arXiv subjects

H. Kimura

Publications and source records attributed to H. Kimura.

At least 19 recordsLinked to original sources

arXiv2024

Magnetic structure of the noncentrosymmetric magnet Sr2MnSi2O7 through irreducible representation and magnetic space group analyses

Magnetic structures of the noncentrosymmetric magnet Sr$_2$MnSi$_2$O$_7$ were examined through neutron diffraction for powder and single-crystalline samples, as well as magnetometry measurements. All allowed magnetic structures under the space group $P\bar{4}2_1 m$ with the magnetic wavevector $\vec{q}_{\rm m}=(0,0,1/2)$~r.l.u., were analysed via irreducible representation and magnetic space group approaches. The compound is refined to have in-plane magnetic moments within the magnetic space group $Cmc2_1.1^{\prime}_c$ (\#36.177) under zero field, which can be altered to $P2_1 2_1 2_1.1^{\prime}_c$ (\#19.28) above $μ_0 H=0.067(5)$~T to align induced weak-ferromagnetic components within one layer on the $ab$-plane. All refined parameters are provided following the recent framework based upon the magnetic space group, which better conveys when exchanging crystallographic information for commensurate magnetic structures.

cond-mat.str-el↗

arXiv2020

Electronic charge transfer driven by spin cycloidal structure

Muon spin rotation and resonant soft X-ray scattering experiments on prototype multiferroics RMn2O5 (R = Y, Sm) are used to demonstrate that the local electric displacements are driven by the spin-current (SC) mechanism. Small local electric displacements were evaluated by observing spin polarization at ligand O ions, for which implanted muons served as an extremely sensitive probe. Our results for YMn2O5 provide evidence that the spin polarization of O ions forming a spin cycloid chain with Mn spins increases in proportion to the vector spin chirality (Si x Sj ) of the Mn ions. This relationship strongly indicates that the charge transfer between O and Mn ions is driven by the SC mechanism, which leads to the ferroelectricity accompanying O spin polarization.

cond-mat.str-el↗

arXiv2016

Proton-proton correlations in distinguishing the two-proton emission mechanism of $^{23}$Al and $^{22}$Mg

The proton-proton momentum correlation functions ($C_{pp}(q)$) for kinematically complete decay channels of $^{23}$Al $\rightarrow$ p + p + $^{21}$Na and $^{22}$Mg $\rightarrow$ p + p + $^{20}$Ne have been measured at the RIKEN RI Beam Factory. From the very different correlation strength of $C_{pp}(q)$ for $^{23}$Al and $^{22}$Mg, the source size and emission time information were extracted from the $C_{pp}(q)$ data by assuming a Gaussian source profile in the correlation function calculation code (CRAB). The results indicated that the mechanism of two-proton emission from $^{23}$Al was mainly sequential emission, while that of $^{22}$Mg was mainly three-body simultaneous emission. By combining our earlier results of the two-proton relative momentum and the opening angle, it is pointed out that the mechanism of two-proton emission could be distinguished clearly.

nucl-ex↗

arXiv2015

High-energy magnetic excitations in overdoped La$_{2-x}$Sr$_{x}$CuO$_{4}$ studied by neutron and resonant inelastic X-ray scattering

