arXiv subjects

H. H. Klauss

Publications and source records attributed to H. H. Klauss.

8 recordsLinked to original sources

arXiv2026

The stripe state at 1/8 Ba doping hosts optimal superconductivity in La-214 cuprates under low in-plane stress

The cuprate system La$_{2-x}$Ba$_{x}$CuO$_{4}$ (LBCO) exhibits a pronounced sensitivity to in-plane uniaxial stress, particularly near the 1/8 doping anomaly, where stripe order strongly suppresses bulk superconductivity. While previous studies have focused on compositions close to 0.125, the commensurate $x$=0.125 phase remains largely unexplored under symmetry-selective lattice tuning. Here, we combine muon-spin rotation ($μ$SR), AC susceptibility, and electrical resistivity to investigate superconductivity, spin-stripe order, and structural response in LBCO-0.125 under in-plane uniaxial stress applied 45$^\circ$ to the Cu-O bond direction. Complementary resistivity measurements on $x$=0.115 and 0.135 track the evolution across both sides of the anomaly. We observe a giant enhancement of the bulk superconducting transition temperature in LBCO-0.125, increasing from 5 K to 37 K under 0.5 GPa. While the onset temperature of spin-stripe order decreases only modestly, the magnetic volume fraction is reduced by about a factor of two, with local order preserved. Simultaneously, the resistivity peak associated with the LTT phase is fully suppressed across all dopings. These results demonstrate that suppression of the LTT phase and reduction of the static spin-stripe-ordered volume fraction are crucial for the development of optimal three-dimensional superconductivity. Strikingly, the composition $x$=0.125, with the most robust stripe stability and the lowest ambient-pressure $T_{\rm c}$ develops the highest $T_{\rm c}$ under stress, reaching a zero-resistance state at 37 K and an onset of the superconducting transition as high as 46 K. This behavior indicates that stripe-related interactions enhance pairing strength, while static stripe order competes with superconductivity primarily at the level of phase coherence rather than pairing itself.

cond-mat.supr-con↗

arXiv2025

Distinct Uniaxial Stress and Pressure Fingerprint of Superconductivity in the 3D Kagome Lattice Compound CeRu2

The exploration of tunable superconductivity in strongly correlated electron systems is a central pursuit in condensed matter physics, with implications for both fundamental understanding and potential applications. The Laves phase CeRu$_{2}$, a pyrochlore compound, exhibits a three-dimensional (3D) Kagome lattice type geometry giving rise to flat bands and degenerate Dirac points, where band structure features intertwine with strong multi-orbital interaction effects deriving from its correlated electronic structure. Here, we combine muon spin rotation ($μ$SR), uniaxial in-plane stress, and hydrostatic pressure to probe the superconducting state of CeRu$_{2}$. Uniaxial stress up to 0.22 GPa induces a dome-shaped evolution of the critical temperature $T_{\rm c}$, with an initial plateau, successively followed by enhancement and suppression without any structural phase transition. Stress is further found to drive a crossover from anisotropic to isotropic $s$-wave pairing. In contrast, hydrostatic pressure up to 2.2 GPa leaves $T_{\rm c}$ largely unchanged but alters the superfluid density from exponential to linear behavior at low temperatures, indicative of nodal superconductivity under hydrostatic pressure. Taken together, these results indicate that CeRu$_{2}$ occupies an ideal position in parameter space, enabling highly responsive and multifold tunability of superconductivity in this three-dimensional correlated electronic system. This warrants further quantitative analysis of the interplay between lattice geometry, electronic correlations, and pairing symmetry.

cond-mat.supr-con↗

arXiv2025

Contrasting $c$-axis and in-plane uniaxial stress effects on superconductivity and stripe order in La$_{1.885}$Ba$_{0.115}$CuO$_4$

The cuprate superconductor La$_{2-x}$Ba$_x$CuO$_4$ (LBCO) near $x=0.125$ is a striking example of intertwined electronic orders, where 3D superconductivity is anomalously suppressed, allowing spin and charge stripe order to develop, in a manner consistent with the emergence of a pair-density-wave (PDW) state. Understanding this interplay remains a key challenge in cuprates, highlighting the necessity of external tuning for deeper insight. While in-plane (within the CuO plane) uniaxial stress enhances superconductivity and suppresses stripe order, the effects of $c$-axis compression (perpendicular to the CuO plane) remains largely unexplored. Here, we use muon spin rotation ($μ$SR) and AC susceptibility with an in situ piezoelectric stress device to investigate the spin-stripe order and superconductivity in LBCO-0.115 under $c$-axis compression. The measurements reveal a gradual suppression of the superconducting transition temperature ($T_{\rm c}$) with increasing $c$-axis stress, in stark contrast to the strong enhancement observed under in-plane stress. We further show that while in-plane stress rapidly reduces both the magnetic volume fraction ($V_{\rm m}$) and the spin-stripe ordering temperature ($T_{\rm so}$), $c$-axis compression has no effect, with $V_{\rm m}$ and $T_{\rm so}$ exhibiting an almost unchanged behavior up to the highest applied stress of 0.21 GPa. These findings demonstrate a strong anisotropy in stress response, underscoring the critical role of crystallographic anisotropy in governing competing electronic phases in LBCO.

cond-mat.supr-con↗

arXiv2019

Emerging superconductivity with broken time reversal symmetry inside a superconducting $s$-wave state

