arXiv subjects

H. Lee

Publications and source records attributed to H. Lee.

At least 73 records · Page 4Linked to original sources

arXiv2020

Purcell enhancement of a single silicon carbide color center with coherent spin control

Silicon carbide has recently been developed as a platform for optically addressable spin defects. In particular, the neutral divacancy in the 4H polytype displays an optically addressable spin-1 ground state and near-infrared optical emission. Here, we present the Purcell enhancement of a single neutral divacancy coupled to a photonic crystal cavity. We utilize a combination of nanolithographic techniques and a dopant-selective photoelectrochemical etch to produce suspended cavities with quality factors exceeding 5,000. Subsequent coupling to a single divacancy leads to a Purcell factor of ~50, which manifests as increased photoluminescence into the zero-phonon line and a shortened excited-state lifetime. Additionally, we measure coherent control of the divacancy ground state spin inside the cavity nanostructure and demonstrate extended coherence through dynamical decoupling. This spin-cavity system represents an advance towards scalable long-distance entanglement protocols using silicon carbide that require the interference of indistinguishable photons from spatially separated single qubits.

quant-ph↗

arXiv2020

Hybridization dynamics in CeCoIn5 revealed by ultrafast optical spectroscopy

We investigate the quasiparticle dynamics in the prototype heavy fermion CeCoIn$_5$ using ultrafast optical pump-probe spectroscopy. Our results indicate that this material system undergoes hybridization fluctuations before full establishment of the heavy electron coherence, as the temperature decreases from $\sim$120 K ($T^\dagger$) to $\sim$55 K ($T^*$ ). We reveal that the observed anomalous phonon softening and damping reduction below $T^*$ are directly associated with opening of an indirect hybridization gap. We also discover a distinct collective mode with an energy of $\sim$8 meV, which may be the experimental evidence of the predicted unconventional density wave. Our observations provide critical informations for understanding the hybridization dynamics in heavy fermion materials.

cond-mat.str-el↗

arXiv2019

Enhancement in hydrogen storage capacities of light metal functionalized Boron Graphdiyne nanosheets

The recent experimental synthesis of the two-dimensional (2D)boron-graphdiyne (BGDY) nanosheet has motivated us to investigate its structural, electronic,and energy storage properties. BGDY is a particularly attractive candidate for this purpose due to uniformly distributed pores which can bind the light-metal atoms. Our DFTcalculations reveal that BGDY can accommodate multiple light-metal dopants (Li, Na, K, Ca)with significantly high binding energies. The stabilities of metal functionalized BGDY monolayers have been confirmed through ab initio molecular dynamics simulations. Furthermore, significant charge-transfer between the dopantsand BGDY sheet renders the metal with a significant positive charge, which is a prerequisite for adsorbing hydrogen (H2) molecules with appropriate binding energies.This results in exceptionally high H2 storage capacities of 14.29, 11.11, 9.10 and 8.99 wt% for the Li, Na, K and Ca dopants, respectively. These H2storage capacities are much higher than many 2D materials such as graphene, graphane, graphdiyne, graphyne, C2N, silicene, and phosphorene. Average H2 adsorption energies for all the studied systems fall within an ideal window of 0.17-0.40 eV/H2. We have also performed thermodynamic analysis to study the adsorption/desorption behavior of H2, which confirmsthat desorption of the H2molecules occurs at practical conditions of pressure and temperature.

cond-mat.mes-hall↗

arXiv2018

Switchable Weyl nodes in topological Kagome ferromagnet Fe3Sn2

The control of topological quantum materials is the prerequisite for novel devices exploiting these materials. Here we propose that the room temperature ferromagnet Fe3Sn2, whose fundamental building blocks are Kagome bilayers of iron, hosts Weyl nodes at the Fermi level which can move in momentum space depending on the direction of the magnetization, itself readily controlled either by modest external fields or temperature. The proposal is derived from density functional calculations, including a mean field treatment of Hubbard repulsion U, which have been validated by comparison with angle-resolved photoemission data. Ferromagnetism with magnetization along certain directions is shown to lift the Weyl degeneracies, while at the same time inducing texture in the quasiparticle spin polarizations mapped in reciprocal space. In particular, the polarization is attenuated and then rotated from parallel to perpendicular to antiparallel to the magnetization as Weyl points derived from crossing of majority and minority spin bands are traversed.