We have performed neutron inelastic scattering and resonant inelastic X-ray scattering (RIXS) at the Cu-$L_3$ edge to study high-energy magnetic excitations at energy transfers of more than 100 meV for overdoped La$_{2-x}$Sr$_{x}$CuO$_{4}$ with $x=0.25$ ($T_c=15$ K) and $x=0.30$ (non-superconducting) using identical single crystal samples for the two techniques. From constant-energy slices of neutron scattering cross-sections, we have identified magnetic excitations up to ~250 meV for $x=0.25$. Although the width in the momentum direction is large, the peak positions along the (pi, pi) direction agree with the dispersion relation of the spin-wave in the non-doped La$_{2}$CuO$_{4}$ (LCO), which is consistent with the previous RIXS results of cuprate superconductors. Using RIXS at the Cu-$L_3$ edge, we have measured the dispersion relations of the so-called paramagnon mode along both (pi, pi) and (pi, 0) directions. Although in both directions the neutron and RIXS data connect with each other and the paramagnon along (pi, 0) agrees well with the LCO spin-wave dispersion, the paramagnon in the (pi, pi) direction probed by RIXS appears to be less dispersive and the excitation energy is lower than the spin-wave of LCO near (pi/2, pi/2). Thus, our results indicate consistency between neutron inelastic scattering and RIXS, and elucidate the entire magnetic excitation in the (pi, pi) direction by the complementary use of two probes. The polarization dependence of the RIXS profiles indicates that appreciable charge excitations exist in the same energy range of magnetic excitations, reflecting the itinerant character of the overdoped sample. A possible anisotropy in the charge excitation intensity might explain the apparent differences in the paramagnon dispersion in the (pi, pi) direction as detected by the X-ray scattering.

cond-mat.supr-con↗

arXiv2015

Different mechanism of two-proton emission from proton-rich nuclei $^{23}$Al and $^{22}$Mg

Two-proton relative momentum ($q_{pp}$) and opening angle ($θ_{pp}$) distributions from the three-body decay of two excited proton-rich nuclei, namely $^{23}$Al $\rightarrow$ p + p + $^{21}$Na and $^{22}$Mg $\rightarrow$ p + p + $^{20}$Ne, have been measured with the projectile fragment separator (RIPS) at the RIKEN RI Beam Factory. An evident peak at $q_{pp}\sim20$ MeV/c as well as a peak in $θ_{pp}$ around 30$^\circ$ are seen in the two-proton break-up channel from a highly-excited $^{22}$Mg. In contrast, such peaks are absent for the $^{23}$Al case. It is concluded that the two-proton emission mechanism of excited $^{22}$Mg is quite different from the $^{23}$Al case, with the former having a favorable diproton emission component at a highly excited state and the latter dominated by the sequential decay process.

nucl-ex↗

arXiv2013

Role of magnetic chirality in polarization flip upon commensurate-incommensurate magnetic phase transition in YMn$_{2}$O$_{5}$

We have performed simultaneous measurements of magnetic chirality by using polarized neutrons and electric polarization along the b-axis of single crystals of YMn$^{4+}$(Mn$_{1-x}$Ga$_{x}$)$^{3+}$O$_{5}$ with $x=0.047$ and 0.12, in which nonmagnetic Ga-ions dilute Mn$^{3+}$ spins. The $x=0.047$ sample exhibits high-temperature incommensurate (HT-ICM), commensurate (CM), and low-temperature incommensurate (LT-ICM) magnetic phases in order of decreasing temperature, whereas the $x=0.12$ sample exhibits only HT-ICM and LT-ICM phases. Here, the CM and LT-ICM phases are ferroelectric and weak-ferroelectric, respectively. Measurements conducted under zero field heating after various field-cooling conditions evidence that the microscopic mechanisms of the spin-driven ferroelectricity in the CM and LT-ICM phases are different: the magnetic chirality of Mn$^{4+}$ cycloidal spins plays a dominant role in the LT-ICM phase, whereas the magnetic exchange striction by the Mn$^{4+}$-Mn$^{3+}$ chain plays a dominant role in the CM phase. The polarization of YMn$_{2}$O$_{5}$ flips upon CM to LT-ICM phase transition because the ferroelectricity driven by the magnetic chirality and the exchange striction provides opposite directions of polarization.

cond-mat.mtrl-sci↗

arXiv2013

Negative magnetostrictive magnetoelectric coupling of BiFeO3

How the magnetoelectric coupling actually occurs on a microscopic level in multiferroic BiFeO3 is not well known. By using the high-resolution single crystal neutron diffraction techniques, we have determined the electric polarization of each individual elements of BiFeO3, and concluded that the magnetostrictive coupling suppresses the electric polarization at the Fe site below TN. This negative magnetoelectric coupling appears to outweigh the spin current contributions arising from the cycloid spin structure, which should produce a positive magnetoelectric coupling.