In general, magnetism and superconductivity are antagonistic to each other. However, there are several families of superconductors, in which superconductivity may coexist with magnetism, and only a few examples are known, when superconductivity itself induces spontaneous magnetism. The most known compounds are Sr$_2$RuO$_4$ and some noncentrosymmetric superconductors. Here, we report the finding of a narrow dome of a novel $s+is'$ superconducting (SC) phase with broken time-reversal symmetry (BTRS) inside the broad $s$-wave SC region of the centrosymmetric multiband superconductor Ba$_{\rm 1-x}$K$_{\rm x}$Fe$_2$As$_2$ ($0.7 \lesssim x \lesssim 0.85$). We observe spontaneous magnetic fields inside this dome using the muon spin relaxation ($μ$SR) technique. Furthermore, our detailed specific heat study reveals that the BTRS dome appears very close to a change in the topology of the Fermi surface (Lifshitz transition). With this, we experimentally demonstrate the emergence of a novel quantum state due to topological changes of the electronic system.

cond-mat.supr-con↗

arXiv2019

Dynamic magnetism in the disordered hexagonal double perovskite BaTi$_{1/2}$Mn$_{1/2}$O$_{3}$

Magnetic frustration and disorder are key ingredients to prevent the onset of magnetic order. In the disordered hexagonal double perovskite BaTi$_{1/2}$Mn$_{1/2}$O$_{3}$, Mn$^{4+}$ cations, with $S=3/2$ spins, can either form highly correlated states of magnetic trimers or dimers or remain as weakly interacting orphan spins. At low temperature ($T$), the dimer response is negligible, and magnetism is dominated by the trimers and orphans. To explore the role of magnetic frustration, disorder and possibly of quantum fluctuations, the low-$T$ magnetic properties of the remaining magnetic degrees of freedom of BaTi$_{1/2}$Mn$_{1/2}$O$_{3}$ are investigated. Heat-capacity data and magnetic susceptibility display no evidence for a phase transition to a magnetically ordered phase but indicate the formation of a correlated spin state. The low-temperature spin dynamics of this state is then explored by $μ$SR experiments. The zero field $μ^{+}$ relaxation rate data show no static magnetism down to $T=19$ mK and longitudinal field experiments support as well that dynamic magnetism persists at low $T$. Our results are interpreted in terms of a spin glass state which stems from a disordered lattice of orphans spins and trimers. A spin liquid state in BaTi$_{1/2}$Mn$_{1/2}$O$_{3}$, however, is not excluded and is also discussed.

cond-mat.str-el↗

arXiv2018

NaYbS$_2$ - a new planar spin-$\frac{1}{2}$ triangular-lattice magnet and putative spin liquid

Platelike high-quality NaYbS$_{2}$ rhombohedral single crystals with lateral dimensions of a few mm have been grown and investigated in great detail by bulk methods like magnetization and specific heat, but also by local probes like nuclear magnetic resonance (NMR), electron-spin resonance (ESR), muon-spin relaxation ($μ$SR), and inelastic neutron scattering (INS) over a wide field and temperature range. Our single-crystal studies clearly evidence a strongly anisotropic quasi-2D magnetism and an emerging spin-orbit entangled $S=1/2$ state of Yb towards low temperatures together with an absence of long-range magnetic order down to 260~mK. In particular, the clear and narrow Yb ESR lines together with narrow $^{23}$Na NMR lines evidence an absence of inherent structural distortions in the system, which is in strong contrast to the related spin-liquid candidate YbMgGaO$_{4}$ falling within the same space group $R\overline{3}m$. This identifies NaYbS$_{2}$ as a rather pure spin-1/2 triangular lattice magnet and a new putative quantum spin liquid.

cond-mat.str-el↗

arXiv2015

Solitonic spin-liquid state due to the violation of the Lifshitz condition in Fe$_{1+y}$Te

A combination of phenomenological analysis and Mössbauer spectroscopy experiments on the tetragonal Fe$_{1+y}$Te system indicates that the magnetic ordering transition in compounds with higher Fe-excess, $y\ge$ 0.11, is unconventional. Experimentally, a liquid-like magnetic precursor with quasi-static spin-order is found from significantly broadened Mössbauer spectra at temperatures above the antiferromagnetic transition. The incommensurate spin-density wave (SDW) order in Fe$_{1+y}$Te is described by a magnetic free energy that violates the weak Lifshitz condition in the Landau theory of second-order transitions. The presence of multiple Lifshitz invariants provides the mechanism to create multidimensional, twisted, and modulated solitonic phases.

cond-mat.supr-con↗

arXiv2008

Strong coupling between magnetic and structural order parameters in SrFe2As2

X-ray and Neutron diffraction as well as muon spin relaxation and Mössbauer experiments performed on SrFe$_2$As$_2$ polycrystalls confirm a sharp first order transition at $T_0 = 205$,K corresponding to an orthorhombic phase distortion and to a columnar antiferromagnetic Fe ordering with a propagation vector (1,0,1), and a larger distortion and larger size of the ordered moment than reported for BaFe$_2$As$_2$. The structural and the magnetic order parameters present an remarkable similarity in their temperature dependence from $T_0$ down to low temperatures, showing that both phenomena are intimately connected. Accordingly, the size of the ordered Fe moments scale with the lattice distortion when going from SrFe$_2$As$_2$ to BaFe$_2$As$_2$. Full-potential band structure calculations confirm that the columnar magnetic order and the orthorhombic lattice distortion are intrinsically tied to each other.

cond-mat.supr-con↗