arXiv subjects

H. Keller

Publications and source records attributed to H. Keller.

At least 37 records · Page 2Linked to original sources

arXiv2013

Lattice and polarizability mediated spin activity in EuTiO_3

EuTiO_3 is shown to exhibit novel strong spin-charge-lattice coupling deep in the paramagnetic phase. Its existence is evidenced by an, until now, unknown response of the paramagnetic susceptibility at temperatures exceeding the structural phase transition temperature T_S = 282K. The "extra" features in the susceptibility follow the rotational soft zone boundary mode temperature dependence above and below T_S. The theoretical modeling consistently reproduces this behavior and provides reasoning for the stabilization of the soft optic mode other than quantum fluctuations.

cond-mat.mtrl-sci↗

arXiv2013

Nonlinear pressure dependence of T_N in almost multiferroic EuTiO_3

The antiferromagnetic (AFM) phase transition temperature T_N of EuTiO_3 has been studied as a function of pressure p. The data reveal a nonlinear dependence of T_N on p with T_N increasing with increasing pressure. The exchange interactions exhibit an analogous dependence on p as T_N (if the absolute value of the nearest neighbor interaction is considered) and there is evidence that the AFM transition is robust with increasing pressure. The corresponding Weiss temperature Θ_W remains anomalous since it always exhibits positive values. The data are analyzed within the Bloch power law model and provide excellent agreement with experiment.

cond-mat.mtrl-sci↗

arXiv2013

Magnetic phase diagram of low-doped La{2-x}SrxCuO4 thin films studied by low-energy muon-spin rotation

The magnetic phase diagram of La2-xSrxCuO4 thin-films grown on single-crystal LaSrAlO4 substrates has been determined by low-energy muon-spin rotation. The diagram shows the same features as the one of bulk La2-xSrxCuO4, but the transition temperatures between distinct magnetic states are significantly different. In the antiferromagnetic phase the Neel temperature TN is strongly reduced, and no hole spin freezing is observed at low temperatures. In the disordered magnetic phase (x>0.02) the transition temperature to the cluster spin-glass state Tg is enhanced. Possible reasons for the pronounced differences between the magnetic phase diagrams of thin-film and bulk samples are discussed.

cond-mat.mtrl-sci↗

arXiv2013

Effect of pressure on the Cu and Pr magnetism in Nd(1-x)Pr(x)Ba2Cu3O7 investigated by muon spin rotation

The effect of pressure on the copper and praseodymium magnetic order in the system Nd(1-x)$Pr(x)Ba2Cu3$O7 with x=0.3, 0.5, 0.7, and 1 was investigated by means of the muon spin rotation (muSR) technique. It was found that the effect of pressure on the Neel temperatures of both copper and praseodymium is positive for the whole range of Pr concentrations (0.3<x<1) studied. These findings are in contrast with a number of previous reports and clarify some of the puzzles related to the effect of pressure on superconductivity and magnetism in the praseodymium-substituted R}(1-x)$Pr(x)Ba2Cu3O7 systems, where R is a rare earth element.

cond-mat.supr-con↗

arXiv2013

Muon-spin rotation and magnetization studies of chemical and hydrostatic pressure effects in EuFe_{2}(As_{1-x}P_{x})_{2}

The magnetic phase diagram of EuFe$_{2}$(As$_{1-x}$P$_{x}$)$_{2}$ was investigated by means of magnetization and muon-spin rotation studies as a function of chemical (isovalent substitution of As by P) and hydrostatic pressure. The magnetic phase diagrams of the magnetic ordering of the Eu and Fe spins with respect to P content and hydrostatic pressure are determined and discussed. The present investigations reveal that the magnetic coupling between the Eu and the Fe sublattices strongly depends on chemical and hydrostatic pressure. It is found that chemical and hydrostatic pressure have a similar effect on the Eu and Fe magnetic order.

cond-mat.supr-con↗

arXiv2013

Tuning the structural instability of SrTiO_3 by Eu doping: The phase diagram of Sr_1-xEu_xTiO_3

