epitaxial and highly stoichiometric films of EuO on yttria-stabilized cubic zirconia (YSZ) (001). The use of the Eu-distillation process during the molecular beam epitaxy assisted growth enables the consistent achievement of stoichiometry. We have also succeeded in growing the films in a layer-by-layer fashion by fine tuning the Eu vs. oxygen deposition rates. The initial stages of growth involve the limited supply of oxygen from the YSZ substrate, but the EuO stoichiometry can still be well maintained. The films grown were sufficiently smooth so that the capping with a thin layer of aluminum was leak tight and enabled ex situ experiments free from trivalent Eu species. The findings were used to obtain recipes for better epitaxial growth of EuO on MgO (001).

cond-mat.str-el↗

arXiv2009

Spin blockade, orbital occupation and charge ordering in La_(1.5)Sr_(0.5)CoO4

Using Co-L_(2,3) and O-K x-ray absorption spectroscopy, we reveal that the charge ordering in La_(1.5)Sr_(0.5)CoO4 involves high spin (S=3/2) Co^2+ and low spin (S=0) Co^3+ ions. This provides evidence for the spin blockade phenomenon as a source for the extremely insulating nature of the La_(2-x)Sr_(x)CoO4 series. The associated e_g^2 and e_g^0 orbital occupation accounts for the large contrast in the Co-O bond lengths, and in turn, the high charge ordering temperature. Yet, the low magnetic ordering temperature is naturally explained by the presence of the non-magnetic (S=0) Co^3+ ions. From the identification of the bands we infer that La_(1.5)Sr_(0.5)CoO4 is a narrow band material.

cond-mat.str-el↗

arXiv2008

Low energy excitations in CoO studied by temperature dependent x-ray absorption spectroscopy

We have measured the intricate temperature dependence of the Co L2,3 x-ray absorption spectra (2p-3d excitations) of CoO. To allow for accurate total electron yield measurements, the material has been grown in thin film form on a metallic substrate in order to avoid charging problems usually encountered during electron spectroscopic studies on bulk CoO samples. The changes in spectra due to temperature are in good agreement with detailed ligand-field calculations indicating that these changes are mostly due to thermal population of closely lying excited states, originating from degenerate t2g levels lifted by the spin-orbit coupling. Magnetic coupling in the ordered phase, modeled as a mean-field exchange field, mixes in excited states inducing a tetragonal charge density. The spin-orbit coupling induced splitting of the low energy states results in a non-trivial temperature dependence for the magnetic susceptibility.

cond-mat.str-el↗

arXiv2008

Aligning spins in antiferromagnetic films using antiferromagnets

We have explored the possibility to orient spins in antiferromagnetic thin films with low magnetocrystalline anisotropy via the exchange coupling to adjacent antiferromagnetic films with high magnetocrystalline anisotropy. We have used MnO as a prototype for a system with negligible single-ion anisotropy. We were able to control its spin direction very effectively by growing it as a film on antiferromagnetic CoO films with different predetermined spin orientations. This result may pave the way for tailoring antiferromagnets with low magnetocrystalline anistropy for applications in exchange bias systems. Very detailed information concerning the exchange coupling and strain effects was obtained from the Mn $L_{2,3}$ soft x-ray absorption spectroscopy.

cond-mat.str-el↗