cond-mat.str-el↗

arXiv2018

Fully gapped $d$-wave superconductivity in CeCu$_2$Si$_2$

The nature of the pairing symmetry of the first heavy fermion superconductor CeCu$_2$Si$_2$ has recently become the subject of controversy. While CeCu$_2$Si$_2$ was generally believed to be a $d$-wave superconductor, recent low temperature specific heat measurements showed evidence for fully gapped superconductivity, contrary to the nodal behavior inferred from earlier results. Here we report London penetration depth measurements, which also reveal fully gapped behavior at very low temperatures. To explain these seemingly conflicting results, we propose a fully gapped $d+d$ band-mixing pairing state for CeCu$_2$Si$_2$, which yields very good fits to both the superfluid density and specific heat, as well as accounting for a sign change of the superconducting order parameter, as previously concluded from inelastic neutron scattering results.

cond-mat.supr-con↗

arXiv2018

Surface reconstruction and charge modulation in BaFe2As2 superconducting film

Whether or not epitaxially grown superconducting films have the same bulk-like superconducting properties is an important concern. We report the structure and the electronic properties of epitaxially grown Ba(Fe1-xCox)2As2 films using scanning tunneling microscopy and scanning tunneling spectroscopy (STS). This film showed a different surface structure, (2sqrtx2sqrt2)R45 reconstruction, from those of as-cleaved surfaces from bulk crystals. The electronic structure of the grown film is different from that in bulk, and it is notable that the film exhibits the same superconducting transport properties. We found that the superconducting gap at the surface is screened at the Ba layer surface in STS measurements, and the charge density wave was observed at the surface in sample in the superconducting state.

cond-mat.supr-con↗

arXiv2018

Band dependent inter-layer $f$-electron hybridization in CeRhIn$_5$

A key issue in heavy fermion research is how subtle changes in the hybridization between the 4$f$ (5$f$) and conduction electrons can result in fundamentally different ground states. CeRhIn$_5$ stands out as a particularly notable example: replacing Rh by either Co or Ir, located above or below Rh in the periodic table, antiferromagnetism gives way to superconductivity. In this photoemission study of CeRhIn$_5$, we demonstrate that the use of resonant ARPES with polarized light allows to extract detailed information on the 4$f$ crystal field states and details on the 4$f$ and conduction electron hybridization which together determine the ground state. We directly observe weakly dispersive Kondo resonances of $f$-electrons and identify two of the three Ce $4f_{5/2}^{1}$ crystal-electric-field levels and band-dependent hybridization, which signals that the hybridization occurs primarily between the Ce $4f$ states in the CeIn$_3$ layer and two more three-dimensional bands composed of the Rh $4d$ and In $5p$ orbitals in the RhIn$_2$ layer. Our results allow to connect the properties observed at elevated temperatures with the unusual low-temperature properties of this enigmatic heavy fermion compound.

cond-mat.str-el↗

arXiv2017

The status of KAGRA underground cryogenic gravitational wave telescope

KAGRA is a 3-km interferometric gravitational wave telescope located in the Kamioka mine in Japan. It is the first km-class gravitational wave telescope constructed underground to reduce seismic noise, and the first km-class telescope to use cryogenic cooling of test masses to reduce thermal noise. The construction of the infrastructure to house the interferometer in the tunnel, and the initial phase operation of the interferometer with a simple 3-km Michelson configuration have been completed. The first cryogenic operation is expected in 2018, and the observing runs with a full interferometer are expected in 2020s. The basic interferometer configuration and the current status of KAGRA are described.