cond-mat.str-el↗

arXiv2013

Resonant inelastic X-ray scattering study of intra-band charge excitations in hole-doped high-Tc cuprates

We have performed resonant inelastic x-ray scattering (RIXS) near the Cu-K edge on cuprate superconductors La(2-x)Sr(x)CuO(4), La(2-x)Ba(x)CuO(4), La(2-x)Sr(x)Cu(1-y)Fe(y)O(4) and Bi(1.76)Pb(0.35)Sr(1.89)CuO(6+d), covering underdoped to heavily overdoped regime and focusing on charge excitations inside the charge-transfer gap. RIXS measurements of the 214 systems with Ei = 8.993 keV have revealed that the RIXS intensity at 1 eV energy transfer has a minimum at (0,0) and maxima at (0.4pi, 0) and $(0, 0.4pi) for all doping points regardless of the stripe ordered state, suggesting that the corresponding structure is not directly related to stripe order. Measurements with Ei = 9.003 keV on metallic La(1.7)Sr(0.3)CuO(4) and Bi(1.76)Pb(0.35)Sr(1.89)CuO(6+d) exhibit a dispersive intra-band excitation below 4 eV, similar to that observed in the electron-doped Nd(1.85)Ce(0.15)CuO(4). This is the first observation of a dispersive intra-band excitation in a hole doped system, evidencing that both electron and hole doped systems have a similar dynamical charge correlation function.

cond-mat.supr-con↗

arXiv2012

Modified Cross-Correlation for Efficient White-Beam Inelastic Neutron Scattering Spectroscopy

We describe a method of white-beam inelastic neutron scattering for improved measurement efficiency. The method consists of matrix inversion and selective extraction. The former is to resolve each incident energy component from the white-beam data, and the latter eliminates contamination by elastic components, which produce strong backgrounds that otherwise obfuscate the inelastic scattering components. In this method, the optimal experimental condition to obtain high efficiency will strongly depend on the specific aim of the individual experiments.

cond-mat.mtrl-sci↗

arXiv2009

Comet dust as a mixture of aggregates and solid particles: model consistent with ground-based and space-mission results

The most successful model of comet dust presents comet particles as aggregates of submicron grains. It qualitatively explains the spectral and angular change in the comet brightness and polarization and is consistent with the thermal infrared data and composition of the comet dust obtained {\it in situ} for comet 1P/Halley. However, it experiences some difficulties in providing a quantitative fit to the observational data. Here we present a model that considers comet dust as a mixture of aggregates and compact particles. The model is based on the Giotto and Stardust mission findings that both aggregates (made mainly of organics, silicates, and carbon) and solid silicate particles are present in the comet dust. We simulate aggregates as {\bf Ballistic Cluster-Cluster Aggregates (BCCA)} and compact particles as polydisperse spheroids with some distribution of the aspect ratio. The particles follow a power-law size distribution with the power -3 that is close to the one obtained for comet dust {\it in situ}, at studies of the Stardust returned samples, and the results of ground-based observations of comets. The model provides a good fit to the angular polarization curve. It also reproduces the positive spectral gradient of polarization, red color of the dust, and {\bf low albedo. It also has the ratio of compact to fluffy particles close to the one found {\it in situ} for comet 1P/Halley} and the mass ratio of silicate to carbonaceous materials equal to unity that is in accordance with the elemental abundances of Halley's dust found by Giotto mission.

astro-ph.EP↗

arXiv2009

Renormalization of Commensurate Magnetic Peak in Ni-doped La$_{1.85}$Sr$_{0.15}$CuO$_{4}$

