arXiv subjects

H. Mori

Publications and source records attributed to H. Mori.

At least 19 recordsLinked to original sources

arXiv2020

Large Enhancement of Thermoelectric Efficiency Due to a Pressure-Induced Lifshitz Transition in SnSe

Lifshitz transition, a change in Fermi surface topology, is likely to greatly influence exotic correlated phenomena in solids, such as high-temperature superconductivity and complex magnetism. However, since the observation of Fermi surfaces is generally difficult in the strongly correlated systems, a direct link between the Lifshitz transition and quantum phenomena has been elusive so far. Here, we report a marked impact of the pressure-induced Lifshitz transition on thermoelectric performance for SnSe, a promising thermoelectric material without strong electron correlation. By applying pressure up to 1.6 GPa, we have observed a large enhancement of thermoelectric power factor by more than 100% over a wide temperature range (10-300 K). Furthermore, the high carrier mobility enables the detection of quantum oscillations of resistivity, revealing the emergence of new Fermi pockets at ~0.86 GPa. The observed thermoelectric properties linked to the multi-valley band structure are quantitatively reproduced by first-principles calculations, providing novel insight into designing the SnSe-related materials for potential valleytronic as well as thermoelectric applications.

cond-mat.mtrl-sci↗

arXiv2019

Multisensory Learning Framework for Robot Drumming

The hype about sensorimotor learning is currently reaching high fever, thanks to the latest advancement in deep learning. In this paper, we present an open-source framework for collecting large-scale, time-synchronised synthetic data from highly disparate sensory modalities, such as audio, video, and proprioception, for learning robot manipulation tasks. We demonstrate the learning of non-linear sensorimotor mappings for a humanoid drumming robot that generates novel motion sequences from desired audio data using cross-modal correspondences. We evaluate our system through the quality of its cross-modal retrieval, for generating suitable motion sequences to match desired unseen audio or video sequences.

cs.RO↗

arXiv2018

Inorbit Performance of the Hard X-ray Telescope (HXT) on board the Hitomi (ASTRO-H) satellite

Hitomi (ASTRO-H) carries two Hard X-ray Telescopes (HXTs) that can focus X-rays up to 80 keV. Combined with the Hard X-ray Imagers (HXIs) that detect the focused X-rays, imaging spectroscopy in the high-energy band from 5 keV to 80 keV is made possible. We studied characteristics of HXTs after the launch such as the encircled energy function (EEF) and the effective area using the data of a Crab observation. The half power diameters (HPDs) in the 5--80 keV band evaluated from the EEFs are 1.59 arcmin for HXT-1 and 1.65 arcmin for HXT-2. Those are consistent with the HPDs measured with ground experiments when uncertainties are taken into account. We can conclude that there is no significant change in the characteristics of the HXTs before and after the launch. The off-axis angle of the aim point from the optical axis is evaluated to be less than 0.5 arcmin for both HXT-1 and HXT-2. The best-fit parameters for the Crab spectrum obtained with the HXT-HXI system are consistent with the canonical values.

astro-ph.IM↗

arXiv2018

Size effects on supercooling phenomena in strongly correlated electron systems: IrTe$_2$ and $θ$-(BEDT-TTF)$_2$RbZn(SCN)$_4$

We report that the sample miniaturization of first-order-phase-transition bulk systems causes a greater degree of supercooling. From a theoretical perspective, the size effects can be rationalized by considering two mechanisms: (i) the nucleation is a rare and stochastic event, and thus, its rate is correlated with the volume and/or surface area of a given sample; (ii) when the sample size decreases, the dominant heterogeneous nucleation sites that play a primary role for relatively large samples are annealed out. We experimentally verified the size effects on the supercooling phenomena for two different types of strongly correlated electron systems: the transition-metal dichalcogenide IrTe$_2$ and the organic conductor $θ$-(BEDT-TTF)$_2$RbZn(SCN)$_4$. The origin of the size effects considered in this study does not depend on microscopic details of the material; therefore, they may often be involved in the first-order-transition behavior of small-volume specimens.

cond-mat.str-el↗

arXiv2017

Direct observation of double valence-band extrema and anisotropic effective masses of the thermoelectric material SnSe

Synchrotron-based angle-resolved photoemission spectroscopy is used to determine the electronic structure of layered SnSe, which was recently turned out to be a potential thermoelectric material. We observe that the top of the valence band consists of two nearly independent hole bands, whose tops differ by ~20 meV in energy, indicating the necessity of a multivalley model to describe the thermoelectric properties. The estimated effective masses are anisotropic, with in-plane values of 0.16-0.39 m$_0$ and an out-of-plane value of 0.71 m$_0$, where m$_0$ is the rest electron mass. Information of the electronic structure is essential to further enhance the thermoelectric performance of hole-doped SnSe.