The phase diagram of Sr_1-xEu_xTiO_3 is determined experimentally by electron paramagnetic resonance and resistivity measurements and analyzed theoretically within the self-consistent phonon approximation as a function of x ([0.03-1.0]). The transition temperature of the structural instability of the system increases nonlinearly to higher temperatures with increasing x. This is interpreted theoretically by a substantial alteration in the dynamics caused by a change in the double-well potential from broad and shallow to narrow and deep.

cond-mat.mtrl-sci↗

arXiv2012

Strong pressure dependence of the magnetic penetration depth in single crystals of the heavy fermion superconductor CeCoIn5 studied by muon spin rotation

In the tetragonal heavy fermion system CeCoIn5 the unconventional superconducting state is probed by means of muon spin rotation. The pressure dependence (0-1 GPa) of the basal-plane magnetic penetration depth (λ_a), the penetration depth anisotropy (γ=λ_c/λ_a) and the temperature dependence of 1/λ_i^2 (i=a,c) were studied in single crystals. A strong decrease of λ_a with pressure was observed, while γand λ_i^2(0)/λ_i^2(T) are pressure independent. A linear relationship between 1/λ_a^2(270 mK) and Tc was also found. The large decrease of λ_a with pressure is the signature of an increase of the number of superconducting quasiparticles by a factor of about 2.

cond-mat.supr-con↗

arXiv2012

Superconductivity and magnetism in RbxFe2-ySe2: Impact of thermal treatment on mesoscopic phase separation

An extended study of the superconducting and normal-state properties of various as-grown and post-annealed RbxFe2-ySe2 single crystals is presented. Magnetization experiments evidence that annealing of RbxFe2-ySe2 at 413 K, well below the onset of phase separation Tp=489 K, neither changes the magnetic nor the superconducting properties of the crystals. In addition, annealing at 563 K, well above Tp, suppresses the superconducting transition temperature Tc and leads to an increase of the antiferromagnetic susceptibility accompanied by the creation of ferromagnetic impurity phases, which are developing with annealing time. However, annealing at T=488K=Tp increases Tc up to 33.3 K, sharpens the superconducting transition, increases the lower critical field, and strengthens the screening efficiency of the applied magnetic field. Resistivity measurements of the as-grown and optimally annealed samples reveal an increase of the upper critical field along both crystallographic directions as well as its anisotropy. Muon spin rotation and scanning transmission electron microscopy experiments suggest the coexistence of two phases below Tp: a magnetic majority phase of Rb2Fe4Se5 and a non-magnetic minority phase of Rb0.5Fe2Se2. Both microscopic techniques indicate that annealing the specimens just at Tp does not affect the volume fraction of the two phases, although the magnetic field distribution in the samples changes substantially. This suggests that the microstructure of the sample, caused by mesoscopic phase separation, is modified by annealing just at Tp, leading to an improvement of the superconducting properties of RbxFe2-ySe2 and an enhancement of Tc.

cond-mat.supr-con↗

arXiv2012

Pressure induced ferromagnetism in antiferromagnetic Fe_1.03Te

The magnetic properties of Fe1.03Te under hydrostatic pressure up to p ~ 5.7 GPa were investigated by means of muon spin rotation, dc magnetization, and neutron depolarization measurements. With increasing pressure the antiferromagnetic ordering temperature TN decreases continuously from 70 K at ambient pressure towards higher pressures. Surprisingly, the commensurate antiferromagnetic order of FeTe enters a region of incommensurate and dynamical magnetic order before at p ~ 1.7 GPa the system turns ferromagnetic. The ferromagnetic ordering temperature TC increases with increasing pressure.