We have studied the magnetic excitations in impurity doped La$_{1.85}$Sr$_{0.15}$Cu$_{1-y}$A$_{y}$O$_{4}$ (A=Ni or Zn) by neutron scattering. The dispersion for Zn:$y=0.017$ is similar to that for the impurity free sample: incommensurate peaks with the incommensurability $δ=0.12\pm0.01$ (rlu) do not change their positions up to 21 meV. On the other hand, for Ni:$y=0.029$, two incommensurate peaks observed at low energies suddenly change into a broad commensurate peak at $E_\mathrm{cross}=15$ meV. Compared to the impurity free sample with a similar Sr-concentration $x=0.16$, [B. Vignolle {\it et al.} Nature Physics {\bf 3} (2007) 163], $E_\mathrm{cross}$ for Ni:$y=0.029$ is decreased by nearly the same factor for the reduction in $T_{c}$. This is very similar to the shift of the resonance energy ($E_\mathrm{res}$) in Ni-doped YBa$_{2}$Cu$_{3}$O$_{7}$.[Y. Sidis {\it et al.}: Phys. Rev. Lett. {\bf 84} (2000) 5900]. These common impurity effects on the shift of $E_\mathrm{cross}$ and $E_\mathrm{res}$ suggest the same magnetic origin for the resonance peak in YBa$_{2}$Cu$_{3}$O$_δ$ and that for a crossing point of upward and downward dispersions in the La$_{2-x}$Sr$_{x}$CuO$_{4}$. We propose that the sudden change in the dispersion is better described by a crossover from incommensurate spin fluctuations to a gapped spin wave rather than a hourglass-like dispersion.

cond-mat.supr-con↗

arXiv2009

Spin chirality and electric polarization in multiferroic compounds $R$Mn$_2$O$_5$ ($R=$Ho, Er)

Polarized neutron diffraction experiments have been performed on multiferroic materials $R$Mn$_{2}$O$_{5}$ ($R=$Ho, Er) under electric fields in the ferroelectric commensurate (CM) and the low-temperature incommensurate (LT-ICM) phases, where the former has the highest electric polarization and the latter has reduced polarization. It is found that, after cooling in electric fields down to the CM phase, the magnetic chirality is proportional to the electric polarization. Also we confirmed that the magnetic chirality can be switched by the polarity of the electric polarization in both the CM and LT-ICM phases. These facts suggest an intimate coupling between the magnetic chirality and the electric polarization. However, upon the transition from the CM to LT-ICM phase, the reduction of the electric polarization is not accompanied by any reduction of the magnetic chirality, implying that the CM and LT-ICM phases contain different mechanisms of the magnetoelectric coupling.

cond-mat.str-el↗

arXiv2008

Optical probe of carrier doping by X-ray irradiation in organic dimer Mott insulator $κ$-(BEDT-TTF)$_{2}$Cu[N(CN)$_{2}]$Cl

We investigated the infrared optical spectra of an organic dimer Mott insulator $κ$-(BEDT-TTF)$_{2}$Cu[N(CN)$_{2}$]Cl, which was irradiated with X-rays. We observed that the irradiation caused a large spectral weight transfer from the mid-infrared region, where interband transitions in the dimer and Mott-Hubbard bands take place, to a Drude part in a low-energy region; this caused the Mott gap to collapse. The increase of the Drude part indicates a carrier doping into the Mott insulator due to irradiation defects. The strong redistribution of the spectral weight demonstrates that the organic Mott insulator is very close to the phase border of the bandwidth-controlled Mott transition.

cond-mat.str-el↗

arXiv2008

Charge excitations associated with charge stripe order in the 214-type nickelate and superconducting cuprate

Charge excitations were studied for stipe-ordered 214 compounds, La$_{5/3}$Sr$_{1/3}$NiO$_{4}$ and 1/8-doped La$_{2}$(Ba, Sr)$_{x}$CuO$_{4}$ using resonant inelastic x-ray scattering in hard x-ray regime. We have observed charge excitations at the energy transfer of 1 eV with the momentum transfer corresponding to the charge stripe spatial period both for the diagonal (nikelate) and parallel (cuprates) stripes. These new excitations can be interpreted as a collective stripe excitation or charge excitonic mode to a stripe-related in-gap state.