cond-mat.mtrl-sci↗

arXiv2017

Crystallization and vitrification of electrons in a glass-forming charge liquid

Charge ordering (CO) is a phenomenon in which electrons in solids crystallize into a periodic pattern of charge-rich and charge-poor sites owing to strong electron correlations. This usually results in long-range order. In geometrically frustrated systems, however, a glassy electronic state without long-range CO has been observed. We found that a charge-ordered organic material with an isosceles triangular lattice shows charge dynamics associated with crystallization and vitrification of electrons, which can be understood in the context of an energy landscape arising from the degeneracy of various CO patterns. The dynamics suggest that the same nucleation and growth processes that characterize conventional glass-forming liquids guide the crystallization of electrons. These similarities may provide insight into our understanding of the liquid-glass transition.

cond-mat.str-el↗

arXiv2017

In-orbit performance of the soft X-ray imaging system aboard Hitomi (ASTRO-H)

We describe the in-orbit performance of the soft X-ray imaging system consisting of the Soft X-ray Telescope and the Soft X-ray Imager aboard Hitomi. Verification and calibration of imaging and spectroscopic performance are carried out making the best use of the limited data of less than three weeks. Basic performance including a large field of view of 38'x38' is verified with the first light image of the Perseus cluster of galaxies. Amongst the small number of observed targets, the on-minus-off pulse image for the out-of-time events of the Crab pulsar enables us to measure a half power diameter of the telescope as about 1.3'. The average energy resolution measured with the onboard calibration source events at 5.89 keV is 179 pm 3 eV in full width at half maximum. Light leak and cross talk issues affected the effective exposure time and the effective area, respectively, because all the observations were performed before optimizing an observation schedule and parameters for the dark level calculation. Screening the data affected by these two issues, we measure the background level to be 5.6x10^{-6} counts s^{-1} arcmin^{-2} cm^{-2} in the energy band of 5-12 keV, which is seven times lower than that of the Suzaku XIS-BI.

astro-ph.IM↗

arXiv2017

Quantum-disordered state of magnetic and electric dipoles in a hydrogen-bonded Mott system

Strongly enhanced quantum fluctuations often lead to a rich variety of quantum-disordered states. A representative case is liquid helium, in which zero-point vibrations of the helium atoms prevent its solidification at low temperatures. A similar behaviour is found for the internal degrees of freedom in electrons. Among the most prominent is a quantum spin liquid (QSL), in which localized spins are highly correlated but fluctuate even at absolute zero. Recently, a coupling of spins with other degrees of freedom has been proposed as an innovative approach to generate even more fascinating QSLs such as orbital--spin liquids. However, such ideas are limited to the internal degrees of freedom in electrons. Here, we demonstrate that a coupling of localized spins with the zero-point motion of hydrogen atoms (proton fluctuations) in a hydrogen-bonded organic Mott insulator provides a new class of QSLs. We find that a divergent dielectric behaviour towards a hydrogen-bond order is suppressed by the quantum proton fluctuations, resulting in a quantum paraelectric (QPE) state. Furthermore, our thermal-transport measurements reveal that a QSL state with gapless spin excitations rapidly emerges upon entering the QPE state. These findings indicate that the quantum proton fluctuations give rise to a novel QSL --- a quantum-disordered state of magnetic and electric dipoles --- through the coupling between the electron and proton degrees of freedom.

cond-mat.str-el↗

arXiv2015

Angular resolution measurements at SPring-8 of a hard X-ray optic for the New Hard X-ray Mission

The realization of X-ray telescopes with imaging capabilities in the hard (> 10 keV) X-ray band requires the adoption of optics with shallow (< 0.25 deg) grazing angles to enhance the reflectivity of reflective coatings. On the other hand, to obtain large collecting area, large mirror diameters (< 350 mm) are necessary. This implies that mirrors with focal lengths >10 m shall be produced and tested. Full-illumination tests of such mirrors are usually performed with on- ground X-ray facilities, aimed at measuring their effective area and the angular resolution; however, they in general suffer from effects of the finite distance of the X-ray source, e.g. a loss of effective area for double reflection. These effects increase with the focal length of the mirror under test; hence a "partial" full-illumination measurement might not be fully representative of the in-flight performances. Indeed, a pencil beam test can be adopted to overcome this shortcoming, because a sector at a time is exposed to the X-ray flux, and the compensation of the beam divergence is achieved by tilting the optic. In this work we present the result of a hard X-ray test campaign performed at the BL20B2 beamline of the SPring-8 synchrotron radiation facility, aimed at characterizing the Point Spread Function (PSF) of a multilayer-coated Wolter-I mirror shell manufactured by Nickel electroforming. The mirror shell is a demonstrator for the NHXM hard X-ray imaging telescope (0.3 - 80 keV), with a predicted HEW (Half Energy Width) close to 20 arcsec. We show some reconstructed PSFs at monochromatic X-ray energies of 15 to 63 keV, and compare them with the PSFs computed from post-campaign metrology data, self-consistently treating profile and roughness data by means of a method based on the Fresnel diffraction theory. The modeling matches the measured PSFs accurately.

