arXiv subjects

H. Klein

Publications and source records attributed to H. Klein.

7 recordsLinked to original sources

arXiv2023

Collective magnetic state induced by charge disorder in the non-Kramers rare-earth pyrochlore Tb$_{2}$ScNbO$_{7}$

Geometrical frustration, as in pyrochlore lattices made of corner-sharing tetrahedra, precludes the onset of conventional magnetic ordering, enabling the stabilization of fluctuating spin states at low temperature. Disorder is a subtle ingredient that can modify the nature of these exotic non-ordered phases. Here, we study the interplay between disorder and magnetic frustration in the new pyrochlore Tb$_{2}$ScNbO$_{7}$ where the non magnetic site presents a charge disorder Nb$^{5+}$/Sc$^{3+}$. Its quantification with sophisticated diffraction techniques (electrons, X-rays, neutrons) allows us to estimate the distribution of the splitting of the magnetic Tb$^{3+}$ non-Kramers ground state doublets and to compare it with excitations measured in inelastic neutron scattering. Combining macroscopic and neutron scattering measurements, we show that a clear spin glass transition at 1 K stems out while retaining strong spin liquid correlations. Our results suggest that Tb$_{2}$ScNbO$_{7}$ stabilizes one of the novel disorder induced quantum spin liquid or topological glassy phases recently proposed theoretically.

cond-mat.str-el↗

arXiv2020

Electrical molecular switch addressed by chemical stimuli

We demonstrate that the conductance switching of benzo-bis(imidazole) molecules upon protonation depends on the lateral functional groups. The protonated H-substituted molecule shows a higher conductance than the neutral one (Gpro>Gneu), while the opposite (Gneu>Gpro) is observed for a molecule laterally functionalized by amino-phenyl groups. These results are demonstrated at various scale lengths : self-assembled monolayer, tiny nanodot-molecule junction and single molecules. From ab-initio theoretical calculations, we conclude that for the H-substituted molecule, the result Gpro>Gneu is correctly explained by a reduction of the LUMO-HOMO gap, while for the amino-phenyl functionnalized molecule, the result Gneu>Gpro is consistent with a shift of HOMO, which reduces the density of states at the Fermi energy.

physics.app-ph↗

arXiv2017

Estimating single molecule conductance from spontaneous evolution of a molecular contact

We present an original method to estimate the conductivity of a single molecule anchored to nanometric-sized metallic electrodes, using a Mechanically Controlled Break Junction (MCBJ) operated at room temperature in liquid. We record the conductance through the metal / molecules / metal nanocontact while keeping the metallic electrodes at a fixed distance. Taking advantage of thermal diffusion and electromigration, we let the contact naturally explore the more stable configurations around a chosen conductance value. The conductance of a single molecule is estimated from a statistical analysis of raw conductance and conductance standard deviation data for molecular contacts containing up to 14 molecules. The single molecule conductance values are interpreted as time-averaged conductance of an ensemble of conformers at thermal equilibrium.

cond-mat.mes-hall↗

arXiv2008

Cross section measurements of $α$-induced reactions on $^{92,94}$Mo and $^{112}$Sn for $p$-process studies

The $^{92}$Mo($α,n$)$^{95}$Ru, $^{94}$Mo($α,n$)$^{97}$Ru, and $^{112}$Sn($α,γ$)$^{116}$Te cross sections were measured at the upper end of the $p$-process Gamow window between 8.2 MeV and 11.1 MeV. Our results are slightly lower than global Hauser-Feshbach calculations from the code NON-SMOKER, but still within the uncertainty of the prediction. The $^{112}$Sn($α,γ$)$^{116}$Te cross section agrees well with a recently measured thick-target cross section in the same energy range. For the $^{92,94}$Mo($α,n$) reactions the present data close to the reaction thresholds could eliminate previous uncertainties within a factor of 20, and we can present now useful comparisons to statistical model calculations with different optical potentials.

astro-ph↗

arXiv2008

Quantum Physics Exploring Gravity in the Outer Solar System: The Sagas Project

We summarise the scientific and technological aspects of the SAGAS (Search for Anomalous Gravitation using Atomic Sensors) project, submitted to ESA in June 2007 in response to the Cosmic Vision 2015-2025 call for proposals. The proposed mission aims at flying highly sensitive atomic sensors (optical clock, cold atom accelerometer, optical link) on a Solar System escape trajectory in the 2020 to 2030 time-frame. SAGAS has numerous science objectives in fundamental physics and Solar System science, for example numerous tests of general relativity and the exploration of the Kuiper belt. The combination of highly sensitive atomic sensors and of the laser link well adapted for large distances will allow measurements with unprecedented accuracy and on scales never reached before. We present the proposed mission in some detail, with particular emphasis on the science goals and associated measurements.

gr-qc↗

arXiv2000

Beam Dynamics Studies for a High Current Ion Injector

Recent ion source developments resulted in the generation of high brilliance, high current beams of protons and light ions. After extraction and transport the beams with large internal space charge forces have to be captured, bunched and preaccelerated for the injection into the following driver part of a new generation of high intensity beam facilities for neutron sources, energy production, transmutation e.g. A combination of RFQ and DTL is considered to be a good solution for such a high current ion injector. Some preliminary beam dynamics layouts have been investigated by multiparticle simulations. Basic parameters like frequency, ion energy and sparking have been varied for the International Fusion Material Irradiation Facility (IFMIF) scenario as an example. The main interest was directed to high transmission, low losses and emittance conservation. The beam matching to the RFQ is shortly discussed as well as the matching between RFQ and DTL.

physics.acc-ph↗

arXiv2000

The Diffraction Model and its Applicability for Wakefield Calculations

The operation of a Free Electron Laser (FEL) in the ultraviolet or in the X-ray regime requires the acceleration of electron bunches with an rms length of 25 to 50 micro meters. The wakefields generated by these sub picosecond bunches extend into the frequency range well beyond the threshold for Cooper pair breakup (about 750 GHz) in superconducting niobium at 2 K. It is shown, that the superconducting cavities can indeed be operated with 25 micro meter bunches without suffering a breakdown of superconductivity (quench), however at the price of a reduced quality factor and an increased heat transfer to the superfluid helium bath. This was first shown by wakefield calculations based on the diffraction model. In the meantime a more conventional method of computing wake fields in the time domain by numerical methods was developed and used for the wakefield calculations. Both methods lead to comparable results: the operation of TESLA with 25 micro meter bunches is possible but leads to an additional heat load due to the higher order modes (HOMs). Therefore HOM dampers for these high frequencies are under construction. These dampers are located in the beam pipes between the 9-cell cavities. So it is of interest, if there are trapped modes in the cavity due to closed photon orbits. In this paper we investigate the existence of trapped modes and the distribution of heat load over the surface of the TESLA cavity by numerical photon tracking.

physics.acc-ph↗