arXiv subjects

H. Jang

Publications and source records attributed to H. Jang.

26 records · Page 2Linked to original sources

arXiv2015

Orbital Reconstruction in a Self-assembled Oxygen Vacancy Nanostructure

We demonstrate the microscopic role of oxygen vacancies spatially confined within nanometer inter-spacing (about 1 nm) in BiFeO3, using resonant soft X-ray scattering techniques and soft X-ray spectroscopy measurements. Such vacancy confinements and total number of vacancy are controlled by substitution of Ca2+ for Bi3+ cation. We found that by increasing the substitution, the in-plane orbital bands of Fe3+ cations are reconstructed without any redox reaction. It leads to a reduction of the hopping between Fe atoms, forming a localized valence band, in particular Fe 3d-electronic structure, around the Fermi level. This band localization causes to decrease the conductivity of the doped BiFeO3 system.

cond-mat.mtrl-sci↗

arXiv2015

Three-Dimensional Charge Density Wave Order in YBa2Cu3O6.67 at High Magnetic Fields

Charge density wave (CDW) correlations have recently been shown to universally exist in cuprate superconductors. However, their nature at high fields inferred from nuclear magnetic resonance is distinct from that measured by x-ray scattering at zero and low fields. Here we combine a pulsed magnet with an x-ray free electron laser to characterize the CDW in YBa2Cu3O6.67 via x-ray scattering in fields up to 28 Tesla. While the zero-field CDW order, which develops below T ~ 150 K, is essentially two-dimensional, at lower temperature and beyond 15 Tesla, another three-dimensionally ordered CDW emerges. The field-induced CDW onsets around the zero-field superconducting transition temperature, yet the incommensurate in-plane ordering vector is field-independent. This implies that the two forms of CDW and high-temperature superconductivity are intimately linked.

cond-mat.str-el↗

arXiv2015

Magnetic-field and doping dependence of low-energy spin fluctuations in the antiferroquadrupolar compound Ce(1-x)La(x)B(6)

CeB(6) is a model compound exhibiting antiferroquadrupolar (AFQ) order, its magnetic properties being typically interpreted within localized models. More recently, the observation of strong and sharp magnetic exciton modes forming in its antiferromagnetic (AFM) state at both ferromagnetic and AFQ wave vectors suggested a significant contribution of itinerant electrons to the spin dynamics. Here we investigate the evolution of the AFQ excitation upon the application of an external magnetic field and the substitution of Ce with non-magnetic La, both parameters known to suppress the AFM phase. We find that the exciton energy decreases proportionally to T_N upon doping. In field, its intensity is suppressed, while its energy remains constant. Its disappearance above the critical field of the AFM phase is preceded by the formation of two modes, whose energies grow linearly with magnetic field upon entering the AFQ phase. These findings suggest a crossover from itinerant to localized spin dynamics between the two phases, the coupling to heavy-fermion quasiparticles being crucial for a comprehensive description of the magnon spectrum.

cond-mat.str-el↗

arXiv2013

Intense low-energy ferromagnetic fluctuations in the antiferromagnetic heavy-fermion metal CeB6

Heavy-fermion metals exhibit a plethora of low-temperature ordering phenomena, among them the so-called hidden-order phases that in contrast to conventional magnetic order are invisible to standard neutron diffraction. One of the oldest and structurally simplest hidden-order compounds, CeB6, became famous for an elusive phase that was attributed to the antiferroquadrupolar ordering of cerium-4f moments. In its ground state, CeB6 also develops a more usual antiferromagnetic (AFM) order. Hence, its essential low-temperature physics was always considered to be solely governed by AFM interactions between the dipolar and multipolar Ce moments. Here we overturn this established perspective by uncovering an intense ferromagnetic (FM) low-energy collective mode that dominates the magnetic excitation spectrum of CeB6. Our inelastic neutron-scattering data reveal that the intensity of this FM excitation by far exceeds that of conventional spin-wave magnons emanating from the AFM wave vectors, thus placing CeB6 much closer to a FM instability than could be anticipated. This propensity of CeB6 to ferromagnetism may account for much of its unexplained behavior, such as the existence of a pronounced electron spin resonance, and should lead to a substantial revision of existing theories that have so far largely neglected the role of FM interactions.

cond-mat.str-el↗

arXiv2011

Interfacial nanostructure induced spin-reorientation transition in Ni/Fe/Ni/W(110)

We investigated the mechanism of the spin-reorientation transition (SRT) in the Ni/Fe/Ni/W(110) system using in situ low-energy electron microscopy, x-ray magnetic circular dichroism measurements, and first principles electronic structure calculations. We discovered that the growth of Fe on a flat Ni film on a W (110) crystal resulted in the formation of nanosized particles, instead of a uniform monolayer of Fe as commonly assumed. This interfacial nanostructure leads to a change of the system's dimensionality from two dimensional- to three dimensional-like, which simultaneously weakens the dipolar interaction and enhances the spin-orbit coupling in the system and drives the observed SRT.

cond-mat.mtrl-sci↗

arXiv2004

Panorama of Nodal Superconductors

Since 1979, many new classes of superconductors have been discovered, including heavy-fermion compounds, organic conductors, high-Tc cuprates, and Sr2RuO4. Most of these superconductors are unconventional and/or nodal. Therefore it is of central importance to determine the symmetry of the order parameter in each of these superconductors. In particular, the angular-controlled thermal conductivity in the vortex state provides a unique means of investigating the nodal structure of the superconducting energy gap when high-quality single crystals in the extremely clean limit are available. Using this method, Izawa et al have recently succeeded in identifying the energy gap symmetry of superconductivity in Sr2RuO4, CeCoIn5, kappa-(ET)2Cu(NCS)2, YNi2B2C, and PrOs4Sb12.

cond-mat.supr-con↗

arXiv2003

Electronic Raman Spectra of Superconducting Borocarbides

Recently we have proposed a s+g-wave model for the superconductivity in borocarbides, YNi2B2C and LuNi2B2C. In the present paper we first summarize thermodynamic properties of s+g-wave model. Then we shall analyse the recent Raman spectra data of RNi2B2C (with R=Lu and Y) by Yang et al. The present model appears to describe salient features of the Raman spectra.

cond-mat.supr-con↗

arXiv1999

Paramagnetic state in d-wave Superconductors

We study theoretically the paramagnetic state in d-wave superconductors. We present the specific heat, the magnetization, superfluid density obtained within the weak-coupling model. At low temperatures and for small magnetic fields they exhibit simple power law behaviors, which should be accessible experimentally in hole-doped high-T_c cuprates and κ-(ET)_2 salts in a magnetic field within the conducting plane.

cond-mat.supr-con↗