astro-ph.IM↗

arXiv2015

Phase-change memory function of correlated electrons in organic conductors

Phase-change memory (PCM), a promising candidate for next-generation non-volatile memories, exploits quenched glassy and thermodynamically stable crystalline states as reversibly switchable state variables. We demonstrate PCM functions emerging from a charge-configuration degree of freedom in strongly correlated electron systems. Non-volatile reversible switching between a high-resistivity charge-crystalline (or charge-ordered) state and a low-resistivity quenched state, charge glass, is achieved experimentally via heat pulses supplied by optical or electrical means in organic conductors $θ$-(BEDT-TTF)$_2$$X$. Switching that is one order of magnitude faster is observed in another isostructural material that requires faster cooling to kinetically avoid charge crystallization, indicating that the material's critical cooling rate can be useful guidelines for pursuing a faster correlated-electron PCM function.

cond-mat.str-el↗

arXiv2014

ASTRO-H White Paper - Low-mass X-ray Binaries

There is still 10-20% uncertainty on the neutron star (NS) mass-radius relation. These uncertainties could be reduced by an order of magnitude through an unambiguous measure of M/R from the surface redshift of a narrow line, greatly constraining the Equation of State for ultra-dense material. It is possible that the SXS on ASTRO-H can detect this from an accreting neutron star with low surface velocity in the line of sight i.e. either low inclination or low spin. Currently there is only one known low inclination LMXB, Ser X-1, and one known slow spin LMXB, J17480-2446 in Terzan 5. Ser X-1 is a persistent source which is always in the soft state (banana branch), where the accreting material should form a equatorial belt around the neutron star. A pole-on view should then allow the NS surface to be seen directly. A 100 ks observation should allow us to measure M/R if there are any heavy elements in the photosphere at the poles. Conversely, J17480-2446 in Terzan 5 is a transient accretion powered millisecond pulsar, where the accreting material is collimated onto the magnetic pole in the hard (island) state (L_x < 0.1 L_Edd). The hotspot where the shock illuminates the NS surface is clearly seen in this state. A 100 ks ToO observation of this (or any other similarly slow spin system) in this state, may again allow the surface redshift to be directly measured. (abstract continues)

astro-ph.HE↗

arXiv2014

Systematic Variations in the Charge-Glass-Forming Ability of Geometrically Frustrated $θ$-(BEDT-TTF)$_2X$ Organic Conductors

The critical cooling rate $R_{\rm c}$ above which charge ordering is kinetically avoided upon cooling, which results in charge-glass formation, was investigated for the geometrically frustrated system $θ$-(BEDT-TTF)$_2X$. X-ray diffraction experiments revealed that $θ$-(BEDT-TTF)$_2$TlCo(SCN)$_4$ exhibits a horizontally charge-ordered state, and kinetic avoidance of this state requires rapid cooling of faster than 150 K/min. This value is markedly higher than that reported for two other isostructural $θ$-type compounds, thus demonstrating the lower charge-glass-forming ability of $X$ $=$ TlCo(SCN)$_4$. In accounting for the systematic variations of $R_{\rm c}$ among the three $θ$-(BEDT-TTF)$_2X$, we found that stronger charge frustration leads to superior charge-glass former. Our results suggest that charge frustration tends to slow the kinetics of charge ordering.

cond-mat.str-el↗

arXiv2013

Multi-command Tactile and Auditory Brain Computer Interface based on Head Position Stimulation

We study the extent to which vibrotactile stimuli delivered to the head of a subject can serve as a platform for a brain computer interface (BCI) paradigm. Six head positions are used to evoke combined somatosensory and auditory (via the bone conduction effect) brain responses, in order to define a multimodal tactile and auditory brain computer interface (taBCI). Experimental results of subjects performing online taBCI, using stimuli with a moderately fast inter-stimulus interval (ISI), validate the taBCI paradigm, while the feasibility of the concept is illuminated through information transfer rate case studies.