gr-qc↗

arXiv2016

Optically switched magnetism in photovoltaic perovskite CH$_3$NH$_3$(Mn:Pb)I$_3$

The demand for ever-increasing density of information storage and speed of manipulation boosts an intense search for new magnetic materials and novel ways of controlling the magnetic bit. Here, we report the synthesis of a ferromagnetic photovoltaic CH$_3$NH$_3$(Mn:Pb)I$_3$ material in which the photo-excited electrons rapidly melt the local magnetic order through the Ruderman-Kittel-Kasuya-Yosida interactions without heating up the spin system. Our finding offers an alternative, very simple and efficient way of optical spin control, and opens an avenue for applications in low power, light controlling magnetic devices.

cond-mat.mtrl-sci↗

arXiv2016

Direct observation of how the heavy fermion state develops in CeCoIn5

Heavy fermion materials gain high electronic masses and expand Fermi surfaces when the high-temperature localized f electrons become itinerant and hybridize with the conduction band at low temperatures. However, despite the common application of this model, direct microscopic verification remains lacking. Here we report high-resolution angle-resolved photoemission spectroscopy measurements on CeCoIn5, a prototypical heavy fermion compound, and reveal the long-sought band hybridization and Fermi surface expansion. Unexpectedly, the localized-to-itinerant transition occurs at surprisingly high temperatures, yet f electrons are still largely localized at the lowest temperature. Moreover, crystal field excitations likely play an important role in the anomalous temperature dependence. Our results paint an comprehensive unanticipated experimental picture of the heavy fermion formation in a periodic multi-level Anderson/Kondo lattice, and set the stage for understanding the emergent properties in related materials.

cond-mat.str-el↗

arXiv2014

Measurement of Muon Antineutrino Quasi-Elastic Scattering on a Hydrocarbon Target at E_ν ~ 3.5 GeV

We have isolated muon anti-neutrino charged-current quasi-elastic interactions occurring in the segmented scintillator tracking region of the MINERvA detector running in the NuMI neutrino beam at Fermilab. We measure the flux-averaged differential cross-section, dσ/dQ^2, and compare to several theoretical models of quasi-elastic scattering. Good agreement is obtained with a model where the nucleon axial mass, M_A, is set to 0.99 GeV/c^2 but the nucleon vector form factors are modified to account for the observed enhancement, relative to the free nucleon case, of the cross-section for the exchange of transversely polarized photons in electron-nucleus scattering. Our data at higher Q^2 favor this interpretation over an alternative in which the axial mass is increased.

hep-ex↗

arXiv2014

Measurement of Muon Neutrino Quasi-Elastic Scattering on a Hydrocarbon Target at E_ν ~ 3.5 GeV

We report a study of muon neutrino charged-current quasi-elastic events in the segmented scintillator inner tracker of the MINERvA experiment running in the NuMI neutrino beam at Fermilab. The events were selected by requiring a μ^- and low calorimetric recoil energy separated from the interaction vertex. We measure the flux-averaged differential cross-section, dσ/dQ^2, and study the low energy particle content of the final state. Deviations are found between the measured dσ/dQ^2 and the expectations of a model of independent nucleons in a relativistic Fermi gas. We also observe an excess of energy near the vertex consistent with multiple protons in the final state.

hep-ex↗

arXiv2013

Neutrinos

This document represents the response of the Intensity Frontier Neutrino Working Group to the Snowmass charge. We summarize the current status of neutrino physics and identify many exciting future opportunities for studying the properties of neutrinos and for addressing important physics and astrophysics questions with neutrinos.

hep-ex↗

arXiv2013

Design, Calibration, and Performance of the MINERvA Detector

The MINERvA experiment is designed to perform precision studies of neutrino-nucleus scattering using $ν_μ$ and ${\barν}_μ$ neutrinos incident at 1-20 GeV in the NuMI beam at Fermilab. This article presents a detailed description of the \minerva detector and describes the {\em ex situ} and {\em in situ} techniques employed to characterize the detector and monitor its performance. The detector is comprised of a finely-segmented scintillator-based inner tracking region surrounded by electromagnetic and hadronic sampling calorimetry. The upstream portion of the detector includes planes of graphite, iron and lead interleaved between tracking planes to facilitate the study of nuclear effects in neutrino interactions. Observations concerning the detector response over sustained periods of running are reported. The detector design and methods of operation have relevance to future neutrino experiments in which segmented scintillator tracking is utilized.