cond-mat.supr-con↗

arXiv2012

Vortex lock-in transition coinciding with the 3D to 2D crossover in YBa2Cu3O7

A vortex lock-in transition was directly detected by torque magnetometry in an overdoped YBa2Cu3O7 single crystal of low anisotropy (\approx 7). The locked-in state was observed below the 3D to 2D crossover temperature Tcr = 76 K, independently of extrinsic pinning effects thanks to a high quality clean crystal and the use of a vortex shaking technique. The shape of the torque signal as a function of the angle between the applied magnetic field and the crystallographic c-axis is in very good agreement with the model developped by Feinberg and Ettouhami [Int. J. Mod. Phys. B 7, 2085 (1993)] for quasi-2D superconductors, despite the low anisotropy of the material.

cond-mat.supr-con↗

arXiv2012

Magnetic field enhanced structural instability in EuTiO_{3}

EuTiO_{3} undergoes a structural phase transition from cubic to tetragonal at T_S = 282 K which is not accompanied by any long range magnetic order. However, it is related to the oxygen ocathedra rotation driven by a zone boundary acoustic mode softening. Here we show that this displacive second order structural phase transition can be shifted to higher temperatures by the application of an external magnetic field (increased by 4 K for mu_{0}H = 9 T). This observed field dependence is in agreement with theoretical predictions based on a coupled spin-anharmonic-phonon interaction model.

cond-mat.mtrl-sci↗

arXiv2012

Hybrid paramagnon phonon modes at elevated temperatures in EuTiO3

EuTiO3 (ETO) has recently experienced an enormous revival of interest because of its possible multiferroic properties which are currently in the focus of research. Unfortunately ETO is an unlikely candidate for enlarged multifunctionality since the mode softening - typical for ferroelectrics - remains incomplete, and the antiferromagnetic properties appear at 5.5K only. However, a strong coupling between lattice and Eu spins exists and leads to the appearance of a magnon-phonon-hybrid mode at elevated temperatures as evidenced by electron paramagnetic resonance (EPR), muon spin rotation (μSR) experiments and model predictions based on a coupled spin-polarizability Hamiltonian. This novel finding supports the notion of strong magneto-dielectric (MD) effects being realized in ETO and opens new strategies in material design and technological applications.

cond-mat.mtrl-sci↗

arXiv2012

Magneto-Electric Coupling in Single Crystal Cu2OSeO3 Studied by a Novel Electron Spin Resonance Technique

The magneto-electric (ME) coupling on spin-wave resonances in single-crystal Cu2OSeO3 was studied by a novel technique using electron spin resonance combined with electric field modulation. An external electric field E induces a magnetic field component μ_0 H^i = γE along the applied magnetic field H with γ=0.7(1) μT/(V/mm) at 10 K. We found that ME coupling strength γis temperature dependent and highly anisotropic. γ(T) nearly follows that of spin susceptibility J(T) and rapidly decreases above the Curie temperature Tc. The ratio γ/J monotonically decreases with increasing temperature without an anomaly at Tc.

cond-mat.str-el↗

arXiv2012

Magnetic-field tuned anisotropy in superconducting Rb(x)Fe(2-y)Se(2)

The anisotropic superconducting properties of a Rb(x)Fe(2-y)Se(2) single crystal with transition temperature 32 K were investigated by means of SQUID and torque magnetometry, probing the effective magnetic penetration depth and the magnetic penetration depth anisotropy. Interestingly, the anisotropy is found to be temperature independent in the superconducting state, but strongly field dependent. This unusual anisotropic behavior, together with a large zero-temperature effective magnetic penetration depth is possibly related to a superconducting state heavily biased by the coexisting antiferromagnetic phase.

cond-mat.supr-con↗

arXiv2012

Magnetism, superconductivity and coupling in cuprate heterostructures probed by low-energy muon-spin rotation

We present a low-energy muon-spin-rotation study of the magnetic and superconducting properties of YBa2Cu3O7/PrBa2Cu3O7 trilayer and bilayer heterostructures. By determining the magnetic-field profiles throughout these structures we show that a finite superfluid density can be induced in otherwise semiconducting PrBa2Cu3O7 layers when juxtaposed to YBa2Cu3O7 "electrodes" while the intrinsic antiferromagnetic order is unaffected.