q-bio.NC↗

arXiv2009

Search for VHE gamma rays from SS433/W50 with the CANGAROO-II telescope

SS433, located at the center of the supernova remnant W50, is a close proximity binary system consisting of a compact star and a normal star. Jets of material are directed outwards from the vicinity of the compact star symmetrically to the east and west. Non-thermal hard X-ray emission is detected from lobes lying on both sides. Shock accelerated electrons are expected to generate sub-TeV gamma rays through the inverse-Compton process in the lobes. Observations of the western X-ray lobe region of SS433/W50 system have been performed to detect sub-TeV gamma-rays using the 10m CANGAROO-II telescope in August and September, 2001, and July and September, 2002. The total observation times are 85.2 hours for ON source, and 80.8 hours for OFF source data. No significant excess of sub-TeV gamma rays has been found at 3 regions of the western X-ray lobe of SS433/W50 system. We have derived 99% confidence level upper limits to the fluxes of gamma rays and have set constraints on the strengths of the magnetic fields assuming the synchrotron/inverse-Compton model for the wide energy range of photon spectrum from radio to TeV. The derived lower limits are 4.3 microgauss for the center of the brightest X-ray emission region and 6.3 microgauss for the far end from SS433 in the western X-ray lobe. In addition, we suggest that the spot-like X-ray emission may provide a major contribution to the hardest X-ray spectrum in the lobe.

astro-ph.HE↗

arXiv2007

X-Ray Observations of the Galactic Center with Suzaku

We report on the diffuse X-ray emissions from the Galactic center (GCDX) observed with the X-ray Imaging Spectrometer (XIS) on board the Suzaku satellite. The highly accurate energy calibrations and extremely low background of the XIS provide many new facts on the GCDX. These are (1) the origin of the 6.7/7.0keV lines is collisional excitation in hot plasma, (2) new SNR and super-bubble candidates are found, (3) most of the 6.4keV line is fluorescence by X-rays, and (4) time variability of the 6.4keV line is found from the SgrB2 complex.

astro-ph↗

arXiv2007

Superconductivity in the vicinity of charge ordered state in organic conductor beta-(meso-DMBEDT-TTF)_2PF_6

We study theoretically competition between the charge ordering and the superconductivity in two-dimensional organic conductor beta-(meso-DMBEDT-TTF)_2PF_6. We analyze the extended Hubbard model on a weakly-dimerized lattice based on the random phase approximation and Eliashberg equations. We found reentrant behavior of the checkerbord-type charge-ordered phase in the phase diagram, and the triplet superconductivity due to the charge fluctuation in the neighboring region. In the low temperature and high pressure region, the singlet superconductivity also appears due to the enhancement of the spin fluctuation.

cond-mat.str-el↗

arXiv2006

Monte-Carlo Simulator and Ancillary Response Generator of Suzaku XRT/XIS System for Spatially Extended Source Analysis

We have developed a framework for the Monte-Carlo simulation of the X-Ray Telescopes (XRT) and the X-ray Imaging Spectrometers (XIS) onboard Suzaku, mainly for the scientific analysis of spatially and spectroscopically complex celestial sources. A photon-by-photon instrumental simulator is built on the ANL platform, which has been successfully used in ASCA data analysis. The simulator has a modular structure, in which the XRT simulation is based on a ray-tracing library, while the XIS simulation utilizes a spectral "Redistribution Matrix File" (RMF), generated separately by other tools. Instrumental characteristics and calibration results, e.g., XRT geometry, reflectivity, mutual alignments, thermal shield transmission, build-up of the contamination on the XIS optical blocking filters (OBF), are incorporated as completely as possible. Most of this information is available in the form of the FITS (Flexible Image Transport System) files in the standard calibration database (CALDB). This simulator can also be utilized to generate an "Ancillary Response File" (ARF), which describes the XRT response and the amount of OBF contamination. The ARF is dependent on the spatial distribution of the celestial target and the photon accumulation region on the detector, as well as observing conditions such as the observation date and satellite attitude. We describe principles of the simulator and the ARF generator, and demonstrate their performance in comparison with in-flight data.

astro-ph↗

arXiv2004

Large dielectric constant and giant nonlinear conduction in the organic conductor theta-(BEDT-TTF)_2CsZn(SCN)_4

The dielectric constant and ac conductivity have been measured for the layered organic conductor theta-(BEDT-TTF)_2CsZn(SCN)_4 along the out-of-plane direction, which show a relaxation behavior similar to those in the charge-density-wave conductor. Most unexpectedly, they exhibit a large bias dependence with a hysteresis, and changes in magnitude by 100-1000 times at a threshold. These findings are very similar to the collective excitation of the charge density wave. theta-$(BEDT-TTF)_2CsZn(SCN)_4 has collective excitations associated with charge ordering, though it shows no clear indication of long range order.

cond-mat.str-el↗