cond-mat.str-el↗

arXiv2008

Complex Spin Structures and Origin of the Magneto-Electric Coupling in YMn2O5

By combining neutron four-circle diffraction and polarized neutron diffraction techniques we have determined the complex spin structures of a multiferroic, YMn2O5, that exhibits two ferroelectric phases at low temperatures. The obtained magnetic structure has spiral components in both the low temperature ferroelectric phases that are magnetically commensurate and incommensurate, respectively. Among proposed microscopic theories for the magneto-electric coupling, our results are consistent with both the spin-current model that requires a magnetic transverse (cycloidal) spiral structure in order to induce a spontaneous electric polarization and the magneto-restriction model. Our results also explain why the electric polarization changes at the commensurate-to-incommensurate phase transition.

cond-mat.str-el↗

arXiv2007

Two different evolutionary types of comets proved by polarimetric and infrared properties of their dust

Comets can be divided into two groups: type I, characterized by high gas/dust ratio, low polarization, and a weak or absent 10 micron silicate feature, and type II, for which a low gas/dust ratio, high polarization, and strong silicate feature are typical. We show that the low polarization is the apparent result of depolarization by gas contamination at low dust concentration, which, in turn, results from the dust in type I comets being concentrated near the nucleus. The simulations of thermal emission show that for more porous particles (BCCA), the silicate feature is more pronounced than more compact ones (BPCA), for which it even vanishes as the particles become larger. We also show that in both types of comets the main contribution to light scattering and emission comes from particles larger than 10 micron. Conclusions: .The strength of the silicate feature in the cometary infrared spectra suggests that the dust in type II comets consists of high-porosity aggregates, whereas the dust of type I comets contains low-porosity ones. This is consistent with the polarimetric features of these comets, which indicate that the dust in type I comets tends to concentrate near the nucleus. This may result from the predominance of highly processed particles in type I comets, whereas in type II comets we see pristine or slightly-processed dust. This conclusion is in accordance with the orbital characteristics of the comets. We have found that the strength of the silicate feature correlates with the semi-major axis of periodic comets and, for short-period comets, with the perihelion distance. Thus, the silicate feature weakens due to compaction of aggregate particles if a comet spends more time in the vicinity of the Sun, which allows the comet to accumulate a mantle on the surface of its nucleus.

astro-ph↗

arXiv2006

Near Infrared Polarization Images of the Orion Nebula

Wide-field (~8' x 8') and deep near-infrared (JHKs bands) polarization images of the Orion nebulae (IRNe) around young stellar objects (YSOs), both massive and low-mass. We found the IRNe around both IRc2 and BN to be very extensive, suggesting that there might be two extended (>0.7 pc) bipolar/monopolar IRNe in these sources. We discovered at least 13 smaller-scale (~0.01-0.1 pc) IRNe around less-massive YSOs including the famous source theta^2 Ori C. We also suggest the presence of many unresolved (<690 AU) systems around low-mass YSOs and young brown dwarfs showing possible intrinsic polarizations. Wide-field infrared polarimetry is thus demonstrated to be a powerful technique in revealing IRNe and hence potential disk/outflow systems among high-mass to substellar YSOs.

astro-ph↗

arXiv2006

Field-induced ferroelectric and commensurate spin state in mutiferroic HoMn$_{2}$O$_{5}$

Neutron diffraction measurements under high magnetic fields have been performed for the multiferroic compound HoMn$_{2}$O$_{5}$. At zero field, high-temperature incommensurate magnetic (HT-ICM) -- commensurate magnetic (CM) -- low-temperature incommensurate magnetic (LT-ICM) orders occur with decreasing temperature, where ferroelectric polarization arises only in the CM phase. Upon applying a magnetic field, the LT-ICM phase completely disappears and the CM phase is induced at the lowest temperature. This field-induced CM state is completely associated with the field-induced electric polarization in this material [Higashiyama {\it et al}., Phys. Rev. B {\bf 72}, 064421 (2005).], strongly indicating that the commensurate spin state is essential to the ferroelectricity in the multiferroic $R$Mn$_{2}$O$_{5}$ system.

cond-mat.str-el↗