cond-mat.supr-con↗

arXiv2011

Coexistence of Superconductivity and Magnetism in FeSe_1-x under Pressure

An extended investigation of the electronic phase diagram of FeSe$_{1-x}$ up to pressures of $p\simeq2.4$\,GPa by means of ac and dc magnetization, zero field muon spin rotation (ZF $μ$SR), and neutron diffraction is presented. ZF $μ$SR indicates that at pressures $p\geq0.8$\,GPa static magnetic order occurs in FeSe$_{1-x}$ and occupies the full sample volume for $p\gtrsim 1.2$\,GPa. ac magnetization measurements reveal that the superconducting volume fraction stays close to 100% up to the highest pressure investigated. In addition, above $p\geq1.2$\,GPa both the superconducting transition temperature $T_{\rm c}$ and the magnetic ordering temperature $T_{\rm N}$ increase simultaneously, and both superconductivity and magnetism are stabilized with increasing pressure. Calculations indicate only one possible muon stopping site in FeSe$_{1-x}$, located on the line connecting the Se atoms along the $c$-direction. Different magnetic structures are proposed and checked by combining the muon stopping calculations with a symmetry analysis, leading to a similar structure as in the LaFeAsO family of Fe-based superconductors. Furthermore, it is shown that the magnetic moment is pressure dependent and with a rather small value of $μ\approx 0.2\,μ_B$ at $p\simeq2.4$\,GPa.

cond-mat.supr-con↗

arXiv2011

Study of the anisotropic magnetic order of the Eu sublattice in single crystals of EuFe_2-xCo_xAs_2 (x = 0, 0.2) by means of magnetization and magnetic torque

Here, we present a combination of magnetization and magnetic torque experiments to investigate the magnetic orders in undoped EuFe2As2 and Co doped EuFe1.8Co0.2As2 single crystals. Although at low temperatures typical results for an antiferromagnetic (AFM) state in EuFe2As2 were found, our data strongly indicate the occurrence of a canted antiferromagnetic (C-AFM) order of the Eu2+ moments between 17 K and 19 K, observed even in the lowest studied magnetic fields. However, unlike in the parent compound, no low-field and low-temperature AFM state of the Eu^2+ moments was observed in the doped EuFe1.8Co0.2As2. Only a C-AFM phase is present at low fields and low temperatures, with a reduced magnetic anisotropy as compared to the undoped system. We present and discuss for both, EuFe2As2 and EuFe1.8Co0.2As2, the experimentally deduced magnetic phase diagrams of the magnetic ordering of the Eu^2+ sublattice with respect to the temperature, the applied magnetic field, and its orientation to the crystallographic axes. It is likely that the magnetic coupling of the Eu and the Fe sublattice is strongly depending on Co doping, having detrimental influence on the magnetic phase diagrams as determined in this work. Their impact on the occurrence of superconductivity with higher Co doping is discussed.

cond-mat.supr-con↗

arXiv2011

Production and characterization of a custom-made 228Th source with reduced neutron source strength for the Borexino experiment

A custom-made 228Th source of several MBq activity was produced for the Borexino experiment for studying the external background of the detector. The aim was to reduce the unwanted neutron emission produced via (alpha,n) reactions in ceramics used typically for commercial 228Th sources. For this purpose a ThCl4 solution was converted chemically into ThO2 and embedded into a gold foil. The paper describes the production and the characterization of the custom-made source by means of gamma-activity, dose rate and neutron source strength measurements. From gamma-spectroscopic measurements it was deduced that the activity transfer from the initial solution to the final source was >91% (at 68% C.L.) and the final activity was (5.41+-0.30) MBq. The dose rate was measured by two dosimeters yielding 12.1 mSv/h and 14.3 mSv/h in 1 cm distance. The neutron source strength of the 5.41 MBq 228Th source was determined as (6.59+-0.85)/sec.

physics.ins-det↗