physics.ins-det↗

arXiv2013

Effects of pressure on the ferromagnetic state of the CDW compound SmNiC2

We report the pressure response of charge-density-wave (CDW) and ferromagnetic (FM) phases of the rare-earth intermetallic SmNiC2 up to 5.5 GPa. The CDW transition temperature (T_{CDW}), which is reflected as a sharp inflection in the electrical resistivity, is almost independent of pressure up to 2.18 GPa but is strongly enhanced at higher pressures, increasing from 155.7 K at 2.2 GPa to 279.3 K at 5.5 GPa. Commensurate with the sharp increase in T_{CDW}, the first-order FM phase transition, which decreases with applied pressure, bifurcates into the upper (T_{M1}) and lower (T_c) phase transitions and the lower transition changes its nature to second order above 2.18 GPa. Enhancement both in the residual resistivity and the Fermi-liquid T^2 coefficient A near 3.8 GPa suggests abundant magnetic quantum fluctuations that arise from the possible presence of a FM quantum critical point.

cond-mat.str-el↗

arXiv2012

Black hole mass and Eddington ratio distribution functions of X-ray selected broad-line AGNs at z~1.4 in the Subaru XMM-Newton Deep Field

In order to investigate the growth of super-massive black holes (SMBHs), we construct the black hole mass function (BHMF) and Eddington ratio distribution function (ERDF) of X-ray-selected broad-line AGNs at z~1.4 in the Subaru XMM-Newton Deep Survey field. In this redshift range, a significant part of the accretion growth of SMBHs is thought to be taking place. Black hole masses of X-ray-selected broad-line AGNs are estimated using the width of the broad MgII line and the 3000A monochromatic luminosity. We supplement the MgII FWHM values with the Ha FWHM obtained from our NIR spectroscopic survey. Using the black hole masses of broad-line AGNs at redshifts between 1.18 and 1.68, the binned broad-line AGN BHMF and ERDF are calculated using the Vmax method. To properly account for selection effects that impact the binned estimates, we derive the corrected broad-line AGN BHMF and ERDF by applying the Maximum Likelihood method, assuming that the ERDF is constant regardless of the black hole mass. We do not correct for the non-negligible uncertainties in virial BH mass estimates. If we compare the corrected broad-line AGN BHMF with that in the local Universe, the corrected BHMF at z~1.4 has a higher number density above 10^8 Msolar but a lower number density below that mass range. The evolution may be indicative of a down-sizing trend of accretion activity among the SMBH population. The evolution of broad-line AGN ERDF from z=1.4 to 0 indicates that the fraction of broad-line AGNs with accretion rate close to the Eddington-limit is higher at higher redshifts.

astro-ph.CO↗

arXiv2012

The MINER$ν$A Data Acquisition System and Infrastructure

MINER$ν$A (Main INjector ExpeRiment $ν$-A) is a new few-GeV neutrino cross section experiment that began taking data in the FNAL NuMI (Fermi National Accelerator Laboratory Neutrinos at the Main Injector) beam-line in March of 2010. MINER$ν$A employs a fine-grained scintillator detector capable of complete kinematic characterization of neutrino interactions. This paper describes the MINER$ν$A data acquisition system (DAQ) including the read-out electronics, software, and computing architecture.

physics.ins-det↗

arXiv2012

Field-induced long-lived supermolecules

We demonstrate that the long-lived bound states (super-molecules) can exist in the dilute limit when we tune the shape of effective potential between polar molecules by an external microwave field. Binding energies, average sizes, and phase diagrams for both s-orbital (bosons) and p-orbital (fermions) dimers are studied, together with bosonic trimer states. We explicitly show that the non- adiabatic transition rate can be easily tuned small for such ground state super-molecules, so that the system can be stable from collapse even near the associated potential resonance. Our results, therefore, suggest a feasible cold molecule system to investigate both novel few-body and many-body physics (for example, the p-wave BCS-BEC crossover for fermions and the paired condensate for bosons) that can not be easily accessed in single species atomic gases.

cond-mat.quant-gas↗